arXiv subjects

Xun Shi

Publications and source records attributed to Xun Shi.

At least 37 records · Page 2Linked to original sources

arXiv2023

Galactic Interstellar Scintillation Observed from Four Globular Cluster Pulsars by FAST

We report detections of scintillation arcs for pulsars in globular clusters M5, M13 and M15 for the first time using the Five-hundred-meter Aperture Spherical radio Telescope (FAST). From observations of these arcs at multiple epochs, we infer that screen-like scattering medium exists at distances $4.1_{-0.3}^{+0.2}$ kpc, $6.7_{-0.2}^{+0.2}$ kpc and $1.3_{-1.0}^{+0.7}$ kpc from Earth in the directions of M5, M13 and M15, respectively. This means M5's and M13's scattering screens are located at $3.0_{-0.2}^{+0.1}$ kpc and $4.4_{-0.1}^{+0.1}$ kpc above the galactic plane, whereas, M15's is at $0.6_{-0.5}^{+0.3}$ kpc below the plane. We estimate the scintillation timescale and decorrelation bandwidth for each pulsar at each epoch using the one-dimensional auto-correlation in frequency and time of the dynamic spectra. We found that the boundary of the Local Bubble may have caused the scattering of M15, and detected the most distant off-plane scattering screens to date through pulsar scintillation, which provides evidence for understanding the medium circulation in the Milky Way.

astro-ph.GA↗

arXiv2023

Nodeless electron pairing in CsV$_3$Sb$_5$-derived kagome superconductors

The newly discovered kagome superconductors represent a promising platform for investigating the interplay between band topology, electronic order, and lattice geometry. Despite extensive research efforts on this system, the nature of the superconducting ground state remains elusive. In particular, consensus on the electron pairing symmetry has not been achieved so far, in part owing to the lack of a momentum-resolved measurement of the superconducting gap structure. Here we report the direct observation of a nodeless, nearly isotropic, and orbital-independent superconducting gap in the momentum space of two exemplary CsV$_3$Sb$_5$-derived kagome superconductors -- Cs(V$_{0.93}$Nb$_{0.07}$)$_3$Sb$_5$ and Cs(V$_{0.86}$Ta$_{0.14}$)$_3$Sb$_5$, using ultrahigh resolution and low-temperature angle-resolved photoemission spectroscopy (ARPES). Remarkably, such a gap structure is robust to the appearance or absence of charge order in the normal state, tuned by isovalent Nb/Ta substitutions of V. Moreover, we observe a signature of the time-reversal symmetry (TRS) breaking inside the superconducting state, which extends the previous observation of TRS-breaking CDW in the kagome lattice. Our comprehensive characterizations of the superconducting state provide indispensable information on the electron pairing of kagome superconductors, and advance our understanding of unconventional superconductivity and intertwined electronic orders.

cond-mat.supr-con↗

arXiv2022

Colossal Nernst power factor in topological semimetal NbSb$_2$

Today solid-state cooling technologies below liquid nitrogen boiling temperature (77 K), crucial to quantum information technology and probing quantum state of matter, are greatly limited due to the lack of good thermoelectric and/or thermomagnetic materials. Here, we report the discovery of colossal Nernst power factor of 3800$\times$10$^{-4}$ W m$^{-1}$ K$^{-2}$ under 5 T at 25 K and high Nernst figure-of-merit of 71$\times$10$^{-4}$ K$^{-1}$ under 5 T at 20 K in topological semimetal NbSb$_2$ single crystals. The observed high thermomagnetic performance is attributed to large Nernst thermopower and longitudinal electrical conductivity, and relatively low transverse thermal conductivity. The large and unsaturated Nernst thermopower is the result of the combination of highly desirable electronic structures of NbSb$_2$ having compensated high mobility electrons and holes near Fermi level and strong phonon-drag effect. This discovery opens an avenue for exploring material option for the solid-state heat pumping below liquid nitrogen temperature.

cond-mat.mtrl-sci↗

arXiv2022

Iterative mean-field approach to the spherical collapse of dark matter halos

Gravitational collapse of dark matter overdensities leads to the formation of dark matter halos which embed galaxies and galaxy clusters. An intriguing feature of dark matter halos is that their density profiles closely follow a universal form irrespective of the initial condition or the corresponding growth history. This represents a class of dynamical systems with emergent universalities. We propose an "iterative mean-field approach" to compute the solutions of the gravitational collapse dynamics. This approach iteratively searches for the evolution of the interaction field $ϕ(t)$ -- in this case the enclosed mass profile $M(r,t)$ -- that is consistent with the dynamics, thus that $ϕ(t)$ is the fix-point of the iterative mapping, $\mathcal{H}(ϕ) = ϕ$. The formalism replaces the N-body interactions with one-body interactions with the coarse-grained interaction field, and thus shares the spirit of the mean-field theory in statistical physics. This "iterative mean-field approach" combines the versatility of numerical simulations and the comprehensiveness of analytical solutions, and is particularly powerful in searching for and understanding intermediate asymptotic states in a wide range of dynamical systems where the solutions can not be obtained through the traditional self-similar analysis.

astro-ph.CO↗

arXiv2022

Direct observation of enhanced electron-phonon coupling in copper nanoparticles in the warm-dense matter regime

Warm-dense matter (WDM) is a highly-excited state that lies at the confluence of solids, plasmas, and liquids and that cannot be described by equilibrium theories. The transient nature of this state when created in a laboratory, as well as the difficulties in probing the strongly-coupled interactions between the electrons and the ions, make it challenging to develop a complete understanding of matter in this regime. In this work, by exciting isolated ~8 nm nanoparticles with a femtosecond laser below the ablation threshold, we create uniformly-excited WDM. We then use photoelectron spectroscopy to track the instantaneous electron temperature and directly extract the strongest electron-ion coupling observed experimentally to date. By directly comparing with state-of-the-art theories, we confirm that the superheated nanoparticles lie at the boundary between hot solids and plasmas, with associated strong electron-ion coupling. This is evidenced both by the fast energy loss of electrons to ions, as well as a strong modulation of the electron temperature by acoustic oscillations in the nanoparticle. This work demonstrates a new route for experimental exploration and theoretical validation of the exotic properties of WDM.

physics.plasm-ph↗

arXiv2022

Bipolaronic nature of the pseudogap in (TaSe4)2I revealed via weak photoexcitation

The origin of the pseudogap in many strongly correlated materials has been a longstanding puzzle. Here, we uncover which many-body interactions underlie the pseudogap in quasi-one-dimensional (quasi-1D) material (TaSe4)2I by weak photo-excitation of the material to partially melt the ground state order and thereby reveal the underlying states in the gap. We observe the appearance of both dispersive and flat bands by using time- and angle-resolved photoemission spectroscopy. We assign the dispersive band to a single-particle bare band, while the flat band to a collection of single-polaron sub-bands. Our results provide direct experimental evidence that many-body interactions among small Holstein polarons i.e., the formation of bipolarons, are primarily responsible for the pseudogap in (TaSe4)2I. Recent theoretical studies of the Holstein model support the presence of such a bipolaron-to-polaron crossover. We also observe dramatically different relaxation times for the excited in-gap states in (TaSe4)2I (~600 fs) compared with another quasi-1D material Rb0.3MoO3 (~60 fs), which provides a new method for distinguishing between pseudogaps induced by polaronic or Luttinger-liquid many-body interactions.

cond-mat.str-el↗

arXiv2021

Plasma microlensing dynamic spectrum probing fine structures in the ionized interstellar medium

Gravitational microlensing has become a mature technique for discovering small gravitational lenses in the Universe which are otherwise beyond our detection limits. Similarly, plasma microlensing can help us explore cosmic plasma lenses. Both pulsar scintillation and extreme scattering events of compact radio sources suggest the existence of $\sim$ AU scale plasma lenses in the ionized interstellar medium (IISM), whose astrophysical correspondence remains a mystery. We demonstrate that plasma microlensing events by these plasma lenses recorded in the form of wide-band dynamic spectra are a powerful probe of their nature. Using the recently developed Picard-Lefschetz integrator for the Kirchhoff-Fresnel integral, we simulate such dynamic spectra for a well-motivated family of single-variable plasma lenses. We demonstrate that the size, strength, and shape of the plasma lens can be measured from the location of the cusp point and the shape of spectral caustics respectively, with a combination of distances and the effective velocity known a priori or measured from the widths of the interference pattern. Future wide-band observations of pulsars, whose plasma microlensing events may be predictable from parabolic arc monitoring, are the most promising ground to apply our results for a deeper insight into the fine structures in the IISM.

astro-ph.GA↗

arXiv2021

Morphology of solar system scale plasma lenses in the interstellar medium: a test from pulsar scintillation parabolic arcs

Scintillation spectra of some pulsars have suggested the existence of $\lesssim$ AU scale density structures in the ionized interstellar medium, whose astrophysical correspondence is still a mystery. The detailed study of Brisken et al. suggested two possible morphologies for these structures: a parallel set of filaments or sheets (the `parallel stripes model'), or a filament broken up into denser knots (the `threaded beads model'). Here we propose a straightforward test that can distinguish these two morphologies: whether the apex of the main parabolic arc created by the scattered images deviates from the origin of the scintillation spectrum or not. In the `parallel stripes' model, the scattered images move along the stripes as the relative position of the pulsar moves. As a result, the pulsar is always co-linear with the scattered images, and thus the apex of the main parabolic arc stays at the origin of the scintillation spectrum. In the `threaded beads' model, the scattered images remain at almost fixed positions relative to the density structures, and thus the pulsar is not co-linear with the scattered images at most times, leading to an offset between the apex and the origin. Looking for this possible offset in a large sample of pulsar scintillation spectra, or monitoring the evolution of parabolic arcs will help pin down the morphology of these tiny density structures and constrain their astrophysical origin.

astro-ph.GA↗

arXiv2021

Molecular contrails -- triggered contraction by passages of massive objects through molecular clouds

We study the effects of passages of compact objects such as stars, star clusters, and black holes through molecular clouds, and propose that the gravitational interaction between the compact object and the ambient gas can lead to the formation of thin and collimated features made of dense gas, which we call "molecular contrails". Supercritical contrails can collapse further leading to triggered star formation. The width of a molecular contrail is determined by the mass and velocity of the compact object and the velocity dispersion of the ambient molecular medium. Under typical conditions in the Milky Way, passages of stellar-mass objects lead to the formation of width $d\gtrsim 0.01\;\rm {parsec}$ contrails, and passages of star clusters lead to the formation of $d\gtrsim 1\;\rm {parsec}$ contrails. We present a few molecular contrail candidates from both categories identified from ALMA 1.3mm continuum observations of star-forming regions and the $^{13}$CO(1-0) map from the Galactic Ring Survey respectively. The contrails represent an overlooked channel where stars and gas in the Galactic disk interact to for structures. They also present a potential way of detecting dark compact objects in the Milky Way.

astro-ph.GA↗

arXiv2020

Creation of a novel inverted charge density wave state

Charge density wave (CDW) order is an emergent quantum phase that is characterized by a periodic lattice distortion and charge density modulation, often present near superconducting transitions. Here we uncover a novel inverted CDW state by using a femtosecond laser to coherently over-drive the unique star-of-David lattice distortion in 1T-TaSe$_2$. We track the signature of this novel CDW state using time- and angle-resolved photoemission spectroscopy and time-dependent density functional theory, and validate that it is associated with a unique lattice and charge arrangement never before realized. The dynamic electronic structure further reveals its novel properties, that are characterized by an increased density of states near the Fermi level, high metallicity, and altered electron-phonon couplings. Our results demonstrate how ultrafast lasers can be used to create unique states in materials, by manipulating charge-lattice orders and couplings.

cond-mat.mtrl-sci↗

arXiv2020

Electronic Origin for the Enhanced Thermoelectric Efficiency of Cu2Se

Thermoelectric materials (TMs) can uniquely convert waste heat into electricity, which provides a potential solution for the global energy crisis that is increasingly severe. Bulk Cu2Se, with ionic conductivity of Cu ions, exhibits a significant enhancement of its thermoelectric figure of merit zT by a factor of ~3 near its structural transition around 400 K. Here, we show a systematic study of the electronic structure of Cu2Se and its temperature evolution using high-resolution angle-resolved photoemission spectroscopy. Upon heating across the structural transition, the electronic states near the corner of the Brillouin zone gradually disappear, while the bands near the centre of Brillouin zone shift abruptly towards high binding energies and develop an energy gap. Interestingly, the observed band reconstruction well reproduces the temperature evolution of the Seebeck coefficient of Cu2Se, providing an electronic origin for the drastic enhancement of the thermoelectric performance near 400 K. The current results not only bridge among structural phase transition, electronic structures, and thermoelectric properties in a condensed matter system, but also provide valuable insights into the search and design of new generation of thermoelectric materials.

cond-mat.mtrl-sci↗

arXiv2020

Dynamical heating of the X-ray emitting intracluster medium: the roles of merger shocks and turbulence dissipation

The diffuse plasma inside clusters of galaxies has X-ray emitting temperatures of a few keV. The physical mechanisms that heat this intracluster medium (ICM) to such temperatures include the accretion shock at the periphery of a galaxy cluster, the shocks driven by merger events, as well as a somewhat overlooked mechanism -- the dissipation of intracluster turbulent motions. We study the relative role of these heating mechanisms using galaxy clusters in Lagrangian tracer particle re-simulations of the Omega500 cosmological simulation. We adopt a novel analysis method of decomposing the temperature increase at each time step into the contribution from dissipative heating and that from adiabatic heating. In the high-resolution spatial-temporal map of these heating rates, merger tracks are clearly visible, demonstrating the dominant role of merger events in heating the ICM. The dissipative heating contributed by each merger event is extended in time and also occurs in the rarefaction regions, suggesting the importance of heating by the dissipation of merger-induced turbulence. Quantitative analysis shows that turbulence heating, rather than direct heating at merger shocks, dominates the temperature increase of the ICM, especially at inner radii $r < r_{\rm 500c}$. In addition, we find that many merger shocks can propagate with almost constant velocity to very large radii $r \gg r_{\rm 500c}$, some even reach and join with the accretion shock and becoming the outer boundary of the ICM. Altogether, these results suggest that the ICM is heated more in an `inside-out' fashion rather than `outside-in' as depicted in the classical smooth accretion picture.

astro-ph.CO↗

arXiv2019

Coherent modulation of the electron temperature and electron-phonon couplings in a 2D material

Ultrashort light pulses can selectively excite charges, spins and phonons in materials, providing a powerful approach for manipulating their properties. Here we use femtosecond laser pulses to coherently manipulate the electron and phonon distributions, and their couplings, in the charge density wave (CDW) material 1T-TaSe$_2$. After exciting the material with a short light pulse, spatial smearing of the electrons launches a coherent lattice breathing mode, which in turn modulates the electron temperature. This indicates a bi-directional energy exchange between the electrons and the strongly-coupled phonons. By tuning the laser excitation fluence, we can control the magnitude of the electron temperature modulation, from ~ 200 K in the case of weak excitation, to ~ 1000 K for strong laser excitation. This is accompanied by a switching of the dominant mechanism from anharmonic phonon-phonon coupling to coherent electron-phonon coupling, as manifested by a phase change of $π$ in the electron temperature modulation. Our approach thus opens up possibilities for coherently manipulating the interactions and properties of quasi-2D and other quantum materials using light.

cond-mat.mtrl-sci↗

arXiv2019

Turbulence decay in the density-stratified intracluster medium

Turbulence evolution in a density-stratified medium differs from that of homogeneous isotropic turbulence described by the Kolmogorov picture. We evaluate the degree of this effect in the intracluster medium (ICM) with hydrodynamical simulations. We find that the buoyancy effect induced by ICM density stratification introduces qualitative changes to the turbulence energy evolution, morphology, and the density fluctuation - turbulence Mach number relation, and likely explains the radial dependence of the ICM turbulence amplitude as found previously in cosmological simulations. A new channel of energy flow between the kinetic and the potential energy is opened up by buoyancy. When the gravitational potential is kept constant with time, this energy flow leaves oscillations to the energy evolution, and leads to a balanced state of the two energies where both asymptote to power-law time evolution with slopes shallower than that for the turbulence kinetic energy of homogeneous isotropic turbulence. We discuss that the energy evolution can differ more significantly from that of homogeneous isotropic turbulence when there is a time variation of the gravitational potential. Morphologically, ICM turbulence can show a layered vertical structure and large horizontal vortical eddies in the central regions with the greatest density stratification. In addition, we find that the coefficient in the linear density fluctuation - turbulence Mach number relation caused by density stratification is in general a variable with position and time.

astro-ph.CO↗

arXiv2019

Ultrafast electron calorimetry uncovers a new long-lived metastable state in 1T-TaSe$_2$ mediated by mode-selective electron-phonon coupling

Quantum materials represent one of the most promising frontiers in the quest for faster, lightweight, energy efficient technologies. However, their inherent complexity and rich phase landscape make them challenging to understand or manipulate in useful ways. Here we present a new ultrafast electron calorimetry technique that can systematically uncover new phases of quantum matter. Using time- and angle-resolved photoemission spectroscopy, we measure the dynamic electron temperature, band structure and heat capacity. We then show that this is a very sensitive probe of phase changes in materials, because electrons react very quickly, and moreover generally are the smallest component of the total heat capacity. This allows us to uncover a new long-lived metastable state in the charge density wave material 1T-TaSe$_2$, that is distinct from all of the known equilibrium phases: it is characterized by a significantly reduced effective heat capacity that is only 30% of the normal value, due to selective electron-phonon coupling to a subset of phonon modes. As a result, significantly less energy is required to melt the charge order and transform the state of the material than under thermal equilibrium conditions.

cond-mat.mtrl-sci↗

arXiv2018

Multi-scale analysis of turbulence evolution in the density stratified intracluster medium

The diffuse hot medium inside clusters of galaxies typically exhibits turbulent motions whose amplitude increases with radius, as revealed by cosmological hydrodynamical simulations. However, its physical origin remains unclear. It could either be due to an excess injection of turbulence at large radii, or faster turbulence dissipation at small radii. We investigate this by studying the time evolution of turbulence in the intracluster medium (ICM) after major mergers, using the Omega500 non-radiative hydrodynamical cosmological simulations. By applying a novel wavelet analysis to study the radial dependence of the ICM turbulence spectrum, we discover that faster turbulence dissipation in the inner high density regions leads to the increasing turbulence amplitude with radius. We also find that the ICM turbulence at all radii decays in two phases after a major merger: an early fast decay phase followed by a slow secular decay phase. The buoyancy effects resulting from the ICM density stratification becomes increasingly important during turbulence decay, as revealed by a decreasing turbulence Froude number $Fr \sim \mathcal{O}(1)$. Our results indicate that the stronger density stratification and smaller eddy turn-over time are the likely causes of the faster turbulence dissipation rate in the inner regions of the cluster.

astro-ph.CO↗

arXiv2018

Revealing the nature of the ultrafast magnetic phase transition in Ni by correlating extreme ultraviolet magneto-optic and photoemission spectroscopies

By correlating time- and angle-resolved photoemission and time-resolved transverse- magneto- optical Kerr effect measurements, both at extreme ultraviolet wavelengths, we uncover the universal nature of the ultrafast photoinduced magnetic phase transition in Ni. This allows us to explain the ultrafast magnetic response of Ni at all laser fluences - from a small reduction of the magnetization at low laser fluences, to complete quenching at high laser fluences. Both probe methods exhibit the same demagnetization and recovery timescales. We further show that the ultrafast demagnetization in Ni is indeed a magnetic phase transition that is launched within 20 fs, followed by demagnetization of the material within ~200 fs, and subsequent recovery of the magnetization on timescales ranging from 500 fs to >70 ps. We also provide evidence of two competing channels with two distinct timescales in the recovery process, that suggest the presence of coexisting phases in the material.

cond-mat.mtrl-sci↗

arXiv2018

Thermoelectric properties of polycrystalline palladium sulfide

A suite measurements of the electrical, thermal, and vibrational properties are conducted on palladium sulfide (PdS) in order to investigate its thermoelectric performance. The tetragonal structure with the space group $P$42/$m$ for PdS is determined from X-ray diffraction measurement. The unique temperature dependence of mobility suggests that acoustic phonons and ion impurity scattering are two dominant scattering mechanisms within the compound. The obtained power factor of $27$ $μ$Wcm$^{-1}$K$^{-2}$ at 800 K is the largest value in the remaining transition-metal sulfides studied so far. The maximum value of the dimensionless figure of merit is 0.33 at 800 K. The observed phonon softening with temperature indicates that the reduction of the lattice thermal conductivity is mainly controlled by the enhanced lattice anharmonicity. These results indicate that the binary bulk PdS has promising potential to have good thermoelectrical performance.

cond-mat.mtrl-sci↗