arXiv subjects

X. C. Wang

Publications and source records attributed to X. C. Wang.

At least 19 recordsLinked to original sources

arXiv2026

Laser-intensity-spike-dominated hot electron generation from two-plasmon decay instability driven by moderate-bandwidth pulses

Our direct-drive-relevant experiments on the low-coherence Kunwu laser facility identify two-plasmon decay (TPD) as the primary source of hot electrons, and demonstrate for the first time that broadband laser pulses enhance TPD. Using particle-in-cell simulations, we attribute this TPD enhancement and the consequent hot electron production to stochastic intensity spikes inherent in broadband laser fields, robust in both weakly- and strongly-driven regimes. These findings suggest that mitigating hot electron generation requires suppressing these intensity spikes.

physics.plasm-ph↗

arXiv2024

Superconductivity Discovered in Niobium Polyhydride at High Pressures

Niobium polyhydride was synthesized at high pressure and high temperature conditions by using diamond anvil cell combined with in situ high pressure laser heating techniques. High pressure electric transport experiments demonstrate that superconducting transition occurs with critical temperature(Tc) 42 K at 187 GPa. The shift of Tc as function of external applied magnetic field is in consistent to the nature of superconductivity while the upper critical field at zero temperature Hc2(0) is estimated to~16.8 Tesla while the GL coherent length ~57 angstrom is estimated. The structure investigation using synchrotron radiation implies that the observed superconductivity may come from Fm-3m phase of NbH3.

cond-mat.supr-con↗

arXiv2024

Superconductivity with Tc 116K discovered in antimony polyhydrides

Superconductivity (SC) was experimentally observed for the first time in antimony polyhydride. The diamond anvil cell combined with laser heating system was used to synthesize the antimony polyhydride sample at high pressure and high temperature conditions. In-situ high pressure transport measurements as function of temperature with applied magnet are performed to study the SC properties. It was found that the antimony polyhydride samples show superconducting transition with critical temperature Tc 116 K at 184 GPa. The investigation of SC at magnetic field revealed that the superconducting coherent length ~40 angstroms based on Ginzburg Landau (GL) equation. Antimony polyhydride superconductor has the second highest Tc in addition to sulfur hydride among the polyhydrides of elements from main group IIIA to VIIA in periodic table.

cond-mat.supr-con↗

arXiv2024

A bright burst from FRB 20200120E in a globular cluster of the nearby galaxy M81

Fast radio bursts (FRBs) are immensely energetic millisecond-duration radio pulses. Observations indicate that nearby FRBs can be produced by old stellar populations, as suggested by the localization of the repeating source FRB 20200120E in a globular cluster of M81. Nevertheless, the burst energies of FRB 20200120E are significantly smaller than those of other cosmological FRBs, even falling below the energy of the Galactic event FRB 20200428. Here, we report the detection of a bright burst from FRB 20200120E in 1.1 -- 1.7 GHz, with a fluence of about 30 Jy ms, which is more than 42 times larger than the previously detected bursts near 1.4 GHz frequency. It reaches one-third of the energy of the weakest burst from FRB 20121102A and is detectable at a distance exceeding 200 Mpc. Our finding bridges the gap between nearby and cosmological FRBs and indicates that FRBs hosted in globular clusters can be bright enough to be observable at cosmological distances.

astro-ph.HE↗

arXiv2023

Superconductivity Observed in Tantalum Polyhydride at High Pressure

We report experimental discovery of tantalum polyhydride superconductor. It was synthesized at high pressure and high temperature conditions using diamond anvil cell combined with in-situ high pressure laser heating techniques. The superconductivity was investigated via resistance measurements at pressures. The highest superconducting transition temperature Tc was found to be ~30 K at 197 GPa in the sample that was synthesized at the same pressure with ~2000 K heating. The transitions are shifted to low temperature upon applying magnetic fields that supports the superconductivity nature. The upper critical field at zero temperature μ0Hc2(0) of the superconducting phase is estimated to be ~20 T that corresponds to GL coherent length ~40 angstroms. Our results suggest that the superconductivity may arise from I-43d phase of TaH3. It is, for the first time to our best knowledge, experimental realization of superconducting hydrides for the VB group of transitional metals.

cond-mat.supr-con↗

arXiv2022

Record High Tc Element Superconductivity Achieved In Titanium

It is challenging to search for high Tc superconductivity (SC) in transition metal elements wherein d electrons are usually not favored by conventional BCS theory. Here we report discovery of surprising SC up to 310 GPa with Tc above 20 K in wide pressure range from 108 GPa to 240 GPa in titanium. The maximum Tc^onset above 26 K and zero resistance Tc^zero of 21 K are record high values hitherto achieved among element superconductors. The Hc2(0) is estimated to be about 32 Tesla with coherence length 32 angstrom. The results show strong s-d transfer and d-band dominance, indicating correlation driven contributions to high Tc SC in dense titanium. This finding is in sharp contrast to the theoretical predications based on pristine electron-phonon coupling scenario. The study opens a fresh promising avenue for rational design and discovery of high Tc superconductors among simple materials via pressure tuned unconventional mechanism.

cond-mat.supr-con↗

arXiv2022

Superconductivity above 80 K in polyhydrides of hafnium

Studies on polyhydrides are attracting growing attentions recently due to their potential high temperature superconductivity (SC). We here report the discovery of SC in hafnium polyhydrides at high pressures. The hafnium superhydrides are synthesized at high pressure and high temperature conditions using diamond anvil cell in combination with in-situ high pressure laser heating technique. The SC was investigated by in-situ high pressure resistance measurements in applied magnetic fields. A superconducting transition with onset Tc ~83 K was observed at 243 GPa. The upper critical field Hc2(0) was estimated to be 24 Tesla by GL theory and the consequent superconducting coherent length to be ~37 angstrom. Our results suggest that the superconducting phase is from C2/m-HfH14. This is the first 5d transition metal polyhydride superconductor with Tc above the liquid nitrogen temperature.

cond-mat.supr-con↗

arXiv2022

Superconductivity above 200 K Observed in Superhydrides of Calcium

Searching for superconductivity with Tc near room temperature is of great interest both for fundamental science & many potential applications. Here we report the experimental discovery of superconductivity with maximum critical temperature (Tc) above 210 K in calcium superhydrides, the new alkali earth hydrides experimentally showing superconductivity above 200 K in addition to sulfur hydride & rare-earth hydride system. The materials are synthesized at the synergetic conditions of 160~190 GPa and ~2000 K using diamond anvil cell combined with in-situ laser heating technique. The superconductivity was studied through in-situ high pressure electric conductance measurements in an applied magnetic field for the sample quenched from high temperature while maintained at high pressures. The upper critical field Hc(0) was estimated to be ~268 T while the GL coherent length is ~11 angstrom. The in-situ synchrotron X-ray diffraction measurements suggest that the synthesized calcium hydrides are primarily composed of CaH6 while there may also exist other calcium hydrides with different hydrogen contents.

cond-mat.supr-con↗

arXiv2022

Superconductivity in Zirconium Polyhydrides with Tc above 70 K

We report the experimental discovery of superconductivity with critical temperature Tc above 70 K in zirconium polyhydrides, the record high so far for 3d transition metal hydrides. The superconducting zirconium polyhydrides are synthesized at the extreme conditions above 200 GPa & 2000 K by using diamond anvil cell combined with in-situ laser heating. Superconductivity was observed in the samples maintained at the same pressure upon quenched from heating.

cond-mat.supr-con↗

arXiv2021

Nodal superconducting gap in LiFeP revealed by NMR: contrast with LiFeAs

Identifying the uniqueness of FeP-based superconductors may shed new lights on the mechanism of superconductivity in iron-pnictides. Here, we report nuclear magnetic resonance(NMR) studies on LiFeP and LiFeAs which have the same crystal structure but different pnictogen atoms. The NMR spectrum is sensitive to inhomogeneous magnetic fields in the vortex state and can provide the information on the superconducting pairing symmetry through the temperature dependence of London penetration depth $λ_L$. We find that $λ_L$ saturates below $T \sim 0.2$ $T_c$ in LiFeAs, where $T_c$ is the superconducting transition temperature, indicating nodeless superconducting gaps. Furthermore, by using a two-gaps model, we simulate the temperature dependence of $λ_L$ and obtain the superconducting gaps of LiFeAs, as $Δ_1 = 1.2$ $k_B T_c$ and $Δ_2 = 2.8$ $k_B T_c$, in agreement with previous result from spin-lattice relaxation. For LiFeP, in contrast, the London penetration depth $λ_L$ does not show any saturation down to $T \sim 0.03 $ $T_c$, indicating nodes in the superconducting energy gap function. Finally, we demonstrate that the strong spin fluctuations with diffusive characteristics exist in LiFeP, as in some cuprate high temperature superconductors.

cond-mat.supr-con↗

arXiv2020

The Hund's Superconductor Li(Fe,Co)As

We combine transport, angle-resolved photoemission spectroscopy and scanning tunneling spectroscopy to investigate several low energy manifestations of the Hund coupling in a canonical FeSC family Li(Fe,Co)As. We determine the doping dependence of the coherent-incoherent crossover temperature and the quasi-particle effective mass enhancement in the normal state. Our tunneling spectroscopy result in the superconducting state supports the idea that superconductivity emerging from Hund's metal state displays a universal maximal superconducting gap vs transition temperature (2$Δ_{max}/k_{B}T_{c}$) value, which is independent of doping level and $T_{c}$.

cond-mat.supr-con↗

arXiv2020

Orbital selectivity of layer resolved tunneling on iron superconductor Ba0.6K0.4Fe2As2

We use scanning tunneling microscopy/spectroscopy (STM/S) to elucidate the Cooper pairing of the iron pnictide superconductor Ba0.6K0.4Fe2As2. By a cold-cleaving technique, we obtain atomically resolved termination surfaces with different layer identities. Remarkably, we observe that the low-energy tunneling spectrum related to superconductivity has an unprecedented dependence on the layer-identity. By cross-referencing with the angle-revolved photoemission results and the tunneling data of LiFeAs, we find that tunneling on each termination surface probes superconductivity through selecting distinct Fe-3d orbitals. These findings imply the real-space orbital features of the Cooper pairing in the iron pnictide superconductors, and propose a new and general concept that, for complex multi-orbital material, tunneling on different terminating layers can feature orbital selectivity.

cond-mat.supr-con↗

arXiv2019

Superconductivity in a unique type of copper oxide

The mechanism of superconductivity in cuprates remains one of the big challenges of condensed matter physics.High Tc cuprates crystallize into layered perovskite structure featuring copper oxygen octahedral coordination. Due to the Jahn Teller effect in combination with the strong static Coulomb interaction, the octahedra in high Tc cuprates are elongated along the c axis, leading to a 3dx2-y2 orbital at the top of the band structure wherein the doped holes reside.This scenario gives rise to two dimensional characteristics in high Tc cuprates that favor d wave pairing symmetry. Here we report superconductivity in a cuprate Ba2CuO4-y wherein the local octahedron is in a very exceptional compressed version.The Ba2CuO4-y compound was synthesized at high pressure at high temperatures, and shows bulk superconductivity with critical temperature Tc above 70 K at ambient conditions. This superconducting transition temperature is more than 30 K higher than the Tc for the isostructural counterparts based on classical La2CuO4. X-ray absorption measurements indicate the heavily doped nature of the Ba2CuO4-y superconductor. In compressed octahedron the 3d3z2-r2 orbital will be lifted above the 3dx2-y2 orbital, leading to significant three dimensional nature in addition to the conventional 3dx2-y2 orbital. This work sheds important new light on advancing our comprehensive understanding of the superconducting mechanism of high Tc in cuprate materials.

cond-mat.supr-con↗

arXiv2018

Electron Mass Enhancement near a Nematic Quantum Critical Point in NaFe$_{1-x}$Co$_{x}$As

A magnetic order can be completely suppressed at zero temperature($T$), by doping carriers or applying pressure, at a quantum critical point(QCP), around which physical properties change drastically. However, the situation is unclear for an electronic nematic order that breaks rotation symmetry. Here we report nuclear magnetic resonance(NMR) studies on NaFe$_{1-x}$Co$_{x}$As where magnetic and nematic transitions are well separated. The NMR spectrum is sensitive to inhomogeneous magnetic fields in the vortex state, which is related to London penetration depth $λ_{\rm L}$ that measures the electron mass $m^*$. We discovered two peaks in the doping dependence of $λ_{\rm L}^2$($T\sim$0); one at $x_{\rm M}$=0.027 where the spin-lattice relaxation rate shows quantum critical behavior, and another at $x_{\rm c}$=0.032 around which the nematic transition temperature extrapolates to zero and the electrical resistivity shows a $T$-linear variation. Our results indicate that a nematic QCP lies beneath the superconducting dome at $x_{\rm c}$ where $m^*$ is enhanced. The impact of the nematic fluctuations on superconductivity is discussed.

cond-mat.supr-con↗

arXiv2018

Single Crystal Growth and Spin Polarization Measurements of Diluted Magnetic Semiconductor (BaK)(ZnMn)2As2

Recently a new type diluted magnetic semiconductor (BaK)(ZnMn)2As2 (BZA) with high Cure temperature (Tc) was discovered showing independent spin and charge doping mechanism. This makes BZA a promising material for spintronics devices. Here we report for the first time the successful growth of BZA single crystal. An Andreev reflection junction that can be used to evaluate spin polarization was fabricated based on the BZA single crystal, a 66% spin polarization of the BZA single crystal was hence obtained by Andreev reflection spectroscopy analysis.

cond-mat.mtrl-sci↗

arXiv2018

Decoupled Pairing Amplitude and Electronic Coherence in Iron-Based Superconductors

Here we use angle-resolved photoemission spectroscopy to study superconductivity that emerges in two extreme cases, from a Fermi liquid phase (LiFeAs) and an incoherent bad-metal phase (FeTe0.55Se0.45). We find that although the electronic coherence can strongly reshape the single-particle spectral function in the superconducting state, it is decoupled from the maximum superconducting pairing amplitude, which shows a universal scaling that is valid for all FeSCs. Our observation excludes pairing scenarios in the BCS and the BEC limit for FeSCs and calls for a universal strong coupling pairing mechanism for the FeSCs.

cond-mat.supr-con↗

arXiv2016

Observation of non-Fermi liquid behavior in hole-doped LiFe$_{1-x}$V$_x$As

We synthesized a series of V-doped LiFe$_{1-x}$V$_x$As single crystals. The superconducting transition temperature $T_c$ of LiFeAs decreases rapidly at a rate of 7 K per 1\% V. The Hall coefficient of LiFeAs switches from negative to positive with 4.2\% V doping, showing that V doping introduces hole carriers. This observation is further confirmed by the evaluation of the Fermi surface volume measured by angle-resolved photoemission spectroscopy (ARPES), from which a 0.3 hole doping per V atom introduced is deduced. Interestingly, the introduction of holes does not follow a rigid band shift. We also show that the temperature evolution of the electrical resistivity as a function of doping is consistent with a crossover from a Fermi liquid to a non-Fermi liquid. Our ARPES data indicate that the non-Fermi liquid behavior is mostly enhanced when one of the hole $d_{xz}/d_{yz}$ Fermi surfaces is well nested by the antiferromagnetic wave vector to the inner electron Fermi surface pocket with the $d_{xy}$ orbital character. The magnetic susceptibility of LiFe$_{1-x}$V$_x$As suggests the presence of strong magnetic impurities following V doping, thus providing a natural explanation to the rapid suppression of superconductivity upon V doping.

cond-mat.supr-con↗

arXiv2016

Coexistence of Clean- and Dirty-limit Superconductivity in LiFeAs

The optical properties of LiFeAs with $T_c \simeq$ 18 K have been determined in the normal and superconducting states. The superposition of two Drude components yields a good description of the low-frequency optical response in the normal state. Below $T_c$, the optical conductivity reveals two isotropic superconducting gaps with $Δ_{1} \simeq 2.9$ $\pm$ 0.2 meV and $Δ_{2} \simeq 5.5$ $\pm$ 0.4 meV. A comparison between the superconducting-state Mattis-Bardeen and the normal-state Drude components, in combination with a spectral weight analysis, indicates that the spectral weight associated with a band which has a very small scattering rate is fully transferred to the superfluid weight upon the superconducting condensate. These observations provide clear evidence for the coexistence of clean- and dirty-limit superconductivity in LiFeAs.

cond-mat.supr-con↗