arXiv subjects

Wolfgang Ketterle

Publications and source records attributed to Wolfgang Ketterle.

At least 37 records · Page 2Linked to original sources

arXiv2022

Many-body spin rotation by adiabatic passage in spin-1/2 XXZ chains of ultracold atoms

Quantum many-body phases offer unique properties and emergent phenomena, making them an active area of research. A promising approach for their experimental realization in model systems is to adiabatically follow the ground state of a quantum Hamiltonian from a product state of isolated particles to one that is strongly-correlated. Such protocols are relevant also more broadly in coherent quantum annealing and adiabatic quantum computing. Here we explore one such protocol in a system of ultracold atoms in an optical lattice. A fully magnetized state is connected to a correlated zero-magnetization state (an xy-ferromagnet) by a many-body spin rotation, realized by sweeping the detuning and power of a microwave field. The efficiency is characterized by applying a reverse sweep with a variable relative phase. We restore up to 50% of the original magnetization independent of the relative phase, evidence for the formation of correlations. The protocol is limited by the many-body gap of the final state, which is inversely proportional to system size, and technical noise. Our experimental and theoretical studies highlight the potential and challenges for adiabatic preparation protocols to prepare many-body eigenstates of spin Hamiltonians.

cond-mat.quant-gas↗

arXiv2022

Magnetic trapping of ultracold molecules at high density

Trapping ultracold molecules in conservative traps is essential for applications -- such as quantum state-controlled chemistry, quantum simulations, and quantum information processing. These applications require high densities or phase-space densities. We report magnetic trapping of NaLi molecules in the triplet ground state at high density ($\approx 10^{11} \; \rm{cm}^{-3}$) and ultralow temperature ($\approx 1\;{\rm μK}$). Magnetic trapping at these densities allows studies on both atom-molecule and molecule-molecule collisions in the ultracold regime in the absence of trapping light, which has often lead to undesired photo-chemistry. We measure the inelastic loss rates in a single spin sample and spin-mixtures of fermionic NaLi as well as spin-stretched NaLi$+$Na mixtures. We demonstrate sympathetic cooling of NaLi molecules in the magnetic trap by radio frequency evaporation of co-trapped Na atoms and observe an increase in the molecules' phase-space density by a factor of $\approx 16$.

physics.atom-ph↗

arXiv2022

Dipolar spin-exchange and entanglement between molecules in an optical tweezer array

Due to their intrinsic electric dipole moments and rich internal structure, ultracold polar molecules are promising candidate qubits for quantum computing and for a wide range of quantum simulations. Their long-lived molecular rotational states form robust qubits while the long-range dipolar interaction between molecules provides quantum entanglement. Using a molecular optical tweezer array, single molecules can be moved and separately addressed for qubit operations using optical and microwave fields, creating a scalable quantum platform. Here, we demonstrate long-range dipolar spin-exchange interactions in pairs of CaF molecules trapped in an optical tweezer array. We control the anisotropic interaction and realize the spin-$\frac{1}{2}$ quantum XY model by encoding an effective spin-$\frac{1}{2}$ system into the rotational states of the molecules. We demonstrate a two-qubit (two-molecule) gate to generate entanglement deterministically, an essential resource for all quantum information applications. Employing interleaved tweezer arrays, we demonstrate high fidelity single site molecular addressability.

physics.atom-ph↗

arXiv2022

Spin dynamics dominated by superexchange via virtual molecules

Simple, paradigmatic systems are important tools in understanding strongly correlated systems. One such system is the Bose-Hubbard model, which can be realized using atoms in optical lattices with delta-function interactions. We report the first experimental observation of two features of the Bose-Hubbard model: superexchange via virtual molecules in excited bands and off-site contact interactions. Adiabatic sweeps confirm the creation of such molecules, exemplifying a new kind of Feshbach resonance.

physics.atom-ph↗

arXiv2022

A Feshbach resonance in collisions between ultracold ground state molecules

Collisional resonances are an important tool which has been used to modify interactions in ultracold gases, for realizing novel Hamiltonians in quantum simulations, for creating molecules from atomic gases and for controlling chemical reactions. So far, such resonances have been observed for atom-atom collisions, atom-molecule collisions and collisions between Feshbach molecules which are very weakly bound. Whether such resonances exist for ultracold ground state molecules has been debated due to the possibly high density of states and/or rapid decay of the resonant complex. Here we report a very pronounced and narrow (25 mG) Feshbach resonance in collisions between two ground state NaLi molecules. This molecular Feshbach resonance has two special characteristics. First, the collisional loss rate is enhanced by more than two orders of magnitude above the background loss rate which is saturated at the $p$-wave universal value, due to strong chemical reactivity. Second, the resonance is located at a magnetic field where two open channels become nearly degenerate. This implies the intermediate complex predominantly decays to the second open channel. We describe the resonant loss feature using a model with coupled modes which is analogous to a Fabry-Pérot cavity. Our observations prove the existence of long-lived coherent intermediate complexes even in systems without reaction barriers and open up the possibility of coherent control of chemical reactions.

cond-mat.quant-gas↗

arXiv2022

Perspectives and Opportunities: A Molecular Toolkit for Fundamental Physics and Matter Wave Interferometry in Microgravity

The study of molecular physics using ultracold gases has provided a unique probe into the fundamental properties of nature and offers new tools for quantum technologies. In this article we outline how the use of a space environment to study ultracold molecular physics opens opportunities for 1) exploring ultra-low energy regimes of molecular physics with high efficiency, 2) providing a toolbox of capabilities for fundamental physics, and 3) enabling new classes of matter-wave interferometers with applications in precision measurement for fundamental and many-body physics.

quant-ph↗

arXiv2022

Fast optical transport of ultracold molecules over long distances

Optically trapped laser-cooled polar molecules hold promise for new science and technology in quantum information and quantum simulation. Large numerical aperture optical access and long trap lifetimes are needed for many studies, but these requirements are challenging to achieve in a magneto-optical trap (MOT) vacuum chamber that is connected to a cryogenic buffer gas beam source, as is the case for all molecule laser cooling experiments so far. Long distance transport of molecules greatly eases fulfilling these requirements as molecules are placed into a region separate from the MOT chamber. We realize a fast transport method for ultracold molecules based on an electronically focus-tunable lens combined with an optical lattice. The high transport speed is achieved by the 1D red-detuned optical lattice, which is generated by interference of a focus-tunable laser beam and a focus-fixed laser beam. Efficiency of 48(8)% is realized in the transport of ultracold calcium monofluoride (CaF) molecules over 46 cm distance in 50 ms, with a moderate heating from 32(2) μK to 53(4) μK. Positional stability of the molecular cloud allows for stable loading of an optical tweezer array with single molecules.

physics.atom-ph↗

arXiv2022

Observation of bosonic stimulation in light scattering

For bosons, the transition rate into an already occupied quantum state is enhanced by its occupation number: the effect of bosonic stimulation. Bosonic enhancement of light scattering has been predicted more than 30 years ago but has not been observed before. Here we theoretically investigate and experimentally demonstrate this effect. We show that the bosonic enhancement factor for a harmonically trapped gas is bounded by a universal constant $ζ(2)/ζ(3)$ above the phase transition to a Bose-Einstein condensate (BEC), and depends linearly on the BEC fraction just below the phase transition. Bosonically enhanced light scattering is observed and characterized above and below the phase transition, and the effect of interactions is discussed. For a multi-level system, bosonic enhancement is reduced because bosonic stimulation occurs only for Rayleigh scattering, but not for Raman scattering.

quant-ph↗

arXiv2022

Control of reactive collisions by quantum interference

In this study, we achieved magnetic control of reactive scattering in an ultracold mixture of $^{23}$Na atoms and $^{23}$Na$^{6}$Li molecules. In most molecular collisions, particles react or are lost near short range with unity probability, leading to the so-called universal rate. By contrast, the Na{+}NaLi system was shown to have only $\sim4\%$ loss probability in a fully spin-polarized state. By controlling the phase of the scattering wave function via a Feshbach resonance, we modified the loss rate by more than a factor of $100$, from far below to far above the universal limit. The results are explained in analogy with an optical Fabry-Perot resonator by interference of reflections at short and long range. Our work demonstrates quantum control of chemistry by magnetic fields with the full dynamic range predicted by our models.

physics.atom-ph↗

arXiv2021

Catching Bethe phantoms and quantum many-body scars: Long-lived spin-helix states in Heisenberg magnets

Exact solutions for quantum many-body systems are rare and provide valuable insight to universal phenomena. Here we show experimentally in anisotropic Heisenberg chains that special helical spin patterns can have very long lifetimes. This finding confirms the recent prediction of phantom Bethe states, exact many-body eigenstates carrying finite momenta yet no energy. We theoretically find analogous stable spin helices in higher dimensions and in other non-integrable systems, where they imply non-thermalizing dynamics associated with quantum many-body scars. We use phantom spin helices to directly measure the interaction anisotropy which has a major contribution from short-range off-site interactions that have not been observed before. Phantom helix states open new opportunities for quantum simulations of spin physics and studies of many-body dynamics.

cond-mat.quant-gas↗

arXiv2021

Preparation of the spin-Mott state: a spinful Mott insulator of repulsively bound pairs

We observe and study a special ground state of bosons with two spin states in an optical lattice: the spin-Mott insulator, a state that consists of repulsively bound pairs which is insulating for both spin and charge transport. Because of the pairing gap created by the interaction anisotropy, it can be prepared with low entropy and can serve as a starting point for adiabatic state preparation. We find that the stability of the spin-Mott state depends on the pairing energy, and observe two qualitatively different decay regimes, one of which exhibits protection by the gap.

cond-mat.quant-gas↗

arXiv2021

Rotational Coherence Times of Polar Molecules in Optical Tweezers

Qubit coherence times are critical to the performance of any robust quantum computing platform. For quantum information processing using arrays of polar molecules, a key performance parameter is the molecular rotational coherence time. We report a 93(7) ms coherence time for rotational state qubits of laser cooled CaF molecules in optical tweezer traps, over an order of magnitude longer than previous systems. Inhomogeneous broadening due to the differential polarizability between the qubit states is suppressed by tuning the tweezer polarization and applied magnetic field to a "magic" angle. The coherence time is limited by the residual differential polarizability, implying improvement with further cooling. A single spin-echo pulse is able to extend the coherence time to nearly half a second. The measured coherence times demonstrate the potential of polar molecules as high fidelity qubits.

physics.atom-ph↗

arXiv2021

Transverse spin dynamics in the anisotropic Heisenberg model realized with ultracold atoms

In Heisenberg models with exchange anisotropy, transverse spin components are not conserved and can decay not only by transport, but also by dephasing. Here we utilize ultracold atoms to simulate the dynamics of 1D Heisenberg spin chains, and observe fast, local spin decay controlled by the anisotropy. Additionally, we directly observe an effective magnetic field created by superexchange which causes an inhomogeneous decay mechanism due to variations of lattice depth between chains, as well as dephasing within each chain due to the twofold reduction of the effective magnetic field at the edges of the chains and due to fluctuations of the effective magnetic field in the presence of mobile holes. The latter is a new coupling mechanism between holes and magnons. All these dephasing mechanisms, corroborated by extensive numerical simulations, have not been observed before with ultracold atoms and illustrate basic properties of the underlying Hubbard model.

cond-mat.quant-gas↗

arXiv2021

Pauli blocking of light scattering in degenerate fermions

Pauli blocking of spontaneous emission is responsible for the stability of atoms. Higher electronic orbitals cannot decay to lower-lying states if they are already occupied -- this is Pauli blocking due to occupation of internal states. Pauli blocking also occurs when free atoms scatter light elastically (Rayleigh scattering) and the final external momentum states are already occupied. A suppression of the total rate of light scattering requires a quantum-degenerate Fermi gas with a Fermi energy larger than the photon recoil energy. This has been predicted more than 30 years ago, but never realized. Here we report the creation of a dense Fermi gas of ultracold lithium atoms and show that at low temperatures light scattering is suppressed. We also explore the suppression of inelastic light scattering when two colliding atoms emit light shifted in frequency.

quant-ph↗

arXiv2021

Observation of Microwave Shielding of Ultracold Molecules

Harnessing the potential wide-ranging quantum science applications of molecules will require control of their interactions. Here, we use microwave radiation to directly engineer and tune the interaction potentials between ultracold calcium monofluoride (CaF) molecules. By merging two optical tweezers, each containing a single molecule, we probe collisions in three dimensions. The correct combination of microwave frequency and power creates an effective repulsive shield, which suppresses the inelastic loss rate by a factor of six, in agreement with theoretical calculations. The demonstrated microwave shielding shows a general route to the creation of long-lived, dense samples of ultracold molecules and evaporative cooling.

physics.atom-ph↗

arXiv2021

Tunable Single-Ion Anisotropy in Spin-1 Models Realized with Ultracold Atoms

Mott insulator plateaus in optical lattices are a versatile platform to study spin physics. Using sites occupied by two bosons with an internal degree of freedom, we realize a uniaxial single-ion anisotropy term proportional to $(S^z)^2$, which plays an important role in stabilizing magnetism for low-dimensional magnetic materials. Here we explore non-equilibrium spin dynamics and observe a resonant effect in the spin anisotropy as a function of lattice depth when exchange coupling and on-site anisotropy are similar. Our results are supported by many-body numerical simulations and are captured by the analytical solution of a two-site model.

cond-mat.quant-gas↗

arXiv2020

Spin-polarized fermions with $p$-wave interactions

We study quantum degenerate Fermi gases of ${^6}$Li atoms at high densities ($10^{15}$ cm$^{-3}$) and observe elastic and inelastic $p$-wave collisions far away from any Feshbach resonance. $P$-wave evaporation reaches temperatures of $T/T_F=0.42$ partially limited by the slow transfer of energy from high to low velocities through $p$-wave collisions. Via cross-dimensional thermalization, the $p$-wave background scattering volume is determined to be $\lvert V_p \rvert =(39^{+1.3}_{-1.6}a_0)^3$. $P$-wave dipolar relaxation creates a metastable mixture of the lowest and highest hyperfine states.

cond-mat.quant-gas↗

arXiv2020

Adiabatic preparation of entangled, magnetically ordered states with cold bosons in optical lattices

We analyze a scheme for preparation of magnetically ordered states of two-component bosonic atoms in optical lattices. We compute the dynamics during adiabatic and optimized time-dependent ramps to produce ground states of effective spin Hamiltonians, and determine the robustness to decoherence for realistic experimental system sizes and timescales. Ramping parameters near a phase transition point in both effective spin-1/2 and spin-1 models produces entangled spin-symmetric states that have potential future applications in quantum enhanced measurement. The preparation of these states and their robustness to decoherence is quantified by computing the Quantum Fisher Information of final states. We identify that the generation of useful entanglement should in general be more robust to heating than it would be implied by the state fidelity, with corresponding implications for practical applications.

cond-mat.quant-gas↗