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Xue-Wen Chen

Publications and source records attributed to Xue-Wen Chen.

At least 19 recordsLinked to original sources

Exclusive Determination of $|V_{cb}|$ from Semileptonic Decays $B\to D^{(*)}\ell ν_{\ell}$

We present an updated exclusive determination of the CKM matrix element \(|V_{cb}|\) from the semileptonic decays \(B\to D^{(*)}\ell\barν_{\ell}\). Our analysis combines the latest Belle II measurements, updated lattice-QCD calculations of the \(B\to D^{(*)}\) form factors at small hadronic recoil, and correlated large-recoil SCET sum-rule predictions incorporating next-to-leading-order QCD corrections and several power-suppressed contributions. We consider three fit scenarios with progressively enlarged input sets and find that the inclusion of the large-recoil sum-rule constraints substantially reduces the form-factor uncertainties. From the full global fit, we obtain\(|V_{cb}|=(39.18 \pm0.47)\times10^{-3}\). Using the combined lattice-QCD and LCSR fit, we predict \(R(D)=0.3069\pm0.0080,\qquad R(D^*)=0.2548\pm0.0043\), and provide differential decay distributions in the momentum transfer and angular variables for both the muon and tau channels. Comparisons of the individual and correlated predictions for \(R(D)\) and \(R(D^*)\) with the experimental averages reveal a persistent tension. In particular, our theoretical 68\% confidence region shows little overlap with the experimental average. All correlations among the fitted parameters are retained in the uncertainty propagation. Our results therefore provide updated Standard Model benchmarks for tests of lepton-flavor universality. Improved lattice-QCD calculations, sum-rule predictions, and Belle II measurements will be essential for determining whether the remaining discrepancies originate from theoretical systematic uncertainties or from physics beyond the Standard Model.

hep-ph

Collective Blinking of Upconversion Emission in Lanthanide-doped Nanocrystals

Fluorescence blinking, often regarded as a limitation for stable emitters, can enable super-resolution localization microscopy and serve as a versatile reporter of the photophysical states of quantum emitters and their interactions with local environment. However, conventional blinking emitters are typically single quantum systems with Stokes-shifted fluorescence, making them susceptible to autofluorescence background, weak signal, and irreversible photodegradation under prolonged excitation. In contrast, single lanthanide-doped upconversion nanocrystals are effectively background-free anti-Stokes emitters and demonstrate robust resistance to photodegradation, yet they are generally considered non-blinking owing to the presence of a large ensemble of uncorrelated emitting lanthanide ions within a single nanocrystal. Here we report the discovery and control of collective blinking in the upconversion luminescence of thousands of lanthanide ions within a single nanocrystal. The blinking exhibits on-off intensity ratio exceeding 10, persists for over 15 hours (over 10,000 cycles) without discernible photodegradation, and can be reversibly controlled by adjusting the excitation power. We elucidate a universal, activator-independent upconversion blinking mechanism, whereby a single quencher, stochastically generated via a cooperative multi-ion process, can intercept delocalized excitation energy within the Yb3+ sensitizer network and darken the whole nanocrystal. Benefiting from the high-contrast, long-term photostable blinking and background-free emission, we achieve robust super-resolution localization microscopy that resolves individual nanocrystals in aggregates with 1.2 nm precision. This work establishes a general strategy to realize and control collective blinking in photostable multi-emitter nanosystems, opening new opportunities in nanoscience, bioimaging, and quantum technologies.

physics.optics

Photothermal Fourier-plane Phase Synchronization for Interferometric Scattering Microscopy

We introduce and experimentally implement Fourier-plane phase synchronization for optical microscopy, and demonstrate its performance with interferometric scattering microscopy. By combining a photothermal phase plate and laser beam scanning, we realize a synchronized phase for all scattering components on the Fourier plane of high numerical-aperture microscopes, where the evanescent waves and optical aberration normally produce highly inhomogeneous phase distributions. We achieve an almost perfect point spread function, exhibiting a tighter focus with 50\% enhancement of the signal and ideal circular symmetry. Particularly, by synchronizing the phase to $π/2$, we demonstrate the background speckles exhibit an anti-symmetric dependence on axial defocus, enabling the effective suppression of the speckles via defocus integration and thus the detection of 10 nm particles immobilized on the substrate. The concept and technique of seamless dynamic phase control on the Fourier plane constitute a key asset for modern optical microscopy.

physics.optics

Roadmap on Nonlocality in Photonic Materials and Metamaterials

Photonic technologies continue to drive the quest for new optical materials with unprecedented responses. A major frontier in this field is the exploration of nonlocal (spatially dispersive) materials, going beyond the local, wavevector-independent assumption traditionally made in optical material modeling. On one end, the growing interest in plasmonic, polaritonic and quantum materials has revealed naturally occurring nonlocalities, emphasizing the need for more accurate models to predict and design their optical responses. This has major implications also for topological, nonreciprocal, and time-varying systems based on these material platforms. Beyond natural materials, artificially structured materials--metamaterials and metasurfaces--can provide even stronger and engineered nonlocal effects, emerging from long-range interactions or multipolar effects. This is a rapidly expanding area in the field of photonic metamaterials, with open frontiers yet to be explored. In the case of metasurfaces, in particular, nonlocality engineering has become a powerful tool for designing strongly wavevector-dependent responses, enabling enhanced wavefront control, spatial compression, multifunctional devices, and wave-based computing. Furthermore, nonlocality and related concepts play a critical role in defining the ultimate limits of what is possible in optics, photonics, and wave physics. This Roadmap aims to survey the most exciting developments in nonlocal photonic materials, highlight new opportunities and open challenges, and chart new pathways that will drive this emerging field forward--toward new scientific discoveries and technological advancements.

cond-mat.mes-hall

Passive and Deterministic Controlled-phase Gate for Single-photon Wavepackets Based on Time-reversal Symmetric Photon Transport

We report the construction of a passive, deterministic and near-unity-fidelity controlled-$π$-phase gate for single-photon wavepackets with a node comprising a two-level emitter and a small number of cavities. The proposed gate is rooted in the concept of time-reversal symmetric photon transport, which makes the entire photon transport process into a perfect absorption and re-emission process. Consequently, it can circumvent the longstanding issue of wavepacket distortion inherent in photonic phase gates employing nonlinear media. Moreover, such time-reversal symmetric transport ensures the nonlinear $π$ phase shift by a single two-level emitter for the two-photon case. We develop analytical solutions to reveal the temporal dynamics of the nonlinear photon transport and to optimize the gate structure. Notably, the gate fidelity can exceed 99\% for a node with only four cavities for both single-photon and two-photon operations. Moreover, the proposed gate architecture is compatible with the platforms of integrated photonics.

quant-ph

Defocus-integration Interferometric Scattering Microscopy for Speckle Suppression and Enhancing Nanoparticle Detection on Substrate

Direct optical detection and imaging of single nanoparticles on substrate in wide field underpin vast applications across different research fields. However, the speckles originating from the unavoidable random surface undulations of the substrate ultimately limit the size of the decipherable nanoparticles by the current optical techniques, including the ultrasensitive interferometric scattering microscopy (iSCAT). Here we report a defocus-integration iSCAT to suppress the speckle noise and to enhance the detection and imaging of single nanoparticles on ultra-flat glass substrate and silicon wafer. In particular, we discover distinct symmetry properties of the scattering phase between the nanoparticle and the surface undulations that cause the speckles. Consequently, we develop the defocus-integration technique to suppress the speckles.We experimentally achieve an enhancement of the signal to noise ratio by 6.9 dB for the nanoparticle detection. We demonstrate that the technique is generally applicable for nanoparticles of various materials and for both low and high refractive-index substrates.

physics.optics

Exploring the Impact of Dissipation Coefficient in Warm Higgs Inflation

In this study, we conducted a detailed analysis of the core parameter of Warm Higgs Inflation (WHI) $-$ the dissipation coefficient ($Q$). As a crucial parameter in the warm inflation process, $Q$ exerts profound influences on the entire evolutionary process. By meticulously deriving the relationships between various quantities and $Q$, we successfully circumvented the common preconceptions regarding strong and weak dissipation, laying the foundation for a more accurate exploration of their interconnections. Taking into account the constraints imposed by Cosmic Microwave Background, we observed that the dissipation coefficient $Q$ remains at extremely low levels throughout the entire warm inflation process, i.e., $Q \ll 1$. This observation indicates that WHI falls under the category of weakly dissipative warm inflation. Despite being weakly dissipative, $Q$ still plays a crucial role in the evolution of temperature, energy, and other quantities, highlighting its significance and non-negligibility. We delved deeper into the impact of the primordial power spectrum on the dissipation coefficient $Q$ during the warm inflation process, discovering that the dependency is not significant. Consequently, this naturally leads to the unobtrusive dependence of the gravitational wave power spectrum on $Q$. Finally, we found that gravitational waves generated by WHI hold the potential for verification in future observational experiments, especially through the SKA100 experiment. These findings provide a theoretical support for a more profound understanding of the early evolution of the universe.

astro-ph.CO

Bright nonblinking photoluminescence with blinking lifetime from a nanocavity-coupled quantum dot

Colloidal semiconductor quantum dots (QDs) are excellent luminescent nanomaterials for a broad range of optoelectronic applications. Their photoluminescence blinking, however, hinders their practical use in many aspects. It has been shown that coupling QDs to plasmonic nanostructures may provide a viable way to suppress blinking. Nevertheless, the underlying mechanism of blinking suppression remains unclear and debated. Here, by deterministically coupling a single QD to a plasmonic nanocavity, we clarify the mechanism of blinking suppression, and demonstrate unprecedentedly bright emission from a single colloidal QD. In particular, we report for the first time that the coupled system exhibits nonblinking photoluminescence with blinking lifetime, which shows that the elimination of photoluminescence blinking originates from enhanced quantum yield of the charged states. We identify that the radiative decay rate is boosted from (48 ns)-1 to (0.7 ns)-1, which outcompetes Auger processes and enables similar quantum yields for charged and neutral excitons. Moreover, we demonstrate ultrabright photoluminescence of up to 17 million detected photons per second from a single QD. This work sheds new light on the goal of achieving ultrabright nonblinking QDs and may benefit a variety of QD-based applications.

physics.optics

Optical Fingerprint of Flat Substrate Surface and Marker-free Lateral Displacement Detection with Angstrom-level Precision

We report that flat substrates such as glass coverslips with surface roughness well below 0.5 nm feature notable speckle patterns when observed with high-sensitivity interference microscopy. We uncover that these speckle patterns unambiguously originate from the subnanometer surface undulations, and develop an intuitive model to illustrate how subnanometer non-resonant dielectric features could generate pronounced interference contrast in the far field. We introduce the concept of optical fingerprint for the deterministic speckle pattern associated with a particular substrate surface area and intentionally enhance the speckle amplitudes for potential applications. We demonstrate such optical fingerprints can be leveraged for reproducible position identification and marker-free lateral displacement detection with an experimental precision of 0.22 nm. The reproducible position identification allows us to detect new nanoscopic features developed during laborious processes performed outside of the microscope. The demonstrated capability for ultrasensitive displacement detection may find applications in the semiconductor industry and super-resolution optical microscopy.

physics.optics

Calibrating quantum hydrodynamic model for noble metals in nanoplasmonics

Quantum hydrodynamic model (QHDM) has become a versatile and efficient tool for studying plasmonics at the nanoscopic length scale. Yet its application to noble metals has not been sufficiently justified, in particular for situations where the metallic structures interface with dielectric material and electrons spill over the interfaces. In a recent work, we developed a refined QHDM, where the near-field effects and static polarization of metal ion lattice, and the electron affinity and static permittivity of the dielectric are incorporated. Here we perform a careful calibration of the model parameters for the refined QHDM. The model parameters are determined by benchmarking with (time-dependent) density functional theory calculations for special cases of simple metal. The predictive power of the refined QHDM with calibrated model parameters is faithfully demonstrated by the calculations of the optical responses from gold nanomatryoshkas of different sizes. The refined QHDM approach allows the quasinormal mode analysis for revealing the intrinsic optical properties of the nanoscopic metallic structures. We expect the well-calibrated refined QHDM would provide the nanoplasmonics community with a useful tool.

physics.optics

A general framework of canonical quasinormal mode analysis for extreme nano-optics

Optical phenomena associated with extremely localized field should be understood with considerations of nonlocal and quantum effects, which pose a hurdle to conceptualize the physics with a picture of eigenmodes. Here we first propose a generalized Lorentz model to describe general nonlocal media under linear mean-field approximation and formulate source-free Maxwell's equations as a linear eigenvalue problem to define the quasinormal modes. Then we introduce an orthonormalization scheme for the modes and establish a canonical quasinormal mode framework for general nonlocal media. Explicit formalisms for metals described by quantum hydrodynamic model and polar dielectrics with nonlocal response are exemplified. The framework enables for the first time direct modal analysis of mode transition in the quantum tunneling regime and provides physical insights beyond usual far-field spectroscopic analysis. Applied to nonlocal polar dielectrics, the framework also unveils the important roles of longitudinal phonon polaritons in optical response.

physics.optics

Quasinormal mode theory for nanoscale electromagnetism with quantum surface responses

We report a self-consistent quasinormal mode theory for nanometer scale electromagnetism where the possible nonlocal and quantum effects are treated through quantum surface responses. With Feibelman's frequency-dependent \textit{d} parameters to describe the quantum surface responses, we formulate the source-free Maxwell's equations into a generalized linear eigenvalue problem to define the quasinormal modes. We then construct an orthonormal relation for the modes and consequently unlock the powerful toolbox of modal analysis. The orthonormal relation is validated by the reconstruction of the full numerical results through modal contributions. Significant changes in the landscape of the modes are observed due to the incorporation of the quantum surface responses for a number of nanostructures. Our semi-analytical modal analysis enables transparent physical interpretation of the spontaneous emission enhancement of a dipolar emitter as well as the near-field and far-field responses of planewave excitations in the nanostructures.

physics.optics

Bright Optical Eigenmode with about 1 nm $^3$ Volume

Concentrating optical field in an eigenmode with a tiny volume is vitally important for light-matter interactions at the fundamental level and underpins new technologies. In the past decades, researchers have investigated various approaches to shrink light and so far managed to reduce the volume of optical eigenmodes, under the quantum-optical definition, down to several ten nm3. Here we report on the discovery, characterization and engineering of a class of extremely localized eigenmodes that are resonances of atomistic protrusions on a metallic host nanoparticle and feature quantum-optical mode volumes of below 1 nm3. We theoretically demonstrate that these extremely localized modes can be made bright with radiation efficiencies reaching 30% and provide up to 4x10^7 times intensity enhancement. The existence of bright eigenmodes with the volume comparable to a photon emitter foresees exciting new optical physics, such as ultrastrong coupling with single optical emitters, angstrom-resolution optical imaging, and atomic-scale single-molecule photochemistry.

physics.optics

The Truncated Metallo-dielectric Omnidirectional Reflector: Collecting Single Photons in the Fundamental Gaussian Mode with 95% Efficiency

We propose a novel antenna structure which funnels single photons from a single emitter with unprecedented efficiency into a low-divergence fundamental Gaussian mode. Our device relies on the concept of creating an omnidirectional photonic bandgap to inhibit unwanted large-angle emission and to enhance small-angle defect-guided-mode emission. The new photon collection strategy is intuitively illustrated, rigorously verified and optimized by implementing an efficient body-of-revolution finite-difference time-domain method for in-plane dipole emitters. We investigate a few antenna designs to cover various boundary conditions posed by fabrication processes or material restrictions and theoretically demonstrate that collection efficiencies into the fundamental Gaussian mode exceeding 95% are achievable. Our antennas are broadband, insensitive to fabrication imperfections and compatible with a variety of solid-state emitters such as organic molecules, quantum dots and defect centers in diamond. Unidirectional and low-divergence Gaussian-mode emission from a single emitter may enable the realization of a variety of photonic quantum computer architectures as well as highly efficient light-matter interfaces.

physics.optics

Multiscale Modeling and Analysis for High-fidelity Interferometric Scattering Microscopy

Interferometric scattering microscopy (iSCAT), as an ultrasensitive fluorescence-free imaging modality, has recently gain enormous attention and been rapidly developing from demonstration of principle to quantitative sensing. Here we report on a theoretical and experimental study for iSCAT with samples having structural dimensions that differ by 4-5 orders of magnitude. In particular, we demonstrate and intuitively explain the profound effects of sub-nanometer surface roughness of a glass coverslip and of a mica surface on the absolute signal and the shape of the point spread function of a gold nanoparticle. These quantities significantly affect the accuracies for determining the target size and position in all three dimensions. Moreover, we investigate a sample system mimicking a gold nanoparticle in a simplified cell environment and show position-dependent and even asymmetric point spread function of the nanoparticle. The multiscale study will facilitate the development of high fidelity iSCAT in real applications.

physics.optics

Single-Molecule Doped Crystalline Nanosheets for Delicate Photophysics Studies and Directional Single-Photon Emitting Devices

Single molecules in solids have been considered as an attractive class of solid-state single quantum systems because they can be chemically synthesized at low cost to have stable narrow transitions at desired wavelengths. Here we report and demonstrate single dibenzoterrylene molecules in crystalline anthracene nanosheets as a robust and versatile solid-state platform for delicate photophysics studies and building blocks of single-photon devices. The high-quality nanosheet sample enables robust studies of delicate single-molecule photophysics at room temperature, including the first real-time observation of single molecule insertion site jump, quantitative measurements of the associated changes of dipole moment orientation and magnitude, unambiguous determination of excitation-power dependent intersystem crossing rate and triplet lifetime. Moreover, we demonstrate the flexible assembly of the nanosheets into a planar antenna device to achieve bright single-molecule emission with a Gaussian emission pattern. The thin thickness, good photostability and mechanical stability make the dibenzoterrylene-in-anthracene nanosheet system an excellent candidate of static quantum nodes in integrated photonic circuit.

physics.app-ph

Towards Simultaneous Observation of Path and Interference of Single Photon in a Modified Mach-Zehnder Interferometer

Classical wisdom of wave-particle duality says that it is impossible to observe simultaneously the wave and particle nature of microscopic object. Mathematically the principle requests that the interference visibility V and which-path distinguishability D satisfy an orthodox limit of square(V)+square(D)<=1. This work presents a new wave-particle duality test experiment with single photon in a modified Mach-Zehnder interferometer and convincingly show the possibility of breaking the limit. The key element of the interferometer is a weakly-scattering total-internal reflection prism surface, which exhibits pronounced single-photon interference with a visibility up to 0.97 and simultaneously provides path distinguishability of 0.83. Apparently square(V)+square(D)=1.63 far exceeds the orthodox limit set by the principle of wave-particle duality for single photon. It is expected that more delicate experiments in future should be able to demonstrate the ultimate regime of square(V)+square(D) approaching 2 and shed new light on the foundations of contemporary quantum mechanics.

quant-ph

Quantum Photonic Node for On-Chip State Transfer

Integrated quantum photonics hold the promise to scale up the system size and form an on-chip quantum network with distributed information processing and simulation units. An outstanding need of such quantum network is to have high fidelity and efficiency on-chip state transfer between distant nodes. Although the nodes are naturally connected via waveguides, it is challenging to fulfill this need because stringent conditions such as spatial mode-matching configuration and time-reversal symmetry have to be satisfied. Here we report a type of quantum photonic nodes consisting of single quantum emitters and cascaded microring resonators for on-chip state transfer. By interfacing the node with a waveguide, we show that all the emission from the node can be funneled into the waveguide and its temporal profile can be synthesized to be time-reversal symmetric. We demonstrate theoretically on-chip quantum state transfer between two distant nodes with near-unity overall success rate can be achieved without any dynamic control. Moreover, we discuss the experimental implementation of our scheme with CMOS compatible integrated photonic platforms and solid-state quantum optics techniques.

quant-ph