arXiv subjects

Yi Chen

Publications and source records attributed to Yi Chen.

At least 181 records · Page 10Linked to original sources

arXiv2024

Magnetostatic effect on spin dynamics properties in antiferromagnetic Van der Waals material CrSBr

Van der Waals (vdW) antiferromagnets are exceptional platforms for exploring the spin dynamics of antiferromagnetic materials owing to their weak interlayer exchange coupling. In this study, we examined the antiferromagnetic resonance spectra of anisotropic Van der Waals antiferromagnet CrSBr. In addition to the ordinary resonance modes, we observed a dipolar spin wave mode when the microwave field was oriented perpendicular to the in-plane easy axis of CrSBr. Furthermore, our results uncovered a pronounced dependency of various resonant modes on the orientation of the microwave field, which is pivotal for the accurate determination of exchange coupling constants. Numerical simulations have elucidated this orientation dependence of spin dynamics arises from the magnetostatic effect. This discovery underscores the previously underappreciated significance of dipolar interactions in shaping the dynamical properties of two-dimensional AFM materials, thereby enhancing our understanding of the intrinsic dynamic properties of vdW magnets.

cond-mat.mtrl-sci↗

arXiv2024

Hard-Label Cryptanalytic Extraction of Neural Network Models

The machine learning problem of extracting neural network parameters has been proposed for nearly three decades. Functionally equivalent extraction is a crucial goal for research on this problem. When the adversary has access to the raw output of neural networks, various attacks, including those presented at CRYPTO 2020 and EUROCRYPT 2024, have successfully achieved this goal. However, this goal is not achieved when neural networks operate under a hard-label setting where the raw output is inaccessible. In this paper, we propose the first attack that theoretically achieves functionally equivalent extraction under the hard-label setting, which applies to ReLU neural networks. The effectiveness of our attack is validated through practical experiments on a wide range of ReLU neural networks, including neural networks trained on two real benchmarking datasets (MNIST, CIFAR10) widely used in computer vision. For a neural network consisting of $10^5$ parameters, our attack only requires several hours on a single core.

cs.CR↗

arXiv2024

LLM-Enhanced Software Patch Localization

Open source software (OSS) is integral to modern product development, and any vulnerability within it potentially compromises numerous products. While developers strive to apply security patches, pinpointing these patches among extensive OSS updates remains a challenge. Security patch localization (SPL) recommendation methods are leading approaches to address this. However, existing SPL models often falter when a commit lacks a clear association with its corresponding CVE, and do not consider a scenario that a vulnerability has multiple patches proposed over time before it has been fully resolved. To address these challenges, we introduce LLM-SPL, a recommendation-based SPL approach that leverages the capabilities of the Large Language Model (LLM) to locate the security patch commit for a given CVE. More specifically, we propose a joint learning framework, in which the outputs of LLM serves as additional features to aid our recommendation model in prioritizing security patches. Our evaluation on a dataset of 1,915 CVEs associated with 2,461 patches demonstrates that LLM-SPL excels in ranking patch commits, surpassing the state-of-the-art method in terms of Recall, while significantly reducing manual effort. Notably, for vulnerabilities requiring multiple patches, LLM-SPL significantly improves Recall by 22.83\%, NDCG by 19.41\%, and reduces manual effort by over 25\% when checking up to the top 10 rankings. The dataset and source code are available at \url{https://anonymous.4open.science/r/LLM-SPL-91F8}.

cs.CR↗

arXiv2024

Long-range near-side correlation in $e^+e^-$ Collisions at 183-209 GeV with ALEPH Archived Data

The first measurement of two-particle angular correlations for charged particles with LEP-II data is presented. The study is performed using archived hadronic $e^+e^-$ data collected by ALEPH at center-of-mass energies up to 209 GeV, above the $W^+W^-$ production threshold, which provide access to unprecedented charged-particle multiplicities and more complex color-string configurations if compared to previous measurements at LEP-I energies. An intriguing long-range near-side excess is observed in the correlation function measured with respect to the thrust axis in the highest multiplicity interval $N_{\mathrm{trk}}\geq 50$. Such a structure is not predicted by the Monte-Carlo simulation. The harmonic anisotropy coefficients $v_n$, which result from the Fourier expansion of the two-particle correlation functions, were also measured for the first time in $e^+e^-$ data, and compared to PYTHIA6 predictions and to the results obtained in proton-proton collisions. The results presented in the Letter provide novel experimental constraints on the formation of collective phenomena in point-like $e^+e^-$ collisions.

hep-ex↗

arXiv2024

Methodological Explainability Evaluation of an Interpretable Deep Learning Model for Post-Hepatectomy Liver Failure Prediction Incorporating Counterfactual Explanations and Layerwise Relevance Propagation: A Prospective In Silico Trial

Artificial intelligence (AI)-based decision support systems have demonstrated value in predicting post-hepatectomy liver failure (PHLF) in hepatocellular carcinoma (HCC). However, they often lack transparency, and the impact of model explanations on clinicians' decisions has not been thoroughly evaluated. Building on prior research, we developed a variational autoencoder-multilayer perceptron (VAE-MLP) model for preoperative PHLF prediction. This model integrated counterfactuals and layerwise relevance propagation (LRP) to provide insights into its decision-making mechanism. Additionally, we proposed a methodological framework for evaluating the explainability of AI systems. This framework includes qualitative and quantitative assessments of explanations against recognized biomarkers, usability evaluations, and an in silico clinical trial. Our evaluations demonstrated that the model's explanation correlated with established biomarkers and exhibited high usability at both the case and system levels. Furthermore, results from the three-track in silico clinical trial showed that clinicians' prediction accuracy and confidence increased when AI explanations were provided.

cs.CV↗

arXiv2024

Controlling structure and interfacial interaction of monolayer TaSe2 on bilayer graphene

Tunability of interfacial effects between two-dimensional (2D) crystals is crucial not only for understanding the intrinsic properties of each system, but also for designing electronic devices based on ultra-thin heterostructures. A prerequisite of such heterostructure engineering is the availability of 2D crystals with different degrees of interfacial interactions. In this work, we report a controlled epitaxial growth of monolayer TaSe2 with different structural phases, 1H and 1T, on a bilayer graphene (BLG) substrate using molecular beam epitaxy, and its impact on the electronic properties of the heterostructures using angle-resolved photoemission spectroscopy. 1H-TaSe2 exhibits significant charge transfer and band hybridization at the interface, whereas 1T-TaSe2 shows weak interactions with the substrate. The distinct interfacial interactions are attributed to the dual effects from the differences of the work functions as well as the relative interlayer distance between TaSe2 films and BLG substrate. The method demonstrated here provides a viable route towards interface engineering in a variety of transition-metal dichalcogenides that can be applied to future nano-devices with designed electronic properties.

cond-mat.mtrl-sci↗

arXiv2024

Operando probing of nanocracking in CuO-derived Cu during CO$_2$ electroreduction

Identifying and controlling active sites in electrocatalysis remains a grand challenge due to restructuring of catalysts in the complex chemical environments during operation. Inactive precatalysts can transform into active catalysts under reaction conditions, such as oxide-derived Cu (OD-Cu) for CO$_2$ electroreduction displaying improved production of multicarbon (C$_{2+}$) chemicals. Revealing the mechanism of active site origin in OD-Cu catalysts requires in situ/operando characterizations of structure, morphology, and valence state evolution with high spatial and temporal resolution. Applying newly developed electrochemical liquid cell transmission electron microscopy combined with X-ray absorption spectroscopy, our multimodal operando techniques unveil the formation pathways of OD-Cu active sites from CuO bicrystal nanowire precatalysts. Rapid reduction of CuO directly to Cu within 60 seconds generates a nanocrack network throughout the nanowire, via formation of "boundary nanocracks" along the twin boundary and "transverse nanocracks" propagating from the surface to the center of the nanowire. The nanocrack network further reconstructs, leading to a highly porous structure rich in Cu nanograins, with a boosted specific surface area and density of active sites for C$_{2+}$ products. These findings suggest a means to optimize active OD-Cu nanostructures through nanocracking by tailoring grain boundaries in CuO precatalysts. More generally, our advanced operando approach opens new opportunities for mechanistic insights to enable improved control of catalyst structure and performance.

cond-mat.mtrl-sci↗

arXiv2024

PAL: Pluralistic Alignment Framework for Learning from Heterogeneous Preferences

Large foundation models pretrained on raw web-scale data are not readily deployable without additional step of extensive alignment to human preferences. Such alignment is typically done by collecting large amounts of pairwise comparisons from humans ("Do you prefer output A or B?") and learning a reward model or a policy with the Bradley-Terry-Luce (BTL) model as a proxy for a human's underlying implicit preferences. These methods generally suffer from assuming a universal preference shared by all humans, which lacks the flexibility of adapting to plurality of opinions and preferences. In this work, we propose PAL, a framework to model human preference complementary to existing pretraining strategies, which incorporates plurality from the ground up. We propose using the ideal point model as a lens to view alignment using preference comparisons. Together with our novel reformulation and using mixture modeling, our framework captures the plurality of population preferences while simultaneously learning a common preference latent space across different preferences, which can few-shot generalize to new, unseen users. Our approach enables us to use the penultimate-layer representation of large foundation models and simple MLP layers to learn reward functions that are on-par with the existing large state-of-the-art reward models, thereby enhancing efficiency of reward modeling significantly. We show that PAL achieves competitive reward model accuracy compared to strong baselines on 1) Language models with Summary dataset ; 2) Image Generative models with Pick-a-Pic dataset ; 3) A new semisynthetic heterogeneous dataset generated using Anthropic Personas. Finally, our experiments also highlight the shortcoming of current preference datasets that are created using rigid rubrics which wash away heterogeneity, and call for more nuanced data collection approaches.

cs.LG↗

arXiv2024

EgoPlan-Bench: Benchmarking Multimodal Large Language Models for Human-Level Planning

The pursuit of artificial general intelligence (AGI) has been accelerated by Multimodal Large Language Models (MLLMs), which exhibit superior reasoning, generalization capabilities, and proficiency in processing multimodal inputs. A crucial milestone in the evolution of AGI is the attainment of human-level planning, a fundamental ability for making informed decisions in complex environments, and solving a wide range of real-world problems. Despite the impressive advancements in MLLMs, a question remains: How far are current MLLMs from achieving human-level planning? To shed light on this question, we introduce EgoPlan-Bench, a comprehensive benchmark to evaluate the planning abilities of MLLMs in real-world scenarios from an egocentric perspective, mirroring human perception. EgoPlan-Bench emphasizes the evaluation of planning capabilities of MLLMs, featuring realistic tasks, diverse action plans, and intricate visual observations. Our rigorous evaluation of a wide range of MLLMs reveals that EgoPlan-Bench poses significant challenges, highlighting a substantial scope for improvement in MLLMs to achieve human-level task planning. To facilitate this advancement, we further present EgoPlan-IT, a specialized instruction-tuning dataset that effectively enhances model performance on EgoPlan-Bench. We have made all codes, data, and a maintained benchmark leaderboard available to advance future research.

cs.CV↗

arXiv2024

Rayleigh surface waves of extremal elastic materials

Extremal elastic materials here refer to a specific class of elastic materials whose elastic matrices exhibit one or more zero eigenvalues, resulting in soft deformation modes that, in principle, cost no energy. They can be approximated through artificially designed solid microstructures. Extremal elastic materials have exotic bulk wave properties unavailable with conventional solids due to the soft modes, offering unprecedented opportunities for manipulating bulk waves, e.g., acting as phonon polarizers for elastic waves or invisibility cloaks for underwater acoustic waves. Despite their potential, Rayleigh surface waves, crucially linked to bulk wave behaviors of such extremal elastic materials, have largely remained unexplored so far. In this paper, we theoretically investigate the propagation of Rayleigh waves in extremal elastic materials based on continuum theory and verify our findings with designed microstructure metamaterials based on pantographic structures. Dispersion relations and polarizations of Rayleigh waves in extremal elastic materials are derived, and the impact of higher order gradient effects is also investigated by using strain gradient theory. This study provides a continuum model for exploring surface waves in extremal elastic materials and may stimulate applications of extremal elastic materials for controlling surface waves.

physics.class-ph↗

arXiv2024

Mott insulating phase and coherent-incoherent crossover across magnetic phase transition in 2D antiferromagnetic CrSBr

In two-dimensional van der Waals magnetic materials, the interplay between magnetism and electron correlation can give rise to new ground states and lead to novel transport and optical properties. A fundamental question in these materials is how the electron correlation manifests and interacts with the magnetic orders. In this study, we demonstrate that the recently discovered 2D antiferromagnetic material, CrSBr, is a Mott insulator, through the combined use of resonant and temperature-dependent angle-resolved photoemission spectroscopy techiniques, supplemented by dynamical mean-field theory analysis. Intriguingly, we found that as the system transitions from the antiferromagnetic to the paramagnetic phases, its Mott bands undergo a reconfiguration, and a coherent-incoherent crossover, driven by the dissolution of the magnetic order. Our findings reveal a distinctive evolution of band structure associated with magnetic phase transitions, shedding light on the investigation of intricate interplay between correlation and magnetic orders in strongly correlated van der Waals magnetic materials.

cond-mat.str-el↗

arXiv2024

Constrained Ensemble Exploration for Unsupervised Skill Discovery

Unsupervised Reinforcement Learning (RL) provides a promising paradigm for learning useful behaviors via reward-free per-training. Existing methods for unsupervised RL mainly conduct empowerment-driven skill discovery or entropy-based exploration. However, empowerment often leads to static skills, and pure exploration only maximizes the state coverage rather than learning useful behaviors. In this paper, we propose a novel unsupervised RL framework via an ensemble of skills, where each skill performs partition exploration based on the state prototypes. Thus, each skill can explore the clustered area locally, and the ensemble skills maximize the overall state coverage. We adopt state-distribution constraints for the skill occupancy and the desired cluster for learning distinguishable skills. Theoretical analysis is provided for the state entropy and the resulting skill distributions. Based on extensive experiments on several challenging tasks, we find our method learns well-explored ensemble skills and achieves superior performance in various downstream tasks compared to previous methods.

cs.LG↗

arXiv2024

Engineering liquid-liquid interfaces for high-entropy alloy synthesis

High-entropy alloys (HEAs) with various promising applications have attracted significant interest. However, alloying immiscible metal elements while controlling the morphology and crystallinity remains extremely challenging. We report a general route, by engineering liquid-liquid interfaces, for the synthesis of HEAs with controlled crystallinity (single crystal, mesocrystal, polycrystal, amorphous), morphology (0-dimension, 2-dimension, 3-dimension), and high composition diversity (20 elements) under mild conditions (room temperature to 80 degrees celsius). As reactions can be spatially confined at the liquid-liquid interface, it provides an opportunity to control the kinetics and reduce the alloying temperature. Our real-time observation of the alloying of HEAs reveals hydrogen-enhanced mixing and isothermal solidification that kinetically traps the mixing states due to composition changes. The concept of liquid-liquid interface engineering can be applied to obtain other high-entropy compounds.

cond-mat.mtrl-sci↗

arXiv2024

SEED-Bench-2-Plus: Benchmarking Multimodal Large Language Models with Text-Rich Visual Comprehension

Comprehending text-rich visual content is paramount for the practical application of Multimodal Large Language Models (MLLMs), since text-rich scenarios are ubiquitous in the real world, which are characterized by the presence of extensive texts embedded within images. Recently, the advent of MLLMs with impressive versatility has raised the bar for what we can expect from MLLMs. However, their proficiency in text-rich scenarios has yet to be comprehensively and objectively assessed, since current MLLM benchmarks primarily focus on evaluating general visual comprehension. In this work, we introduce SEED-Bench-2-Plus, a benchmark specifically designed for evaluating \textbf{text-rich visual comprehension} of MLLMs. Our benchmark comprises 2.3K multiple-choice questions with precise human annotations, spanning three broad categories: Charts, Maps, and Webs, each of which covers a wide spectrum of text-rich scenarios in the real world. These categories, due to their inherent complexity and diversity, effectively simulate real-world text-rich environments. We further conduct a thorough evaluation involving 34 prominent MLLMs (including GPT-4V, Gemini-Pro-Vision and Claude-3-Opus) and emphasize the current limitations of MLLMs in text-rich visual comprehension. We hope that our work can serve as a valuable addition to existing MLLM benchmarks, providing insightful observations and inspiring further research in the area of text-rich visual comprehension with MLLMs. The dataset and evaluation code can be accessed at https://github.com/AILab-CVC/SEED-Bench.

cs.CV↗

arXiv2024

Variance-Dependent Regret Bounds for Non-stationary Linear Bandits

We investigate the non-stationary stochastic linear bandit problem where the reward distribution evolves each round. Existing algorithms characterize the non-stationarity by the total variation budget $B_K$, which is the summation of the change of the consecutive feature vectors of the linear bandits over $K$ rounds. However, such a quantity only measures the non-stationarity with respect to the expectation of the reward distribution, which makes existing algorithms sub-optimal under the general non-stationary distribution setting. In this work, we propose algorithms that utilize the variance of the reward distribution as well as the $B_K$, and show that they can achieve tighter regret upper bounds. Specifically, we introduce two novel algorithms: Restarted Weighted$\text{OFUL}^+$ and Restarted $\text{SAVE}^+$. These algorithms address cases where the variance information of the rewards is known and unknown, respectively. Notably, when the total variance $V_K$ is much smaller than $K$, our algorithms outperform previous state-of-the-art results on non-stationary stochastic linear bandits under different settings. Experimental evaluations further validate the superior performance of our proposed algorithms over existing works.

cs.LG↗

arXiv2024

Enhancing Large Language Models Against Inductive Instructions with Dual-critique Prompting

Numerous works are proposed to align large language models (LLMs) with human intents to better fulfill instructions, ensuring they are trustful and helpful. Nevertheless, some human instructions are often malicious or misleading and following them will lead to untruthful and unsafe responses. Previous work rarely focused on understanding how LLMs manage instructions based on counterfactual premises, referred to here as \textit{inductive instructions}, which may stem from users' false beliefs or malicious intents. In this paper, we aim to reveal the behaviors of LLMs towards \textit{inductive instructions} and enhance their truthfulness and helpfulness accordingly. Specifically, we first introduce a benchmark of \underline{\textbf{Indu}}ctive {In\underline{\textbf{st}}ruct}ions (\textsc{\textbf{INDust}}), where the false knowledge is incorporated into instructions in multiple different styles. After extensive human and automatic evaluations, we uncovered a universal vulnerability among LLMs in processing inductive instructions. Additionally, we identified that different inductive styles affect the models' ability to identify the same underlying errors, and the complexity of the underlying assumptions also influences the model's performance. Motivated by these results, we propose \textsc{Dual-critique} prompting to improve LLM robustness against inductive instructions. Our experiments demonstrate that \textsc{Dual-critique} prompting significantly bolsters the robustness of a diverse array of LLMs, even when confronted with varying degrees of inductive instruction complexity and differing inductive styles.

cs.CL↗

arXiv2024

Role Prompting Guided Domain Adaptation with General Capability Preserve for Large Language Models

The growing interest in Large Language Models (LLMs) for specialized applications has revealed a significant challenge: when tailored to specific domains, LLMs tend to experience catastrophic forgetting, compromising their general capabilities and leading to a suboptimal user experience. Additionally, crafting a versatile model for multiple domains simultaneously often results in a decline in overall performance due to confusion between domains. In response to these issues, we present the RolE Prompting Guided Multi-Domain Adaptation (REGA) strategy. This novel approach effectively manages multi-domain LLM adaptation through three key components: 1) Self-Distillation constructs and replays general-domain exemplars to alleviate catastrophic forgetting. 2) Role Prompting assigns a central prompt to the general domain and a unique role prompt to each specific domain to minimize inter-domain confusion during training. 3) Role Integration reuses and integrates a small portion of domain-specific data to the general-domain data, which are trained under the guidance of the central prompt. The central prompt is used for a streamlined inference process, removing the necessity to switch prompts for different domains. Empirical results demonstrate that REGA effectively alleviates catastrophic forgetting and inter-domain confusion. This leads to improved domain-specific performance compared to standard fine-tuned models, while still preserving robust general capabilities.

cs.CL↗

arXiv2024

DSS-o-SAGE: Direction-Scan Sounding-Oriented SAGE Algorithm for Channel Parameter Estimation in mmWave and THz Bands

Investigation of millimeter (mmWave) and Terahertz (THz) channels relies on channel measurements and estimation of multi-path component (MPC) parameters. As a common measurement technique in the mmWave and THz bands, direction-scan sounding (DSS) resolves angular information and increases the measurable distance. Through mechanical rotation, the DSS creates a virtual multi-antenna sounding system, which however incurs signal phase instability and large data sizes, which are not fully considered in existing estimation algorithms and thus make them ineffective. To tackle this research gap, in this paper, a DSS-oriented space-alternating generalized expectation-maximization (DSS-o-SAGE) algorithm is proposed for channel parameter estimation in mmWave and THz bands. To appropriately capture the measured data in mmWave and THz DSS, the phase instability is modeled by the scanning-direction-dependent signal phases. Furthermore, based on the signal model, the DSS-o-SAGE algorithm is developed, which not only addresses the problems brought by phase instability, but also achieves ultra-low computational complexity by exploiting the narrow antenna beam property of DSS. Simulations in synthetic channels are conducted to demonstrate the efficacy of the proposed algorithm and explore the applicable region of the far-field approximation in DSS-o-SAGE. Last but not least, the proposed DSS-o-SAGE algorithm is applied in real measurements in an indoor corridor scenario at 300~GHz. Compared with results using the baseline noise-elimination method, the channel is characterized more correctly and reasonably based on the DSS-o-SAGE.

cs.IT↗