arXiv subjects

X. Xu

Publications and source records attributed to X. Xu.

At least 91 records · Page 5Linked to original sources

arXiv2019

Spin-Liquid-Like State in Pure and Mn-Doped TbInO3 with Nearly Triangular Lattice

Inelastic neutron scattering studies in single crystals of TbInO3 and TbIn0.95Mn0.05O3 with nearly-triangular antiferromagnetic lattice are reported. At low energies, a broad and apparently gapless continuum of magnetic excitations, located at the triangular lattice (TL) Brillouin zone boundary, is observed. The data are well described by the uncorrelated nearest-neighbor valence bonds model. At higher energies, a broad excitation branch dispersing from the TL zone boundary is observed. No signs of static magnetic order are found down to the temperatures two orders of magnitude smaller than the effective interaction energy. The fluctuating magnetic moment exceeds two thirds of the Tb3+ free-ion value and is confined to the TL plane. These observations are consistent with a TL-based spin liquid state in TbInO3.

cond-mat.str-el↗

arXiv2019

Masses of neutron-rich $^{\operatorname{52-54}}$Sc and $^{54,56}$Ti nuclides: The $N=32$ subshell closure in scandium

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the neutron-rich $^{\operatorname{52-54}}$Sc and $^{54,56}$Ti nuclei. The new mass excess values $ME$($^{52}$Sc) $=$ $-40525(65)$ keV, $ME$($^{53}$Sc) $=$ $-38910(80)$ keV, and $ME$($^{54}$Sc) $=$ $-34485(360)$ keV, deviate from the Atomic Mass Evaluation 2012 by 2.3$σ$, 2.8$σ$, and 1.7$σ$, respectively. These large deviations significantly change the systematics of the two-neutron separation energies of scandium isotopes. The empirical shell gap extracted from our new experimental results shows a significant subshell closure at $N = 32$ in scandium, with a similar magnitude as in calcium. Moreover, we present $ab$ $initio$ calculations using the valence-space in-medium similarity renormalization group based on two- and three-nucleon interactions from chiral effective field theory. The theoretical results confirm the existence of a substantial $N = 32$ shell gap in Sc and Ca with a decreasing trend towards lighter isotones, thus providing a consistent picture of the evolution of the $N = 32$ magic number from the $pf$ into the $sd$ shell.

nucl-ex↗

arXiv2019

Improving the resolving power of Isochronous Mass Spectrometry by employing an in-ring mechanical slit

Isochronous Mass Spectrometry (IMS) in heavy-ion storage rings is an excellent experimental method for precision mass measurements of exotic nuclei. In the IMS, the storage ring is tuned in a special isochronous ion-optical mode. Thus, the mass-over-charge ratios of the stored ions are directly reflected by their respective revolution times in first order. However, the inevitable momentum spread of secondary ions increases the peak widths in the measured spectra and consequently limits the achieved mass precision. In order to achieve a higher mass resolving power, the ring aperture was reduced to 60 mm by applying a mechanical slit system at the dispersive straight section. The momentum acceptance was reduced as well as better isochronous conditions were achieved. The results showed a significant improvement of the mass resolving power reaching $5.2 \times 10^{5}$, though at the cost of about 40\% ion loss.

nucl-ex↗

arXiv2019

Towards the Limits of Existence of Nuclear Structure: Observation and First spectroscopy of the Isotope $^{31}$K by measuring its three-proton Decay

The most-remote from stability isotope $^{31}$K, which is located four atomic mass units beyond the proton drip line, has been observed. It is unbound in respect to three-proton (${3p}$) emission, and its decays have been detected in flight by measuring trajectories of all decay products using micro-strip detectors. The $3p$-emission processes have been studied by means of angular correlations $^{28}$S+3$p$ and the respective decay vertexes. The energies of the previously-unknown ground and excited states of $^{31}$K have been determined. This provides its $3p$ separation-energy value $S_{3p}$ of $-4.6(2)$ MeV. Upper half-life limits of 10 ps of the observed $^{31}$K states have been derived from distributions of the measured decay vertexes.

nucl-ex↗

arXiv2019

How Robust is the N = 34 Subshell Closure? First Spectroscopy of $^{52}$Ar

The first $γ$-ray spectroscopy of $^{52}$Ar, with the neutron number N = 34, was measured using the $^{53}$K(p,2p) one-proton removal reaction at $\sim$210 MeV/u at the RIBF facility. The 2$^{+}_{1}$ excitation energy is found at 1656(18) keV, the highest among the Ar isotopes with N $>$ 20. This result is the first experimental signature of the persistence of the N = 34 subshell closure beyond $^{54}$Ca, i.e., below the magic proton number Z = 20. Shell-model calculations with phenomenological and chiral-effective-field-theory interactions both reproduce the measured 2$^{+}_{1}$ systematics of neutron-rich Ar isotopes, and support a N = 34 subshell closure in $^{52}$Ar.

nucl-ex↗

arXiv2019

Spectral content of a single non-Brownian trajectory

Time-dependent processes are often analysed using the power spectral density (PSD), calculated by taking an appropriate Fourier transform of individual trajectories and finding the associated ensemble-average. Frequently, the available experimental data sets are too small for such ensemble averages, and hence it is of a great conceptual and practical importance to understand to which extent relevant information can be gained from $S(f,T)$, the PSD of a single trajectory. Here we focus on the behavior of this random, realization-dependent variable, parametrized by frequency $f$ and observation-time $T$, for a broad family of anomalous diffusions---fractional Brownian motion (fBm) with Hurst-index $H$---and derive exactly its probability density function. We show that $S(f,T)$ is proportional---up to a random numerical factor whose universal distribution we determine---to the ensemble-averaged PSD. For subdiffusion ($H<1/2$) we find that $S(f,T)\sim A/f^{2H+1}$ with random-amplitude $A$. In sharp contrast, for superdiffusion $(H>1/2)$ $S(f,T)\sim BT^{2H-1}/f^2$ with random amplitude $B$. Remarkably, for $H>1/2$ the PSD exhibits the same frequency-dependence as Brownian motion, a deceptive property that may lead to false conclusions when interpreting experimental data. Notably, for $H>1/2$ the PSD is ageing and is dependent on $T$. Our predictions for both sub- and superdiffusion are confirmed by experiments in live cells and in agarose hydrogels, and by extensive simulations.

cond-mat.stat-mech↗

arXiv2019

High-resolution, accurate MR-TOF-MS for short-lived, exotic nuclei of few events in their ground and low-lying isomeric states

Mass measurements of fission and projectile fragments, produced via $^{238}$U and $^{124}$Xe primary beams, have been performed with the multiple-reflection time-of-flight mass spectrometer (MR-TOF-MS) of the FRS Ion Catcher with a mass resolving powers (FWHM) up to 410,000 and an uncertainty of $6\cdot 10^{-8}$. The nuclides were produced and separated in-flight with the fragment separator FRS at 300 to 1000 MeV/u and thermalized in a cryogenic stopping cell. The data-analysis procedure was developed to determine with highest accuracy the mass values and the corresponding uncertainties for the most challenging conditions: down to a few events in a spectrum and overlapping distributions, characterized only by a broader common peak shape. With this procedure, the resolution of low-lying isomers is increased by a factor of up to three compared to standard data analysis. The ground-state masses of 31 short-lived nuclides of 15 different elements with half-lives down to 17.9~ms and count rates as low as 11 events per nuclide were determined. This is the first direct mass measurement for seven nuclides. The excitation energies and the isomer-to-ground state ratios of six isomeric states with excitation energies down to about 280~keV were measured. For nuclides with known mass values, the average relative deviation from the literature values is $(2.9 \pm 6.2) \cdot 10^{-8}$. The measured two-neutron separation energies and their slopes near and at the N=126 and Z=82 shell closures indicate a strong element-dependent binding energy of the first neutron above the closed proton shell Z=82. The experimental results deviate strongly from the theoretical predictions, especially for N=126 and N=127.

nucl-ex↗

arXiv2018

Experimental Investigation of the Transition Energy $γ_t$ in the Isochronous Mode of the HIRFL-CSRe

The Isochronous Mass Spectrometry (IMS) based on storage rings is a powerful technique for mass measurement of short-lived exotic nuclei. The transition energy $γ_t$ of the storage ring is a vital parameter of the IMS technique. It is difficult to measure the $γ_t$ and its relation to momentum spread or circulating length, especially to monitor the variation of $γ_t$ during experiments. An experimental investigation on the $γ_t$ has been performed for the IMS experiment at the Cooler Storage Ring of the Heavy Ion Research Facility in Lanzhou (HIRFL-CSRe). With the velocity measured by two time-of-flight (TOF) detectors, the $γ_t$ as a function of orbital length can be determined. The influences of higher order magnetic field components on the $γ_t$ function were inferred for isochronous correction. This paper introduces and investigates the influence of dipole magnetic fields, quadrupole magnetic fields and sextupole magnetic fields on the $γ_t$ function. With the quadrupole magnets and sextupole magnets corrections, a mass resolution of 171332 (FWHM) and $σ(T)/T=1.34\times10^{-6}$ were reached, which shall be compared with 31319 (FWHM) and $σ(T)/T=7.35\times10^{-6}$ obtained without correction.

physics.acc-ph↗

arXiv2018

Application of isochronous mass spectrometry for the study of angular momentum population in projectile fragmentation reactions

Isochronous mass spectrometry was applied to measure isomeric yield ratios of fragmentation reaction products. This approach is complementary to conventional gamma-ray spectroscopy in particular for measuring yield ratios for long-lived isomeric states. Isomeric yield ratios for the high-spin I = 19/2 states in the mirror nuclei 53Fe and 53Co are measured to study angular momentum population following the projectile fragmentation of 78Kr at energies of 480A MeV on a beryllium target. The 19/2 state isomeric ratios of 53Fe produced from different projectiles in the literature have also been extracted as a function of mass number difference between projectile and fragment (mass loss). The results are compared to ABRABLA07 model calculations. The isomeric ratios of 53Fe produced using different projectiles suggest that the theory underestimates not only the previously reported dependence on the spin but also the dependence on the mass loss.

nucl-ex↗

arXiv2018

A method to measure the transition energy $γ_{t}$ of the isochronously tuned storage ring

The Isochronous Mass Spectrometry (IMS) is a powerful technique developed in heavy-ion storage rings for measuring masses of very short-lived exotic nuclei. The IMS is based on the isochronous setting of the ring. One of the main parameters of this setting is the transition energy $γ_{t}$. %The transition energy $γ_{t}$ plays an important role in the isochronous mass spectrometry (IMS). It has been a challenge to determine the $γ_{t}$ and especially to monitor the variation of $γ_{t}$ during experiments. In this paper we introduce a method to measure the $γ_{t}$ online during IMS experiments by using the acquired experimental data. Furthermore, since the storage ring has (in our context) a relatively large momentum acceptance, the variation of the $γ_{t}$ across the ring acceptance is a source of systematic uncertainty of measured masses. With the installation of two time-of-flight (TOF) detectors, the velocity of each stored ion and its revolution time are simultaneously available for the analysis. These quantities enabled us to determine the $γ_{t}$ as a function of orbital length in the ring. The presented method is especially important for future IMS experiments planned at the new-generation storage ring facilities FAIR in Germany and HIAF in China.

physics.ins-det↗

arXiv2018

Isochronous mass measurements of $T_z=-1$ $fp$-shell nuclei from projectile fragmentation of $^{58}$Ni

Atomic masses of seven $T_z=-1$, $fp$-shell nuclei from $^{44}$V to $^{56}$Cu and two low-lying isomers, $^{44m}$V ($J^π=6^+$) and $^{52m}$Co ($J^π=2^+$), have been measured with relative precisions of $1-4\times 10^{-7}$ with Isochronous Mass Spectrometry (IMS) at CSRe. The masses of $^{56}$Cu, $^{52g,52m}$Co, and $^{44m}$V were measured for the first time in this experiment. The Mass Excesses ($ME^{\prime}$s) of $^{44}$V, $^{48}$Mn, $^{50}$Fe, and $^{54}$Ni are determined with an order of magnitude improved precision compared to the literature values. $^{52g,52m}$Co and $^{56}$Cu are found to be $370$~keV and $400$~keV more bound, respectively, while $^{44g,44m}$V are $\sim 300$~keV less bound than the extrapolations in the Atomic-Mass Evaluation 2012 (AME$^{\prime}$12). The masses of the four $T_z=-1/2$ nuclei $^{45}$V, $^{47}$Cr, $^{49}$Mn, and $^{51}$Fe are re-determined to be in agreement, within the experimental errors, with the recent JYFLTRAP measurements or with the previous IMS measurements in CSRe. Details of the measurements and data analysis are described, and the impact of the new $ME$ values on different aspects in nuclear structure are investigated and discussed.

nucl-ex↗

arXiv2018

HST/COS observations of the newly discovered obscuring outflow in NGC 3783

To understand the nature of transient obscuring outflows in active galactic nuclei, we observed the Seyfert 1 galaxy NGC 3783 on two occasions in December 2016 triggered by Swift monitoring indicating strong soft X-ray absorption in November. We obtained ultraviolet spectra using COS on HST and optical spectra using FEROS on the MPG/ESO 2.2-m telescope that were simultaneous with X-ray spectra from XMM-Newton and NuSTAR. We find new components of broad, blue-shifted absorption associated with Ly$α$, \ion{N}{v}, \ion{Si}{iv}, and \ion{C}{iv} in our COS spectra. The absorption extends from velocities near zero in the rest-frame of the host galaxy to $-6200$ $\rm km~s^{-1}$. These features appear for the first time in NGC 3783 at the same time as the heavy soft X-ray absorption seen in the XMM-Newton X-ray spectra. The X-ray absorption has a column density of $\sim 10^{23}~\rm cm^{-2}$, and it partially covers the X-ray continuum source. The X-ray absorption becomes more transparent in the second observation, as does the UV absorption. Combining the X-ray column densities with the UV spectral observations yields an ionization parameter for the obscuring gas of log $ξ=1.84^{+0.4}_{-0.2}$ $\rm erg~cm~s^{-1}$. Despite the high intensity of the UV continuum in NGC 3783, F(1470 Å)=$8 \times 10^{-14}~\rm erg~cm^{-2}~s^{-1}~Å^{-1}$, the well known narrow UV absorption lines are deeper than in earlier observations in unobscured states, and low ionization species such as \ion{C}{iii} appear, indicating that the narrow-line gas is more distant from the nucleus and is being shadowed by the gas producing the obscuration. Despite the high continuum flux levels in our observations of NGC 3783, moderate velocities in the UV broad line profiles have substantially diminished. We suggest that a collapse of the broad line region has led to the outburst and triggered the obscuring event.

astro-ph.GA↗

arXiv2018

Magnetic excitations in bulk multiferroic two-dimensional triangular lattice antiferromagnet (Lu,Sc)FeO$_3$

Non-collinear two-dimensional triangular lattice antiferromagnets (2D TLAF) are currently an area of very active research due to their unique magnetic properties, which lead to non-trivial quantum effects that experimentally manifest themselves in the spin excitation spectra. Recent examples of such insulating 2D TLAF include (Y,Lu)MnO$_3$, LiCrO$_2$, and CuCrO$_2$. Hexagonal LuFeO3 is a recently synthesized 2D TLAF which exhibits properties of an ideal multiferroic material, partially because of the high spin ($S=5/2$) and strong magnetic super-exchange interactions. We report the full range of spin dynamics in a bulk single crystal of (Lu$_{0.6}$Sc$_{0.4}$)FeO$_3$ (Sc doping to stabilize the hexagonal structure) measured via time-of-flight inelastic neutron scattering. Modeling with linear spin wave theory yields a nearest neighbor exchange coupling of $J$ = 4.0(2) meV (DFT calculations for $h$-LuFeO$_3$ predicted a value of 6.31 meV) and anisotropy values of $K_D$ = 0.17(1) meV (easy plane) and $K_A$~=~-0.05(1)~meV (local easy axis). It is observed that the magnon bandwidth of the spin wave spectra is twice as large for $h$-(Lu,Sc)FeO$_3$ as it is for $h$-LuMnO$_3$.

cond-mat.str-el↗

arXiv2018

Deep excursion beyond the proton dripline. I. Argon and chlorine isotope chains

The proton-unbound argon and chlorine isotopes have been studied by measuring trajectories of their decay-in-flight products by using a tracking technique with micro-strip detectors. The proton ($1p$) and two-proton ($2p$) emission processes have been detected in the measured angular correlations "heavy-fragment"+$p$ and "heavy-fragment"+$p$+$p$, respectively. The ground states of the previously unknown isotopes $^{30}$Cl and $^{28}$Cl have been observed for the first time, providing the $1p$-separation energies $S_p$ of $-0.48(2)$ and $-1.60(8)$ MeV, respectively. The relevant systematics of $1p$ and $2p$ separations energies have been studied theoretically in the core+$p$ and core+$p$+$p$ cluster models. The first-time observed excited states of $^{31}$Ar allow to infer the $2p$-separation energy $S_{2p}$ of 6(34) keV for its ground state. The first-time observed state in $^{29}$Ar with $S_{2p} = -5.50(18)$ MeV can be identified either as a ground or an excited state according to different systematics.

nucl-ex↗

arXiv2018

Deep excursion beyond the proton dripline. II. Toward the limits of existence of nuclear structure

Prospects of experimental studies of argon and chlorine isotopes located far beyond the proton dripline are studied by using systematics and cluster models. The deviations from the widespread systematics observed in $^{28,29}$Cl and $^{29,30}$Ar have been theoretically substantiated, and analogous deviations predicted for the lighter chlorine and argon isotopes. The limits of nuclear structure existence are predicted for Ar and Cl isotopic chains, with $^{26}$Ar and $^{25}$Cl found to be the lightest sufficiently long-living nuclear systems. By simultaneous measurements of protons and $γ$-rays following decays of such systems as well as their $β$-delayed emission, an interesting synergy effect may be achieved, which is demonstrated by the example of $^{30}$Cl and $^{31}$Ar ground state studies. Such synergy effect may be provided by the new EXPERT setup (EXotic Particle Emission and Radioactivity by Tracking), being operated inside the fragment separator and spectrometer facility at GSI, Darmstadt.

nucl-ex↗

arXiv2018

Detection of thermodynamic "valley noise" in monolayer semiconductors: access to intrinsic valley relaxation timescales

Together with charge and spin degrees of freedom, many new 2D materials also permit information to be encoded in an electron's valley degree of freedom - that is, in particular momentum states in the material's Brillouin zone. With a view towards future generations of valley-based (opto)electronic technologies, the intrinsic timescales of scattering and relaxation between valleys therefore represent fundamental parameters of interest. Here we introduce and demonstrate an entirely passive, noise-based approach for exploring intrinsic valley dynamics in atomically-thin transition-metal dichalcogenide (TMD) semiconductors. Exploiting the valley-specific optical selection rules in monolayer TMDs, we use optical Faraday rotation to detect, under conditions of strict thermal equilibrium, the stochastic thermodynamic fluctuations of the valley polarization in a Fermi sea of resident carriers. Frequency spectra of this spontaneous "valley noise" reveal narrow Lorentzian lineshapes and therefore long exponentially-decaying intrinsic valley relaxation. Moreover, the valley noise signals are shown to validate both the relaxation times and the spectral dependence of conventional (perturbative) pump-probe measurements. These results provide a viable route toward quantitative measurements of intrinsic valley dynamics, free from any external perturbation, pumping, or excitation.

cond-mat.mes-hall↗

arXiv2018

The Masses of the $T_z=-3/2$ Nuclei $^{27}$P and $^{29}$S

Isochronous mass spectrometry has been applied in the storage ring CSRe to measure the masses of the $T_z=-3/2$ nuclei $^{27}$P and $^{29}$S. The new mass excess value $ME$($^{29}$S) $=-3094(13)$~keV is 66(52)~keV larger than the result of the previous $^{32}$S($^3$He,$^{6}$He)$^{29}$S reaction measurement in 1973 and a factor of 3.8 more precise. The new result for $^{29}$S, together with those of the $T=3/2$ isobaric analog states (IAS) in $^{29}$P, $^{29}$Si, and $^{29}$Al, fit well into the quadratic form of the Isobaric Multiplet Mass Equation IMME. The mass excess of $^{27}$P has been remeasured to be $ME(^{27}$P$)=-685(42)$ keV. By analyzing the linear and quadratic coefficients of the IMME in the $T_z=-3/2$ $sd$-shell nuclei, it was found that the ratio of the Coulomb radius parameters is $R\approx0.96$ and is nearly the same for all $T=3/2$ isospin multiplets. Such a nearly constant $R$-value, apparently valid for the entire light mass region with $A>9$, can be used to set stringent constraints on the isovector and isotensor components of the isospin non-conserving forces in theoretical calculations.

nucl-ex↗

arXiv2018

First application of combined isochronous and Schottky mass spectrometry: Half-lives of fully ionized 49Cr24+ and 53Fe26+ atoms

Lifetime measurements of b -decaying highly charged ions have been performed in the storage ring CSRe by applying the isochronous Schottky mass spectrometry. The fully ionized 49Cr and 53Fe ions were produced in projectile fragmentation of 58Ni primary beam and were stored in the CSRe tuned into the isochronous ion-optical mode. The new resonant Schottky detector was applied to monitor the intensities of stored uncooled 49Cr24+ and 53Fe26+ ions. The extracted half-lives T1/2(49Cr24+) = 44.0(27) min and T1/2(53Fe26+) = 8.47(19) min are in excellent agreement with the literature half-life values corrected for the disabled electron capture branchings. This is an important proof-of-principle step towards realizing the simultaneous mass and lifetime measurements on exotic nuclei at the future storage ring facilities.

nucl-ex↗