arXiv subjects

Xiunian Jing

Publications and source records attributed to Xiunian Jing.

14 recordsLinked to original sources

arXiv2025

Intrinsic Non-linearity of Josephson Junctions as an Alternative Origin of the Missing First Shapiro Step

The missing first Shapiro step in microwave-irradiated Josephson junctions has been widely interpreted as a hallmark of Majorana bound states. However, conventional mechanisms like junction underdamping or Joule heating can produce similar signatures. Here, we demonstrate that the intrinsic non-linear current-voltage characteristic of low-to-moderate transparency junctions can also suppress the first step, accompanied by distinctive zigzag boundaries between the zeroth and first step at intermediate driving frequencies. Microwave measurements on Al/WTe2 junctions and numerical simulations of a non-linear resistively and capacitively shunted junction model reveal the first step collapse induced by switching jumps of current, together with zigzag features absent in scenarios solely driven by finite \b{eta} or Joule heating. This zigzag signature therefore provides a crucial diagnostic tool, emphasizing the necessity of comprehensive analysis of microwave spectra before attributing the absence of the first Shapiro step to Majorana physics.

cond-mat.mes-hall↗

arXiv2022

1T-FeS$_2$$:$ a new type of two-dimensional metallic ferromagnet

Discovery of intrinsic two-dimensional (2D) magnetic materials is crucial for understanding the fundamentals of 2D magnetism and realizing next-generation magnetoelectronic and magneto-optical devices. Although significant efforts have been devoted to identifying 2D magnetism by exfoliating bulk magnetic layered materials, seldom studies are performed to synthesize ultra-thin magnetic materials directly for non-layered magnetic materials. Here, we report the successful synthesis of a new type of theoretically proposed 2D metallic ferromagnet 1T FeS2, through the molten-salt-assisted chemical vapor deposition (CVD) method. The long-range 2D ferromagnetic order is confirmed by the observation of a large anomalous Hall effect (AHE) and a hysteretic magnetoresistance. The experimentally detected out-of-plane ferromagnetic ordering is theoretically suported with Stoner criterion. Our findings open up new possibilities to search novel 2D ferromagnets in non-layered compounds and render opportunities for realizing realistic ultra-thin spintronic devices.

cond-mat.mtrl-sci↗

arXiv2021

Controlled synthesis of MoxW1-xTe2 atomic layers with emergent quantum states

Recently, new states of matter like superconducting or topological quantum states were found in transition metal dichalcogenides (TMDs) and manifested themselves in a series of exotic physical behaviors. Such phenomena have been demonstrated to exist in a series of transition metal tellurides including MoTe2, WTe2 and alloyed MoxW1-xTe2. However, the behaviors in the alloy system have been rarely addressed due to their difficulty in obtaining atomic layers with controlled composition, albeit the alloy offers a great platform to tune the quantum states. Here, we report a facile CVD method to synthesize the MoxW1-xTe2 with controllable thickness and chemical composition ratios. The atomic structure of monolayer MoxW1-xTe2 alloy was experimentally confirmed by scanning transmission electron microscopy (STEM). Importantly, two different transport behaviors including superconducting and Weyl semimetal (WSM) states were observed in Mo-rich Mo0.8W0.2Te2 and W-rich Mo0.2W0.8Te2 samples respectively. Our results show that the electrical properties of MoxW1-xTe2 can be tuned by controlling the chemical composition, demonstrating our controllable CVD growth method is an efficient strategy to manipulate the physical properties of TMDCs. Meanwhile, it provides a perspective on further comprehension and shed light on the design of device with topological multicomponent TMDCs materials.

cond-mat.mtrl-sci↗

arXiv2020

Dimensionality-dependent type-II Weyl semimetal state in Mo$_{0.25}$W$_{0.75}$Te$_{2}$

Weyl nodes and Fermi arcs in type-II Weyl semimetals (WSMs) have led to lots of exotic transport phenomena. Recently, Mo$_{0.25}$W$_{0.75}$Te$_{2}$ has been established as a type-II WSM with Weyl points located near Fermi level, which offers an opportunity to study its intriguing band structure by electrical transport measurements. Here, by selecting a special sample with the thickness gradient across two- (2D) and three-dimensional (3D) regime, we show strong evidences that Mo$_{0.25}$W$_{0.75}$Te$_{2}$ is a type-II Weyl semimetal by observing the following two dimensionality-dependent transport features: 1) A chiral-anomaly-induced anisotropic magneto-conductivity enhancement, proportional to the square of in-plane magnetic field (B$_{in}$$^{2}$); 2) An additional quantum oscillation with thickness-dependent phase shift. Our theoretical calculations show that the observed quantum oscillation originates from a Weyl-orbit-like scenario due to the unique band structure of Mo$_{0.25}$W$_{0.75}$Te$_{2}$. The in situ dimensionality-tuned transport experiment offers a new strategy to search for type-II WSMs.

cond-mat.mes-hall↗

arXiv2020

Magnitude and Spatial Distribution Control of the Supercurrent in Bi2O2Se-Based Josephson Junction

Many proposals in exploring topological quantum computation are based on superconducting quantum devices constructed on materials with strong spin-orbit coupling (SOC). For these devices, a full control on both the magnitude and the spatial distribution of the supercurrent would be highly demanded, but has been elusive up to now. We constructed proximity-type Josephson junction on nanoplates of Bi2O2Se, a new emerging semiconductor with strong SOC. Through electrical gating, we show that the supercurrent can be fully turned ON and OFF, and its real-space pathways can be configured either through the bulk or along the edges. Our work demonstrates Bi2O2Se as a promising platform for constructing multifunctional hybrid superconducting devices as well as for searching for topological superconductivity.

cond-mat.mes-hall↗

arXiv2019

Gate-tunable h/e-period magnetoresistance oscillations in Bi2O2Se nanowires

We report on the successful synthesis and low-temperature electron transport investigations of a new form of material - Bi2O2Se semiconducting nanowires. Gate-tunable 0- and $π$-h/e (h is the Planck constant and e the elementary charge) periodic resistance oscillations in longitudinal magnetic field were observed unexpectedly, demonstrating novel quasi-ballistic, phase-coherent surface states in Bi2O2Se nanowires. By reaching a very good agreement between the calculated density of states and the experimental data, we clarified the mechanism to be the one dimensional subbands formed along the circumference of the nanowire rather than the usually considered Aharonov-Bohm interference. A qualitative physical picture based on downward band bending associated with the complex band structure is proposed to describe the formation of the surface states.

cond-mat.mes-hall↗

arXiv2019

Phase evolution and superconductivity enhancement in Se-substituted MoTe$_2$ thin films

The strong spin$-$orbit coupling (SOC) and numerous crystal phases in few$-$layer transition metal dichalcogenides (TMDCs) MX$_2$ (M$=$W, Mo, and X$=$Te, Se, S) has led to a variety of novel physics, such as Ising superconductivity and quantum spin Hall effect realized in monolayer 2H$-$ and Td$-$MX$_2$, respectively. Consecutive tailoring of the MX$_2$ structure from 2H to Td phase may realize the long$-$sought topological superconductivity in one material system by incorporating superconductivity and quantum spin Hall effect together. In this work, by combing Raman spectrum, X-ray photoelectron spectrum (XPS), scanning transmission electron microscopy imaging (STEM) as well as electrical transport measurements, we demonstrate that a consecutively structural phase transitions from Td to 1T$'$ to 2H polytype can be realized as the Se-substitution concentration increases. More importantly, the Se$-$substitution has been found to notably enhance the superconductivity of the MoTe$_2$ thin film, which is interpreted as the introduction of the two$-$band superconductivity. The chemical constituent induced phase transition offers a new strategy to study the s$_{+-}$ superconductivity and the possible topological superconductivity as well as to develop phase$-$sensitive devices based on MX$_2$ materials.

cond-mat.mes-hall↗

arXiv2019

Evidence of Majorana Zero Modes in Josephson Trijunctions

In search of fault-tolerant topological quantum computation (TQC), zero-bias conductance peak as a necessary signature of Majorana zero modes (MZMs) has been observed in a number of solid-state systems. Here, we present the signature of MZMs from a phase-sensitive experiment on Josephson trijunctions constructed on the surface of three-dimensional topological insulators. We observed that the minigap at the center of the trijunction is protected to close over extended regions in phase space, supporting in principle the Majorana phase diagram proposed by Fu and Kane in 2008. Our study paves the way for further braiding MZMs and exploring TQC on a scalable two-dimensional platform.

cond-mat.mes-hall↗

arXiv2018

Transport evidence of asymmetric spin-orbit coupling in few$-$layer superconducting 1Td$-$MoTe$_2$

Two-dimensional (2D) transition metal dichalcogenides (TMDCs) MX2 (M=W, Mo, Nb, and X=Te, Se, S) with strong spin-orbit coupling (SOC) possess plenty of novel physics including superconductivity. Due to the Ising SOC, monolayer NbSe$_2$ and gated MoS$_2$ of 2H structure can realize the Ising superconductivity phase, which manifests itself with in-plane upper critical field far exceeding Pauli paramagnetic limit. Surprisingly, we find that a few-layer 1Td structure MoTe$_2$ also exhibits an in-plane upper critical field ($H_{c2,//}$) which goes beyond the Pauli paramagnetic limit. Importantly, the in-plane upper critical field shows an emergent two-fold symmetry which is different from the isotropic $H_{c2,//}$ in 2H structure TMDCs. We show that this is a result of an asymmetric SOC in 1Td structure TMDCs. The asymmetric SOC is very strong and estimated to be on the order of tens of meV. Our work provides the first transport evidence of a new type of asymmetric SOC in TMDCs which may give rise to novel superconducting and spin transport properties. Moreover, our findings mostly depend on the symmetry of the crystal and apply to a whole class of 1Td TMDCs such as 1Td-WTe$_2$ which is under intense study due to its topological properties.

cond-mat.supr-con↗

arXiv2018

Protected gap closing in Josephson junctions constructed on Bi$_2$Te$_3$ surface

On the road of searching for Majorana zero modes (MZMs) in topological insulator-based Josephson junctions, a highly-sought signature is the protected full transparency of electron transport through the junctions due to the existence of the MZMs, associated with complete gap closing between the electron-like and hole-like Andreev bound states (ABSs). Here, we present direct experimental evidence of gap closing and full transparency in single Josephson junctions constructed on the surface of three-dimensional topological insulator (3D TI) Bi$_2$Te$_3$. Our results demonstrate that the 2D surface of 3D TIs provides a promising platform for hosting and manipulating MZMs.

cond-mat.mes-hall↗

arXiv2016

Observation of Anomalous Magnetic Moments in Superconducting Bi/Ni Bilayer

There have been continuous efforts in searching for unconventional superconductivity over the past five decades. Compared to the well-established d-wave superconductivity in cuprates, the existence of superconductivity with other high-angular-momentum pairing symmetries is less conclusive. Bi/Ni epitaxial bilayer is a potential unconventional superconductor with broken time reversal symmetry (TRS), for that it demonstrates superconductivity and ferromagnetism simultaneously at low temperatures. We employ a specially designed superconducting quantum interference device (SQUID) to detect, on the Bi/Ni bilayer, the orbital magnetic moment which is expected if the TRS is broken. An anomalous hysteretic magnetic response has been observed in the superconducting state, providing the evidence for the existence of chiral superconducting domains in the material.

cond-mat.supr-con↗

arXiv2016

Majorana fermions in a superconducting Mobius strip

Recently, much attention has been paid to search for Majorana fermions in solid-state systems. Among various proposals there is one based on radio-frequency superconducting quantum interference devices (rf-SQUIDs), in which the appearance of 4$π$-period energy-phase relations is regarded as smoking-gun evidence of Majorana fermion states. Here we report the observation of truncated 4$π$-period (i.e., 2$π$-period but fully skewed) oscillatory patterns of contact resistance on rf-SQUIDs constructed on the surface of three-dimensional topological insulator Bi$_2$Te$_3$. The results reveal the existence of 1/2 fractional modes of Cooper pairs and the occurrence of parity switchings, both of which are necessary signatures accompanied with the formation of Majorana fermion states.

cond-mat.mes-hall↗

arXiv2013

Anomalous Cooper pair interference on Bi2Te3 surface

It is believed that the edges of a chiral p-wave superconductor host Majorana modes, relating to a mysterious type of fermions predicted seven decades ago. Much attention has been paid to search for p-wave superconductivity in solid-state systems, including recently those with strong spin-orbit coupling (SOC). However, smoking-gun experiments are still awaited. In this work, we have performed phase-sensitive measurements on particularly designed superconducting quantum interference devices constructing on the surface of topological insulators Bi2Te3, in such a way that a substantial portion of the interference loop is built on the proximity-effect-induced superconducting surface. Two types of Cooper interference patterns have been recognized at low temperatures. One is s-wave like and is contributed by a zero-phase loop inhabited in the bulk of Bi2Te3. The other, being identified to relate to the surface states, is anomalous for that there is a phase shift between the positive and negative bias current directions. The results support that the Cooper pairs on the surface of Bi2Te3 have a 2πBerry phase which makes the superconductivity p_x+ip_y-wave-like. Mesoscopic hybrid rings as constructed in this experiment are presumably arbitrary-phase loops good for studying topological quantum phenomena.

cond-mat.mes-hall↗

arXiv2011

Strong Superconducting Proximity Effect in Pb-Bi2Te3 Hybrid Structures

Majarona fermions (MFs) were predicted more than seven decades ago but are yet to be identified [1]. Recently, much attention has been paid to search for MFs in condensed matter systems [2-10]. One of the seaching schemes is to create MF at the interface between an s-wave superconductor (SC) and a 3D topological insulator (TI) [11-13]. Experimentally, progresses have been achieved in the observations of a proximity-effect-induced supercurrent [14-16], a perfect Andreev reflection [17] and a conductance peak at the Fermi level [18]. However, further characterizations are still needed to clarify the nature of the SC-TI interface. In this Letter, we report on a strong proximity effect in Pb-Bi2Te3 hybrid structures, based on which Josephson junctions and superconducting quantum interference devices (SQUIDs) can be constructed. Josephson devices of this type would provide a test-bed for exploring novel phenomena such as MFs in the future.

cond-mat.mes-hall↗