arXiv subjects

Xitong Xu

Publications and source records attributed to Xitong Xu.

At least 19 recordsLinked to original sources

arXiv2026

Electrical Transport and Quantum Oscillations in the Metallic Spin Supersolid EuCo2Al9

The discovery of spin supersolid and its giant magnetocaloric effect has opened a new arena in frustrated quantum magnets and cutting-edge cryogenics. The intermetallic EuCo2Al9 (ECA), for the first time, extends this intriguing phase from Mott insulators to a highly conductive metal [1]. In this work, we systematically study the electrical transport properties of ECA, where itinerant electrons serve as a sensitive probe for the spin supersolid states. We observe anomalies both in the temperature-dependent resistivity and field-dependent magnetoresistance and Hall signals, which are attributed to response of electrons to the Eu2+ spins and their fluctuations. Moreover, Shubnikov-de Haas quantum oscillations at high magnetic field reveal pronounced band splitting in the spin polarized state. Our results reveal an intimate correspondence between electrical transport and magnetic transitions in ECA, deepening the understanding of this metallic spin supersolid.

cond-mat.str-el↗

arXiv2026

RKKY-dipolar Interactions and 3D Spin Supersolid on Stacked Triangular Lattice

Inspired by the recent discovery of metallic spin supersolidity and its giant magnetocaloric effect in the rare-earth alloy EuCo$_2$Al$_9$ [Nature 651, 61 (2026)], we perform a combined study through electronic structure analysis, effective spin model, and Monte Carlo simulations on a stacked triangular lattice, and reveal a novel mechanism for the emergence of 3D spin supersolid in a metallic antiferromagnet. From first-principles inputs, we derive a minimal spin model on a stacked triangular lattice (STL), which arises from the interplay between Ruderman-Kittel-Kasuya-Yosida (RKKY) and dipolar interactions and accurately reproduces the experimental thermodynamics. Based on the STL model, we identify a ground state that simultaneously breaks discrete lattice translational symmetry and continuous spin-rotational symmetry -- the hallmark of a spin supersolid. Furthermore, we present the field-temperature phase diagram of the 3D STL model and discuss the various magnetic phases and associated phase transitions. Under zero field, the spin supersolid Y order establishes in two steps: an upper transition at $T_{N1}$, where an emergent U(1) symmetry appears and the system enters a fluctuating collinear regime, followed by a lower transition at $T_{N2}$ into the spin supersolid Y phase. In contrast, the supersolid V phase undergoes a single phase transition at $T_N^V$. Our results not only provide a comprehensive theoretical understanding of the metallic spin supersolid reported for EuCo$_2$Al$_9$ but also pave the way for further experimental investigations into its supersolid transitions and universality class.

cond-mat.str-el↗

arXiv2025

Stable skyrmion bundles at room temperature and zero magnetic field in a chiral magnet

Topological spin textures are characterized by topological magnetic charges, Q, which govern their electromagnetic properties. Recent studies have achieved skyrmion bundles with arbitrary integer values of Q, opening possibilities for exploring topological spintronics based on Q. However, the realization of stable skyrmion bundles in chiral magnets at room temperature and zero magnetic field - the prerequisite for realistic device applications - has remained elusive. Here, through the combination of pulsed currents and reversed magnetic fields, we experimentally achieve skyrmion bundles with different integer Q values - reaching a maximum of 24 at above room temperature and zero magnetic field - in the chiral magnet Co8Zn10Mn2. We demonstrate the field-driven annihilation of high-Q bundles and present a phase diagram as a function of temperature and field. Our experimental findings are consistently corroborated by micromagnetic simulations, which reveal the nature of the skyrmion bundle as that of skyrmion tubes encircled by a fractional Hopfion.

cond-mat.mes-hall↗

arXiv2025

Phase-sensitive evidence for pair density waves in a kagome superconductor

Pair density wave (PDW) exhibits periodic amplitude and sign modulations of the superconducting order parameter. Such a pairing state has long been proposed to be highly sensitive to nonmagnetic scattering, but its experimental realization remains elusive. Here we discover a nonmagnetic PDW-breaking effect in a kagome superconductor, using designer atomic nonmagnetic impurities and high-precision scanning tunneling microscopy (STM) at a base temperature of 30mK. We detect 2x2 pair density modulations by Josephson STM with a superconducting tip and 2x2 pairing gap modulations by normal STM. We find that the pairing modulations in both cases are substantially suppressed upon doping the kagome lattice with dilute isovalent nonmagnetic impurities, whereas the charge order and uniform superconductivity remain robust. We further identify the correlation between atomic dopants and the local suppression of PDW. We attribute these findings to a nonmagnetic pair-breaking effect, arising from the phase modulation of PDW in the kagome d-orbital. Taken together with its signatures in other state-of-the-art spectroscopy and transport measurements linked by theory, our findings support the ground state of the kagome superconductor as a correlated topological phase with superconducting loop currents.

cond-mat.supr-con↗

arXiv2025

Giant Self Spin-Valve Effect in the Kagome Helimagnet

Kagome magnets can combine non-trivial band topology and electron correlations, offering a versatile playground for various quantum phenomena. In this work we propose that kagome magnets with frustrated interlayer interactions can intrinsically support a self spin-valve effect, and experimentally confirm this in the kagome helimagnet TmMn$_6$Sn$_6$. Under a magnetic field perpendicular to the helical axis, using magnetic force microscopy we observed stripe domains that stack strictly along the helical axis, which we attribute to the stability loss of the kagome helimagnetic state. Such a domain pattern spontaneously mimics the artificial multilayered structure in traditional spin valves, which, combined with the high spin polarization, leads to a giant magnetoresistance (GMR) ratio over 160%. This discovery opens an avenue to realize inherent spin valves in a variety of quantum magnets, and can hold promise in future spintronics.

cond-mat.str-el↗

arXiv2024

Chiral kagome superconductivity modulations with residual Fermi arcs in KV3Sb5 and CsV3Sb5

Superconductivity involving finite momentum pairing can lead to spatial gap and pair density modulations, as well as Bogoliubov Fermi states within the superconducting gap. However, the experimental realization of their intertwined relations has been challenging. Here, we detect chiral kagome superconductivity modulations with residual Fermi arcs in KV3Sb5 and CsV3Sb5 by normal and Josephson scanning tunneling microscopy down to 30mK with resolved electronic energy difference at microelectronvolt level. We observe a U-shaped superconducting gap with flat residual in-gap states. This gap exhibits chiral 2 by 2 spatial modulations with magnetic field tunable chirality, which align with the chiral 2 by 2 pair density modulations observed through Josephson tunneling. These findings demonstrate a chiral pair density wave (PDW) that breaks time-reversal symmetry. Quasiparticle interference imaging of the in-gap zero-energy states reveals segmented arcs, with high-temperature data linking them to parts of the reconstructed V d-orbital states within the charge order. The detected residual Fermi arcs can be explained by the partial suppression of these d-orbital states through an interorbital 2 by 2 PDW and thus serve as candidate Bogoliubov Fermi states. Additionally, we differentiate the observed PDW order from impurity-induced gap modulations. Our observations not only uncover a chiral PDW order with orbital-selectivity, but also illuminate the fundamental space-momentum correspondence inherent in finite momentum paired superconductivity.

cond-mat.supr-con↗

arXiv2023

Quantum oscillations in kagome metals (Ti, Zr, Hf)V6Sn6 at Van Hove filling

Kagome materials have recently drawn great attention due to the interplay between nontrivial band topology, electron correlations, and Van Hove singularities related many-body orders. Here we report three new vanadium-based kagome metals, TiV6Sn6, ZrV6Sn6, and HfV6Sn6, and conduct a comprehensive investigation of their structural, magnetic, and electrical transport properties. All three compounds exhibit large unsaturated magnetoresistances and multiband Hall effects at low temperatures, indicating the existence of multiple highly mobile carriers. Both the diagonal and off-diagonal resistivity show quantum oscillations with nontrivial Berry phases and high quantum mobilities. First-principles calculations together with quantum oscillation analyses suggest the Van Hove singularities at the M point for the three compounds all located in close vicinity of the Fermi level, and there also exist multiple topological nontrivial band crossings, including a nodal ring and a massive Dirac cone. Our work extends the kagome AM6X6 family and paves the way for searching possible Van Hove physics in the V kagome lattice.

cond-mat.str-el↗

arXiv2023

Quantum Interactions in Topological R166 Kagome Magnet

Kagome magnet has been found to be a fertile ground for the search of exotic quantum states in condensed matter. Arising from the unusual geometry, the quantum interactions in the kagome lattice give rise to various quantum states, including the Chern-gapped Dirac fermion, Weyl fermion, flat band and van Hove singularity. Here we review recent advances in the study of the R166 kagome magnet (RT6E6, R = rare earths; T = transition metals; and E = Sn, Ge, etc.) whose crystal structure highlights the transition-metal-based kagome lattice and rare-earth sublattice. Compared with other kagome magnets, the R166 family owns the particularly strong interplays between the d electrons on the kagome site and the localized f electrons on the rare-earth site. In the form of spin-orbital coupling, exchange interaction and many-body effect, the quantum interactions play an essential role in the Berry curvature field in both the reciprocal and real spaces of R166 family. We discuss the spectroscopic and transport visualization of the topological electrons hosted in the Mn kagome layer of RMn6Sn6 and the various topological effects due to the quantum interactions, including the Chern-gap opening, the exchange-biased effect, the topological Hall effect and the emergent inductance. We hope this work serves as a guide for future explorations of quantum magnets.

cond-mat.str-el↗

arXiv2023

Observation of Kondo lattice and Kondo-enhanced anomalous Hall effect in an itinerant ferromagnet

The interplay between Kondo screening and magnetic interactions is central to comprehending the intricate phases in heavy-fermion compounds. However, the role of the itinerant magnetic order, which is driven by the conducting (c) electrons, has been largely uncharted in the context of heavy-fermion systems due to the scarcity of material candidates. Here we demonstrate the coexistence of the coherent Kondo screening and d-orbital ferromagnetism in material system La$_{1-x}$Ce$_x$Co$_2$As$_2$, through comprehensive thermodynamic and electrical transport measurements. Additionally, using angle-resolved photoemission spectroscopy (ARPES), we further observe the f-orbit-dominated bands near the Fermi level ($E_f$) and signatures of the f-c hybridization below the magnetic transition temperature, providing strong evidence of Kondo lattice state in the presence of ferromagnetic order. Remarkably, by changing the ratio of Ce/La, we observe a substantial enhancement of the anomalous Hall effect (AHE) in the Kondo lattice regime. The value of the Hall conductivity quantitatively matches with the first-principle calculation that optimized with our ARPES results and can be attributed to the large Berry curvature (BC) density engendered by the topological nodal rings composed of the Ce-4f and Co-3d orbitals at $E_f$. Our findings point to the realization of a new platform for exploring correlation-driven topological responses in a novel Kondo lattice environment.

cond-mat.str-el↗

arXiv2021

Topological charge-entropy scaling in kagome Chern magnet TbMn$_6$Sn$_6$

In ordinary materials, electrons conduct both electricity and heat, where their charge-entropy relations observe the Mott formula and the Wiedemann-Franz law. In topological quantum materials, the transverse motion of relativistic electrons can be strongly affected by the quantum field arising around the topological fermions, where a simple model description of their charge-entropy relations remains elusive. Here we report the topological charge-entropy scaling in the kagome Chern magnet TbMn$_6$Sn$_6$, featuring pristine Mn kagome lattices with strong out-of-plane magnetization. Through both electric and thermoelectric transports, we observe quantum oscillations with a nontrivial Berry phase, a large Fermi velocity and two-dimensionality, supporting the existence of Dirac fermions in the magnetic kagome lattice. This quantum magnet further exhibits large anomalous Hall, anomalous Nernst, and anomalous thermal Hall effects, all of which persist to above room temperature. Remarkably, we show that the charge-entropy scaling relations of these anomalous transverse transports can be ubiquitously described by the Berry curvature field effects in a Chern-gapped Dirac model. Our work points to a model kagome Chern magnet for the proof-of-principle elaboration of the topological charge-entropy scaling.

cond-mat.str-el↗

arXiv2021

Helicoid-arc van Hove singularities in topological chiral crystals

Van Hove singularity are electronic instabilities that lead to many fascinating interactions, such as superconductivity and charge-density waves. And despite much interest, the nexus of emergent correlation effects from van Hove singularities and topological states of matter remains little explored in experiments. By utilizing synchrotron-based angle-resolved photoemission spectroscopy and Density Functional Theory, here we provide the first discovery of the helicoid quantum nature of topological Fermi arcs inducing van Hove singularities. In particular, in topological chiral conductors RhSi and CoSi we directly observed multiple types of inter- and intra-helicoid-arc mediated singularities, which includes the type-I and type-II van Hove singularity. We further demonstrate that the energy of the helicoid-arc singularities are easily tuned by chemical engineering. Taken together, our work provides a promising route to engineering new electronic instabilities in topological quantum materials.

cond-mat.mtrl-sci↗

arXiv2021

Anomalous Hall effect in distorted kagome magnets (Nd, Sm)Mn$_6$Sn$_6$

We report magnetic and electrical properties for single crystals of NdMn$_6$Sn$_6$ and SmMn$_6$Sn$_6$. They crystallize into a structure which has distorted, Mn-based kagome lattices, compared to the pristine kagome lattices in heavy-rare-earth-bearing RMn$_6$Sn$_6$ compounds. They are hightemperature ferromagnets of which the R moment is parallel with the Mn moment. We observed a large intrinsic anomalous Hall effect (AHE) that is comparable to the ferrimagnetic, heavy-R siblings in a wide range of temperature. We conclude that their intrinsic AHE is stemming from the Mn-based kagome lattice, just as in the heavy RMn$_6$Sn$_6$.

cond-mat.str-el↗

arXiv2021

Rare earth engineering in RMn$_6$Sn$_6$ topological kagome magnets

Exploration of the topological quantum materials with electron correlation is at the frontier of physics, as the strong interaction may give rise to new topological phases and transitions. Here we report that a family of kagome magnets RMn$_6$Sn$_6$ manifest the quantum transport properties analogical to those in the quantum-limit Chern magnet TbMn$_6$Sn$_6$. The topological transport in the family, including quantum oscillations with nontrivial Berry phase and large anomalous Hall effect arising from Berry curvature field, points to the existence of massive Dirac fermions. Our observation demonstrates a close relationship between rare-earth magnetism and topological electron structure, indicating the rare-earth elements can effectively engineer the Chern quantum phase in kagome magnets.

cond-mat.mtrl-sci↗

arXiv2020

Observation of Weyl fermions in a magnetic non-centrosymmetric crystal

Characterized by the absence of inversion symmetry, non-centrosymmetric materials are of great interest because they exhibit ferroelectricity, second harmonic generation, emergent Weyl fermions, and other fascinating phenomena. It is expected that if time-reversal symmetry is also broken, additional magneto-electric effects can emerge from the interplay between magnetism and electronic order. Here we report topological conducting properties in the non-centrosymmetric magnet PrAlGe. By photoemission spectroscopy, we observe an arc parametrizing surface-localized states---a topological arc. Using the bulk-boundary correspondence, we conclude that these arcs correspond to projected topological charges of $\pm{1}$ in the surface Brillouin zone, demonstrating the presence of magnetic Weyl quasiparticles in bulk. We further observe a large anomalous Hall response, arising from diverging bulk Berry curvature fields associated with the magnetic Weyl band structure. Our results demonstrate a topological phase with robust electronic surface states and anomalous transport in a non-centrosymmetric magnet for the first time, providing a novel material platform to study the interplay between magnetic order, band topology and transport.

cond-mat.mtrl-sci↗

arXiv2020

Discovery of a quantum limit Chern magnet TbMn6Sn6

The quantum level interplay between geometry, topology, and correlation is at the forefront of fundamental physics. Owing to the unusual lattice geometry and breaking of time-reversal symmetry, kagome magnets are predicted to support intrinsic Chern quantum phases. However, quantum materials hosting ideal spin-orbit coupled kagome lattices with strong out-of-plane magnetization have been lacking. Here we use scanning tunneling microscopy to discover a new topological kagome magnet TbMn6Sn6, which is close to satisfying the above criteria. We visualize its effectively defect-free purely Mn-based ferromagnetic kagome lattice with atomic resolution. Remarkably, its electronic state exhibits distinct Landau quantization upon the application of a magnetic field, and the quantized Landau fan structure features spin-polarized Dirac dispersion with a large Chern gap. We further demonstrate the bulk-boundary correspondence between the Chern gap and topological edge state, as well as the Berry curvature field correspondence of Chern gapped Dirac fermions. Our results point to the realization of a quantum-limit Chern phase in TbMn6Sn6, opening up an avenue for discovering topological quantum phenomena in the RMn6Sn6 (R = rare earth element) family with a variety of magnetic structures. Our visualization of the magnetic bulk-boundary-Berry correspondence covering real and momentum space demonstrates a proof-of-principle method revealing topological magnets.

cond-mat.mtrl-sci↗

arXiv2020

Enhanced Anomalous Hall Effect in Magnetic Topological Semimetal Co$_3$Sn$_{2-x}$In$_x$S$_2$

We study the anomalous Hall Effect (AHE) of single-crystalline Co$_3$Sn$_{2-x}$In$_x$S$_2$ over a large range of indium concentration x from 0 to 1. Their magnetization reduces progressively with increasing x while their ground state evolves from a ferromagnetic Weyl semimetal into a nonmagnetic insulator. Remarkably, after systematically scaling the AHE, we find that their intrinsic anomalous Hall conductivity (AHC) features an unexpected maximum at around x = 0.15. The change of the intrinsic AHC corresponds with the doping evolution of Berry curvature and the maximum arises from the magnetic topological nodal-ring gap. Our experimental results show a larger AHC in a fundamental nodal-ring gap than that of Weyl nodes.

cond-mat.mtrl-sci↗

arXiv2019

Highly Mobile Carriers in a Candidate of Quasi-Two-Dimensional Topological Semimetal AuTe$_2$Br

We report the crystal and electronic structures of a non-centrosymmetric quasi-two-dimensional (2D), candidate of topological semimetal AuTe2Br. The Fermi surface of this layered compound consists of 2D-like, topological trivial electron and non-trivial hole pockets which host a Dirac cone along the kz direction. Our transport measurements on the single crystals show highly anisotropic, compensated low-density electrons and holes, both of which exhibit ultrahigh mobility at a level of 10^5cm^2V^-1s^-1 at low temperature. The highly mobile, compensated carriers lead a non-saturated, parabolic magnetoresistance as large as 3*10^5 in single-crystalline AuTe2Br in a magnetic field up to 58 T.

cond-mat.mtrl-sci↗

arXiv2019

Crystal growth and quantum oscillations in the topological chiral semimetal CoSi

We survey the electrical transport properties of the single-crystalline, topological chiral semimetal CoSi which was grown via different methods. High-quality CoSi single crystals were found in the growth from tellurium solution. The sample's high carrier mobility enables us to observe, for the first time, quantum oscillations (QOs) in its thermoelectrical signals. Our analysis of QOs reveals two spherical Fermi surfaces around the R point in the Brillouin zone corner. The extracted Berry phases of these electron orbits are consistent with the -2 chiral charge as reported in DFT calculations. Detailed analysis on the QOs reveals that the spin-orbit coupling induced band-splitting is less than 2 meV near the Fermi level, one order of magnitude smaller than our DFT calculation result. We also report the phonon-drag induced large Nernst effect in CoSi at intermediate temperatures.

cond-mat.mtrl-sci↗