arXiv subjects

Y. Uwatoko

Publications and source records attributed to Y. Uwatoko.

At least 55 records · Page 3Linked to original sources

arXiv2015

Pressure-Induced Valence Crossover and Novel Metamagnetic Behavior near the Antiferromagnetic Quantum Phase Transition of YbNi$_{3}$Ga$_{9}$

We report electrical resistivity, ac magnetic susceptibility and X-ray absorption spectroscopy measurements of intermediate valence YbNi$_{3}$Ga$_{9}$ under pressure and magnetic field. We have revealed a characteristic pressure-induced Yb valence crossover within the temperature-pressure phase diagram, and a first-order metamagnetic transition is found below $P_{\rm c}$ $\sim$ 9 GPa where the system undergoes a pressure-induced antiferromagnetic transition. As a possible origin of the metamagnetic behavior, a critical valence fluctuation emerging near the critical point of the first-order valence transition is discussed on the basis of the temperature-field-pressure phase diagram.

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arXiv2014

Pressure induced superconductivity on the border of magnetic order in MnP

We report the discovery of superconductivity on the border of long-range magnetic order in the itinerant-electron helimagnet MnP via the application of high pressure. Superconductivity with Tsc~1 K emerges and exists merely near the critical pressure Pc~8 GPa, where the long-range magnetic order just vanishes. The present finding makes MnP the first Mn-based superconductor. The close proximity of superconductivity to a magnetic instability suggests an unconventional pairing mechanism. Moreover, the detailed analysis of the normal-state transport properties evidenced non-Fermi-liquid behavior and the dramatic enhancement of the quasi-particle effective mass near Pc associated with the magnetic quantum fluctuations.

cond-mat.supr-con↗

arXiv2014

Quantum Criticality Based on Large Ising Spins: YbCo$_2$Ge$_4$ with New 1-2-4 Structure Type

We present a new type of quantum critical material YbCo$_2$Ge$_4$, having the largest quantum-critical pseudospin size ever. The YbCo$_2$Ge$_4$-type structure is new, forms in the orthorhombic $Cmcm$ system, and is related to the well-known ThCr$_2$Si$_2$ structure. Heavy rare earth (Tm,Yb,Lu, or Y) members are also possible to be grown. YbCo$_2$Ge$_4$ possesses the Ising-type ground-state doublet, namely the simplest ones of uniaxially up or down, $|\pm \sim 7/2\rangle$. It is clearly manifested through comprehensive resistivity, magnetization, specific heat, and NQR/NMR experiments. Large pseudospin state usually tends to order in simple magnetisms, or hard to be screened by Kondo effect. Therefore, the discovery of the quantum criticality of the fluctuating large spins opens a new door to new-material search and theoretical studies.

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arXiv2012

Microwave Surface Impedance Measurements of the Electronic State and Dissipation of Magnetic Vortices in Superconducting Iron-Based LiFeAs Single Crystals

LiFeAs is one of the iron-based superconductors having multiple gaps with the possible sign reversal. To clarify how those novel natures affect the energy dissipation of magnetic vortices, we investigated the microwave surface impedance of LiFeAs single crystals under finite magnetic fields. The flux-flow resistivity enhanced rapidly at low magnetic fields, which is similar to the case of MgB$_{2}$. This is probably the consequence of the multiple-gap nature and the gap anisotropy. This suggest that the sign-reversal is not important for the flux-flow even for multiple-gap superconductors. As for the electronic state, the vortex core of LiFeAs turned out to be "moderately clean". Furthermore, the mean free path inside the vortex core was much shorter than that outside, and was close to the core radius. These results strongly suggest a process specific to the core boundary is important for a scattering mechanism inside the vortex core.

cond-mat.supr-con↗

arXiv2012

Scanning Tunneling Microscopy/Spectroscopy of Vortices in LiFeAs

We investigate vortices in LiFeAs using scanning tunneling microscopy/spectroscopy. Zero-field tunneling spectra show two superconducting gaps without detectable spectral weight near the Fermi energy, evidencing fully-gapped multi-band superconductivity. We image vortices in a wide field range from 0.1 T to 11 T by mapping the tunneling conductance at the Fermi energy. A quasi-hexagonal vortex lattice at low field contains domain boundaries which consist of alternating vortices with unusual coordination numbers of 5 and 7. With increasing field, the domain boundaries become ill-defined, resulting in a uniformly disordered vortex matter. Tunneling spectra taken at the vortex center are characterized by a sharp peak just below the Fermi energy, apparently violating particlehole symmetry. The image of each vortex shows energy-dependent 4-fold anisotropy which may be associated with the anisotropy of the Fermi surface. The vortex radius shrinks with decreasing temperature and becomes smaller than the coherence length estimated from the upper critical field. This is direct evidence of the Kramer-Pesch effect expected in a clean superconductor.

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arXiv2011

Pressure-induced changes in the magnetic and valence state of EuFe2As2

We present the results of electrical resistivity, ac specific heat, magnetic susceptibility, X-ray absorption spectroscopy (XAS) and X-ray magnetic circular dichroism (XMCD) of the ternary iron arsenide EuFe2As2 single crystal under pressure. Applying pressure leads to a continuous suppression of the antiferromagnetism associated with Fe moments and the antiferromagnetic transition temperature becomes zero in the vicinity of a critical pressure Pc ~2.5-2.7 GPa. Pressure-induced re-entrant superconductivity, which is highly sensitive to the homogeneity of the pressure, only appears in the narrow pressure region in the vicinity of Pc due to the competition between superconductivity and the antiferromagnetic ordering of Eu2+ moments. The antiferromagnetic state of Eu2+ moments changes to the ferromagnetic state above 6 GPa. We also found that the ferromagnetic order is suppressed with further increasing pressure, which is connected with a valence change of Eu ions.

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arXiv2011

Control of ferroelectric polarization via uniaxial pressure in the spin-lattice-coupled multiferroic CuFe1-xGaxO2

We have demonstrated that ferroelectric polarization in a spin-driven multiferroic CuFe1-xGaxO2 with x = 0.035 can be controlled by the application of uniaxial pressure. Our neutron diffraction and in-situ ferroelectric polarization measurements have revealed that the pressure dependence of the ferroelectric polarization is explained by repopulation of three types of magnetic domains originating from the trigonal symmetry of the crystal. We conclude that the spin-driven anisotropic lattice distortion and the fixed relationship between the directions of the magnetic modulation wave vector and the ferroelectric polarization are the keys to this spin-mediated piezoelectric effect.

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arXiv2010

Determination of the Upper Critical Field of a Single Crystal LiFeAs: The Magnetic Torque Study up to 35 Tesla

We report on the upper critical field B_c2 of a superconducting LiFeAs single crystal with T_c~16 K, determined from magnetic torque measurements in dc-magnetic fields up to 35 T and at temperatures down to 0.3 K. B_c2 at 0.3 K is obtained to be 26.4 T and 15.5 T for the applied field B_a||ab and B_a||c, respectively. The anisotropy parameter $Γ$=$B_c2^ab / B_c2^c$ is ~ 3 at T_c and decreases to 1.7 as $T \rightarrow 0$, showing rather isotropic superconductivity. While B_c2 is orbitally-limited for B_a||c, the spin-paramagnetic effect is evident in the temperature dependence of B_c2 for B_a||ab

cond-mat.supr-con↗

arXiv2009

Spontaneous formation of a superconducting and antiferromagnetic hybrid state in SrFe2As2 under high pressure

We report a novel superconducting (SC) and antiferromagnetic (AF) hybrid state in SrFe2As2 revealed by 75As nuclear magnetic resonance (NMR) experiments on a single crystal under highly hydrostatic pressure up to 7 GPa. The NMR spectra at 5.4 GPa indicate simultaneous development of the SC and AF orders below 30 K. The nuclear spin-lattice relaxation rate in the SC domains shows a substantial residual density of states, suggesting proximity effects due to spontaneous formation of a nano-scale SC/AF hybrid structure. This entangled behavior is a remarkable example of a self-organized heterogeneous structure in a clean system.

cond-mat.supr-con↗

arXiv2009

Novel phase transition and the pressure effect in YbFe2Al10-type CeT2Al10 (T=Fe, Ru, Os)

We have succeeded in growing single crystals of orthorhombic CeT2Al10 (T=Fe, Ru, Os) by Al self-flux method for the first time, and measured the electrical resistivity at pressures up to 8 GPa, the magnetic susceptibility and specific heat at ambient pressure. These results indicate that CeT2Al10 belongs to the heavy fermion compounds. CeRu2Al10 and CeOs2Al10 show a similar phase transition at T0 = 27.3 and 28.7 K, respectively. The temperature dependences in the ordered phases are well described by the thermally activated form, suggesting that partial gap opens over the Fermi surfaces below T0. When pressure is applied to CeRu2Al10, T0 disappears suddenly between 3 and 4 GPa, and CeRu2Al10 turns into a Kondo insulator, followed by a metal. The similarity of CeT2Al10 under respective pressures suggests a scaling relation by some parameter controlling the unusual physics in these compounds.

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arXiv2009

NMR and NQR study of pressure-induced superconductivity and the origin of critical-temperature enhancement in the spin-ladder cuprate Sr$_2$Ca$_{12}$Cu$_{24}$O$_{41}$

Pressure-induced superconductivity was studied for a spin-ladder cuprate Sr$_2$Ca$_{12}$Cu$_{24}$O$_{41}$ using nuclear magnetic resonance (NMR) under pressures up to the optimal pressure 3.8 GPa. Pressure application leads to a transitional change from a spin-gapped state to a Fermi-liquid state at temperatures higher than $T_c$. The relaxation rate $1/T_1$ shows activated-type behavior at an onset pressure, whereas Korringa-like behavior becomes predominant at the optimal pressure, suggesting that an increase in the density of states (DOS) at the Fermi energy leads to enhancement of $T_c$. Nuclear quadrupole resonance (NQR) spectra suggest that pressure application causes transfer of holes from the chain to the ladder sites. The transfer of holes increases DOS below the optimal pressure. A dome-shaped $T_c$ versus pressure curve arises from naive balance between the transfer of holes and broadening of the band width.

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arXiv2008

Pressure-induced superconductivity in Iron pnictide compound SrFe2As2

Electrical resistivity under high pressure have been measured on nominally pure SrFe2As2 up to 14 GPa. The resistivity drop appeared with increasing pressure, and we clearly observed zero resistivity. The maximum of superconducting transition temperature (Tc) is 38 K. The value is corresponding to the one of optimally doping AFe2As2 (A=Sr, Ba) system with K+ ions at the A2+ site.

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arXiv2008

Superconductivity under high pressure in LaFeAsO

Electrical resistivity measurements under high pressures up to 29 GPa were performed for oxypnictide compound LaFeAsO. We found a pressure-induced superconductivity in LaFeAsO. The maximum value of Tc is 21 K at ~12 GPa. The pressure dependence of the Tc is similar to those of LaFeAsO1-xFx series reported previously.

cond-mat.supr-con↗

arXiv2008

Magneto-transport properties governed by the antiferromagnetic fluctuations in heavy fermion superconductor CeIrIn$_{5}$

In quasi-two dimensional Ce(Ir,Rh)In$_5$ system, it has been suggested that the phase diagram contains two distinct domes with different heavy fermion superconducting states. We here report the systematic pressure dependence of the electron transport properties in the normal state of CeRh$_{0.2}$Ir$_{0.8}$In$_{5}$ and CeIrIn$_{5}$, which locates in first and second superconducting dome, respectively. We observed non-Fermi liquid behavior at low temperatures in both compounds, including non-quadratic $T-$dependence of the resistivity, large enhancement of the Hall coefficient, and the violation of the Kohler's rule in the magnetoresistance. We show that the cotangent of Hall angle $\cot Θ_H$ varies as $T^2$, and the magnetoresistance is quite well scaled by the Hall angle as $Δρ_{xx}/ρ_{xx}\propto \tan^2Θ_H$. The observed transport anomalies are common features of Ce$M$In$_{5}$ ($M$=Co, Rh, and Ir) and high-$T_c$ cuprates, suggesting that the anomalous transport properties observed in CeIrIn$_{5}$ are mainly governed by the antiferromagnetic spin fluctuations, not by the Ce-valence fluctuations which has been proposed to be the possible origin for the second superconducting dome.

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arXiv2007

Positive and negative pressure effects on the magnetic ordering and the Kondo effect in the compound Ce2RhSi3

The competition between magnetic ordering and the Kondo effect in Ce2RhSi3, ordering antiferromagnetically at 7 K, is investigated by the measurements of magnetization, heat capacity and electrical resistivity on the solid solutions, Ce(2-x)La(x)RhSi3, Ce(2-y)Y(y)RhSi3, and Ce2RhSi(3-z)Ge(z), as well as by high pressure studies on this compound. The trends in the Kondo and Neel temperature variations among these alloys are compared to infer the roles of unit-cell volume and electronic structure changes. On the basis of the results, we infer that this compound lies at the peak of Doniach-magnetic-phase-diagram. The high pressure electrical resistivity data indicate that the quantum critical point for this compound is in the vicinity of 4 GPa.

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arXiv2007

Softening of Magnetic Excitations Leading to Pressure-Induced Quantum Phase Transition in Gapped Spin System KCuCl$_3$

KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar. Magnetic excitations in KCuCl$_3$ at a hydrostatic pressure of 4.7 kbar have been investigated by conducting neutron inelastic scattering experiments using a newly designed cylindrical high-pressure clamp cell. A well-defined single excitation mode is observed. The softening of the excitation mode due to the applied pressure is clearly observed. From the analysis of the dispersion relations, it is found that an intradimer interaction decreases under hydrostatic pressure, while most interdimer interactions increase.

cond-mat.str-el↗

arXiv2006

Non-Fermi liquid behavior in the magnetotransport of CeMIn5 (M: Co and Rh): Striking similarity between quasi 2D heavy fermion and high-Tc cuprates

We present a systematic study of the dc-resistivity, Hall effect, and magnetoresistance in the normal state of quasi 2D heavy fermion superconductors CeMIn5 (M: Rh and Co) under pressure. Here the electronic system evolves with pressure from an antiferromagnetic (AF) metal, through a highly unconventional non-Fermi liquid, and finally into a Fermi-liquid state. The amplitude of the Hall coefficient increases dramatically with decreasing T, reaching at low temperatures a value significantly larger than 1/ne. Furthermore, the magnetoresistance is characterized by T- and H-dependence which clearly violate Kohler's rule. We found that the Hall angle cotΘvaries as T^2, and the magnetoresistance is well scaled by the Hall angle as Δρ_{xx}/ρ_{xx}\propto \tan^2Θ. These non-Fermi liquid properties in the electron transport are remarkably pronounced when the AF fluctuations are enhanced in the vicinity of the QCP. We lay particular emphasis on the striking resemblance of these anomalous magnetotransport with those of the high-Tc cuprates. We argue that features commonly observed in quasi 2D heavy fermion and cuprates very likely capture universal features of strongly correlated electron systems.

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arXiv2006

Stoner gap in the superconducting ferromagnet UGe2

We report the temperature ($T$) dependence of ferromagnetic Bragg peak intensities and dc magnetization of the superconducting ferromagnet UGe2 under pressure ($P$). We have found that the low-$T$ behavior of the uniform magnetization can be explained by a conventional Stoner model. A functional analysis of the data produces the following results: The ferromagnetic state below a critical pressure can be understood as the perfectly polarized state, in which heavy quasiparticles occupy only majority spin bands. A Stoner gap $Δ(P)$ decreases monotonically with increasing pressure and increases linearly with magnetic field. We show that the present analysis based on the Stoner model is justified by a consistency check, i.e., comparison of density of states at the Fermi energy deduced from the analysis with observed electronic specific heat coeffieients. We also argue the influence of the ferromagnetism on the superconductivity.

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