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Xiangdong Zhang

Publications and source records attributed to Xiangdong Zhang.

At least 163 records · Page 9Linked to original sources

Topolectrical-circuit octupole insulator with topologically protected corner states

Recent theoretical studies have extended the Berry phase framework to account for higher electric multipole moments, quadrupole and octupole topological phases have been proposed. Although the two-dimensional quantized quadrupole insulators have been demonstrated experimentally, octupole topological phases have not previously been observed experimentally. Here we report on the experimental realization of classical analog of octupole topological insulator in the electric circuit system. Three-dimensional topolectrical circuits for realizing such topological phases are constructed experimentally. We observe octupole topological states protected by the topology of the bulk, which are localized at the corners. Our results provide conclusive evidence of a form of robustness against disorder and deformation, which is characteristic of octupole topological insulators. Our study opens a new route toward higher-order topological phenomena in three-dimensions and paves the way for employing topolectrical circuitry to study complex topological phenomena.

cond-mat.mes-hall↗

Efficient verification of Dicke states

Among various multipartite entangled states, Dicke states stand out because their entanglement is maximally persistent and robust under particle losses. Although much attention has been attracted for their potential applications in quantum information processing and foundational studies, the characterization of Dicke states remains as a challenging task in experiments. Here, we propose efficient and practical protocols for verifying arbitrary $n$-qubit Dicke states in both adaptive and nonadaptive ways. Our protocols require only two distinct settings based on Pauli measurements besides permutations of the qubits. To achieve infidelity $ε$ and confidence level $1-δ$, the total number of tests required is only $O(nε^{-1}\lnδ^{-1})$. This performance is exponentially more efficient than all previous protocols based on local measurements, including quantum state tomography and direct fidelity estimation, and is comparable to the best global strategy. Our protocols are readily applicable with current experimental techniques and are able to verify Dicke states of hundreds of qubits.

quant-ph↗

Locally distinguish unextendible product bases by efficiently using entanglement resource

Any set of states which cannot be perfectly distinguished by local operations and classical communication (LOCC) alone, can always be locally distinguished using quantum teleportation with enough entanglement resource. However, in quantum information theory, entanglement is a very valuable resource, so it leaves the following open question: how to accomplish this task more efficiently than teleportation, that is, design the local discrimination protocol using less entanglement resource. In this paper, we first present two protocols to locally distinguish a set of unextendible product bases (UPB) in $5\otimes 5$ by using different entanglement resource. Then, we generalize the distinguishing methods for a class of UPB in $d\otimes d$, where $d$ is odd and $d\geqslant 3$. Furthermore, for a class of UPB in $d\otimes d$, where $d$ is even and $d\geqslant 4$, we prove that these states can also be distinguished by LOCC with multiple copies of low-dimensional entanglement resource. These results offer rather general insight into how to use entanglement resource more efficiently, and also reveal the phenomenon of less nonlocality with more entanglement.

quant-ph↗

Observation of novel robust edge states without bulk-boundary correspondence in non-Hermitian quantum walks

Recently, the study of non-Hermitian physics has attracted considerable attention. The modified bulk-boundary correspondence has been proposed to understand topological edge states in non-Hermitian static systems. Here we report a new experimental observation of edge states in non-Hermitian periodically driven systems. Some unconventional edge states are found not to be satisfied with the bulk-boundary correspondence when the system belongs to the broken parity-time (PT) symmetric phase. The experiments are performed in our constructed non-Hermitian light quantum walk platform with left and right boundaries, where the beams outside system boundary are blocked subtly at the end of each step. The robust properties of these edge states against to static perturbations and disorder have also been demonstrated experimentally. The finding of robust edge states in broken PT-symmetric phase inspires us to explore a robust transport channel in ubiquitously complex systems with strong dissipation.

physics.optics↗

Coherence Depletion in Quantum Algorithms

Besides the superior efficiency compared to their classical counterparts, quantum algorithms known so far are basically task-dependent, and scarcely any common features are shared between them. In this work, however, we show that the depletion of quantum coherence turns out to be a common phenomenon in these algorithms. For all the quantum algorithms that we investigated including Grover's algorithm, Deutsch-Jozsa algorithm and Shor's algorithm, quantum coherence of the system states reduces to the minimum along with the successful execution of the respective processes. Notably, a similar conclusion cannot be drawn using other quantitative measures such as quantum entanglement. Thus, we expect that coherence depletion as a common feature can be useful for devising new quantum algorithms in the future.

quant-ph↗

Kerr-de Sitter and Kerr-anti-de Sitter black holes as accelerators for spinning particles

It is shown that the Kerr black hole could act as accelerators for spinning particles. In principle, it could obtain arbitrarily high energy for extremal Kerr black hole. In this paper, we extend the previous research to the Kerr-(anti-)de Sitter background and find that the cosmological constant plays an important role in the result. For the case of Kerr-anti-de Sitter black holes, like the Kerr background, only the extremal Kerr-anti-de Sitter black holes can have a divergent center-of-mass energy of collision. While, for the case of Kerr-de Sitter black holes, the collision of two spinning particles can take place on the outer horizon of the black holes and the center-of-mass energy of collision can blow up if one of the collision particle takes the critical angular momentum. Hence, non-extremal Kerr-de Sitter black holes could also act as accelerators with arbitrarily high center-of-mass energy for spinning particles.

gr-qc↗

Long-lived quantum speedup based on plasmonic hot spot systems

Long-lived quantum speedup serves as a fundamental component for quantum algorithms. The quantum walk is identified as an ideal scheme to realize the long-lived quantum speedup. However, one finds that the duration of quantum speedup is very short in real systems implementing quantum walk. The speedup can last only dozens of femtoseconds in the photosynthetic light-harvesting system, which was regarded as the best candidate for quantum information processing. Here, we construct one plasmonic system with two-level molecules embodied in the hot spots of one-dimensional nanoparticle chains to realize the long-lived quantum speedup. The coherent and incoherent coupling parameters in the system are obtained by means of Green's tensor technique. Our results reveal that the duration of quantum speedup in our scheme can exceed 500 fs under strong coherent coupling conditions, which is several times larger than that in the photosynthetic light-harvesting system. Our proposal presents a competitive scheme to realize the long-lived quantum speedup, which is very beneficial for quantum algorithms.

physics.optics↗

Plasmon-induced strong interaction between chiral molecules and orbital angular momentum of light

Whether or not chiral interaction exists between the optical orbital angular momentum (OAM) and a chiral molecule remains unanswered. So far, such an interaction has not been observed experimentally. Here we present a T-matrix method to study the interaction between optical OAM and the chiral molecule in a cluster of nanoparticles. We find that strong interaction between the chiral molecule and OAM can be induced by the excitation of plasmon resonances. An experimental scheme to observe such an interaction has been proposed. Furthermore, we have found that the signal of the OAM dichroism can be either positive or negative, depending on the spatial positions of nanocomposites in the cross-sections of OAM beams. The cancellation between positive and negative signals in the spatial average can explain why the interaction has not been observed in former experiments.

physics.optics↗

Competition of Chiroptical Effect Caused by Nanostructure and Chiral Molecules

The theory to calculate circular dichroism (CD) of chiral molecules in a finite cluster with arbitrarily disposed objects has been developed by means of T-matrix method. The interactions between chiral molecules and nanostructures have been investigated. Our studies focus on the case of chiral molecules inserted into plasmonic hot spots of nanostructures. Our results show that the total CD of the system with two chiral molecules is not sum for two cases when two chiral molecules inserted respectively into the hot spots of nanoparticle clusters as the distances among nanoparticles are small, although the relationship is established at the case of large interparticle distances. The plasmonic CD arising from structure chirality of nanocomposites depends strongly on the relative positions and orientations of nanospheroids, and are much greater than that from molecule-induced chirality. However, the molecule-induced plasmonic CD effect from the molecule-NP nanocomposites with special chiral structures can be spectrally distinguishable from the structure chirality-based optical activity. Our results provide a new theoretical framework for understanding the two different aspects of plasmonic CD effect in molecule-NP nanocomposites, which would be helpful for the experimental design of novel biosensors to realize ultrasensitive probe of chiral information of molecules by plasmon-based nanotechnology.

physics.optics↗

Multifrequency multi-qubit entanglement based on plasmonic hot spots

The theoretical method to study strong coupling between an ensemble of quantum emitters (QEs) and surface plasmons excited by the nanoparticle cluster has been presented by using a rigorous first-principles electromagnetic Green's tensor technique. We have demonstrated that multi-qubit entanglement for two-level QEs can be produced at different frequencies simultaneously, when they locate in hot spots of metallic nanoparticle clusters. The duration of quantum beats for such an entanglement can reach two orders longer than that for the entanglement in a photonic cavity. The phenomenon originates from collective coupling resonance excitation of the cluster. At the frequency of single scattering resonance, the entanglement cannot be produced although the single QE spontaneous decay rate is very big

quant-ph↗

Engineering topological edge states in two dimensional magnetic photonic crystal

Based on a perturbative approach, we propose a simple and efficient method to engineer topological edge states in two dimensional magnetic photonic crystals. The topological edge states in the microstructures can be constructed and varied by altering the parameters of the microstructure according to the fieldenergy distributions of the Bloch states at the related Bloch wave vectors. The validity of the proposed method has been demonstrated by exact numerical calculations through three concrete examples. Our method makes the topological edge states 'designable'.

physics.optics↗

Ultrafast coherent energy transfer with high efficiency based on plasmonic nanostructures

The theory of energy transfer dynamics of a pair of donor and acceptor molecules located in the plasmonic hot spots is developed by means of the master equation approach and the electromagnetic Green's tensor technique. A nonlocal effect has been considered by using a hydrodynamic model. The coherent interaction between the two molecules in plasmonic nanostructures is investigated under some strong coupling conditions. It is shown that the energy transfer efficiency of a pair of molecules can be improved largely and the transfer time decreases to dozens of femtoseconds when the contribution of quantum coherence is considered. The physical origin for such a phenomenon has also been analyzed. This ultrafast and high-efficiency energy transfer mechanism could be beneficial for artificial light-harvesting devices.

physics.optics↗

Simultaneously giant enhancement of Forster resonance energy transfer rate and efficiency based on plasmonic excitations

We present a first-principles calculation on the rate and efficiency of Förster resonance energy transfer (FRET) from a donor to an acceptor when they are located in the hotspots of nanoparticle clusters. Nonlocal effect has been considered by using a hydrodynamic model. It is found that FRET rate and efficiency can be enhanced simultaneously by more than 9 and 3 orders of magnitude, respectively. The physical origins for these phenomena have been disclosed. Two opposite phenomena, the energy transfer rate is independent or dependent of the local density of optical states (LDOS), have been observed in the same system under different conditions. These findings not only help us to understand the unresolved debate on how the FRET rate depends on the LDOS, but also provide a new way to realize ultrafast energy transfer process with ultrahigh efficiency.

physics.optics↗

Implementing Quantum Search Algorithm with Metamaterials

Metamaterials, artificially structured electromagnetic (EM) materials, have enabled the realization of many unconventional electromagnetic properties not found in nature, such as negative refractive index, magnetic response, invisibility cloaking and so on. Based on these man-made materials with novel EM properties, various devices have been designed and realized. However, quantum analog devices based on metamaterials have not been achieved so far. Here we designed and printed metamaterials to perform quantum search algorithm. The structures, comprising of an array of two-dimensional (2D) sub-wavelength air holes with different radii perforated on the dielectric layer, have been fabricated by using 3D printing technique. When an incident wave enters in the designed metamaterials, the profile of beam wavefront is processed iteratively as it propagates through the metamaterial periodically. After roundtrips, precisely the same as the efficiency of quantum search algorithm, searched items will be found with the incident wave all focusing on the marked positions. Such a metamaterial-based quantum searching simulator may lead to remarkable achievements in wave-based signal processors.

physics.optics↗

Strongly Enhanced Raman Optical Activity in Molecules by Magnetic Response of Nanoparticles

An analytical theory for the surface-enhanced Raman optical activity (SEROA) with the magnetic response of the substrate particle has been presented. We have demonstrated that the SEROA signal is proportional to the magnetic polarizability of the substrate particle, which can be significantly enhanced due to the existence of the magnetic response. At the same time, a large circular intensity difference (CID) for the SEROA can also be achieved in the presence of the magnetic response. Taking Si nanoparticles as examples, we have found that the CID enhanced by a Si nanoparticle is 10 times larger than that of Au. Furthermore, when the molecule is located in the hotspot of a Si dimer, CID can be 60 times larger. The phenomena originate from large magnetic fields concentrated near the nanoparticle and boosted magnetic dipole emission of the molecule. The symmetric breaking of the electric fields caused by the magnetic dipole response of the nanoparticle also plays an important role. Our findings provide a new way to tailor theRaman optical activity by designing metamaterials with the strong magnetic response.

physics.optics↗

Surface Enhanced Circular Dichroism of Oriented Chiral Molecules by Plasmonic Nanostructures

We present a rigorous finite element method to calculate circular dichroism (CD) in various systems consisting of nanostructures and oriented chiral molecules with electric quadrupole transitions. The interaction between oriented molecule materials, which are regarded as anisotropic chiral media, and metallic nanostructures has been investigated. Our results show that the plasmon-induced CD is sensitive to the orientations of the molecules. In many cases, the contribution of molecular electric quadrupole transitions to the total CD signal can play a key role. More interesting, we have demonstrated that both the quadrupole- and dipole-based CD signals can be improved greatly by matching the phases for the electromagnetic fields and their gradients at different regions around the nanostructures, which are occupied by the oriented chiral molecules. Different regions might produce CD of opposite sign. When integrating over regions with only one side of the proposed nanostructure, we find that the CD-peak may be nearly hundreds-fold over the case of integrating both sides. We believe that these findings would be helpful for realizing ultrasensitive probing of chiral information for oriented molecules by plasmon-based nanotechnology.

physics.optics↗

Giant chiroptical effect caused by the electric quadrupole

Recently, there is a great interest in studying ultrasensitive detection and characterization of biomolecules using plasmonic particles, because they are of considerable importance in biomedical science and pharmaceutics. So far, all the theories on plasmoninduced circular dichroism (CD) are based on the dipole approximation, the electric quadrupolar contribution is generally considered to be relatively small and neglected. Here we demonstrate that the electric quadrupolar contribution not only cannot be ignored, but also plays a key role in many cases. Particularly, for the chiral medium that possesses preferential molecular orientations and is located at the hotspot of plasmonic nanostructures, the plasmonic CD strength contributed by molecular electric quadrupoles (EQ) can be two orders of magnitude higher than that contributed by molecular electric/magnetic dipoles. Unlike the case of dipole approximation, molecular EQ associated plasmonic CD activity appears mainly at the plasmonic resonance absorptions that facilitate the optically enhanced near-field with steep electric filed gradients, and is correlated with the boosted emission rate of a molecular EQ. Based on such physical understandings, we can design nanostructures to realize giant chiroptical effect using the EQ contribution according to the requirements,2 which provide a new strategy for ultrasensitive detection and quantification of molecular chirality.

physics.optics↗

Amplification of Molecular Chiroptical Effect by Low-loss Dielectric Nanoantennas

We report here chiroptical amplification effect occurring in the hybrid systems consisting of chiral molecules and Si nanostructures. Under resonant excitation of circularly polarized light, the hybrid systems show strong CD induction signals at optical frequency, which arise from both the electric and magnetic responses of the Si nanostructures. More interestingly, the induced CD signals from Si-based dielectric nanoantennas are always larger than that from Au-based plasmonic counterparts. The related physical origin was disclosed. Furthermore, compared to the Au-based high-loss plasmonic nanoantenas, Si-based low-loss structures would generate negligible photothermal effect, which makes Si nanoantennas become an optimized candidate to amplify molecular CD signals with ultralow thermal damages. Our findings may provide a guideline for the design of novel chiral nanosensors for applications in the fields of biomedicine and pharmaceutics.

physics.optics↗