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Xiangzhuo Xing

Publications and source records attributed to Xiangzhuo Xing.

25 records · Page 2Linked to original sources

Disorder-robust high-field superconducting phase of FeSe single crystals

When exposed to high magnetic fields, certain materials manifest an exotic superconducting (SC) phase that has attracted considerable attention. A proposed explanation for the origin of the high-field SC phase is the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state. This state is characterized by inhomogeneous superconductivity, where the Cooper pairs have finite center-of-mass momenta. Recently, the high-field SC phase was observed in FeSe, and it was deemed to originate from the FFLO state. Here, we synthesize FeSe single crystals with different levels of disorder. The level of disorder is expressed by the ratio of the mean free path to the coherence length and ranges between 35 and 1.2. The upper critical field \textit{B}$_{\rm{c}2}$ was obtained by both resistivity and magnetic torque measurements over a wide range of temperatures, which went as low as $\sim$0.5 K, and magnetic fields, which went up to $\sim$38 T along the \textit{c} axis and in the \textit{ab} plane. In the high-field region parallel to the \textit{ab} plane, an unusual SC phase was confirmed in all the crystals, and the phase was found to be robust against disorder. This result suggests that the high-field SC phase in FeSe is not a conventional FFLO state.

cond-mat.supr-con↗

Comparative study of superconducting and normal-state anisotropy in Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ superconductors with controlled amounts of interstitial excess Fe

We report a systematic study of the superconducting (SC) and normal-state anisotropy of Fe$_{1+y}$Te$_{0.6}$Se$_{0.4}$ single crystals with controlled amounts of excess Fe ($y$ = 0, 0.07, and 0.14). The SC state anisotropy $γ_{H}$ was obtained by measuring the upper critical fields under high magnetic fields over 50 T for both $H\parallel ab$ and $H\parallel c$. On the other hand, the normal state anisotropy $γ_ρ$ was obtained by measuring the resistivity with current flowing in the $ab$ plane ($ρ_{ab}$) and along the $c$ axis ($ρ_c$). To precisely measure $ρ_{ab}$ and $ρ_c$ in the same part of a specimen avoiding the variation dependent on pieces or parts, we adopt a new method using a micro-fabricated bridge with an additional neck part along $c$ axis. The $γ_{H}$ decreases from a value dependent on the amount of excess Fe at $T_{\rm{c}}$ to a common value $\sim$ 1 at 2 K. The different $γ_{H}$ at $T_{\rm{c}}$ ($\sim$1.5 for $y$ = 0, and 2.5 for $y$ = 0.14) suggests that the anisotropy of effective mass $m_c^*/m_{ab}^*$ increases from $\sim$ 2.25 ($y$ = 0) to 6.25 ($y$ = 0.14) with the excess Fe. The almost isotropic $γ_{H}$ at low temperatures is due to the strong spin paramagnetic effect at $H\parallel ab$. By contrast, the $γ_ρ$ shows a much larger value of $\sim$ 17 ($y$ = 0) to $\sim$ 50 ($y$ = 0.14) at the temperature just above $T_{\rm{c}}$. Combined the results of $γ_{H}$ and $γ_ρ$ near $T_{\rm{c}}$, we found out that the discrepant anisotropies between the SC and normal states originates from a large anisotropy of scattering time $τ_{ab}$/$τ_c$ $\sim$ 7.8. The $τ_{ab}$/$τ_c$ is found to be independent of the excess Fe.

cond-mat.supr-con↗

Electronic transport properties and hydrostatic pressure effect of FeSe$_{0.67}$Te$_{0.33}$ single crystals free of phase separation

FeSe$_{1-x}$Te$_{x}$ superconductors manifest some intriguing electronic properties depending on the value of $x$. In FeSe single crystal, the nematic phase and Dirac band structure have been observed, while topological surface superconductivity with the Majorana bound state was found in the crystal of $x \sim 0.55$. Therefore, the electronic properties of single crystals with $0 < x \leq 0.5$ are crucial for probing the evolution of those intriguing properties as well as their relations. However, this study is still left blank due to the lack of single crystals because of phase separation. Here, we report the synthesis, magnetization, electronic transport properties, and hydrostatic pressure effect of FeSe$_{0.67}$Te$_{0.33}$ single crystals free of phase separation. A structural (nematic) transition is visible at $T_{s} = 39$ K, below which the resistivity exhibits a Fermi-liquid behavior. Analysis of upper critical fields suggests that spin-paramagnetic effect should be taken into account for both $H \parallel c$ axis and $H \parallel ab$ plane. A crossover from the low-$H$ quadratic to the high-$H$ quasi-linear behavior is observed in the magnetoresistance, signifying the possible existence of Dirac-cone state. Besides, the strong temperature dependence of Hall coefficient, violation of (modified) Kohler's rule, and two-band model analysis indicate the multiband effects in FeSe$_{0.67}$Te$_{0.33}$ single crystals. Hydrostatic pressure measurements reveal that $T_{s}$ is quickly suppressed with pressure while $T_{c}$ is monotonically increased up to 2.31 GPa, indicating the competition between nematicity and superconductivity. No signature of magnetic order that has been detected in FeSe$_{1-x}$S$_{x}$ is observed. Our findings fill up the blank of the knowledge on the basic properties of FeSe$_{1-x}$Te$_{x}$ system with low-Te concentrations.

cond-mat.supr-con↗

Hydrothermal synthesis and complete phase diagram of FeSe$_{1-x}$S$_{x}$ $(0 \leq x \leq 1)$ single crystals

We report the successful synthesis of FeSe$_{1-x}$S$_{x}$ single crystals with $x$ ranging from 0 to 1 via a hydrothermal method. A complete phase diagram of FeSe$_{1-x}$S$_{x}$ has been obtained based on resistivity and magnetization measurements. The nematicity is suppressed with increasing $x$, and a small superconducting dome appears within the nematic phase. Outside the nematic phase, the superconductivity is continuously suppressed and reaches a minimum $T_c$ at $x$ = 0.45; beyond this point, $T_c$ slowly increases until $x$ = 1. Intriguingly, an anomalous resistivity upturn with a characteristic temperature $T^*$ in the intermediate region of $0.31 \leq x \leq 0.71$ is observed. $T^{*}$ shows a dome-like behavior with a maximum value at $x$ = 0.45, which is opposite the evolution of $T_c$, indicating competition between $T^*$ and superconductivity. The origin of $T^*$ is discussed in detail. Furthermore, the normal state resistivity evolves from non-Fermi-liquid to Fermi-liquid behavior with S doping at low temperatures, accompanied by a reduction in electronic correlations. Our study addresses the lack of single crystals in the high-S doping region and provides a complete phase diagram, which will promote the study of relations among nematicity, superconductivity, and magnetism.

cond-mat.supr-con↗

Fully gapped superconductivity without sign reversal in the topological superconductor PbTaSe$_2$

We investigate the superconducting gap function of topological superconductor PbTaSe$_2$. Temperature, magnetic field, and three-dimensional (3D) field-angle dependences of the specific heat prove that the superconductivity of PbTaSe$_2$ is fully-gapped, with two isotropic $s$-wave gaps. The pair-breaking effect is probed by systematically increasing non-magnetic disorders through H$^+$-irradiations. The superconducting transition temperature, $T_{\rm{c}}$, is found to be robust against disorders, which suggests that the pairing should be sign-preserved rather than sign-reversed.

cond-mat.supr-con↗

Anisotropic Ginzburg-Landau scaling of Hc2 and transport properties of 112-type Ca0.8La0.2Fe0.98Co0.02As2 single crystal

High-quality single crystal of Ca0.8La0.2Fe0.98Co0.02As2 has been successfully synthesized using a self-flux method. The magnetization measurement reveals a second peak effect and high critical current density exceeding 2*10^6 A/cm2 at 5 K(self-field). The upper critical field anisotropy was systematically studied by measuring the electrical resistivity under various magnetic fields and angles. The angle dependent magnetoresistance, by choosing an appropriate anisotropy parameter within the framework of the anisotropic Ginzburg Landau (AGL) theory, can be scaled onto one single curve. In the normal state, the negative Hall coefficient shows strong but nonmonotonic T-dependence through a minimum at 175 K. Moreover, it is shown that the magnetoresistance apparently violates the semiclassical Kohler's rule below 175 K but can be well scaled by the Hall angle instead. This suggests either the change of carriers with T or the exotic anisotropic scattering in the system.

cond-mat.supr-con↗

Anisotropic Superconductivity of Ca1-xLaxFeAs2 (x ~ 0.18) Single Crystal

Anisotropic superconducting properties including the upper critical field Hc2, thermal activation energy U0, and critical current density Jc are systematically studied in a large Ca1-xLaxFeAs2 single crystal (x ~ 0.18). The obtained Hc2 bears a moderate anisotropy gamma of approximately 2-4.2, located between those of '122' Ba1-xKxFe2As2 (1 < gamma < 2) and '1111' NdFeAsO1-xFx (5 < gamma < 9.2). Both the magnitude of U0 and its field dependence are very similar to those of NdFeAsO1-xFx, also indicating anisotropic superconductivity. Moreover, high and anisotropic Jc's exceeding 10^5 A/cm2 have been calculated from the magnetization hysteresis loops, indicating the existence of strong bulk-dominated pinning in the present superconducting material.

cond-mat.supr-con↗