arXiv subjects

X. G. Luo

Publications and source records attributed to X. G. Luo.

At least 73 records · Page 4Linked to original sources

arXiv2011

Pressure effect on superconductivity of $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs)

We performed the high hydrostatic pressure resistivity measurements (up to 1.7 GPa) on the newly discovered superconductors $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs) single crystals. Two batches of single crystals $K_xFe_2Se_2$ with different transition temperatures ($T_c$) were used to study the effect of pressure. The $T_c$ of the first one gradually decreases with increasing pressure from 32.6 K at ambient pressure. While a dome-like behavior was observed for the crystal with $T_c=31.1$ K, and $T_c$ reaches its maximum value of 32.7 K at the pressure of 0.48 GPa. It indicates that there exists a optimal doping with maximum $T_c$ of 32.7K in $K_xFe_2Se_2$ system. The behavior of $T_c$ vs. pressure for $Cs_xFe_2Se_2$ also shows a dome-like behavior, and $T_c$ reaches its maximum value of 31.1 K at the pressure of 0.82 GPa. The hump observed in temperature dependence of resistivity for all the samples tends to shift to high temperature with increasing pressure. The resistivity hump could arise from the vacancy of Fe or Se.

cond-mat.supr-con↗

arXiv2010

Superconductivity and Magnetic Properties of high-quality single crystals of $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs)

We successfully grew the high-quality single crystals of $A_{x}$Fe$_2$Se$_2$ ($A$ = K and Cs) by self-flux method. Sharp superconducting transition was observed for both types of crystals. The crystals show the onset superconducting transition temperatures ($T_{\rm c}$) of 31 K and 30 K for K- and Cs-compounds, respectively, with nearly 100% shielding fraction. The crystals show quite high resistivity in the normal state of more than 160 m$Ω$ cm and 1300 m$Ω$ cm maximum resistivity for $K_{0.86}Fe_2Se_{1.82}$ and $Cs_{0.86}Fe_{1.66}Se_{2}$ single crystals, respectively. Much larger upper critical field $H_{\rm c2}$ is inferred from low-temperature iso-magnetic-field magnetoresistance in these crystals than in FeSe. The anisotropy $H^{ab}_{\rm c2}$(0)/$H^{c}_{\rm c2}$(0) is around 3 for both of the two materials. Anisotropic peculiar magnetic behavior in normal state has been found for $Cs_{0.86}Fe_{1.66}Se_{2}$

cond-mat.supr-con↗

arXiv2010

Superconductivity at 32 K in single crystal Rb$_{0.78}$Fe$_2$Se$_{1.78}$}

We successfully grew the high-quality single crystal of Rb$_{0.78}$Fe$_2$Se$_{1.78}$, which shows sharp superconducting transition in magnetic susceptibility and electrical resistivity. Resistivity measurements show the onset superconducting transition ($T_{\rm c}$) at 32.1 K and zero resistivity at 30 K. From the low-temperature iso-magnetic-field magnetoresistance, large upper critical field $H_{\rm c2}$(0) has been estimated as high as 180 T for in-plane field and 59 T for out-of-plane field. The anisotropy $H^{ab}_{\rm c2}$(0)/$H^{c}_{\rm c2}$(0) is around 3.0, right lying between those observed in K$_x$Fe$_2$Se$_2$ and Cs$_x$Fe$_2$Se$_2$.

cond-mat.supr-con↗

arXiv2010

Reentrant spin-glass behavior in $TlFe_{2-x}Se_2$ with the $ThCr_2Si_2$-type structure

We investigated the physical properties of $TlFe_{2-x}Se_2$ single crystals. The resistivity of $TlFe_{2-x}Se_2$ shows typical semiconductor behavior with an activation energy of 25 meV. DC susceptibility indicates an antiferromagnetic transition at about 450 K. Reentrant spin-glass (RSG) behavior was found at about 130 K through DC and AC magnetic measurements. The RSG behavior suggests the existence of a strong competition between ferromagnetic (FM) and antiferromagnetic (AFM) interactions due to Fe deficiencies. Strong electron-electron correlation may exist in this material and it is possibly a candidate of parent compound for high $T_c$ superconductors.

cond-mat.str-el↗

arXiv2010

Nodes in the gap structure of the iron-arsenide superconductor Ba(Fe_{1-x}Co_x)_2As_2 from c-axis heat transport measurements

The thermal conductivity k of the iron-arsenide superconductor Ba(Fe_{1-x}Co_x)_2As_2 was measured down to 50 mK for a heat current parallel (k_c) and perpendicular (k_a) to the tetragonal c axis, for seven Co concentrations from underdoped to overdoped regions of the phase diagram (0.038 < x < 0.127). A residual linear term k_c0/T is observed in the T = 0 limit when the current is along the c axis, revealing the presence of nodes in the gap. Because the nodes appear as x moves away from the concentration of maximal T_c, they must be accidental, not imposed by symmetry, and are therefore compatible with an s_{+/-} state, for example. The fact that the in-plane residual linear term k_a0/T is negligible at all x implies that the nodes are located in regions of the Fermi surface that contribute strongly to c-axis conduction and very little to in-plane conduction. Application of a moderate magnetic field (e.g. H_c2/4) excites quasiparticles that conduct heat along the a axis just as well as the nodal quasiparticles conduct along the c axis. This shows that the gap must be very small (but non-zero) in regions of the Fermi surface which contribute significantly to in-plane conduction. These findings can be understood in terms of a strong k dependence of the gap Delta(k) which produces nodes on a Fermi surface sheet with pronounced c-axis dispersion and deep minima on the remaining, quasi-two-dimensional sheets.

cond-mat.supr-con↗

arXiv2010

Doping dependence of heat transport in the iron-arsenide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$: from isotropic to strongly $k$-dependent gap structure

The temperature and magnetic field dependence of the in-plane thermal conductivity $κ$ of the iron-arsenide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ was measured down to $T \simeq 50$ mK and up to $H = 15$ T as a function of Co concentration $x$ in the range 0.048 $ \leq x \leq $ 0.114. In zero magnetic field, a negligible residual linear term in $κ/T$ as $T \to 0$ at all $x$ shows that there are no zero-energy quasiparticles and hence the superconducting gap has no nodes in the $ab$-plane anywhere in the phase diagram. However, the field dependence of $κ$ reveals a systematic evolution of the superconducting gap with doping $x$, from large everywhere on the Fermi surface in the underdoped regime, as evidenced by a flat $κ(H)$ at $T \to 0$, to strongly $k$-dependent in the overdoped regime, where a small magnetic field can induce a large residual linear term, indicative of a deep minimum in the gap magnitude somewhere on the Fermi surface. This shows that the superconducting gap structure has a strongly $k$-dependent amplitude around the Fermi surface only outside the antiferromagnetic/orthorhombic phase.

cond-mat.supr-con↗

arXiv2009

Quasiparticle Heat Transport in Ba$_{1-x}$K$_x$Fe$_2$As$_2$: Evidence for a k-dependent Superconducting Gap without Nodes

The thermal conductivity $κ$ of the iron-arsenide superconductor Ba$_{1-x}$K$_x$Fe$_2$As$_2$ ($T_c \simeq$ 30 K) was measured in single crystals at temperatures down to $T \simeq 50$ mK ($\simeq T_c$/600) and in magnetic fields up to $H = 15$ T ($\simeq H_{c2}$/4). A negligible residual linear term in $κ/T$ as $T \to 0$ shows that there are no zero-energy quasiparticles in the superconducting state. This rules out the existence of line and in-plane point nodes in the superconducting gap, imposing strong constraints on the symmetry of the order parameter. It excludes d-wave symmetry, drawing a clear distinction between these superconductors and the high-$T_c$ cuprates. However, the fact that a magnetic field much smaller than $H_{c2}$ can induce a residual linear term indicates that the gap must be very small on part of the Fermi surface, whether from strong anisotropy or band dependence, or both.

cond-mat.supr-con↗

arXiv2008

Novel electronic structure induced by a highly strained oxide interface with incommensurate crystal fields

The misfit oxide, Bi$_{2}$Ba$_{1.3}$K$_{0.6}$Co$_{2.1}$O$_{y}$, made of alternating rocksalt-structured [BiO/BaO] layers and hexagonal CoO$_{2}$ layers, was studied by angle-resolved photoemission spectroscopy. Detailed electronic structure of such a highly strained oxide interfaces is revealed for the first time. We found that under the two incommensurate crystal fields, electrons are confined within individual sides of the interface, and scattered by umklapp scattering of the crystal field from the other side. In addition, the high strain on the rocksalt layer raises its chemical potential and induces large charge transfer to the CoO$_{2}$ layer. Furthermore, a novel interface effects, the interfacial enhancement of electron-phonon interactions, is discovered. Our findings of these electronic properties lay a foundation for designing future functional oxide interfaces.

cond-mat.str-el↗

arXiv2007

Transport properties and magnetic field induced localization in the misfit cobaltite [Bi$_2$Ba$_{1.3}$K$_{0.6}$Co$_{0.1}$]$^{RS}$[CoO$_2$]$_{1.97}$ single crystal

Resistivity under magnetic field, thermopower and Hall coefficient are systematically studied for [Bi$_2$Ba$_{1.3}$K$_{0.6}$Co$_{0.1}$]$^{RS}$[CoO$_2$]$_{1.97}$ single crystal. In-plane resistivity ($ρ_{ab}$(T)) shows metallic behavior down to 2 K with a $T^2$ dependence below 30 K; while out-of-plane resistivity ($ρ_{c}(T)$) shows metallic behavior at high temperature and a thermal activation semiconducting behavior below about 12 K. Striking feature is that magnetic field induces a ln(1/$T$) diverging behavior in both $ρ_{ab}$ and $ρ_{c}(T)$ at low temperature. The positive magnetoresistance (MR) could be well fitted by the formula based on multi-band electronic structure. The ln(1/$T$) diverging behavior in $ρ_{ab}$ and $ρ_{c}(T)$ could arise from the magnetic-field-induced 2D weak localization or spin density wave.

cond-mat.str-el↗

arXiv2007

Intergrowth and thermoelectric properties in the Bi-Ca-Co-O system

Single crystals of the Bi-Ca-Co-O system have been grown using the flux method with cooling from 900$\celsius$ and 950$\celsius$, respectively. The single crystals are characterized by transmission electron microscopy and X-ray diffraction. The misfit cobaltite [Ca$_2$Bi$_{1.4}$Co$_{0.6}$O$_4$]$^{RS}$[CoO$_2$]$_{1.69}$ single crystals with quadruple ($n$=4) rocksalt (RS) layer are achieved with cooling from 900$\celsius$. Such crystal exhibits room-temperature thermoelectric power (TEP) of 180$μ$V/K, much larger than that in Sr-based misfit cobaltites with quadruple RS layer. However, intergrowth of single crystals of quadruple ($n$=4) and triple ($n$=3) RS-type layer-based misfit cobaltites is observed with cooling from 950$\celsius$. Both of TEP and resistivity were obviously enhanced by the intergrowth compared to [Ca$_2$Bi$_{1.4}$Co$_{0.6}$O$_4$]$^{RS}$[CoO$_2$]$_{1.69}$ single crystal, while the power factor at room temperature remains unchanged.

cond-mat.mtrl-sci↗

arXiv2007

Transport properties in Cu$_{x}$TiSe$_{2}$ (0.015$\leq$x$\leq$0.110) Single Crystal

Transport properties are systematically studied for the single crystals Cu$_{x}$TiSe$_{2}$ (0.015$\leq$x$\leq$0.110). Both of in-plane and out-of-plane resistivity show the coexistence of superconducting transition and charge density wave (CDW) for the single crystals with $x \leq 0.025$. After CDW state is completely suppressed around x=0.055, the superconductivity is apparently enhanced by Cu doping. No superconducting transition is observed above 1.8 K for Cu$_{0.11}$TiSe$_{2}$. Anisotropy in resistivity increases with increasing Cu content, and is nearly $T$-independent. CDW state has a strong effect on Hall coefficient and thermopower. A large thermopower, comparable to the triangle lattice $NaxCoO_2$, is observed in Cu$_{x}$TiSe$_{2}$. Intercalation of Cu induces a negative MR due to the interaction between conducting carries and localized magnetic moments.

cond-mat.supr-con↗

arXiv2007

Origin of superconductivity in nominally "undoped" T'-La$_{2-x}$Y$_{x}$CuO$_{4}$ films

We have systematically studied the transport properties of the La$_{2-x}$Y$_{x}$CuO$_{4}$(LYCO) films of T'-phase ($0.05\leq x \leq 0.30$). In this nominally "undoped" system, superconductivity was acquired in certain Y doping range ($0.10\leq x \leq 0.20$). Measurements of resistivity, Hall coefficients in normal states and resistive critical field ($H^ρ_{c2}$)in superconducting states of the T'-LYCO films show the similar behavior as the known Ce-doped n-type cuprate superconductors, indicating the intrinsic electron-doping nature. The charge carriers are induced by oxygen deficiency. Non-superconducting Y-doped Pr- or Nd-based T'-phase cuprate films were also investigated for comparison, suggesting the crucial role of the radii of A-site cations in the origin of superconductivity in the nominally "undoped" cuptates. Based on a reasonable scenario in the microscopic reduction process, we put forward a self-consistent interpretation of these experimental observations.

cond-mat.supr-con↗

arXiv2007

Magnetic field induced spin-flop transition in Na$_x$CoO$_2$ (0.5$<$x$<$0.55)

The isothermal magnetoresistance (MR) with magnetic field (H) parallel to and perpendicular to ab plane is systematically studied on the single crystal Na$_{0.52}$CoO$_2$ with charge ordering at $\sim 50$ K and an in-plane ferromagnetism below 25 K. The isothermal MR behavior with H $\parallel$ ab plane and H $\perp$ ab plane is quite different. When H $\parallel$ ab plane, the MR is always negative and the in-plane ferromagnetic behavior is enhanced. While the MR with H $\perp$ ab plane changes from negative to positive with decreasing temperature or increasing H, and the in-plane ferromagnetic behavior is suppressed. A striking feature is that the MR with H $\perp$ ab plane shows a hysteresis behavior below 25 K, which is absent for the case of H $\parallel$ ab plane. These results provide strong evidence for a spin-flop transition of small moments of Co$^{3.5-δ}$ sites induced by H $\perp$ ab plane, leading to a metamagnetic transition for small moments of Co$^{3.5-δ}$ sites. These complex magnetism suggests an unconventional superconductivity in Na$_x$CoO$_2$ system because the Na$_x$CoO$_2$ around x=0.5 is considered to be the parent compound of superconductivity.

cond-mat.str-el↗

arXiv2007

Novel dynamical effects and glassy response in strongly correlated electronic system

We find an unconventional nucleation of low temperature paramagnetic metal (PMM) phase with monoclinic structure from the matrix of high-temperature antiferromagnetic insulator (AFI) phase with tetragonal structure in strongly correlated electronic system $BaCo_{0.9}Ni_{0.1}S_{1.97}$. Such unconventional nucleation leads to a decease in resistivity by several orders with relaxation at a fixed temperature without external perturbation. The novel dynamical process could arise from the competition of strain fields, Coulomb interactions, magnetic correlations and disorders. Such competition may frustrate the nucleation, giving rise to a slow, nonexponential relaxation and "physical aging" behavior.

cond-mat.str-el↗

arXiv2006

Giant isotope effect and spin state transition induced by oxygen isotope exchange in ($Pr_{1-x}Sm_x)_{0.7}Ca_{0.3}CoO_3$

We systematically investigate effect of oxygen isotope in $(Pr_{1-x}Sm_x)_{0.7}Ca_{0.3}CoO_3$ which shows a crossover with x from ferromagnetic metal to the insulator with spin-state transition. A striking feature is that effect of oxygen isotope on the ferromagnetic transition is negligible in the metallic phase, while replacing $^{16}O$ with $^{18}O$ leads to a giant up-shift of the spin-state transition temperature ($T_s$) in the insulating phase, especially $T_s$ shifts from 36 to 54 K with isotope component $α_S=-4.7$ for the sample with x=0.175. A metal-insulator transition is induced by oxygen isotope exchange in the sample x=0.172 being close to the insulating phase. The contrasting behaviors observed in the two phases can be well explained by occurrence of static Jahn-Teller distortions in the insulating phase, while absence of them in the metallic phase.

cond-mat.str-el↗

arXiv2006

Magnetic and transport properties in Gd$_{1-x}$Sr$_x$CoO$_{3}$ ($x$= 0.10-0.70)

Magnetic and transport properties of polycrystalline Gd$_{1-x}$Sr$_x$CoO$_{3}$ ($x$= 0.10-0.70) are investigated systemically. Cluster-glass magnetism for $x \leq$ 0.45 and long-range ferromagnetic order in higher doping level are observed. Transport measurements indicate insulator-like behaviors for the samples with $x \leq$ 0.30, and an insulator-metal (IM) transition around $x$ = 0.35, and metallic behaviors for higher $x$ samples. In contrast to La$_{1-x}$Sr$_{x}$COO$_{3}$, the striking feature is that the system reenters insulator-like state for $x \geq$ 0.60, and the long-range ferromagnetic order and IM transition take place in samples with higher Sr content. It could be attributed to the enhancement of low-spin state stability for the trivalent Co ions due to the small radius of Gd$^{3+}$ ion.

cond-mat.str-el↗

arXiv2005

In-plane ferromagnetism in charge-ordering $Na_{0.55}CoO_2$

The magnetic and transport properties are systematically studied on the single crystal $Na_{0.55}CoO_2$ with charge ordering and divergency in resistivity below 50 K. A long-range ferromagnetic ordering is observed in susceptibility below 20 K with the magnetic field parallel to Co-O plane, while a negligible behavior is observed with the field perpendicular to the Co-O plane. It definitely gives a direct evidence for the existence of in-plane ferromagnetism below 20 K. The observed magnetoresistance (MR) of 30 % at the field of 6 T at low temperatures indicates an unexpectedly strong spin-charge coupling in triangle lattice systems.

cond-mat.str-el↗

arXiv2005

Influence of doping level on the Hall coefficient and on the thermoelectric power in $Nd_{2-x}Ce_xCuO_4$

Hall coefficient $R_H$ and thermoelectric power TEP are studied systematically in the single crystals $Nd_{2-x}Ce_xCuO_{4+δ}$ (NCCO) with different x from underdoped to overdoped regime. With increasing doping level, both $R_H$ and TEP decrease and change their sign from negative to positive. A striking feature is that the temperature dependence of the Hall angle follows a $T^4$ behavior in the underdoped regime, while a $T^2$ in the overdoped regime. These behaviors are closely related to the evolution of Fermi surface with doping level observed by ARPES.

cond-mat.str-el↗