arXiv subjects

Y. J. Choi

Publications and source records attributed to Y. J. Choi.

27 records · Page 2Linked to original sources

arXiv2010

Surface Reconstruction of Hexagonal Y-doped HoMnO3 and LuMnO3 studied using low-energy electron diffraction

We have investigated the (0001) surfaces of several hexagonal manganite perovskites by low-energy electron diffraction (LEED) in order to determine if the surface periodicity is different from that of the bulk materials. These LEED studies were conducted using near-normal incidence geometry with a low energy electron microscope (LEEM)/LEED apparatus from room temperature to 1200 degrees Celsius and with an electron energy in the range of 15-50 eV. Diffraction patterns showed features of bulk-terminated periodicity as well as a 2\times2 surface reconstruction. Possible origins for this surface reconstruction structure are discussed and comparisons are made with surface studies of other complex oxides.

cond-mat.str-el↗

arXiv2010

Origin of Electric Field Induced Magnetization in Multiferroic HoMnO3

We have performed polarized and unpolarized small angle neutron scattering experiments on single crystals of HoMnO3 and have found that an increase in magnetic scattering at low momentum transfers begins upon cooling through temperatures close to the spin reorientation transition at TSR ~ 40 K. We attribute the increase to an uncompensated magnetization arising within antiferromagnetic domain walls. Polarized neutron scattering experiments performed while applying an electric field show that the field suppresses magnetic scattering below T ~ 50 K, indicating that the electric field affects the magnetization via the antiferromagnetic domain walls rather than through a change to the bulk magnetic order.

cond-mat.str-el↗

arXiv2009

Magnetic excitations and optical transitions in the multiferroic spin-1/2 system LiCu$_2$O$_2$

Magnetic excitations in cycloidal magnet LiCu$_2$O$_2$ are explored using THz absorption spectroscopy in magnetic fields up to 12 T. Below the spin ordering temperature we observe eight optically active transitions in the spin system of LiCu$_2$O$_2$ in the energy range from 4 to 30 cm$^{-1}$. In magnetic field the number of modes increases and the electric polarization flop is seen as a change in magnetic field dependence of mode energies. The polarization dependence of two of the modes in zero magnetic field fits the selection rules for the cycloid tilted by $θ=41\pm1^{\circ}$ from the bc plane. For the remaining six modes electric and magnetic dipole approximations cannot explain the observed polarization dependence. We do not see the electromagnon in the explored energy range although there is evidence that it could exist below 4 cm$^{-1}$.

cond-mat.str-el↗

arXiv2009

Origin of electromagnon excitations in \textit{R}MnO$_3$

The origin of electromagnon excitations in cycloidal \textit{R}MnO$_3$ is explained in terms of the Heisenberg coupling between spins despite the fact that the static polarization arises from the much weaker Dzyaloshinskii-Moriya (DM) exchange interaction. We present a model that incorporates structural characteristics of this family of manganites that is confirmed by far infrared transmission data as a function of temperature and magnetic field and inelastic neutron scattering results. A deep connection is found between the magnetoelectric dynamics of the spiral phase and the static magnetoelectric coupling in the collinear E-phase of this family of manganites.

cond-mat.str-el↗

arXiv2008

3:1 magnetization plateau and suppression of ferroelectric polarization in an Ising chain multiferroic

Ferroelectric Ising chain magnet Ca$_3$Co$_{2-x}$Mn$_x$O$_6$ ($x\simeq$0.96) was studied in magnetic fields up to 33 T. Magnetization and neutron scattering measurements reveal successive metamagnetic transitions from the zero-field $\uparrow \uparrow \downarrow \downarrow$ spin configuration to the $\uparrow \uparrow \uparrow \downarrow$ state with a broad magnetization plateau, and then to the $\uparrow \uparrow \uparrow \uparrow$ state. The absence of hysteresis in these plateaus reveals an intriguing coupling between the intra-chain state and the three-dimensional geometrically frustrated magnetic system. Inversion symmetry, broken in the $\uparrow \uparrow \downarrow \downarrow$ state, is restored in the $\uparrow \uparrow \uparrow \downarrow$ state, leading to the complete suppression of the electric polarization driven by symmetric superexchange.

cond-mat.str-el↗

arXiv2008

Multiferroicity in the spin-1/2 quantum matter of LiCu2O2

Multiferroicity in LiCu2O2 single crystals is studied using resonant soft x-ray magnetic scattering, hard x-ray diffraction, heat capacity, magnetic susceptibility, and electrical polarization. Two magnetic transitions are found at 24.6 K (T1) and 23.2 K (T2). Our data are consistent with a sinusoidal spin structure at T2<T<T1 and with a helicoidal spin structure at T<T2 giving rise to ferroelectricity. Surprisingly, above T2 the correlation lengths of the spin structures increase as the temperature increases with dramatic changes of ~42% along the c-axis. Our results demonstrate the interplay of the geometrical frustration and the electronic and magnetic polarizations.

cond-mat.str-el↗

arXiv2008

Spin phonon coupling in frustrated magnet CdCr$_2$O$_4$

The infrared phonon spectrum of the spinel CdCr2O4 is measured as a function temperature from 6 K to 300K. The triply degenerate Cr phonons soften in the paramagnetic phase as temperature is lowered below 100 K and then split into a singlet and doublet in the low T antiferromagnetic phase which is tetragonally distorted to relieve the geometric frustration in the pyrochlore lattice of Cr$^{3+}$ ions. The phonon splitting is inconsistent with the simple increase (decrease) in the force constants due to deceasing (increasing) bond lengths in the tetragonal phase. Rather they correspond to changes in the force constants due to the magnetic order in the antiferromagnetic state. The phonon splitting in this system is opposite of that observed earlier in ZnCr2O4 as predicted by theory. The magnitude of the splitting gives a measure of the spin phonon coupling strength which is smaller than in the case of ZnCr2O4.

cond-mat.mtrl-sci↗

arXiv2007

Colossal magnon-phonon coupling in multiferroic Eu$_{0.75}$Y$_{0.25}$MnO$_3$

We report the spectra of magnetically induced electric dipole absorption in Eu$_{0.75}$Y$_{0.25}$MnO$_3$ from temperature dependent far infrared spectroscopy (10-250 cm$^{-1}$). These spectra, which occur only in the $e||a$ polarization, consist of two relatively narrow electromagnon features that onset at $T_{FE}=30$ K and a broad absorption band that persists to temperatures well above $T_N=47$ K. The observed excitations account for the step up of the static dielectric constant in the ferroelectric phase. The electromagnon at 80 cm$^{-1}$ is observed to be strongly coupled to the nearby lowest optical phonon which transfers more than 1/2 of its spectral weight to the magnon. We attribute the origin of the broad background absorption to the two magnon emission decay process of the phonon.

cond-mat.mtrl-sci↗

arXiv2000

Topology of the Galaxy Distribution in the Hubble Deep Fields

We have studied topology of the distribution of the high redshift galaxies identified in the Hubble Deep Field (HDF) North and South. The two-dimensional genus is measured from the projected distributions of the HDF galaxies at angular scales from $3.8''$ to $ 6.1''$. We have also divided the samples into three redshift slices with roughly equal number of galaxies using photometric redshifts to see possible evolutionary effects on the topology. The genus curve of the HDF North clearly indicates clustering of galaxies over the Poisson distribution while the clustering is somewhat weaker in the HDF South. This clustering is mainly due to the nearer galaxies in the samples. We have also found that the genus curve of galaxies in the HDF is consistent with the Gaussian random phase distribution with no significant redshift dependence.

astro-ph↗