arXiv subjects

Yan Sun

Publications and source records attributed to Yan Sun.

At least 271 records · Page 15Linked to original sources

arXiv2020

Local Molecular Gas toward the Aquila Rift Region

We present the results of a ~250 square degrees CO mapping (+26d 4.1x10^5 Msun in the whole region. In fact, the mass of the molecular gas is dominated by the W40 giant molecular cloud (GMC) at ~474 pc (~1.4x10^5 Msun) and the GMC complex G036.0+01.0 at ~560-670 pc (~2.0x10^5 Msun), while the MCs at ~220-260pc have gas masses of 10^2-10^3 Msun. Interestingly, an ~80pc long filamentary MC G044.0-02.5 at a distance of ~404 pc shows a systematic velocity gradient along and perpendicular to the major axis of the filament. The HI gas with the enhanced emission has the similar spatial morphologies and velocity features compared to the corresponding CO structure, indicating that the large-scale converging HI flows are probably responsible for the formation of the MC. Meanwhile, the long filamentary MC consists of many sub-filaments with the lengths ranging from ~0.5 pc to several pc, as well as prevalent networks of filaments in other large-scale local MCs.

astro-ph.SR↗

arXiv2020

Searching for Molecular Outflows with Support Vector Machines: Dark Cloud Complex in Cygnus

We present a survey of molecular outflows across the dark cloud complex in the Cygnus region, based on 46.75 deg^2 field of CO isotopologues data from Milky Way Imaging Scroll Painting (MWISP) survey. A supervised machine learning algorithm, Support Vector Machine (SVM), is introduced to accelerate our visual assessment of outflow features in the data cube of 12CO and 13CO J = 1-0 emission. A total of 130 outflow candidates are identified, of which 77 show bipolar structures and 118 are new detections. Spatially, these outflows are located inside dense molecular clouds and some of them are found in clusters or in elongated linear structures tracing the underlying gas filament morphology. Along the line of sight, 97, 31, and 2 candidates reside in the Local, Perseus, and Outer arm, respectively. Young stellar objects as outflow drivers are found near most outflows, while 36 candidates show no associated source. The clusters of outflows that we detect are inhomogeneous in their properties; nevertheless, we show that the outflows cannot inject turbulent energy on cloud scales. Instead, at best, they are restricted to affecting the so called "clump" and "core" scales, and this only on short (~0.3 Myr) estimated timescales. Combined with outflow samples in the literature, our work shows a tight outflow mass-size correlation.

astro-ph.SR↗

arXiv2020

Spin-orbitronic materials with record spin-charge conversion from high-throughput ab initio calculations

The spin Hall effect (SHE) is an important spintronics phenomenon, which allows transforming a charge current into a spin current and vice versa without the use of magnetic materials or magnetic fields. To gain new insight into the physics of the SHE and to identify materials with a substantial spin Hall conductivities (SHC), we performed high-precision, high-throughput ab initio electronic structure calculations of the intrinsic SHC for over 20,000 non-magnetic crystals. The calculations reveal a strong and unexpected relation of the magnitude of the SHC with the crystalline symmetry, which we show exists because large SHC is typically associated with mirror symmetry protected nodal lines in the band structure. From the new developed database, we identify new promising materials. This includes eleven materials with a SHC comparable or even larger than that the up to now record Pt as well as materials with different types of spin currents, which could allow for new types of spin-obitronics devices.

cond-mat.mtrl-sci↗

arXiv2020

Thickness dependence of the anomalous Nernst effect and the Mott relation of Weyl-semimetal Co2MnGa thin films

We report a robust anomalous Nernst effect in Co2MnGa thin films in the thickness regime between 20 and 50 nm. The anomalous Nernst coefficient varied in the range of -2.0 to -3.0 uV/K at 300 K. We demonstrate that the anomalous Hall and Nernst coefficients exhibit similar behavior and fulfill the Mott relation. We simultaneously measure all four transport coefficients of the longitudinal resistivity, transversal resistivity, Seebeck coefficient, and anomalous Nernst coefficient. We connect the values of the measured and calculated Nernst conductivity by using the remaining three magneto-thermal transport coefficients, where the Mott relation is still valid. The intrinsic Berry curvature dominates the transport due to the relation between the longitudinal and transversal transport. Therefore, we conclude that the Mott relationship is applicable to describe the magneto-thermoelectric transport in Weyl semimetal Co2MnGa as a function of film thickness.

cond-mat.mes-hall↗

arXiv2020

Giant anomalous Hall and Nernst effect in magnetic cubic Heusler compounds

The interplay of magnetism and topology opens up the possibility for exotic linear response effects, such as the anomalous Hall effect and the anomalous Nernst effect, which can be strongly enhanced by designing a strong Berry curvature in the electronic structure. It is even possible to utilize this to create a quantum anomalous Hall state at high temperatures by reducing the dimensionality. Magnetic Heusler compounds are a promising class of materials for this purpose because they grow in thin films, have a high Curie temperature, and their electronic structure hosts strong topological features. Here, we provide a comprehensive study of the intrinsic anomalous transport for magnetic cubic full Heusler compounds and we illustrate that several Heusler compounds outperform the best so far reported materials. The results reveal the importance of symmetries, especially mirror planes, in combination with magnetism for giant anomalous Hall and Nernst effects, which should be valid in general for linear responses (spin Hall effect, spin orbital torque, etc.) dominated by intrinsic contributions.

cond-mat.mtrl-sci↗

arXiv2020

Strong anomalous Nernst effect in collinear magnetic Weyl semimetals without net magnetic moments

We predict a large anomalous Nernst effect in the inverse Heusler compensated ferrimagnets Ti$_2$Mn$X$ ($X$=Al,Ga,In) with vanishing net magnetic moments. Though the net magnetic moment is zero, the Weyl points in these systems lead to a large anomalous Nernst conductivity (ANC) due to the lack of a magnetic sublattice that inverses the sign of the Berry curvature. In comparison to the noncollinear antiferromagnets Mn$_3$Sn and Mn$_3$Ge, the high ANC stems almost entirely from the Weyl points in this class of compounds, and thus, it is topologically protected. This work shows for the first time a large ANC with zero net magnetic moments in collinear systems, which is helpful for comprehensive understanding of the thermoelectric effect in zero-moment magnetic materials and its further applications.

cond-mat.mtrl-sci↗

arXiv2020

Large Nernst Power Factor over a Broad Temperature Range in Polycrystalline Weyl Semimetal NbP

The discovery of topological materials has provided new opportunities to exploit advanced materials for heat-to-electricity energy conversion as they share many common characteristics with thermoelectric materials. In this work, we report the magneto-thermoelectric properties and Nernst effect of the topological Weyl semimetal NbP. We find that polycrystalline, bulk NbP shows a significantly larger Nernst thermopower than its conventional thermopower under magnetic field. As a result, a maximum Nernst power factor of ~ 35*10-4 Wm-1K-2 is achieved at 9 T and 136 K, which is 4 times higher than its conventional power factor and is also comparable to that of state-of-the-art thermoelectrics. Moreover, the Nernst power factor maintains relatively large value over a broad temperature range. These results highlight that the enhancement of thermoelectric performance can be achieved in topological semimetals based on the Nernst effect and transverse transport.

cond-mat.mtrl-sci↗

arXiv2020

Synergistically creating sulfur vacancies in semimetal-supported amorphous MoS2 for efficient hydrogen evolution

The presence of elemental vacancies in materials is inevitable according to statistical thermodynamics, which will decide the chemical and physical properties of the investigated system. However, the controlled manipulation of vacancies for specific applications is a challenge. Here we report a facile method for creating large concentrations of S vacancies in the inert basal plane of MoS2 supported on semimetal CoMoP2. With a small applied potential, S atoms can be removed in the form of H2S due to the optimized free energy of formation. The existence of vacancies favors electron injection from the electrode to the active site by decreasing the contact resistance. As a consequence, the activity is increased by 221 % with the vacancy-rich MoS2 as electrocatalyst for hydrogen evolution reaction (HER). A small overpotential of 75 mV is needed to deliver a current density of 10 mA cm-2, which is considered among the best values achieved for MoS2. It is envisaged that this work may provide a new strategy for utilizing the semimetal phase for structuring MoS2 into a multi-functional material.

cond-mat.mtrl-sci↗

arXiv2020

In situ modification of delafossite type PdCoO2 bulk single crystal for reversible hydrogen sorption and fast hydrogen evolution

The observation of extraordinarily high conductivity in delafossite-type PdCoO2 is of great current interest, and there is some evidence that electrons behave like a fluid when flowing in bulk crystals of PdCoO2. Thus, this material is an ideal platform for the study of the electron transfer processes in heterogeneous reactions. Here, we report the use of bulk single crystal PdCoO2 as a promising electrocatalyst for hydrogen evolution reactions (HERs). An overpotential of only 31 mV results in a current density of 10 mA cm^(-2), accompanied by high long-term stability. We have precisely determined that the crystal surface structure is modified after electrochemical activation with the formation of strained Pd nanoclusters in the surface layer. These nanoclusters exhibit reversible hydrogen sorption and desorption, creating more active sites for hydrogen access. The bulk PdCoO2 single crystal with ultra-high conductivity, which acts as a natural substrate for the Pd nanoclusters, provides a high-speed channel for electron transfer

cond-mat.mtrl-sci↗

arXiv2020

Zero-field Nernst effect in a ferromagnetic kagome-lattice Weyl-semimetal Co3Sn2S2

The discovery of magnetic topological semimetals recently attracted significant attention in the field of topology and thermoelectrics. In a thermoelectric device based on the Nernst geometry, an external magnet is required as an integral part. We report a zero-field Nernst effect in a newly discovered hard-ferromagnetic kagome-lattice Weyl-semimetal Co3Sn2S2. A maximum Nernst thermopower of 3 microvolt/K at 80 K in zero field is achieved in this magnetic Weyl-semimetal. Our results demonstrate the possibility of application of topological hard magnetic semimetals for low-power thermoelectric devices based on the Nernst effect and are thus valuable for the comprehensive understanding of transport properties in this class of materials.

cond-mat.mtrl-sci↗

arXiv2020

Comprehensive scan for nonmagnetic Weyl semimetals with nonlinear optical response

As the development of topological band theory, comprehensive databases about time reversal and crystalline symmetries protected nonmagnetic topological materials were developed via first-principles calculations recently. However, owing to the low symmetry requirement of Weyl points, the symmetry-based topological indicator cannot be applied to Weyl semimetals (WSMs). Hitherto, the WSMs with Weyl points in arbitrary positions are still absent in the well-known databases. In this work, we develop an efficient algorithm to search for Weyl points automatically and establish a database of nonmagnetic WSMs with Weyl points near Fermi level based on the total experimental noncentrosymmetric crystal structures in the Inorganic Crystal Structure Database (ICSD). Totally 46 Weyl semimetals were discovered to have nearly clean Fermi surface and Weyl points near Fermi level within 300 meV, and 9 of them are chiral structures which may host the quantized circular photogalvanic effect. In addition, the nonlinear optical response is studied and giant shift current is explored in the end. Besides nonmagnetic WSMs, our powerful tools can also be used in the discovery of magnetic topological materials.

cond-mat.mtrl-sci↗

arXiv2020

Chiral Topological Semimetal with Multifold Band Crossings and Long Fermi arcs

Topological semimetals in crystals with a chiral structure (which possess a handedness due to a lack of mirror and inversion symmetries) are expected to display numerous exotic physical phenomena, including fermionic excitations with large topological charge [1], long Fermi arc surface states [2,3], unusual magnetotransport [4] and lattice dynamics [5], as well as a quantized response to circularly polarized light [6]. To date, all experimentally confirmed topological semimetals exist in crystals that contain mirror operations, meaning that these properties do not appear. Here, we show that AlPt is a structurally chiral topological semimetal that hosts new fourfold and sixfold fermions, which can be viewed as a higher spin eneralization of Weyl fermions without equivalence in elementary particle physics. These multifold fermions are located at high symmetry points and have Chern numbers larger than those in Weyl semimetals, thus resulting in multiple Fermi arcs that span the full diagonal of the surface Brillouin zone. By imaging these long Fermi arcs, we experimentally determine the magnitude and sign of their Chern number, allowing us to relate their dispersion to the handedness of their host crystal.

cond-mat.mes-hall↗

arXiv2020

Emerging chiral edge states from the confinement of a magnetic Weyl semimetal in Co$_3$Sn$_2$S$_2$

The quantum anomalous Hall effect (QAHE) and magnetic Weyl semimetals (WSMs) are topological states induced by intrinsic magnetic moments and spin-orbit coupling. Their similarity suggests the possibility of achieving the QAHE by dimensional confinement of a magnetic WSM along one direction. In this study, we investigate the emergence of the QAHE in the two-dimensional (2D) limit of magnetic WSMs due to finite size effects in thin films and step-edges. We demonstrate the feasibility of this approach with effective models and real materials. To this end, we have chosen the layered magnetic WSM Co$_3$Sn$_2$S$_2$, which features a large anomalous Hall conductivity and anomalous Hall angle in its 3D bulk, as our material candidate. In the 2D limit of Co$_3$Sn$_2$S$_2$ two QAHE states exist depending on the stoichiometry of the 2D layer. One is a semimetal with a Chern number of 6, and the other is an insulator with a Chern number of 3. The latter has a band gap of 0.05 eV, which is much larger than that in magnetically doped topological insulators. Our findings naturally explain the existence of chiral states in step edges of bulk Co$_3$Sn$_2$S$_2$ which habe been reported in a recent experiment at $T = 4K$ and present a realistic avenue to realize QAH states in thin films of magnetic WSMs.

cond-mat.str-el↗

arXiv2020

Anisotropic electrical and thermal magnetotransport in the magnetic semimetal GdPtBi

The half-Heusler rare-earth intermetallic GdPtBi has recently gained attention due to peculiar magnetotransport phenomena that have been associated with the possible existence of Weyl fermions, thought to arise from the crossings of spin-split conduction and valence bands. On the other hand, similar magnetotransport phenomena observed in other rare-earth intermetallics have often been attributed to the interaction of itinerant carriers with localized magnetic moments stemming from the $4f$-shell of the rare-earth element. In order to address the origin of the magnetotransport phenomena in GdPtBi, we performed a comprehensive study of the magnetization, electrical and thermal magnetoresistivity on two single-crystalline GdPtBi samples. In addition, we performed an analysis of the Fermi surface via Shubnikov-de Haas oscillations in one of the samples and compared the results to \emph{ab initio} band structure calculations. Our findings indicate that the electrical and thermal magnetotransport in GdPtBi cannot be solely explained by Weyl physics and is strongly influenced by the interaction of both itinerant charge carriers and phonons with localized magnetic Gd-ions and possibly also paramagnetic impurities.

cond-mat.mes-hall↗

arXiv2020

Dirac Fermions in Antiferromagnetic FeSn Kagome Lattices with Combined Space Inversion and Time Reversal Symmetry

Symmetry principles play a critical role in formulating the fundamental laws of nature, with a large number of symmetry-protected topological states identified in recent studies of quantum materials. As compelling examples, massless Dirac fermions are jointly protected by the space inversion symmetry $P$ and time reversal symmetry $T$ supplemented by additional crystalline symmetry, while evolving into Weyl fermions when either $P$ or $T$ is broken. Here, based on first-principles calculations, we reveal that massless Dirac fermions are present in a layered FeSn crystal containing antiferromagnetically coupled ferromagnetic Fe kagome layers, where each of the $P$ and $T$ symmetries is individually broken but the combined $PT$ symmetry is preserved. These stable Dirac fermions protected by the combined $PT$ symmetry with additional non-symmorphic $S_{\rm{2z}}$ symmetry can be transformed to either massless/massive Weyl or massive Dirac fermions by breaking the $PT$ or $S_{\rm{2z}}$ symmetry. Our angle-resolved photoemission spectroscopy experiments indeed observed the Dirac states in the bulk and two-dimensional Weyl-like states at the surface. The present study substantially enriches our fundamental understanding of the intricate connections between symmetries and topologies of matter, especially with the spin degree of freedom playing a vital role.

cond-mat.mtrl-sci↗

arXiv2020

Observation of giant spin-split Fermi-arc with maximal Chern number in the chiral topological semimetal PtGa

Non-symmorphic chiral topological crystals host exotic multifold fermions, and their associated Fermi arcs helically wrap around and expand throughout the Brillouin zone between the high-symmetry center and surface-corner momenta. However, Fermi-arc splitting and realization of the theoretically proposed maximal Chern number rely heavily on the spin-orbit coupling (SOC) strength. In the present work, we investigate the topological states of a new chiral crystal, PtGa, which has the strongest SOC among all chiral crystals reported to date. With a comprehensive investigation using high-resolution angle-resolved photoemission spectroscopy, quantum-oscillation measurements, and state-of-the-art ab initio calculations, we report a giant SOC-induced splitting of both Fermi arcs and bulk states. Consequently, this study experimentally confirms the realization of a maximal Chern number equal to |4| for the first time in multifold fermionic systems, thereby providing a platform to observe large-quantized photogalvanic currents in optical experiments.

cond-mat.mtrl-sci↗

arXiv2020

Resource Allocation for IRS-assisted Full-Duplex Cognitive Radio Systems

In this paper, we investigate the resource allocation design for intelligent reflecting surface (IRS)-assisted full-duplex (FD) cognitive radio systems. In particular, a secondary network employs an FD base station (BS) for serving multiple half-duplex downlink (DL) and uplink (UL) users simultaneously. An IRS is deployed to enhance the performance of the secondary network while helping to mitigate the interference caused to the primary users (PUs). The DL transmit beamforming vectors and the UL receive beamforming vectors at the FD BS, the transmit power of the UL users, and the phase shift matrix at the IRS are jointly optimized for maximization of the total sum rate of the secondary system. The design task is formulated as a non-convex optimization problem taking into account the imperfect knowledge of the PUs' channel state information (CSI) and their maximum interference tolerance. Since the maximum interference tolerance constraint is intractable, we apply a safe approximation to transform it into a convex constraint. To efficiently handle the resulting approximated optimization problem, which is still non-convex, we develop an iterative block coordinate descent (BCD)-based algorithm. This algorithm exploits semidefinite relaxation, a penalty method, and successive convex approximation and is guaranteed to converge to a stationary point of the approximated optimization problem. Our simulation results do not only reveal that the proposed scheme yields a substantially higher system sum rate for the secondary system than several baseline schemes, but also confirm its robustness against CSI uncertainty. Besides, our results illustrate the tremendous potential of IRS for managing the various types of interference arising in FD cognitive radio networks.

cs.IT↗

arXiv2020

A combined laser-based ARPES and 2PPES study of Td-WTe$_2$

Laser-based angle-resolved photoemission spectroscopy (ARPES) and two-photon photoemission spectroscopy (2PPES) are employed to study the valence electronic structure of the Weyl semimetal candidate Td-WTe$_2$ along two high symmetry directions and for binding energies between $\approx$ -1 eV and 5 eV. The experimental data show a good agreement with band structure calculations. Polarization dependent measurements provide furthermore information on initial and intermediate state symmetry properties with respect to the mirror plane of the Td structure of WTe$_2$.

cond-mat.mtrl-sci↗