arXiv subjects

Xiaoli Dong

Publications and source records attributed to Xiaoli Dong.

At least 19 recordsLinked to original sources

arXiv2026

Decoupled domain-texture switching from magnetic easy axis in kagome ferromagnet EuTi3Bi4

Magnetic anisotropy defines the easy axis of a magnetic material and governs the spatial arrangement of its domains. To date, anisotropy engineering has focused on reorienting the easy axis or tuning the anisotropy energy, both of which demand substantial energy input. Here, we demonstrate that magnetic domain textures can be switched without reorienting the easy axis, as observed in a kagome ferromagnet EuTi3Bi4 crystal. Using low-temperature magnetic force microscopy, we observe that the preferred orientation of magnetic domains switches from the a-axis to the b-axis upon temperature variation, and that this switching can also be triggered by an out-of-plane magnetic-field reset. Magnetization measurements and density functional theory calculations confirm a robust c-axis easy magnetization, ruling out a conventional spin-reorientation transition. Instead, the texture switching is governed by the temperature dependence of the in-plane variation of the Magnetic anisotropy energy landscape, which arises from two competing interactions with different decay rates: single-ion anisotropy favors a-oriented spin components, while nearest-neighbor anisotropic exchange favors b-oriented ones. Furthermore, the critical switching temperature is substantially elevated in a mechanically exfoliated EuTi3Bi4 flake. Our findings establish that macroscopic magnetic textures can be effectively manipulated by tuning the competition between in-plane anisotropic interactions, without the energy cost of reorienting the easy axis.

cond-mat.mtrl-sci↗

arXiv2026

Tunable bifurcation of magnetic anisotropy and bi-oriented antiferromagnetic order in kagome metal GdTi3Bi4

The novel kagome family RTi3Bi4 (R: rare-earth) offers a unique platform for exploring distinctive physical phenomena such as anisotropy, spin density wave, and anomalous Hall effect. In particular, the magnetic frustration and behavior of magnetic anisotropy in antiferromagnetic (AFM) kagome materials are of great interest for the fundamental studies and hold promise for next-generation device applications. Here, we report a tunable bifurcation of magnetic anisotropic and bi-oriented AFM order observed in the quasi-1D kagome antiferromagnet GdTi3Bi4. The magnetic domain evolutions during two plateau transition processes are directly visualized, unveiling a pronounced in-plane anisotropy along the a-axis. Temperature-dependent characterization reveals a bifurcation transition of anisotropy at approximately 2 K, where the a-axis anisotropy splits into two special orientations, revealing a hidden bi-oriented in-plane AFM order deviating from the high-symmetry direction by 7 degree. More intriguingly, the characteristics of the bifurcated anisotropy are clearly illustrated through vector magnetic field modulation, revealing three distinct in-plane domain phases in the transverse magnetic field phase diagram. Our results not only provide valuable insights into the tunable bifurcation of magnetic anisotropic in GdTi3Bi4, but also pave a novel pathway for AFM spintronics development.

cond-mat.str-el↗

arXiv2026

Cs$_4$Cr$_7$Te$_{10}$: Interwoven Reconstructed Archimedean and Kagome Lattices with a Possible Phase Transition near 130 K

Chromium-based materials with complex lattice geometries provide an important platform for investigating correlated electronic and magnetic states. However, Cr-based compounds with unusual crystal geometries are still rarely reported. Here, we report a new Cr-based compound, Cs$_4$Cr$_7$Te$_{10}$, featuring interwoven Cr and Te sublattices that can be viewed as reconstructed networks derived from Archimedean (3.4.6.4) tiling and the kagome lattice, respectively. Transport measurements reveal the semiconducting nature in Cs$_4$Cr$_7$Te$_{10}$. Magnetization measurements show a weak anisotropy between H//b and H//ac planes, and uncover an anomaly near 130 K that is insensitive to the applied magnetic fields. Specific-heat measurements further confirm this transition, indicating its bulk thermodynamic nature. The associated entropy change is as small as 0.41 J mol^-1 K^-1, ruling out a structural phase transition and pointing to a possible electronic and/or magnetic phase transition. These results provide a new route for designing complex crystal geometries and exploring their associated emergent phenomena.

cond-mat.mtrl-sci↗

arXiv2025

Prevailing orbital excitations in paramagnetic kagome superconductor Cs(V$_{0.95}$Ti$_{0.05}$)$_3$Sb$_5$

Using the muon as a sensitive local magnetic probe, we investigated the layered kagome superconductor Cs(V$_{0.95}$Ti$_{0.05}$)$_3$Sb$_5$, a material notably devoid of both static magnetic moments and long-range charge order. Our transverse-field $\mu$SR measurements reveal that the local magnetic susceptibility, obtained via the muon Knight shift, is dominated by orbital excitations with a split energy levels around 20 meV. Meanwhile, the persistence of itinerant electron paramagnetism down to 5 K and 7 T confirms the absence of static magnetism within this regime. In addition, zero-field (ZF) $\mu$SR experiments detect a significant increase in the inhomogeneous nuclear dipolar field distribution below a featured temperature at 70 K. We attribute this ZF-$\mu$SR feature to the emergence of local lattice distortions at low temperatures, potentially arising from orbital ordering. Significantly, our study establishes that orbital excitations constitute an intrinsic property of the layered V-Sb kagome lattice. Despite its small magnitude, spin-orbit coupling plays a crucial role in governing the lattice dynamics, potentially driving the emergence of novel phenomena such as phonon carrying angular momentum in crystals with non-chiral point groups.

cond-mat.str-el↗

arXiv2025

Extracting intrinsic superconducting properties in intercalated layered superconductors using an extended 2D Tinkham model

Bulk two dimensional (2D) superconductivity has gained considerable attention due to its intricate interplay between symmetry breaking, nontrivial topology, 2D phase fluctuations, and unconventional superconductivity. However, certain intercalated layered superconductors, despite their short c-axis superconducting coherence length, have been misclassified as anisotropic three-dimensional (3D) superconductors. Here, we investigate (Li,Fe)OHFeSe superconductors with varying degrees of interlayer misalignment, revealing sample-dependent superconducting dimensionality while consistently observing Berezinskii Kosterlitz Thouless (BKT) transitions. To resolve this discrepancy, we develop an extended 2D Tinkham model that quantitatively captures the blurring effects induced by interlayer misalignment. We further demonstrate the validity of this model in both (Li,Fe)OHFeSe and cetyltrimethyl ammonium (CTA+) intercalated (CTA)0.5SnSe2 superconductors, highlighting its broad applicability. This work provides valuable insights into bulk 2D superconductivity and establishes an extended 2D Tinkham model for quantitatively extracting intrinsic superconducting properties in intercalated layered superconductors, particularly those exhibiting significant interlayer misalignments.

cond-mat.supr-con↗

arXiv2025

Absence of diode effect in chiral type-I superconductor NbGe2

Symmetry elegantly governs the fundamental properties and derived functionalities of condensed matter. For instance, realizing the superconducting diode effect (SDE) demands breaking space-inversion and time-reversal symmetries simultaneously. Although the SDE is widely observed in various platforms, its underlying mechanism remains debated, particularly regarding the role of vortices. Here, we systematically investigate the nonreciprocal transport in the chiral type-I superconductor NbGe2. Moreover, we induce type-II superconductivity with elevated superconducting critical temperature on the artificial surface by focused ion beam irradiation, enabling control over vortex dynamics in NbGe2 devices. Strikingly, we observe negligible diode efficiency (Q < 2%) at low magnetic fields, which rises significantly to Q ~ 50% at high magnetic fields, coinciding with an abrupt increase in vortex creep rate when the superconductivity of NbGe2 bulk is suppressed. These results unambiguously highlight the critical role of vortex dynamics in the SDE, in addition to the established symmetry rules.

cond-mat.supr-con↗

arXiv2024

Bulk high-temperature superconductivity in the high-pressure tetragonal phase of bilayer La2PrNi2O7

The Ruddlesden-Popper (R-P) bilayer nickelate, La3Ni2O7, was recently found to show signatures of high-temperature superconductivity (HTSC) at pressures above 14 GPa. Subsequent investigations achieved zero resistance in single- and poly-crystalline samples under hydrostatic pressure conditions. Yet, obvious diamagnetic signals, the other hallmark of superconductors, are still lacking owing to the filamentary nature with low superconducting volume fraction. The presence of a novel "1313" polymorph and competing R-P phases obscured proper identification of the phase for HTSC. Thus, achieving bulk HTSC and identifying the phase at play are the most prominent tasks at present. Here, we address these issues in the praseodymium (Pr)-doped La2PrNi2O7 polycrystalline samples. We find that the substitutions of Pr for La effectively inhibits the intergrowth of different R-P phases, resulting in nearly pure bilayer structure. For La2PrNi2O7, pressure-induced orthorhombic-to-tetragonal structural transition takes place at Pc ~ 11 GPa, above which HTSC emerges gradually upon further compression. The superconducting transition temperatures at 18-20 GPa reach Tconset = 82.5 K and Tczero = 60 K, which are the highest values among known nickelate superconductors. More importantly, bulk HTSC was testified by detecting clear diamagnetic signals below ~75 K corresponding to an estimated superconducting volume fraction ~ 57(5)% at 20 GPa. Our results not only resolve the existing controversies but also illuminate directions for exploring bulk HTSC in the bilayer nickelates.

cond-mat.supr-con↗

arXiv2024

Quantum Oscillations in kagome metals CsTi3Bi5 and RbTi3Bi5

We report quantum oscillation measurements on the kagome compounds ATi$_3$Bi$_5$ (A=Rb, Cs) in magnetic fields up to 41.5 T and temperatures down to 350 mK. In addition to the frequencies observed in previous studies, we have observed multiple unreported frequencies above 2000 T in CsTi$_3$Bi$_5$ using a tunnel diode oscillator technique. We compare these results against density functional theory calculations and find good agreement with the calculations in the number of peaks observed, frequency, and the dimensionality of the Fermi surface. For RbTi$_3$Bi$_5$ we have obtained a different quantum oscillation spectrum, although calculated quantum oscillation frequencies for the Rb compound are remarkably similar to the Cs compound, calling for further studies.

cond-mat.str-el↗

arXiv2024

A Novel Paradigm for Neural Computation: X-Net with Learnable Neurons and Adaptable Structure

Multilayer perception (MLP) has permeated various disciplinary domains, ranging from bioinformatics to financial analytics, where their application has become an indispensable facet of contemporary scientific research endeavors. However, MLP has obvious drawbacks. 1), The type of activation function is single and relatively fixed, which leads to poor `representation ability' of the network, and it is often to solve simple problems with complex networks; 2), the network structure is not adaptive, it is easy to cause network structure redundant or insufficient. In this work, we propose a novel neural network paradigm X-Net promising to replace MLPs. X-Net can dynamically learn activation functions individually based on derivative information during training to improve the network's representational ability for specific tasks. At the same time, X-Net can precisely adjust the network structure at the neuron level to accommodate tasks of varying complexity and reduce computational costs. We show that X-Net outperforms MLPs in terms of representational capability. X-Net can achieve comparable or even better performance than MLP with much smaller parameters on regression and classification tasks. Specifically, in terms of the number of parameters, X-Net is only 3% of MLP on average and only 1.1% under some tasks. We also demonstrate X-Net's ability to perform scientific discovery on data from various disciplines such as energy, environment, and aerospace, where X-Net is shown to help scientists discover new laws of mathematics or physics.

cs.AI↗

arXiv2023

Observation of high-temperature superconductivity in the high-pressure tetragonal phase of La2PrNi2O7-δ

The recent discovery of high-temperature superconductivity in the Ruddlesden-Popper phase La3Ni2O7 under high pressure marks a significant breakthrough in the field of 3d transition-metal oxide superconductors. For an emerging novel class of high-Tc superconductors, it is crucial to find more analogous superconducting materials with a dedicated effort toward broadening the scope of nickelate superconductors. Here, we report on the observation of high-Tc superconductivity in the high-pressure tetragonal I4/mmm phase of La2PrNi2O7 above ~10 GPa, which is distinct from the reported orthorhombic Fmmm phase of La3Ni2O7 above 14 GPa. For La2PrNi2O7, the onset and the zero-resistance temperatures of superconductivity reach Tconset = 78.2 K and Tczero = 40 K at 15 GPa. This superconducting phase shares the samilar structural symmetry as many cuprate superconductors, providing a fresh platform to investigate underlying mechanisms of nickelate superconductors.

cond-mat.supr-con↗

arXiv2023

Phase shift and magnetic anisotropy induced field splitting of impurity states in (Li1-xFex)OHFeSe superconductor

Revealing the energy and spatial characteristics of impurity induced states in superconductors is essential for understanding their mechanism and fabricating new quantum state by manipulating impurities. Here by using high-resolution scanning tunneling microscopy/spectroscopy, we investigated the spatial distribution and magnetic field response of the impurity states in (Li1-xFex)OHFeSe. We detected two pairs of strong in-gap states on the "dumbbell" shaped defects. They display clear damped oscillations with different phase shifts and a direct phase-energy correlation. These features have long been predicted for classical Yu-Shiba-Rusinov (YSR) state, which are demonstrated here with unprecedented resolution for the first time. Moreover, upon applying magnetic field, all the in-gap state peaks remarkably split into two rather than shift, and the splitting strength is field orientation dependent. Via detailed numerical model calculations, we found such anisotropic splitting behavior can be naturally induced by a high-spin impurity coupled to anisotropic environment, highlighting how magnetic anisotropy affects the behavior of YSR states.

cond-mat.supr-con↗

arXiv2023

Charge order driven by multiple-Q spin fluctuations in heavily electron-doped iron selenide superconductors

Intertwined spin and charge orders have been widely studied in high-temperature superconductors, since their fluctuations may facilitate electron pairing; however, they are rarely identified in heavily electron-doped iron selenides. Here, using scanning tunneling microscopy, we show that when the superconductivity of (Li0.84Fe0.16OH)Fe1-xSe is suppressed by introducing Fe-site defects, a short-ranged checkerboard charge order emerges, propagating along the Fe-Fe directions with an approximately 2aFe period. It persists throughout the whole phase space tuned by Fe-site defect density, from a defect-pinned local pattern in optimally doped samples to an extended order in samples with lower Tc or non-superconducting. Intriguingly, our simulations indicate that the charge order is likely driven by multiple-Q spin density waves originating from the spin fluctuations observed by inelastic neutron scattering. Our study proves the presence of a competing order in heavily electron-doped iron selenides, and demonstrates the potential of charge order as a tool to detect spin fluctuations.

cond-mat.supr-con↗

arXiv2023

Percolation-induced resistivity drop in cold-pressed LuH2

The stoichiometric bulk LuH2 is a paramagnetic metal with high electrical conductivity comparable to simple metals. Here we show that the resistivity of cold-pressed (CP) LuH2 samples varies sensitively upon modifying the grain size or surface conditions via the grinding process, i.e., the CP pellets made of commercially purchased LuH2 powder remain metallic but exhibit thousands of times higher resistivity, while additional grinding of LuH2 powders in air further enhances the resistivity and even results in weakly localized behaviors. For these CP samples, interestingly, we can occasionally observe abrupt resistivity drops at high temperatures, which also show dependences on magnetic fields and electrical current. Measurements of variable-temperature XRD, magnetic susceptibility, and specific heat exclude the possibilities of structural, magnetic, and superconducting transitions for the observed resistivity drops. Instead, we tentatively attribute these above observations to the presence of insulating layers on the grain surface due to the modification of hydrogen stoichiometry or the pollution by oxygen/nitrogen. Percolation of the metallic grains through the insulating surfaces can explain the sudden drop in resistivity. The present results thus call for caution in asserting the resistivity drops as superconductivity and invalidate the background subtraction in analyzing the resistivity data.

cond-mat.supr-con↗

arXiv2023

Fe$_{1+y}$Te$_{x}$Se$_{1-x}$: a delicate and tunable Majorana material

We report the observation for the p$_{z}$ electron band and the band inversion in Fe$_{1+y}$Te$_{x}$Se$_{1-x}$ with angle-resolved photoemission spectroscopy. Furthermore, we found that excess Fe (y>0) inhibits the topological band inversion in Fe$_{1+y}$Te$_{x}$Se$_{1-x}$, which explains the absence of Majorana zero modes in previous reports for Fe$_{1+y}$Te$_{x}$Se$_{1-x}$ with excess Fe. Based on our analysis of different amounts of Te doping and excess Fe, we propose a delicate topological phase in this material. Thanks to this delicate phase, one may be able to tune the topological transition via applying lattice strain or carrier doping.

cond-mat.supr-con↗

arXiv2022

Non-trivial band topology and orbital-selective electronic nematicity in a new titanium-based kagome superconductor

Electronic nematicity that spontaneously breaks rotational symmetry has been shown as a generic phenomenon in correlated quantum systems including high-temperature superconductors and the AV3Sb5 (A = K, Rb, Cs) family with a kagome network. Identifying the driving force has been a central challenge for understanding nematicity. In iron-based superconductors, the problem is complicated because the spin, orbital and lattice degrees of freedom are intimately coupled. In vanadium-based kagome superconductors AV3Sb5, the electronic nematicity exhibits an intriguing entanglement with the charge density wave order (CDW), making understanding its origin difficult. Recently, a new family of titanium-based kagome superconductors ATi3Bi5 has been synthesized. In sharp contrast to its vanadium-based counterpart, the electronic nematicity occurs in the absence of CDW. ATi3Bi5 provides a new window to explore the mechanism of electronic nematicity and its interplay with the orbital degree of freedom. Here, we combine polarization-dependent angle-resolved photoemission spectroscopy with density functional theory to directly reveal the band topology and orbital characters of the multi-orbital RbTi3Bi5. The promising coexistence of flat bands, type-II Dirac nodal line and nontrivial Z2 topological states is identified in RbTi3Bi5. Remarkably, our study clearly unveils the orbital character change along the G-M and G-K directions, implying a strong intrinsic inter-orbital coupling in the Ti-based kagome metals, reminiscent of iron-based superconductors. Furthermore, doping-dependent measurements directly uncover the orbital-selective features in the kagome bands, which can be well explained by the d-p hybridization. The suggested d-p hybridization, in collaboration with the inter-orbital coupling, could account for the electronic nematicity in ATi3Bi5.

cond-mat.supr-con↗

arXiv2022

Quasi two-dimensional nature of high-Tc superconductivity in iron-based (Li,Fe)OHFeSe

The intercalated iron selenide (Li,Fe)OHFeSe has a strongly layered structure analogous to the quasi two-dimensional (2D) bismuth cuprate superconductors, and exhibits both high-temperature (Tc) and topological superconductivity. However, the issue of its superconductivity dimensionality has not yet been fully investigated so far. Here we report that the quasi-2D superconductivity features, including the high anisotropy γ = 151 and the associated quasi-2D vortices, are also revealed for (Li,Fe)OHFeSe, based on systematic experiments of the electrical transport and magnetization and model fittings. Thus, we establish a new vortex phase diagram for (Li,Fe)OHFeSe, which delineates an emergent quasi-2D vortex-liquid state, and a subsequent vortex-solid dimensional crossover from a pancake-like to a three-dimensional state with decreasing temperature and magnetic field. Furthermore, we find that all the quasi-2D characteristics revealed here for the high-Tc iron selenide superconductor are very similar to those reported for the high-Tc bismuth cuprate superconductors.

cond-mat.supr-con↗

arXiv2022

Superconductivity and orbital-selective nematic order in a new titanium-based kagome metal CsTi3Bi5

Fabrication of new types of superconductors with novel physical properties has always been a major thread in the research of superconducting materials. An example is the enormous interests generated by the cascade of correlated topological quantum states in the newly discovered vanadium-based kagome superconductors AV3Sb5 (A=K, Rb, and Cs) with a Z2 topological band structure. Here we report the successful fabrication of single-crystals of titanium-based kagome metal CsTi3Bi5 and the observation of superconductivity and electronic nematicity. The onset of the superconducting transition temperature Tc is around 4.8 K. In sharp contrast to the charge density wave superconductor AV3Sb5, we find that the kagome superconductor CsTi3Bi5 preserves translation symmetry, but breaks rotational symmetry and exhibits an electronic nematicity. The angular-dependent magnetoresistivity shows a remarkable two-fold rotational symmetry as the magnetic field rotates in the kagome plane. The scanning tunneling microscopy and spectroscopic imaging detect rotational-symmetry breaking C2 quasiparticle interference patterns (QPI) at low energies, providing further microscopic evidence for electronic nematicity. Combined with first-principle calculations, we find that the nematic QPI is orbital-selective and dominated by the Ti dxz and dyz orbitals, possibly originating from the intriguing orbital bond nematic order. Our findings in the new "135" material CsTi3Bi5 provide new directions for exploring the multi-orbital correlation effect and the role of orbital or bond order in the electron liquid crystal phases evidenced by the symmetry breaking states in kagome superconductors.

cond-mat.supr-con↗

arXiv2022

Titanium doped kagome superconductor CsV3-xTixSb5 and two distinct phases

The vanadium-based kagome superconductor CsV3Sb5 has attracted tremendous attention due to its unexcepted anomalous Hall effect (AHE), charge density waves (CDWs), nematicity, and a pseudogap pair density wave (PDW) coexisting with unconventional strong-coupling superconductivity (SC). The origins of CDWs, unconventional SC, and their correlation with different electronic states in this kagome system are of great significance, but so far, are still under debate. Chemical doping in the kagome layer provides one of the most direct ways to reveal the intrinsic physics, but remains unexplored. Here, we report, for the first time, the synthesis of Ti-substituted CsV3Sb5 single crystals and its rich phase diagram mapping the evolution of intertwining electronic states. The Ti atoms directly substitute for V in the kagome layers. CsV3-xTixSb5 shows two distinct SC phases upon substitution. The Ti slightly-substituted phase displays an unconventional V-shaped SC gap, coexisting with weakening CDW, PDW, AHE, and nematicity. The Ti highly-substituted phase has a U-shaped SC gap concomitant with a short-range rotation symmetry breaking CDW, while long-range CDW, twofold symmetry of in-plane resistivity, AHE, and PDW are absent. Furthermore, we also demonstrate the chemical substitution of V atoms with other elements such as Cr and Nb, showing a different modulation on the SC phase and CDWs. These findings open up a way to synthesise a new family of doped CsV3Sb5 materials, and further representing a new platform for tuning the different correlated electronic states and superconducting pairing in kagome superconductors.

cond-mat.supr-con↗