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Wolfgang Ketterle

Publications and source records attributed to Wolfgang Ketterle.

At least 55 records · Page 3Linked to original sources

Dynamics of rotated spin states and magnetic ordering with two-component bosonic atoms in optical lattices

The microscopic control available over cold atoms in optical lattices has opened new opportunities to study the properties of quantum spin models. While a lot of attention is focussed on experimentally realizing ground or thermal states via adiabatic loading, it would often be more straightforward to prepare specific simple product states and to probe the properties of interacting spins by observing their dynamics. We explore this possibility for spin-1/2 and spin-1 models that can be realized with bosons in optical lattices, and which exhibit \textit{XY}-ferromagnetic (or counterflow spin superfluid) phases. We consider the dynamics of initial spin-rotated states corresponding to a mean-field version of the phases of interest. Using matrix product state methods in one dimension, we compute both non-equilibrium dynamics and ground/thermal states for these systems. We compare and contrast their behaviour in terms of correlation functions and induced spin currents, which should be directly observable with current experimental techniques. We find that although spin correlations decay substantially at large distances and on long timescales, for induction of spin currents, the rotated states behave similarly to the ground states on experimentally observable timescales.

cond-mat.quant-gas↗

Spin transport in a tunable Heisenberg model realized with ultracold atoms

Simple models of interacting spins play an important role in physics. They capture the properties of many magnetic materials, but also extend to other systems, such as bosons and fermions in a lattice, systems with gauge fields, high-Tc superconductors, and systems with exotic particles such as anyons and Majorana fermions. In order to study and compare these models, a versatile platform is needed. Realizing such a system has been a long-standing goal in the field of ultracold atoms. So far, spin transport has only been studied in the isotropic Heisenberg model. Here we implement the Heisenberg XXZ model with adjustable anisotropy and use this system to study spin transport far from equilibrium after quantum quenches from imprinted spin helix patterns. In the non-interacting XX model, we find ballistic behavior of spin dynamics, while in the isotropic XXX model, we find diffusive behavior. For positive anisotropies, the dynamics ranges from anomalous super-diffusion to sub-diffusion depending on anisotropy, whereas for negative anisotropies, we observe a crossover in the time domain from ballistic to diffusive transport. This behavior contrasts with expectations for the linear response regime and raises new questions in understanding quantum many-body dynamics far away from equilibrium.

cond-mat.quant-gas↗

Enhanced Superexchange in a Tilted Mott Insulator

In an optical lattice entropy and mass transport by first-order tunneling is much faster than spin transport via superexchange. Here we show that adding a constant force (tilt) suppresses first-order tunneling, but not spin transport, realizing new features for spin Hamiltonians. Suppression of the superfluid transition can stabilize larger systems with faster spin dynamics. For the first time in a many-body spin system, we vary superexchange rates by over a factor of 100 and tune spin-spin interactions via the tilt. In a tilted lattice, defects are immobile and pure spin dynamics can be studied.

cond-mat.quant-gas↗

Observation of Collisions between Two Ultracold Ground-State CaF Molecules

We measure inelastic collisions between ultracold CaF molecules by combining two optical tweezers, each containing a single molecule. We observe collisions between $^2Σ$ CaF molecules in the absolute ground state $|X,v=0, N=0,F=0\rangle$, and in excited hyperfine and rotational states. In the absolute ground state, we find a two-body loss rate of $7(4) \times 10^{-11} \text{cm}^{3}/\text{s}$, which is below, but close to the predicted universal loss rate.

physics.atom-ph↗

High-precision analysis of Feshbach resonances in a Mott insulator

We show that recent high-precision measurements of relative on-site interaction energies $ΔU$ in a Mott insulator require a theoretical description beyond the standard Hubbard-model interpretation, when combined with an accurate coupled-channels calculation. In contrast to more sophisticated lattice models, which can be elaborate especially for parameter optimization searches, we introduce an easy to use effective description of $U$ valid over a wide range of interaction strengths modeling atomic pairs confined to single lattice sites. This concise model allows for a straightforward combination with a coupled-channels analysis. With this model we perform such a coupled-channels analysis of high-precision $^7$Li spectroscopic data on the on-site interaction energy $U$, which spans over four Feshbach resonances and provide an accurate and consistent determination of the associated resonance positions. Earlier experiments on three of the Feshbach resonances are consistent with this new analysis. Moreover, we verify our model with a more rigorous numerical treatment of the two atom system in an optical lattice.

cond-mat.quant-gas↗

Enhancing the capture velocity of a Dy magneto-optical trap with two-stage slowing

Magneto-optical traps (MOTs) based on the $626\;{\rm nm}$, $136\;{\rm kHz}$-wide intercombination line of Dy, which has an attractively low Doppler temperature of $3.3\;μ{\rm K}$, have been implemented in a growing number of experiments over the last several years. A challenge in loading these MOTs comes from their low capture velocities. Slowed atomic beams can spread out significantly during free-flight from the Zeeman slower to the MOT position, reducing the fraction of the beam captured by the MOT. Here we apply, for the first time in a Dy experiment, a scheme for enhancing the loading rate of the MOT wherein atoms are Zeeman-slowed to a final velocity larger than the MOT's capture velocity, and then undergo a final stage of slowing by a pair of near-detuned beams addressing the $421\;{\rm nm}$ transition directly in front of the MOT. By reducing the free-flight time of the Zeeman-slowed atomic beam, we greatly enhance the slowed flux delivered to the MOT, leading to more than an order of magnitude enhancement in the final MOT population.

cond-mat.quant-gas↗

Floquet Heating in Interacting Atomic Gases with an Oscillating Force

We theoretically investigate the collisional heating of a cold atom system subjected to time-periodic forces. We show within the Floquet framework that this heating rate due to two-body collisions has a general semiclassical expression $\mathcal{P}\propto ρσv_{\rm col} E_0$, depending on the kinetic energy $E_0$ associated with the shaking, particle number density $ρ$, elastic collision cross section $σ$, and an effective collisional velocity $v_{\rm col}$ determined by the dominant energy scale in the system. We further show that the collisional heating is suppressed by Pauli blocking in cold fermionic systems, and by the modified density of states in systems in lower dimensions. Our results provide an exactly solvable example and reveal some general features of Floquet heating in interacting systems.

physics.atom-ph↗

An Optical Tweezer Array of Ultracold Molecules

Arrays of single ultracold molecules promise to be a powerful platform for many applications ranging from quantum simulation to precision measurement. Here we report on the creation of an optical tweezer array of single ultracold CaF molecules. By utilizing light-induced collisions during the laser cooling process, we trap single molecules. The high densities attained inside the tweezer traps have also enabled us to observe in the absence of light molecule-molecule collisions of laser cooled molecules for the first time.

physics.atom-ph↗

Observation of two-beam collective scattering phenomena in a Bose-Einstein condensate

New phenomena of collective light scattering are observed when an elongated Bose-Einstein condensate is pumped by two non-interfering beams counterpropagating along its long axis. In the limit of small Rayleigh scattering rates, the presence of a second pump beam suppresses superradiance, whereas at large Rayleigh scattering rates it lowers the effective threshold power for collective light scattering. In the latter regime, the quench dynamics of the two-beam system are oscillatory, compared to monotonic in the single-beam case. In addition, the dependence on power, detuning, and atom number is explored. The observed features of the two-beam system qualitatively agree with the recent prediction of a supersolid crystalline phase of light and matter at large Rayleigh scattering rates [S. Ostermann, F. Piazza, and H. Ritsch, Phys. Rev. X 6, 021026 (2016).]

cond-mat.quant-gas↗

Interaction Spectroscopy of a Two-component Mott Insulator

We prepare and study a two-component Mott insulator of bosonic atoms with two particles per site. The mapping of this system to a magnetic spin model, and the subsequent study of its quantum phases, require a detailed knowledge of the interaction strengths of the two components. In this work, we use radio frequency (RF) transitions and an on-site interaction blockade for precise, empirical determination of the interaction strengths of different combinations of hyperfine states on a single lattice site. We create a map of the interactions of the lowest two hyperfine states of $^7$Li as a function of magnetic field, including measurements of several Feshbach resonances with unprecedented sensitivity, and we identify promising regions for the realization of magnetic spin models.

cond-mat.quant-gas↗

How to dress radio-frequency photons with tunable momentum

We demonstrate how the combination of oscillating magnetic forces and radio-frequency (RF) pulses endows RF photons with tunable momentum. We observe velocity-selective spinflip transitions and the associated Doppler shift. This realizes the key component of purely magnetic spin-orbit coupling schemes for ultracold atoms, which does not involve optical transitions and therefore avoids the problem of heating due to spontaneous emission.

physics.atom-ph↗

$Λ$-Enhanced Imaging of Molecules in an Optical Trap

We report non-destructive imaging of optically trapped calcium monofluoride (CaF) molecules using in-situ $Λ$-enhanced gray molasses cooling. $200$ times more fluorescence is obtained compared to destructive on-resonance imaging, and the trapped molecules remain at a temperature of $20\,μ\text{K}$. The achieved number of scattered photons makes possible non-destructive single-shot detection of single molecules with high fidelity.

physics.atom-ph↗

Laser Cooling of Optically Trapped Molecules

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an ODT. Enhanced loading by a factor of five is obtained when sub-Doppler cooling light and trapping light are on simultaneously. For trapped molecules, we directly observe efficient sub-Doppler cooling to a temperature of $60(5)$ $μ\text{K}$. The trapped molecular density of $8(2)\times10^7$ cm$^{-3}$ is an order of magnitude greater than in the initial sub-Doppler cooled sample. The trap lifetime of 750(40) ms is dominated by background gas collisions.

physics.atom-ph↗

Photoassociation of Ultracold NaLi

We perform photoassociation spectroscopy in an ultracold $^{23}$Na-$^6$Li mixture to study the $c^3Σ^+$ excited triplet molecular potential. We observe 50 vibrational states and their substructure to an accuracy of 20 MHz, and provide line strength data from photoassociation loss measurements. An analysis of the vibrational line positions using near-dissociation expansions and a full potential fit is presented. This is the first observation of the $c^3Σ^+$ potential, as well as photoassociation in the NaLi system.

physics.atom-ph↗

Two-Photon Spectroscopy of the NaLi Triplet Ground State

We employ two-photon spectroscopy to study the vibrational states of the triplet ground state potential ($a^3Σ^+$) of the $^{23}$Na$^{6}$Li molecule. Pairs of Na and Li atoms in an ultracold mixture are photoassociated into an excited triplet molecular state, which in turn is coupled to vibrational states of the triplet ground potential. Vibrational state binding energies, line strengths, and potential fitting parameters for the triplet ground $a^3Σ^+$ potential are reported. We also observe rotational splitting in the lowest vibrational state.

physics.atom-ph↗

Long-Lived Ultracold Molecules with Electric and Magnetic Dipole Moments

We create fermionic dipolar $^{23}$Na$^6$Li molecules in their triplet ground state from an ultracold mixture of $^{23}$Na and $^6$Li. Using magneto-association across a narrow Feshbach resonance followed by a two-photon STIRAP transfer to the triplet ground state, we produce $3\,{\times}\,10^4$ ground state molecules in a spin-polarized state. We observe a lifetime of $4.6\,\text{s}$ in an isolated molecular sample, approaching the $p$-wave universal rate limit. Electron spin resonance spectroscopy of the triplet state was used to determine the hyperfine structure of this previously unobserved molecular state.

cond-mat.quant-gas↗

Radio Frequency Magneto-Optical Trapping of CaF with High Density

We demonstrate significantly improved magneto-optical trapping of molecules using a very slow cryogenic beam source and RF modulated and DC magnetic fields. The RF MOT confines $1.1(3) \times 10^5$ CaF molecules at a density of $4(1) \times 10^6$ cm$^{-3}$, which is an order of magnitude greater than previous molecular MOTs. Near Doppler-limited temperatures of $340(20)$ $μ$K are attained. The achieved density enables future work to directly load optical tweezers and create optical arrays for quantum simulation.

physics.atom-ph↗

Observation of the supersolid stripe phase in spin-orbit coupled Bose-Einstein condensates

Supersolidity is an intriguing concept. It combines the property of superfluid flow with the long-range spatial periodicity of solids, two properties which are often mutually exclusive. The original discussion of quantum crystals and supersolidity focuses on solid Helium-4 where it was predicted that vacancies could form dilute weakly interacting Bose-Einstein condensates. In this system, direct observation of supersolidity has been elusive. The concept of supersolidity was then generalized to include other superfluid systems which break the translational symmetry of space. One of such systems is a Bose-Einstein condensate with spin-orbit coupling which has a supersolid stripe phase. Despite several recent studies of this system, the stripe phase has not been observed. Here we report the direct observation of the predicted density modulation of the stripe phase using Bragg reflection. Our work establishes a system with unique symmetry breaking properties. Of future interest is further spatial symmetry breaking through the introduction of vortices, solitons, impurities or disorder.

cond-mat.quant-gas↗