arXiv subjects

Y. J. Choi

Publications and source records attributed to Y. J. Choi.

At least 19 recordsLinked to original sources

arXiv2023

Spin-phonon interactions and magnetoelectric coupling in Co$_4$$B_2$O$_9$ ($B$ = Nb, Ta)

In order to explore the consequences of spin-orbit coupling on spin-phonon interactions in a set of chemically-similar mixed metal oxides, we measured the infrared vibrational properties of Co$_4B_2$O$_9$ ($B$ = Nb, Ta) as a function of temperature and compared our findings with lattice dynamics calculations and several different models of spin-phonon coupling. Frequency vs. temperature trends for the Co$^{2+}$ shearing mode near 150 cm$^{-1}$ reveal significant shifts across the magnetic ordering temperature that are especially large in relative terms. Bringing these results together and accounting for noncollinearity, we obtain spin-phonon coupling constants of -3.4 and -4.3 cm$^{-1}$ for Co$_4$Nb$_2$O$_9$ and the Ta analog, respectively. Analysis reveals that these coupling constants derive from interlayer (rather than intralayer) exchange interactions and that the interlayer interactions contain competing antiferromagnetic and ferromagnetic contributions. At the same time, beyond-Heisenberg terms are minimized due to fortuitous symmetry considerations, different than most other 4$d$- and 5$d$-containing oxides. Comparison with other contemporary oxides shows that spin-phonon coupling in this family of materials is among the strongest ever reported, suggesting an origin for magnetoelectric coupling.

cond-mat.mtrl-sci↗

arXiv2021

Rotation acceleration of asteroids (10115) 1992 SK, (1685) Toro, and (1620) Geographos due to the YORP effect

The rotation state of small asteroids is affected by the Yarkovsky-O'Keefe-Radzievskii-Paddack (YORP) effect, which is a net torque caused by solar radiation directly reflected and thermally reemitted from the surface. Due to this effect, the rotation period slowly changes, which can be most easily measured in light curves because the shift in the rotation phase accumulates over time quadratically. We collected archived light curves and carried out new photometric observations for asteroids (10115) 1992 SK, (1620) Geographos, and (1685) Toro. We applied the method of light curve inversion to fit observations with a convex shape model. The YORP effect was modeled as a linear change of the rotation frequency $\upsilon \equiv \mathrm{d}ω/ \mathrm{d}t$ and optimized together with other spin and shape parameters. We detected the acceleration $\upsilon = (8.3 \pm 0.6) \times 10^{-8}\,\mathrm{rad}\,\mathrm{d}^{-2}$ of the rotation for asteroid (10115) 1992 SK. This observed value agrees well with the theoretical value of YORP-induced spin-up computed for our shape and spin model. For (1685) Toro, we obtained $\upsilon = (3.3 \pm 0.3) \times 10^{-9}\,\mathrm{rad}\,\mathrm{d}^{-2}$, which confirms an earlier tentative YORP detection. For (1620) Geographos, we confirmed the previously detected YORP acceleration and derived an updated value of $\upsilon$ with a smaller uncertainty. We also included the effect of solar precession into our inversion algorithm, and we show that there are hints of this effect in Geographos' data. The detected change of the spin rate of (10115) 1992 SK has increased the total number of asteroids with YORP detection to ten. In all ten cases, the $\mathrm{d}ω/ \mathrm{d}t$ value is positive, so the rotation of these asteroids is accelerated. It is unlikely to be just a statistical fluke, but it is probably a real feature that needs to be explained.

astro-ph.EP↗

arXiv2019

Strong magnetoelectric coupling in mixed ferrimagnetic-multiferroic phases of a double perovskite

Exploring new magnetic materials is essential for finding advantageous functional properties such as magnetoresistance, magnetocaloric effect, spintronic functionality, and multiferroicity. Versatile classes of double perovskite compounds have been recently investigated because of intriguing physical properties arising from the proper combination of several magnetic ions. In this study, it is observed that the dominant ferrimagnetic phase is coexisted with a minor multiferroic phase in single-crystalline double-perovskite Er2CoMnO6. The majority portion of the ferrimagnetic order is activated by the long-range order of Er3+ moments below TEr = 10 K in addition to the ferromagnetic order of Co2+ and Mn4+ moments arising at TC = 67 K, characterized by compensated magnetization at TComp = 3.15 K. The inverted magnetic hysteresis loop observed below TComp can be described by an extended Stoner-Wohlfarth model. The additional multiferroic phase is identified by the ferroelectric polarization of 0.9 uC/m2 at 2 K. The coexisting ferrimagnetic and multiferroic phases appear to be strongly correlated in that metamagnetic and ferroelectric transitions occur simultaneously. The results based on intricate magnetic correlations and phases in Er2CoMnO6 enrich fundamental and applied research on magnetic materials through the scope of distinct magnetic characteristics in double perovskites.

cond-mat.str-el↗

arXiv2018

Anisotropic magnetic properties and giant rotating magnetocaloric effect in double-perovskite Tb2CoMnO6

We investigated the anisotropy of the magnetic and magnetocaloric properties of singlecrystalline double perovskite Tb2CoMnO6, which crystallizes in a monoclinic P21/n structure. Due to dissimilar magnetic anisotropy, the ferromagnetic order of the Co2+ and Mn4+ moments emerges along the c-axis at TC = 100 K, and the larger Tb3+ moments align perpendicular to the c-axis, below TTb = 15 K. The intricate temperature development of the metamagnetism along the c-axis results in a large negative change in the magnetic entropy at low temperature. On the other hand, the larger but almost reversible magnetization, perpendicular to the c-axis, results in a small and positive entropy change. This highly anisotropic magnetocaloric effect (MCE) leads to a giant rotational MCE, estimated to be 20.8 J/kg K. Our findings, based on the magnetic anisotropy in Tb2CoMnO6, enrich fundamental and applied research on magnetic materials, considering the distinct magnetic characteristics of double perovskites.

cond-mat.str-el↗

arXiv2016

Electric polarization observed in single crystals of multiferroic Lu2MnCoO6

We report electric polarization and magnetization measurements in single crystals of double perovskite Lu2MnCoO6 using pulsed magnetic fields and optical second harmonic generation (SHG) in DC magnetic fields. we observe well-resolved magnetic field-induced changes in the electric polarization in single crystals and thereby resolve the question about whether multiferroic behavior is intrinsic to these materials or an extrinsic feature of polycrystals. We find electric polarization along the crystalline b-axis, that is suppressed by applying a magnetic fields along c-axis and advance a model for the origin of magnetoelectric coupling. We furthermore map the phase diagram using both capacitance and electric polarization to identify regions of ordering and regions of magnetoelectric hysteresis. This compound is a rare example of coupled hysteretic behavior in the magnetic and electric properties. The ferromagnetic-like magnetic hysteresis loop that couples to hysteretic polarization can be attributed not to ordinary ferromagnetic domains, but to the rich physics of magnetic frustration of Ising-like spins in the axial next-nearest neighbor interaction model.

cond-mat.mtrl-sci↗

arXiv2015

Signature of high temperature superconductivity in electron doped Sr2IrO4

Sr2IrO4 was predicted to be a high temperature superconductor upon electron doping since it highly resembles the cuprates in crystal structure, electronic structure and magnetic coupling constants. Here we report a scanning tunneling microscopy/spectroscopy (STM/STS) study of Sr2IrO4 with surface electron doping by depositing potassium (K) atoms. At the 0.5-0.7 monolayer (ML) K coverage, we observed a sharp, V-shaped gap with about 95% loss of density of state (DOS) at EFand visible coherence peaks. The gap magnitude is 25-30 meV for 0.5-0.6 ML K coverage and it closes around 50 K. These behaviors exhibit clear signature of superconductivity. Furthermore, we found that with increased electron doping, the system gradually evolves from an insulating state to a normal metallic state, via a pseudogap-like state and possible superconducting state. Our data suggest possible high temperature superconductivity in electron doped Sr2IrO4, and its remarkable analogy to the cuprates.

cond-mat.supr-con↗

arXiv2014

Strong ferromagnetic-dielectric coupling in multiferroic Lu2CoMnO6 single crystals

We have grown single crystals of multiferroic double-perovskite Lu2CoMnO6 and studied the directional dependence of their magnetic and dielectric properties. The ferromagnetic order emerges below TC ~ 48K along the crystallographic c axis. Dielectric anomaly arises along the b axis at TC, contrary to the polycrystalline work suggesting ferroelectricity along the c axis. Through the strongly coupled ferromagnetic and dielectric states, the highly non-linear variation of both dielectric constant and magnetization was achieved in application of magnetic fields. This concurrent tunability provides an efficient route to manipulation of multiple order parameters in multiferroics.

cond-mat.str-el↗

arXiv2013

Giant Magnetic Fluctuations at the Critical Endpoint in Insulating HoMnO3

Although abundant research has focused recently on the quantum criticality of itinerant magnets, critical phenomena of insulating magnets in the vicinity of critical endpoints (CEP's) have rarely been revealed. Here we observe an emergent CEP at 2.05 T and 2.2 K with a suppressed thermal conductivity and concomitant strong critical fluctuations evident via a divergent magnetic susceptibility (e.g., chi''(2.05 T, 2.2 K)/chi''(3 T, 2.2 K)=23,500 %, comparable to the critical opalescence in water) in the hexagonal insulating antiferromagnet HoMnO3.

cond-mat.str-el↗

arXiv2012

A next generation Ultra-Fast Flash Observatory (UFFO-100) for IR/optical observations of the rise phase of gamma-ray bursts

The Swift Gamma-ray Burst (GRB) observatory responds to GRB triggers with optical observations in ~ 100 s, but cannot respond faster than ~ 60 s. While some ground-based telescopes respond quickly, the number of sub-60 s detections remains small. In mid- to late-2013, the Ultra-Fast Flash Observatory-Pathfinder is to be launched on the Lomonosov spacecraft to investigate early optical GRB emission. This pathfinder mission is necessarily limited in sensitivity and event rate; here we discuss a next generation rapid-response space observatory. We list science topics motivating our instruments, those that require rapid optical-IR GRB response, including: A survey of GRB rise shapes/times, measurements of optical bulk Lorentz factors, investigation of magnetic dominated (vs. non-magnetic) jet models, internal vs. external shock origin of prompt optical emission, the use of GRBs for cosmology, and dust evaporation in the GRB environment. We also address the impacts of the characteristics of GRB observing on our instrument and observatory design. We describe our instrument designs and choices for a next generation observatory as a second instrument on a low-earth orbit spacecraft, with a 120 kg instrument mass budget. Restricted to relatively modest mass and power, we find that a coded mask X-ray camera with 1024 cm2 of detector area could rapidly locate about 64 GRB triggers/year. Responding to the locations from the X-ray camera, a 30 cm aperture telescope with a beam-steering system for rapid (~ 1 s) response and a near-IR camera should detect ~ 29 GRB, given Swift GRB properties. Am additional optical camera would give a broadband optical-IR slope, allowing dynamic measurement of dust extinction at the source, for the first time.

astro-ph.IM↗

arXiv2012

Collective magnetism at multiferroic vortex domain walls

Topological defects have been playgrounds for many emergent phenomena in complex matter such as superfluids, liquid crystals, and early universe. Recently, vortex-like topological defects with six interlocked structural antiphase and ferroelectric domains merging into a vortex core were revealed in multiferroic hexagonal manganites. Numerous vortices are found to form an intriguing self-organized network. Thus, it is imperative to find out the magnetic nature of these vortices. Using cryogenic magnetic force microscopy, we discovered unprecedented alternating net moments at domain walls around vortices that can correlate over the entire vortex network in hexagonal ErMnO3 The collective nature of domain wall magnetism originates from the uncompensated Er3+ moments and the correlated organization of the vortex network. Furthermore, our proposed model indicates a fascinating phenomenon of field-controllable spin chirality. Our results demonstrate a new route to achieving magnetoelectric coupling at domain walls in single-phase multiferroics, which may be harnessed for nanoscale multifunctional devices.

cond-mat.str-el↗

arXiv2011

Data Acquisition System for the UFFO Pathfinder

The Ultra-Fast Flash Observatory (UFFO) Pathfinder is a payload on the Russian Lomonosov satellite, scheduled to be launched in November 2011. The Observatory is designed to detect early UV/Optical photons from Gamma-Ray Bursts (GRBs). There are two telescopes and one main data acquisition system: the UFFO Burst Alert & Trigger Telescope (UBAT), the Slewing Mirror Telescope (SMT), and the UFFO Data Acquisition (UDAQ) system. The UDAQ controls and manages the operation and communication of each telescope, and is also in charge of the interface with the satellite. It will write the data taken by each telescope to the NOR flash memory and sends them to the satellite via the Bus-Interface system (BI). It also receives data from the satellite including the coordinates and time of an external trigger from another payload, and distributes them to two telescopes. These functions are implemented in field programmable gates arrays (FPGA) for low power consumption and fast processing without a microprocessor. The UDAQ architecture, control of the system, and data flow will be presented.

astro-ph.IM↗

arXiv2011

Design and Fabrication of Detector Module for UFFO Burst Alert & Trigger Telescope

The Ultra-Fast Flash Observatory (UFFO) pathfinder is a space mission devoted to the measurement of Gamma-Ray Bursts (GRBs), especially their early light curves which will give crucial information on the progenitor stars and central engines of the GRBs. It consists of two instruments: the UFFO Burst Alert & Trigger telescope (UBAT) for the detection of GRB locations and the Slewing Mirror Telescope (SMT) for the UV/optical afterglow observations, upon triggering by UBAT. The UBAT employs a coded-mask γ/X-ray camera with a wide field of view (FOV), and is comprised of three parts: a coded mask, a hopper, and a detector module (DM). The UBAT DM consists of a LYSO scintillator crystal array, multi-anode photo multipliers, and analog and digital readout electronics. We present here the design and fabrication of the UBAT DM, as well as its preliminary test results.

astro-ph.CO↗

arXiv2011

The UFFO (Ultra Fast Flash Observatory) Pathfinder: Science and Mission

Hundreds of gamma-ray burst (GRB) optical light curves have been measured since the discovery of optical afterglows. However, even after nearly 7 years of operation of the Swift Observatory, only a handful of measurements have been made soon (within a minute) after the gamma ray signal. This lack of early observations fails to address burst physics at short time scales associated with prompt emissions and progenitors. Because of this lack of sub-minute data, the characteristics of the rise phase of optical light curve of short-hard type GRB and rapid-rising GRB, which may account for ~30% of all GRB, remain practically unknown. We have developed methods for reaching sub-minute and sub-second timescales in a small spacecraft observatory. Rather than slewing the entire spacecraft to aim the optical instrument at the GRB position, we use rapidly moving mirror to redirect our optical beam. As a first step, we employ motorized slewing mirror telescope (SMT), which can point to the event within 1s, in the UFFO Pathfinder GRB Telescope onboard the Lomonosov satellite to be launched in Nov. 2011. UFFO's sub-minute measurements of the optical emission of dozens of GRB each year will result in a more rigorous test of current internal shock models, probe the extremes of bulk Lorentz factors, provide the first early and detailed measurements of fast-rise GRB optical light curves, and help verify the prospect of GRB as a new standard candle. We will describe the science and the mission of the current UFFO Pathfinder project, and our plan of a full-scale UFFO-100 as the next step.

astro-ph.HE↗

arXiv2011

Implementation of the readout system in the UFFO Slewing Mirror Telescope

The Ultra-Fast Flash Observatory (UFFO) is a new space-based experiment to observe Gamma-Ray Bursts (GRBs). GRBs are the most luminous electromagnetic events in the universe and occur randomly in any direction. Therefore the UFFO consists of two telescopes; UFFO Burst Alert & Trigger Telescope (UBAT) to detect GRBs using a wide field-of-view (FOV), and a Slewing Mirror Telescope (SMT) to observe UV/optical events rapidly within the narrow, targeted FOV. The SMT is a Ritchey-Chretien telescope that uses a motorized mirror system and an Intensified Charge-Coupled Device (ICCD). When the GRB is triggered by the UBAT, the SMT receives the position information and rapidly tilts the mirror to the target. The ICCD start to take the data within a second after GRB is triggered. Here we give the details about the SMT readout electronics that deliver the data.

astro-ph.IM↗

arXiv2011

Temperature-dependent properties of the magnetic order in single-crystal BiFeO3

We report neutron diffraction and magnetization studies of the magnetic order in multiferroic BiFeO3. In ferroelectric monodomain single crystals, there are three magnetic cycloidal domains with propagation vectors equivalent by crystallographic symmetry. The cycloid period slowly grows with increasing temperature. The magnetic domain populations do not change with temperature except in the close vicinity of the N¶eel temperature, at which, in addition, a small jump in magneti- zation is observed. No evidence for the spin-reorientation transitions proposed in previous Raman and dielectric studies is found. The magnetic cycloid is slightly anharmonic for T=5 K. The an- harmonicity is much smaller than previously reported in NMR studies. At room temperature, a circular cycloid is observed, within errors. We argue that the observed anharmonicity provides important clues for understanding electromagnons in BiFeO3.

cond-mat.str-el↗

arXiv2011

Optical identification of hybrid magnetic and electric excitations in Dy3Fe5O12 garnet

Far-infrared spectra of magneto-dielectric Dy3Fe5O12 garnet were studied between 13 and 100 cm-1 and at low temperatures between 5 and 80 K. A combination of transmission, reflectivity, and rotating analyzer ellipsometry was used to unambiguously identify the type of the dipole activity of the infrared modes. In addition to purely dielectric and magnetic modes, we observed several hybrid modes with a mixed magnetic and electric dipole activity. These modes originate from the superexchange between magnetic moments of Fe and Dy ions. Using 4x4 matrix formalism for materials with Mu=/=1, we modeled the experimental optical spectra and determined the far-infrared dielectric and magnetic permeability functions. The matching condition Mu(Wh)*Se=Eps(Wh)*Sm for the oscillator strengths Se(m) explains the observed vanishing of certain hybrid modes at Wh in reflectivity.

cond-mat.str-el↗

arXiv2010

Observation of Anomalous Phonons in E-Type Orthorhombic REMnO3

We observe the appearance of a phonon near the lock-in temperature in orthorhombic REMnO3 (RE: Lu and Ho) and anomalous phonon hardening in orthorhombic LuMnO3. The anomalous phonon occurs at the onset of spontaneous polarization. No such changes were found in incommensurate orthorhombic DyMnO3. These observations directly reveal different electric polarization mechanisms in the E-type and IC-type REMnO3.

cond-mat.str-el↗

arXiv2010

Coupling between magnon and ligand-field excitations in magnetoelectric Tb3Fe5O12 garnet

The spectra of far-infrared transmission in Tb3Fe5O12 magnetoelectric single crystals have been studied in the range between 15 and 100 cm-1, in magnetic fields up to 10 T, and for temperatures between 5 and 150 K. We attribute some of the observed infrared-active excitations to electric-dipole transitions between ligand-field split states of Tb3+ ions. Anticrossing between the magnetic exchange excitation and the ligand-field transition occurs at the temperature between 60 and 80 K. The corresponding coupling energy for this interaction is 6 cm-1. Temperature-induced softening of the hybrid IR excitation correlates with the increase of the static dielectric constant. We discuss the possibility for hybrid excitations of magnons and ligand-field states and their possible connection to the magnetoelectric effect in Tb3Fe5O12.

cond-mat.str-el↗