arXiv subjects

Y. Zhu

Publications and source records attributed to Y. Zhu.

At least 91 records · Page 5Linked to original sources

arXiv2014

Glass-like recovery of antiferromagnetic spin ordering and dimensional crossover in a photo-excited manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$

Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr$_{0.7}$Ca$_{0.3}$MnO$_3$ following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

cond-mat.str-el↗

arXiv2014

Ultrafast structural and electronic dynamics of the metallic phase in a layered manganite

The transition between different states in manganites can be driven by various external stimuli. Controlling these transitions with light opens the possibility to investigate the microscopic path through which they evolve. We performed femtosecond (fs) transmission electron microscopy on a bi-layered manganite to study its response to ultrafast photoexcitation. We show that a photoinduced temperature jump launches a pressure wave that provokes coherent oscillations of the lattice parameters, detected via ultrafast electron diffraction. Their impact on the electronic structure are monitored via ultrafast electron energy loss spectroscopy (EELS), revealing the dynamics of the different orbitals in response to specific structural distortions.

cond-mat.str-el↗

arXiv2013

Energy, momentum and mass outflows and feedback from thick accretion discs around rotating black holes

Using long-duration general relativistic magnetohydrodynamic simulations of radiatively inefficient accretion discs, the energy, momentum and mass outflow rates from such systems are estimated. Outflows occur via two fairly distinct modes: a relativistic jet and a sub-relativistic wind. The jet power depends strongly on the black hole spin and on the magnetic flux at the horizon. Unless these are very small, the energy output in the jet dominates over that in the wind. For a rapidly spinning black hole accreting in the magnetically arrested limit, it is confirmed that jet power exceeds the total rate of accretion of rest mass energy. However, because of strong collimation, the jet probably does not have a significant feedback effect on its immediate surroundings. The power in the wind is more modest and shows a weaker dependence on black hole spin and magnetic flux. Nevertheless, because the wind subtends a large solid angle, it is expected to provide efficient feedback on a wide range of scales inside the host galaxy. Empirical formulae are obtained for the energy and momentum outflow rates in the jet and the wind.

astro-ph.HE↗

arXiv2013

LaAlO3 stoichiometry found key to electron liquid formation at LaAlO3/SrTiO3 interfaces

Emergent phenomena, including superconductivity and magnetism, found in the two-dimensional electron liquid (2-DEL) at the interface between the insulators LaAlO3 and SrTiO3 distinguish this rich system from conventional two-dimensional electron gases at compound semiconductor interfaces. The origin of this 2-DEL, however, is highly debated with focus on the role of defects in the SrTiO3 while the LaAlO3 has been assumed perfect. Our experiments and first principles calculations show that the cation stoichiometry of the nominal LaAlO3 layer is key to 2-DEL formation: only Al-rich LaAlO3 results in a 2-DEL. While extrinsic defects including oxygen deficiency are known to render LaAlO3/SrTiO3 samples conducting, our results show that in the absence of such extrinsic defects, an interface 2-DEL can form. Its origin is consistent with an intrinsic electronic reconstruction occurring to counteract a polarization catastrophe. This work provides a roadmap for identifying other interfaces where emergent behaviors await discovery.

cond-mat.mtrl-sci↗

arXiv2013

Real-time manifestation of strongly coupled spin and charge order parameters in stripe-ordered nickelates via time-resolved resonant x-ray diffraction

We investigate the order parameter dynamics of the stripe-ordered nickelate, La$_{1.75}$Sr$_{0.25}$NiO$_4$, using time-resolved resonant X-ray diffraction. In spite of distinct spin and charge energy scales, the two order parameters' amplitude dynamics are found to be linked together due to strong coupling. Additionally, the vector nature of the spin sector introduces a longer re-orientation time scale which is absent in the charge sector. These findings demonstrate that the correlation linking the symmetry-broken states does not unbind during the non-equilibrium process, and the time scales are not necessarily associated with the characteristic energy scales of individual degrees of freedom.

cond-mat.str-el↗

arXiv2012

Phase Fluctuations and the Absence of Topological Defects in Photo-excited Charge Ordered Nickelate

The dynamics of an order parameter's amplitude and phase determines the collective behaviour of novel states emerged in complex materials. Time- and momentum-resolved pump-probe spectroscopy, by virtue of its ability to measure material properties at atomic and electronic time scales and create excited states not accessible by the conventional means can decouple entangled degrees of freedom by visualizing their corresponding dynamics in the time domain. Here, combining time-resolved femotosecond optical and resonant x-ray diffraction measurements on striped La1.75Sr0.25NiO4, we reveal unforeseen photo-induced phase fluctuations of the charge order parameter. Such fluctuations preserve long-range order without creating topological defects, unlike thermal phase fluctuations near the critical temperature in equilibrium10. Importantly, relaxation of the phase fluctuations are found to be an order of magnitude slower than that of the order parameter's amplitude fluctuations, and thus limit charge order recovery. This discovery of new aspect to phase fluctuation provides more holistic view for the importance of phase in ordering phenomena of quantum matter.

cond-mat.str-el↗

arXiv2011

The ultraviolet limit and sum rule for the shear correlator in hot Yang-Mills theory

We determine a next-to-leading order result for the correlator of the shear stress operator in high-temperature Yang-Mills theory. The computation is performed via an ultraviolet expansion, valid in the limit of small distances or large momenta, and the result is used for writing operator product expansions for the Euclidean momentum and coordinate space correlators as well as for the Minkowskian spectral density. In addition, our results enable us to confirm and refine a shear sum rule originally derived by Romatschke, Son and Meyer.

hep-ph↗

arXiv2011

Graded Orbital Occupation near Interfaces in a La2NiO4 - La2CuO4 Superlattice

X-ray absorption spectroscopy and resonant soft x-ray reflectivity show a non-uniform distribution of oxygen holes in a La2NiO4 - La2CuO4 (LNO-LCO) superlattice, with excess holes concentrated in the LNO layers. Weak ferromagnetism with Tc = 160 K suggests a coordinated tilting of NiO6 octahedra, similar to that of bulk LNO. Ni d3z2-r2 orbitals within the LNO layers have a spatially variable occupation. This variation of the Ni valence near LNO-LCO interfaces is observed with resonant soft x-ray reflectivity at the Ni L edge, at a reflection suppressed by the symmetry of the structure, and is possible through graded doping with holes, due to oxygen interstitials taken up preferentially by inner LNO layers. Since the density of oxygen atoms in the structure can be smoothly varied with standard procedures, this orbital occupation, robust up to at least 280 K, is tunable.

cond-mat.str-el↗

arXiv2011

On the Correlations between Galaxy Properties and Supermassive Black Hole Mass

We use a large sample of upper limits and accurate estimates of supermassive black holes masses coupled with libraries of host galaxy velocity dispersions, rotational velocities and photometric parameters extracted from Sloan Digital Sky Survey i-band images to establish correlations between the SMBH and host galaxy parameters. We test whether the mass of the black hole, MBH, is fundamentally driven by either local or global galaxy properties. We explore correlations between MBH and stellar velocity dispersion sigma, bulge luminosity, bulge mass Sersic index, bulge mean effective surface brightness, luminosity of the galaxy, galaxy stellar mass, maximum circular velocity Vc, galaxy dynamical and effective masses. We verify the tightness of the MBH-sigma relation and find that correlations with other galaxy parameters do not yield tighter trends. We do not find differences in the MBH-sigma relation of barred and unbarred galaxies. The MBH-sigma relation of pseudo-bulges is also coarser and has a different slope than that involving classical bulges. The MBH-bulge mass is not as tight as the MBH-sigma relation, despite the bulge mass proving to be a better proxy of MBH than bulge luminosity. We find a rather poor correlation between MBH and Sersic index suggesting that MBH is not related to the bulge light concentration. The correlations between MBH and galaxy luminosity or mass are not a marked improvement over the MBH sigma relation. If Vc is a proxy for the dark matter halo mass, the large scatter of the MBH-Vc relation then suggests that MBH is more coupled to the baryonic rather than the dark matter. We have tested the need for a third parameter in the MBH scaling relations, through various linear correlations with bulge and galaxy parameters, only to confirm that the fundamental plane of the SMBH is mainly driven by sigma, with a small tilt due to the effective radius. (Abridged)

astro-ph.CO↗

arXiv2011

Next-to-leading order thermal spectral functions in the perturbative domain

Motivated by applications in thermal QCD and cosmology, we elaborate on a general method for computing next-to-leading order spectral functions for composite operators at vanishing spatial momentum, accounting for real, virtual as well as thermal corrections. As an example, we compute these functions (together with the corresponding imaginary-time correlators which can be compared with lattice simulations) for scalar and pseudoscalar densities in pure Yang-Mills theory. Our results may turn out to be helpful in non-perturbative estimates of the corresponding transport coefficients, which are the bulk viscosity in the scalar channel and the rate of anomalous chirality violation in the pseudoscalar channel. We also mention links to cosmology, although the most useful results in that context may come from a future generalization of our methods to other correlators.

hep-ph↗

arXiv2011

Performance of a large TeO2 crystal as a cryogenic bolometer in searching for neutrinoless double beta decay

Bolometers are ideal devices in the search for neutrinoless Double Beta Decay. Enlarging the mass of individual detectors would simplify the construction of a large experiment, but would also decrease the background per unit mass induced by alpha-emitters located close to the surfaces and background arising from external and internal gamma's. We present the very promising results obtained with a 2.13 kg TeO2 crystal. This bolometer, cooled down to a temperature of 10.5 mK in a dilution refrigerator located deep underground in the Gran Sasso National Laboratories, represents the largest thermal detector ever operated. The detector exhibited an energy resolution spanning a range from 3.9 keV (at 145 keV) to 7.8 keV (at the 2615 gamma-line of 208Tl) FWHM. We discuss the decrease in the background per unit mass that can be achieved increasing the mass of a bolometer.

nucl-ex↗

arXiv2011

Ferromagnetic Enhancement of CE-type Spin Ordering in (Pr,Ca)MnO$_3$

We present resonant soft X-ray scattering (RSXS) results from small band width manganites (Pr,Ca)MnO$_3$, which show that the CE-type spin ordering (SO) at the phase boundary is stabilized only below the canted antiferromagnetic transition temperature and enhanced by ferromagnetism in the macroscopically insulating state (FM-I). Our results reveal the fragility of the CE-type ordering that underpins the colossal magnetoresistance (CMR) effect in this system, as well as an unexpected cooperative interplay between FM-I and CE-type SO which is in contrast to the competitive interplay between the ferromagnetic metallic (FM-M) state and CE-type ordering.

cond-mat.str-el↗

arXiv2010

Response of a TeO_2 bolometer to alpha particles

$TeO_2$ crystals are used as bolometers in experiments searching for Double Beta Decay without emission of neutrinos. One of the most important issues in this extremely delicate kind of experiments is the characterization of the background. The knowledge of the response to $α$ particles in the energy range where the signal is expected is therefore a must. In this paper we report the results on the response function of a $TeO_2$ bolometer to $α$'s emitted by $^{147}$Sm dissolved in the crystal at the growth phase. A Quenching Factor of ($1.0076\pm 0.0005$) is found, independent of the temperature in the investigated range. The energy resolution on $α$ peaks shows a standard calorimeter energy dependence: $σ\; [\rm{keV}] = (0.56 \pm 0.02) \oplus (0.010 \pm 0.002)\sqrt{E[\rm{keV}]} $. Signal pulses show no difference between $α$ and $βγ$ particles

nucl-ex↗

arXiv2010

Atomic Imaging Using Secondary Electrons in a Scanning Transmission Electron Microscope : Experimental Observations and Possible Mechanisms

We report our detailed investigation of high-resolution imaging using secondary electrons (SE) with a subnanometer probe in an aberration-corrected transmission electron microscope, Hitachi HD2700C. This instrument also allows us to acquire the corresponding annular-dark-field (ADF) images simultaneously and separately. We demonstrate that atomic SE imaging is achievable for a wide range of elements, from uranium to carbon. Using the ADF images as a reference, we study the SE image intensity and contrast as a function of applied bias, atomic number, crystal tilt and thickness to shed light on the origin of the unexpected ultrahigh resolution in SE imaging. We have also demonstrated that the SE signal is sensitive to the terminating species at a crystal surface. Possible mechanisms for atomicscale SE imaging are proposed. The ability to image both the surface and bulk of a sample at atomic scale is unprecedented, and could revolutionize the field of electron microscopy and imaging.

cond-mat.mtrl-sci↗

arXiv2010

Production of high purity TeO2 single crystals for the study of neutrinoless double beta decay

High purity TeO2 crystals are produced to be used for the search for the neutrinoless double beta decay of 130Te. Dedicated production lines for raw material synthesis, crystal growth and surface processing were built compliant with radio-purity constraints specific to rare event physics experiments. High sensitivity measurements of radio-isotope concentrations in raw materials, reactants, consumables, ancillaries and intermediary products used for TeO2 crystals production are reported. Production and certification protocols are presented and resulting ready-to-use TeO2 crystals are described.

cond-mat.mtrl-sci↗

arXiv2009

The Structural Phase Transition in FeSe (Fe1+dSe)

In this letter we show that superconducting Fe1.01Se undergoes a structural transition at 90 K from a tetragonal to an orthorhombic phase but that non-superconducting Fe1.03Se does not. Further, high resolution electron microscopy study at low temperatures reveals an unexpected additional modulation of the crystal structure of the superconducting phase involving displacements of the Fe atoms, and that the non-superconducting material shows a distinct, complex nanometer-scale structural modulation. Finally, we show that magnetism is not the driving force for the phase transition in the superconducting phase.

cond-mat.supr-con↗

arXiv2008

Interface and electronic characterization of thin epitaxial Co3O4 films

The interface and electronic structure of thin (~20-74 nm) Co3O4(110) epitaxial films grown by oxygen-assisted molecular beam epitaxy on MgAl2O4(110) single crystal substrates have been investigated by means of real and reciprocal space techniques. As-grown film surfaces are found to be relatively disordered and exhibit an oblique low energy electron diffraction (LEED) pattern associated with the O-rich CoO2 bulk termination of the (110) surface. Interface and bulk film structure are found to improve significantly with post-growth annealing at 820 K in air and display sharp rectangular LEED patterns, suggesting a surface stoichiometry of the alternative Co2O2 bulk termination of the (110) surface. Non-contact atomic force microscopy demonstrates the presence of wide terraces separated by atomic steps in the annealed films that are not present in the as-grown structures; the step height of ~ 2.7 A corresponds to two atomic layers and confirms a single termination for the annealed films, consistent with the LEED results. A model of the (1 * 1) surfaces that allows for compensation of the polar surfaces is presented.

cond-mat.mtrl-sci↗

arXiv2008

Tuning the Charge Density Wave and Superconductivity in CuxTaS2

We report the characterization of layered, 2H-type CuxTaS2, for x between 0 and 0.12. The charge density wave (CDW), at 70 K for TaS2, is destabilized with Cu doping. The sub-1K superconducting transition in undoped 2H-TaS2 jumps quickly to 2.5 K at low x, increases to 4.5 K at the optimal composition Cu0.04TaS2, and then decreases at higher x. The electronic contribution to the specific heat, first increasing and then decreasing as a function of Cu content, is 12 mJ mol-1 K-2 at Cu0.04TaS2. Electron diffraction studies show that the CDW remains present at the optimal superconducting composition, but with both a changed q vector and decreased coherence length. We present an electronic phase diagram for the system.

cond-mat.supr-con↗