arXiv subjects

Xiangzhuo Xing

Publications and source records attributed to Xiangzhuo Xing.

At least 19 recordsLinked to original sources

arXiv2026

Observation of Magnetic-Anisotropy Crossover and High-Temperature Skyrmions in the Dirac Magnet Fe3Ge with a Distorted Kagome Lattice

Topological materials that simultaneously host robust high-temperature skyrmions and nontrivial electronic band structures have attracted tremendous interest owing to their distinctive advantages for both fundamental research and prospective technological applications. Here, we report the observation of robust skyrmions in the Dirac kagome magnet Fe3Ge, which exhibits a high Curie temperature of ~ 650 K. At room temperature, Fe3Ge shows a large intrinsic anomalous Hall conductivity of ~ 380 {\Omega}-1cm-1, originating from its nontrivial electronic band topology. Systematic magnetization measurements reveal a spin reorientation transition at ~ 375 K, indicating a crossover from easy-plane to easy-axis magnetic anisotropy. Below the spin reorientation temperature, a large topological Hall effect is observed, arising from microscopic noncoplanar spin structures. Lorentz transmission electron microscopy shows that mesoscopic skyrmions are stabilized in the easy-axis magnetic anisotropy regime and persist over an exceptionally wide temperature window of 375-650 K, far exceeding that of most previously reported skyrmion-hosting materials. These results establish Fe3Ge as a promising platform for exploring diverse topological properties, with strong potential for advancing future high-temperature spintronic applications, ranging from next-generation information storage to logic computing devices.

cond-mat.mtrl-sci↗

arXiv2026

Superconductivity in the pressure-amorphized topological insulator CrP$_4$

The interplay among superconductivity, magnetism, and nontrivial band topology represents one of the most compelling frontiers in condensed matter physics. The exploration of novel superconductivity in 3d transition-metal compounds, particularly the rare Cr-based systems containing strongly magnetic Cr ions, has long attracted attention owing to their unconventional pairing mechanisms that challenge conventional wisdom. Yet, Cr-based superconductors remain scarce, especially those possessing nontrivial topological character, underscoring the urgent need to uncover new members. Here we report the observation of superconductivity in pressure-amorphized Cr-based topological insulator CrP$_4$. Upon compression, CrP$_4$ undergoes an anomalous quantum phase transition from a metallic to a semiconducting-like state at around 15 GPa, driven by significant changes in the electronic structure. At approximately 70 GPa, re-metallization with superconductivity occurs alongside an irreversible amorphization. The superconducting transition temperature Tc increases monotonically with pressure, reaching 4.8 K at 141.3 GPa. Furthermore, theoretical calculations predict multiple topological phase transitions from a strong topological insulator to a trivial state and finally back to a strong topological state under pressure. Our study not only establishes CrP$_4$ as the first Cr-based amorphous superconductor but also opens a new paradigm for exploring superconducting and topological properties in amorphous materials.

cond-mat.supr-con↗

arXiv2026

Pressure-induced reentrant superconductivity in a misfit layered compound $\mathrm{(SnS)_{1.15}(TaS_2)}$

Misfit layered compounds are natural van der Waals heterostructures in which electronically active transition-metal dichalcogenide layers are decoupled by incommensurate blocking layers, enabling bulk realization of quasi-two-dimensional quantum states. Here we investigate the superconducting, transport,and structural properties of the misfit compound $\mathrm{(SnS)_{1.15}(TaS_2)}$ under pressures up to 150 GPa. The low-pressure superconducting phase is gradually suppressed and disappears near 14.7 GPa,accompanied by increasing residual resistance. Remarkably, a distinct superconducting phase reemerges above 80 GPa and persists to the highest pressures achieved. This reentrant superconductivity follows a pressure-induced sign reversal of the Hall coefficient near 60 GPa and a nonmonotonic evolution of the normal-state resistance, indicating an electronic reconstruction. No structural phase transition is detected over the entire pressure range. Our results demonstrate a pressure-driven electronic reconstruction leading to reentrant superconductivity in a misfit layered compound, establishing pressure as an effective route to engineer superconductivity and electronic states in natural van der Waals heterostructures.

cond-mat.supr-con↗

arXiv2026

Weakly anisotropic superconductivity of Pr4Ni3O10 single crystals

Since the discovery of high-temperature superconductivity, studying the upper critical field and its anisotropy has been crucial for understanding superconducting mechanism and guiding applications. Here we perform in situ high-pressure angular-dependent electrical transport measurements on Pr4Ni3O10 single crystals using a custom diamond anvil cell (DAC) rotator and confirming its anisotropic superconductivity. The anisotropy parameter is approximately 1.6, decreasing with increasing temperature and approaches 1 near Tc. Comparing effective mass anisotropy and inter-block distance in cuprates and iron-based superconductors (FeSCs) reveals that Pr4Ni3O10 single crystals superconductors are consistent with a two-band model, where intralayer quantum confinement within the unit cell induces interlayer coherence, thereby leading to three-dimensional (3D) superconductivity. This study not only establishes the existence of anisotropic superconductivity in bulk Ruddlesden-Popper nickelates, but also provide critical insight into the role of dimensionality in high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2025

Boost of critical current density near quantum critical points in FeSe-Based superconductors with two superconducting domes

Recent studies have identified two superconducting domes in FeSe-based superconductors. It was discovered that each dome is accompanied by a distinct nematic quantum critical point (QCP): one associated with a pure nematic QCP, and the other with a nematic QCP entangled with antiferromagnetism (AFM). In this study, we delve into the evolution of the critical current density ($J_{\rm{c}}$) with doping in FeSe${_{1-x}}$(Te/S)${_{x}}$ single crystals, focusing on the behavior within the two superconducting domes. Surprisingly, three maxima of $J_{\rm{c}}$ were found in the two superconducting domes, with two sharp peaks in $J_{\rm{c}}$ observed precisely at the endpoints of the nematic phases, at $x$(Te) $\sim$ 0.5 for Te-doped and $x$(S) $\sim$ 0.17 for S-doped FeSe. The mechanisms of vortex pinning and the influence of quantum critical fluctuations have been extensively explored, emphasizing the contribution of quantum critical fluctuations in modulating $J_{\rm{c}}$. Additionally, an increase in $J_{\rm{c}}$ was also noted near FeSe$_{0.1}$Te$_{0.9}$, where its origin has been explored and discussed. This finding provides crucial clues about the existence of an ordered phase endpoint beneath the superconducting dome, offering an initial basis for further investigation into the potential presence of a QCP beneath it.

cond-mat.supr-con↗

arXiv2025

Diamond quantum sensing at record high pressure up to 240 GPa

Quantum sensing utilizing nitrogen-vacancy (NV) centers in diamond has emerged as a transformative technology for probing magnetic phase transition1-4, evidencing Meissner effect of superconductors1,5-9, and visualizing stress distribution3,9 under extreme conditions. Recent development in NV configurations and hydrostatic environments have raised the operational pressures of NV centers to 140 GPa2,6,10,11, but substantial challenges remain in extending sensing capabilities into multi-megabar range, critical for research in hydrogen-rich superconductors like La-Sc-H ($T_{\text{c}}$ of 271-298 K at 195-266 GPa)12 and evolution of minerals near Earth's core13. Here we report the fabrication of shallow NV centers through ion implantation followed by high-pressure and high-temperature (HPHT) annealing, leading to increased density, improved coherence, and mitigated internal stresses, a pre-requisite for reducing their degradation under compression. This NV magnetometry enable breakthrough of pressure capabilities exceeding 240 GPa, constrained by structural integrity of the 50 um diamond anvils, suggesting that the untapped pressure limit may enable further advancements with smaller cutlets or more robust diamonds. We present compelling evidence of the Meissner effect and trapped flux at record-high pressure of 180 GPa for superconducting transition in elemental titanium (Ti) as benchmark, establishing a solid foundation for high-pressure magnetometry in exploring complex quantum phenomena at previously unreachable pressures.

quant-ph↗

arXiv2025

In-Plane Magnetic Anisotropy and Large topological Hall Effect in Self-Intercalated Ferromagnet Cr1.61Te2

Self-intercalated chromium tellurides Cr1+xTe2 have garnered growing attention due to their high-temperature ferromagnetism, tunable spin structures and air stability, all of which are vital for versatile applications in next-generation memory and information technology. Here, we report strong magnetic anisotropy and a large topological Hall effect (THE) in self-intercalated Cr1.61Te2 single crystals, which are both highly desirable properties for future spintronic applications. Our results demonstrate that Cr1.61Te2 is a soft ferromagnet with strong in-plane magnetic anisotropy. Remarkably, distinct THE behaviors are observed in different temperature regimes, reflecting the intricate spin structures and competing exchange interactions. More interestingly, a large topological Hall resistivity, induced by microscopic non-coplanar spin structures, emerges in the temperature range 70-240 K, reaching a maximum value of 0.93 μΩ cm at 150 K. Moreover, a sign-reversed and weak THE is observed at low temperatures below ~70 K, indicating the emergence of an additional topological spin structure with opposite topological charges. This work not only offers valuable insights into the correlation between magnetocrystalline anisotropy and topological phenomena in Cr1+xTe2 systems, but also provides a robust platform for engineering the evolution of complex spin textures that can be leveraged in diverse spintronic device applications.

cond-mat.mtrl-sci↗

arXiv2025

Pressure-driven superconductivity in the topological insulator GeBi4Te7

The van der Waals, pseudo-binary chalcogenides (ACh)m(Pn2Ch3)n (A = Ge, Mn, Pb, etc.; Pn = Sb or Bi; Ch = Te, Se) have recently been reported to host a vast landscape of topological phases of matter, including the quantum anomalous Hall state and topological axion state with quantized magnetoelectric effect. A subgroup in this series, like MnSb4Te7 and GeSb4Te7, can be driven to a superconducting state by applying a physical pressure, making them viable candidates to realize so-called topological superconductivity. However, the role of magnetic fluctuations in this pressure-induced superconductivity remains unclear. Here, we report the pressure-induced multiple superconducting phases in the nonmagnetic GeBi4Te7, accompanied by corresponding structural transitions evidenced from the high-pressure Raman scattering. In comparison with other members in this family, we find the superconducting transition temperature of the nonmagnetic subgroup is significantly higher than their magnetic homologues, possibly hinting at the detrimental role played by the magnetic fluctuations in the superconductivity formation, at least in this pseudo-binary chalcogenide family.

cond-mat.supr-con↗

arXiv2025

Abnormal Normal State and Pressure-driven Reentrant Superconductivity in the Heavy $d$-electron Superconductor Rh$_{17}$S$_{15}$

Superconductivity beyond the conventional Bardeen-Cooper-Schrieffer (BCS) framework often emerges out of a normal state that is accompanied by exotic magnetism and thereby displays many exceptional transport and thermodynamic properties. Here we report that the normal state of the heavy $d$-electron superconductor Rh$_{17}$S$_{15}$ is characterized by a weak \textit{ferromagnetism} that persists up to room temperature. We show that the broad hump in its resistivity likely results from the Kondo interaction of the conduction electrons with this novel magnetism. By applying pressure, superconductivity is fully suppressed first. In the high-pressure regime, however, we observe a second dome of superconductivity with its maximum $T_c$ greater than the ambient pressure value, highlighting the possible \textit{unconventional} superconductivity in this heavy $d$-electron sulfide.

cond-mat.supr-con↗

arXiv2025

Critical Current Density and AC Magnetic Susceptibility of High-quality FeTe$_{0.5}$Se$_{0.5}$ Superconducting Tapes

Iron telluride-selenium superconducting materials, known for their non-toxicity, ease of preparation, simple structure, and high upper critical fields, have attracted much research interest in practical application. In this work, we conducted electrical transport measurements, magneto-optical imaging, and AC magnetic susceptibility measurements on FeTe$_{0.5}$Se$_{0.5}$ superconducting long tapes fabricated via reel-to-reel pulsed laser deposition. Our transport measurements revealed a high critical current density that remains relatively stable even with increasing external magnetic fields, reaching over $1\times 10^5$ A/cm$^2$ at 8 K and 9 T. The calculated pinning force density indicates that normal point pinning is the primary mechanism in these tapes. The magneto-optical images demonstrated that the tapes show homogeneous superconductivity and uniform distribution of critical current density. The AC magnetic susceptibility measurements also confirmed their strong flux pinning nature of withstanding high magnetic field. Based on these characteristics, FeTe$_{0.5}$Se$_{0.5}$ superconducting tapes show promising prospects for applications under high magnetic fields.

cond-mat.supr-con↗

arXiv2024

Bulk and surface Dirac states accompanied by two superconducting domes in FeSe-based superconductors

Recent investigations of FeSe-based superconductors have revealed the presence of two superconducting domes, and suggest possible distinct pairing mechanisms. Two superconducting domes are commonly found in unconventional superconductors and exhibit unique normal states and electronic structures. In this study, we conducted electromagnetic transport measurements to establish a complete phase diagram, successfully observing the two superconducting domes in FeSe$_{1-x}$S$_x$ (0 $\le x \le$ 0.25) and FeSe$_{1-x}$Te$_x$ (0 $\le x \le$ 1) superconductors. The normal state resistivity on SC1 shows the strange metal state, with a power exponent approximately equal to 1 ($ρ(T)\propto T^n$ with $n\sim 1$), whereas the exponent on SC2 is less than 1. A bulk Dirac state observed on SC1, completely synchronized with the strange metal behavior, indicating a close relationship between them. While a topological surface Dirac state is witnessed on SC2, and undergoes a sign change near the pure nematic quantum critical point. The evolution of the Dirac states indicates that the appearance of the two superconducting domes may originate from the Fermi surface reconstruction. Our findings highlight distinct Dirac states and normal state resistivity across the two superconducting domes, providing convincing evidence for the existence of the two different pairing mechanisms in FeSe-based superconductors.

cond-mat.supr-con↗

arXiv2024

Unusually weak irradiation effects in anisotropic iron-based superconductor RbCa2Fe4As4F2

We report on the effects of 3.5 MeV proton irradiation in RbCa$_2$Fe$_4$As$_4$F$_2$, an iron-based superconductor with unusual properties in between those of the pnictides and of the cuprate high-temperature superconductors. We studied how structural disorder introduced by ion bombardment affects the critical temperature, superfluid density and gap values by combining a coplanar waveguide resonator technique, electric transport measurements and point-contact Andreev-reflection spectroscopy. We find an unusually weak dependence of the superconducting properties on the amount of disorder in this material when compared to other iron-based superconductors under comparable irradiation conditions. The nodal multigap state exhibited by pristine RbCa$_2$Fe$_4$As$_4$F$_2$ is also robust against proton irradiation, with a two-band $d-d$ model being the one that best fits the experimental data.

cond-mat.supr-con↗

arXiv2023

Observation of non-superconducting phase changes in LuH$_{2\pm\text{x}}$N$_y$

The recent report of near-ambient superconductivity in nitrogen doped lutetium hydride has triggered a worldwide fanaticism and raised major questions about the latest claims. An intriguing phenomenon of color changes in pressurized samples from blue to pink to red was observed and correlated with the claimed superconducting transition, but the origin and underlying physics of these color changes have yet to be elucidated. Here we report synthesis and characterization of high-purity nitrogen doped lutetium hydride LuH$_{2\pm\text{x}}$N$_y$ with the same structure and composition as in the main phase of near-ambient superconductor1. We find a new purple phase of LuH$_{2\pm\text{x}}$N$_y$ between blue and pink phase, and reveal that the sample color changes likely stem from pressure-driven redistribution of nitrogen and its interaction with the LuH$_2$ framework. No superconducting transition is found in all blue, purple, pink and red phases at temperatures 1.8-300 K and pressures 0-30 GPa. Instead, we identify a notable temperature-induced resistance anomaly of structural and/or electronic origin in LuH$_{2\pm\text{x}}$N$_y$, which is most pronounced in the pink phase and may have been erroneously interpreted as a sign of superconducting transition. This work establishes key benchmarks for nitrogen doped lutetium hydrides, allowing an in-depth understanding of the novel pressure-induced phase changes.

cond-mat.supr-con↗

arXiv2023

Anomalous second magnetization peak in 12442-type RbCa$_2$Fe$_4$As$_4$F$_2$ superconductors

The second magnetization peak (SMP) appears in most superconductors and is crucial for the understanding of vortex physics as well as the application. Although it is well known that the SMP is related to the type and quantity of disorder/defects, the mechanism has not been universally understood. In this work, we selected three stoichiometric superconducting RbCa$_2$Fe$_4$As$_4$F$_2$ single crystals with identical superconducting critical temperature $T_c$ $\sim$ 31 K and similar self-field critical current density $J_c$, but with different amounts of disorder/defects, to study the SMP effect. It is found that only the sample S2 with a moderate disorder/defects shows a significant SMP effect. The evolution of the normalized pinning force density $f_p$ demonstrates that the dominant pinning mechanism changes from weak pinning at low temperatures to strong pinning at high temperatures. The microstructure study for sample S2 reveals some expanded Ca$_2$F$_2$ layers and dislocation defects in RbFe$_2$As$_2$ layers. The normalized magnetic relaxation results indicate that the SMP is strongly associated with the elastic to plastic (E-P) vortex transition. As temperature increases, the SMP gradually evolves into a step-like shape and then becomes a sharp peak near the irreversibility field similar to what is usually observed in low-temperature superconductors. Our findings connect the low field SMP of high-temperature superconductors and the high field peak of low-temperature superconductors, revealing the possible universal origin related to the E-P phase transition.

cond-mat.supr-con↗

arXiv2023

Significant enhancement of critical current density in H+-intercalated FeSe single crystal

Superconducting transition temperature (Tc) and critical current density (Jc) are two key factors that are not only crucial for probing high-temperature superconducting mechanisms, but also for practical applications. The simple crystal structure of FeSe is very favorable for the fabrication of thin films and wires, but its application is limited by the relatively low Tc and small Jc. A previous study has found that the Tc of FeSe can be significantly enhanced over 40 K by using the protonation method. Here, we present a systematic study of Jc and vortex properties of H+-intercalated FeSe (Hx-FeSe) single crystals. The value of Jc for Hx-FeSe single crystal is significantly enhanced, exceeding 1.3*10^6 A/cm2 at 4 K, which is more than two orders of magnitude larger than 1.1*10^4 A/cm2 of pristine FeSe. The vortex pinning mechanism of Hx-FeSe is found to be surface pinning, which is different from the dominant strong point-like pinning in pristine FeSe. Moreover, the systematic study of the vortex phase transition and the underlying mechanism provides a wealth of information for the vortex phase diagram of Hx-FeSe single crystal. Our results confirm that the introduction of H+ intercalations into FeSe not only enhances the Tc, but also significantly increases the value of Jc, which is favorable for practical applications.

cond-mat.supr-con↗

arXiv2022

Nodal multigap superconductivity in the anisotropic iron-based compound RbCa2Fe4As4F2

The 12442 compounds are a recently discovered family of iron-based superconductors, that share several features with the cuprates due to their strongly anisotropic structure, but are so far poorly understood. Here, we report on the gap structure and anisotropy of RbCa2(Fe1-xNix)4As4F2 single crystals, investigated by a combination of directional point-contact Andreev-reflection spectroscopy and coplanar waveguide resonator measurements. Two gaps were identified, with clear signatures of d-wave-like nodal structures which persist upon Ni doping, well described by a two-band d-d state with symmetry-imposed nodes. A large London penetration depth anisotropy was revealed, weakly dependent on temperature and fully compatible with the d-d model.

cond-mat.supr-con↗

arXiv2021

Protonation-induced discrete superconducting phases in bulk FeSe single crystals

The superconducting transition temperature, $T_{\rm{c}}$, of FeSe can be significantly enhanced several-fold by applying pressure, electron doping, intercalating spacing layer, and reducing dimensionality. Various ordered electronic phases, such as nematicity and spin density waves, have also been observed accompanying high-$T_{\rm{c}}$ superconductivity. Investigation on the evolution of the electronic structure with $T_{\rm{c}}$ is essential to understanding electronic behavior and high-$T_{\rm{c}}$ superconductivity in FeSe and its derived superconductors. In this report, we have found a series of discrete superconducting phases, with a maximum $T_{\rm{c}}$ up to 44 K, in H$^+$-intercalated FeSe single crystals using an ionic liquid gating method. Accompanied with the increase of $T_{\rm{c}}$, suppression of the nematic phase and evolution from non-Fermi-liquid to Fermi-liquid behavior was observed. An abrupt change in the Fermi surface topology was proposed to explain the discrete superconducting phases. A band structure that favors the high-$T_{\rm{c}}$ superconducting phase was also revealed.

cond-mat.supr-con↗

arXiv2021

Disorder-robust high-field superconducting phase of FeSe single crystals

When exposed to high magnetic fields, certain materials manifest an exotic superconducting (SC) phase that has attracted considerable attention. A proposed explanation for the origin of the high-field SC phase is the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. This state is characterized by inhomogeneous superconductivity, where the Cooper pairs have finite center-of-mass momenta. Recently, the high-field SC phase was observed in FeSe, and it was deemed to originate from the FFLO state. Here, we synthesize FeSe single crystals with different levels of disorder. The level of disorder is expressed by the ratio of the mean free path to the coherence length and ranges between 35 and 1.2. The upper critical field \textit{B}$_{\rm{c}2}$ was obtained by both resistivity and magnetic torque measurements over a wide range of temperatures, which went as low as $\sim$0.5 K, and magnetic fields, which went up to $\sim$38 T along the \textit{c} axis and in the \textit{ab} plane. In the high-field region parallel to the \textit{ab} plane, an unusual SC phase was confirmed in all the crystals, and the phase was found to be robust against disorder. This result suggests that the high-field SC phase in FeSe is not a conventional FFLO state.

cond-mat.supr-con↗