arXiv subjects

X. G. Qiu

Publications and source records attributed to X. G. Qiu.

At least 19 recordsLinked to original sources

arXiv2024

Visualization of Skyrmion-Superconducting Vortex Pairs in a Chiral-Magnet-Superconductor Heterostructure

Magnetic skyrmions, the topological states possessing chiral magnetic structure with nontrivial topology, have been widely investigated as a promising candidate for spintronic devices. They can also couple with superconducting vortices to form skyrmion-vortex pairs, hosting Majorana zero mode, which is a potential candidate for topological quantum computing. Many theoretical proposals have been put forward on constructing skyrmion-vortex pairs in heterostructures of chiral magnets and superconductors. Nevertheless, how to generate skyrmion-vortex pairs in a controllable way experimentally remains a significant challenge. We have designed a heterostructure of a chiral magnet and superconductor [Ta/Ir/CoFeB/MgO]7/Nb in which zero field Néel-type skyrmions can be stabilized and the superconducting vortices can couple with the skyrmions when Nb is in the superconducting state. We have directly observed the formation of skyrmion-superconducting vortex pairs that is dependent on the direction of the applied magnetic field. Our results provide an effective method to manipulate the quantum states of skyrmions with the help of superconducting vortices, which can be used to explore new routines to control the skyrmions for spintronics devices.

cond-mat.supr-con↗

arXiv2022

Direct Observation of Coherent Longitudinal and Shear Acoustic Phonons in TaAs Using Ultrafast X-ray Diffraction

Using femtosecond time-resolved X-ray diffraction, we investigated optically excited coherent acoustic phonons in the Weyl semimetal TaAs. The low symmetry of the (112) surface probed in our experiment enables the simultaneous excitation of longitudinal and shear acoustic modes, whose dispersion closely matches our simulations. We observed an asymmetry in the spectral lineshape of the longitudinal mode that is notably absent from the shear mode, suggesting a time-dependent frequency chirp that is likely driven by photoinduced carrier diffusion. We argue on the basis of symmetry that these acoustic deformations can transiently alter the electronic structure near the Weyl points and support this with model calculations. Our study underscores the benefit of using off-axis crystal orientations when optically exciting acoustic deformations in topological semimetals, allowing one to transiently change their crystal and electronic structures.

cond-mat.mtrl-sci↗

arXiv2021

Photocurrent-driven transient symmetry breaking in the Weyl semimetal TaAs

Symmetry plays a central role in conventional and topological phases of matter, making the ability to optically drive symmetry change a critical step in developing future technologies that rely on such control. Topological materials, like the newly discovered topological semimetals, are particularly sensitive to a breaking or restoring of time-reversal and crystalline symmetries, which affect both bulk and surface electronic states. While previous studies have focused on controlling symmetry via coupling to the crystal lattice, we demonstrate here an all-electronic mechanism based on photocurrent generation. Using second-harmonic generation spectroscopy as a sensitive probe of symmetry change, we observe an ultrafast breaking of time-reversal and spatial symmetries following femtosecond optical excitation in the prototypical type-I Weyl semimetal TaAs. Our results show that optically driven photocurrents can be tailored to explicitly break electronic symmetry in a generic fashion, opening up the possibility of driving phase transitions between symmetry-protected states on ultrafast time scales.

cond-mat.mtrl-sci↗

arXiv2019

Optical and photoemission investigation of structural and magnetic transitions in the iron-based superconductor Sr$_\mathbf{0.67}$Na$_\mathbf{0.33}$Fe$_\mathbf{2}$As$_\mathbf{2}$

We report the temperature-dependent optical conductivity and ARPES studies of the iron-based superconductor (SC) Sr$_{0.67}$Na$_{0.33}$Fe$_2$As$_2$ in the high-temperature tetragonal paramagnetic phase; below the structural and magnetic transitions at $T_{\rm N}\simeq$125 K in the orthorhombic spin-density-wave (SDW)-like phase, and $T_r\simeq$42 K in the reentrant tetragonal double-Q magnetic phase where both charge and SDW order exist; and below the SC transition at $T_c\simeq$10 K. The free-carrier component in the optical conductivity is described by two Drude contributions; one strong and broad, the other weak and narrow. The broad Drude component decreases dramatically below $T_{\rm N}$ and $T_r$, with much of its strength being transferred to a bound excitation in the mid-infrared, while the narrow Drude component shows no anomalies at either of the transitions, actually increasing in strength at low temperature while narrowing dramatically. The behavior of an infrared-active mode suggests zone-folding below $T_r$. Below $T_c$ the dramatic decrease in the low-frequency optical conductivity signals the formation of a SC energy gap. ARPES reveals hole-like bands at the center of the Brillouin zone (BZ), with both electron- and hole-like bands at the corners. Below $T_{\rm N}$, the hole pockets at the center of the BZ decrease in size, consistent with the behavior of the broad Drude component; while below $T_r$ the electron-like bands shift and split, giving rise to a low-energy excitation in the optical conductivity at ~20 meV. The magnetic states, with resulting SDW and charge-SDW order, respectively, lead to a significant reconstruction of the Fermi surface that has profound implications for the transport originating from the electron and hole pockets, but appears to have relatively little impact on the SC in this material.

cond-mat.str-el↗

arXiv2019

Tracking ultrafast photocurrents in the Weyl semimetal TaAs using THz emission spectroscopy

We investigate polarization-dependent ultrafast photocurrents in the Weyl semimetal TaAs using terahertz (THz) emission spectroscopy. Our results reveal that highly directional, transient photocurrents are generated along the non-centrosymmetric c-axis regardless of incident light polarization, while helicity-dependent photocurrents are excited within the ab-plane. This is consistent with earlier static photocurrent experiments, and demonstrates on the basis of both the physical constraints imposed by symmetry and the temporal dynamics intrinsic to current generation and decay that optically induced photocurrents in TaAs are inherent to the underlying crystal symmetry of the transition metal monopnictide family of Weyl semimetals.

cond-mat.str-el↗

arXiv2018

Temperature-driven Topological Phase Transition and Intermediate Dirac Semimetal Phase in ZrTe$_5$

We present an infrared spectroscopy study of ZrTe$_5$, which confirms a recent theoretical proposal that this material exhibits a temperature-driven topological quantum phase transition from a weak to a strong topological insulating state with an intermediate Dirac semimetal state around $T_p \simeq$ 138K. Our study details the temperature evolution of the energy gap in the bulk electronic structure. We found that the energy gap closes around $T_p$ where the optical response exhibits characteristic signatures of a Dirac semimetal state, i.e. a linear frequency-dependent optical conductivity extrapolating to the origin (after subtracting a weak Drude response). This finding allows us to reconcile previous diverging reports about the topological nature of ZrTe$_5$ in terms of a variation of $T_p$ that depends on the crystal growth condition.

cond-mat.mtrl-sci↗

arXiv2018

Scaling of the Fano effect of the in-plane Fe-As phonon and the superconducting critical temperature in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

By means of infrared spectroscopy we determine the temperature-doping phase diagram of the Fano effect for the in-plane Fe-As stretching mode in Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$. The Fano parameter $1/q^2$, which is a measure of the phonon coupling to the electronic particle-hole continuum, shows a remarkable sensitivity to the magnetic/structural orderings at low temperatures. More strikingly, at elevated temperatures in the paramagnetic/tetragonal state we find a linear correlation between $1/q^2$ and the superconducting critical temperature $T_c$. Based on theoretical calculations and symmetry considerations, we identify the relevant interband transitions that are coupled to the Fe-As mode. In particular, we show that a sizable $xy$ orbital component at the Fermi level is fundamental for the Fano effect and possibly also for the superconducting pairing.

cond-mat.supr-con↗

arXiv2017

Infrared probe of the gap evolution across the phase diagram of Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$

We measured the optical conductivity of superconducting single crystals of Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ with $x$ ranging from 0.40 (optimal doping, $T_c = 39$ K) down to 0.20 (underdoped, $T_c = 16$ K), where a magnetic order coexists with superconductivity. In the normal state, the low-frequency optical conductivity can be described by an incoherent broad Drude component and a coherent narrow Drude component: the broad one is doping-independent, while the narrow one shows strong scattering in the heavily underdoped compound. In the superconducting state, the formation of the condensate leads to a low-frequency suppression of the optical conductivity spectral weight. In the heavily underdoped region, the superfluid density is significantly suppressed, and the weight of unpaired carriers rapidly increases. We attribute these results to changes in the superconducting gap across the phase diagram, which could show a nodal-to-nodeless transition due to the strong interplay between magnetism and superconductivity in underdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$.

cond-mat.supr-con↗

arXiv2016

Temperature-tunable Fano resonance induced by strong coupling between Weyl fermions and phonons in TaAs

Strong coupling between discrete phonon and continuous electron-hole pair excitations can give rise to a pronounced asymmetry in the phonon line shape, known as the Fano resonance. This effect has been observed in a variety of systems, such as stripe-phase nickelates, graphene and high-$T_{c}$ superconductors. Here, we reveal explicit evidence for strong coupling between an infrared-active $A_1$ phonon and electronic transitions near the Weyl points (Weyl fermions) through the observation of a Fano resonance in the recently discovered Weyl semimetal TaAs. The resultant asymmetry in the phonon line shape, conspicuous at low temperatures, diminishes continuously as the temperature increases. This anomalous behavior originates from the suppression of the electronic transitions near the Weyl points due to the decreasing occupation of electronic states below the Fermi level ($E_{F}$) with increasing temperature, as well as Pauli blocking caused by thermally excited electrons above $E_{F}$. Our findings not only elucidate the underlying mechanism governing the tunable Fano resonance, but also open a new route for exploring exotic physical phenomena through the properties of phonons in Weyl semimetals.

cond-mat.str-el↗

arXiv2016

Optical observation of spin-density-wave fluctuations in Ba122 iron-based superconductors

In iron-based superconductors, a spin-density-wave (SDW) magnetic order is suppressed with doping and unconventional superconductivity appears in close proximity to the SDW instability. The optical response of the SDW order shows clear gap features: substantial suppression in the low-frequency optical conductivity, alongside a spectral weight transfer from low to high frequencies. Here, we study the detailed temperature dependence of the optical response in three different series of the Ba122 system [Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$, Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ and BaFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$]. Intriguingly, we found that the suppression of the low-frequency optical conductivity and spectral weight transfer appear at a temperature $T^{\ast}$ much higher than the SDW transition temperature $T_{SDW}$. Since this behavior has the same optical feature and energy scale as the SDW order, we attribute it to SDW fluctuations. Furthermore, $T^{\ast}$ is suppressed with doping, closely following the doping dependence of the nematic fluctuations detected by other techniques. These results suggest that the magnetic and nematic orders have an intimate relationship, in favor of the magnetic-fluctuation-driven nematicity scenario in iron-based superconductors.

cond-mat.supr-con↗

arXiv2015

Spin-flop transition and magnetic phase diagram in CaCo$_{2}$As$_{2}$ revealed by torque measurements

The magnetic properties of CaCo$_{2}$As$_{2}$ single crystal was systematically studied by using dc magnetization and magnetic torque measurements. A paramagnetic to antiferromagnetic transition occurs at $T_N$ = 74 K with Co spins being aligned parallel to the c axis. For $H \parallel c$, a field-induced spin-flop transition was observed below $T_N$ and a magnetic transition from antiferromagnetic to paramagnetic was inferred from the detailed analysis of magnetization and magnetic torque. Finally, we summarize the magnetic phase diagram of CaCo$_{2}$As$_{2}$ based on our results in the \emph{H-T} plane.

cond-mat.supr-con↗

arXiv2015

Optical Signatures of Weyl Points in TaAs

We present a systematic study of both the temperature and frequency dependence of the optical response in TaAs, a material that has recently been realized to host the Weyl semimetal state. Our study reveals that the optical conductivity of TaAs features a narrow Drude response alongside a conspicuous linear dependence on frequency. The width of the Drude peak decreases upon cooling, following a $T^{2}$ temperature dependence which is expected for Weyl semimetals. Two linear components with distinct slopes dominate the 5-K optical conductivity. A comparison between our experimental results and theoretical calculations suggests that the linear conductivity below $\sim$230~cm$^{-1}$ is a clear signature of the Weyl points lying in very close proximity to the Fermi energy.

cond-mat.mtrl-sci↗

arXiv2015

Spin-Fluctuation-Induced Non-Fermi-Liquid Behavior with suppressed superconductivity in LiFe$_{1-x}$Co$_{x}$As

A series of LiFe$_{1-x}$Co$_{x}$As compounds with different Co concentrations have been studied by transport, optical spectroscopy, angle-resolved photoemission spectroscopy and nuclear magnetic resonance. We observed a Fermi liquid to non-Fermi liquid to Fermi liquid (FL-NFL-FL) crossover alongside a monotonic suppression of the superconductivity with increasing Co content. In parallel to the FL-NFL-FL crossover, we found that both the low-energy spin fluctuations and Fermi surface nesting are enhanced and then diminished, strongly suggesting that the NFL behavior in LiFe$_{1-x}$Co$_{x}$As is induced by low-energy spin fluctuations which are very likely tuned by Fermi surface nesting. Our study reveals a unique phase diagram of LiFe$_{1-x}$Co$_{x}$As where the region of NFL is moved to the boundary of the superconducting phase, implying that they are probably governed by different mechanisms.

cond-mat.supr-con↗

arXiv2015

Anomalous phonon redshift in K-doped BaFe2As2 iron pnictides

The effect of K, Co and P dopings on the lattice dynamics in the BaFe$_2$As$_2$ system is studied by infrared spectroscopy. We focus on the phonon at $\sim$ 253 cm$^{-1}$, the highest energy in-plane infrared-active Fe-As mode in BaFe$_2$As$_2$. Our studies show that the Co and P dopings lead to a blue shift of this phonon in frequency, which can be simply interpreted by the change of lattice parameters induced by doping. In sharp contrast, an unusual red shift of the same mode was observed in the K-doped compound, at odds with the above explanation. This anomalous behavior in K-doped BaFe$_2$As$_2$ is more likely associated with the coupling between lattice vibrations and other channels, such as charge or spin. This coupling scenario is also supported by the asymmetric line shape and intensity growth of the phonon in the K-doped compound.

cond-mat.supr-con↗

arXiv2015

Optical conductivity of Ba0.6 K0.4 Fe2 As2 : The effect of in-plane and out-of-plane doping in the superconducting gap

We measured the in-plane optical conductivity of a nearly optimally doped (Ba,K)Fe2As2 single crystal with Tc = 39.1 K. Upon entering the superconducting state the optical conductivity below ~20 meV vanishes, strongly suggesting a fully gapped system. A BCS-like fit requires two different isotropic gaps to describe the optical response of this material. The temperature dependence of the gaps and the penetration depth suggest a strong interband coupling, but no impurity scattering induced pair breaking is present. This contrasts to the large residual conductivity observed in optimally doped Ba(Fe,Co)2As2 and strongly supports an s(+/-) gap symmetry for these compounds.

cond-mat.supr-con↗

arXiv2014

Electron-phonon coupling in the superconducting single crystal Rb$_{0.8}$Fe$_{1.68}$Se$_2$

The optical properties of the superconducting single crystal Rb$_{0.8}$Fe$_{1.68}$Se$_2$ with $T_{c}$ $\simeq$ 31 K have been measured over a wide frequency range in the $ab$ plane. We found that the optical conductivity is dominated by a series of infrared-active phonon modes at low-frequency region as well as several other high-frequency bound excitations. The low-frequency optical conductivity has rather low value and shows quite small Drude-like response, indicating low carriers density in this material. Furthermore, the phonon modes increase continuously in frequency with decreasing temperature; specifically, the phonon mode around 200 cm$^{-1}$ shows an enhanced asymmetry effect at low temperatures, suggesting an increasing electron-phonon coupling in this system.

cond-mat.supr-con↗

arXiv2013

Pseudogap in underdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ as seen via optical conductivity

We report the observation of a pseudogap in the \emph{ab}-plane optical conductivity of underdoped Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ ($x = 0.2$ and 0.12) single crystals. Both samples show prominent gaps opened by a spin density wave (SDW) order and superconductivity at the transition temperatures $T_{\it SDW}$ and $T_c$, respectively. In addition, we observe an evident pseudogap below $T^{\ast} \sim$ 75 K, a temperature much lower than $T_{\it SDW}$ but much higher than $T_{c}$. A spectral weight analysis shows that the pseudogap is closely connected to the superconducting gap, indicating the possibility of its being a precursor of superconductivity. The doping dependence of the gaps is also supportive of such a scenario.

cond-mat.supr-con↗

arXiv2013

Hidden $T$-Linear Scattering Rate in Ba$_{0.6}$K$_{0.4}$Fe$_2$As$_2$ Revealed by Optical Spectroscopy

The optical properties of Ba$_{0.6}$K$_{0.4}$Fe$_{2}$As$_{2}$ have been determined in the normal state for a number of temperatures over a wide frequency range. Two Drude terms, representing two groups of carriers with different scattering rates ($1/τ$), well describe the real part of the optical conductivity, $σ_{1}(ω)$. A "broad" Drude component results in an incoherent background with a $T$-independent $1/τ_b$, while a "narrow" Drude component reveals a $T$-linear $1/τ_n$ resulting in a resistivity $ρ_n \equiv 1/σ_{1n}(ω\rightarrow 0)$ also linear in temperature. An arctan($T$) low-frequency spectral weight is also a strong evidence for a $T$-linear 1/$τ$. Comparison to other materials with similar behavior suggests that the $T$-linear $1/τ_n$ and $ρ_n$ in Ba$_{0.6}$K$_{0.4}$Fe$_{2}$As$_{2}$ originate from scattering from spin fluctuations and hence that an antiferromagnetic quantum critical point is likely to exist in the superconducting dome.

cond-mat.supr-con↗