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Yongcheng Deng

Publications and source records attributed to Yongcheng Deng.

13 recordsLinked to original sources

Orbital Hall Effect Enables Field-Free Magnetization Reversal in Ferrimagnets without Additional Conversion Layer

The spin Hall effect provides a well-established route for electrical magnetization control, while the orbital Hall effect offers a powerful yet less explored source of angular momentum. Achieving field-free deterministic switching in straightforward orbital-torque architectures remains challenging. Here, we demonstrate orbital-Hall-current-driven switching in a Mo/CoGd bilayer without the need for a separate orbital-to-spin conversion layer across a wide temperature range. In this simplified geometry, Mo serves as both an orbital and spin current source. However, the spin contribution is insufficient due to weak spin-orbit coupling, which is consistent with first-principles calculations predicting a large orbital Hall conductivity. The adjacent ferrimagnetic CoGd layer provides both orbital-to-spin conversion and the perpendicular switching medium. Planar Hall and current-induced loop-shift measurements reveal a substantial unconventional z-polarized damping-like torque originating from interfacial symmetry breaking. Increasing the Mo thickness from 0.2 to 2 nm increases torque efficiency by approximately 31% (y-polarized) and 71% (z-polarized) components. This enhancement enables field-free deterministic switching with a critical current density down to 2.51 x 10^6 A cm^-2. Our results establish Mo/CoGd bilayers as a compact platform for orbital-current switching and point toward low-power orbitronic memory devices.

cond-mat.mtrl-sci

Harnessing hidden quantum metric response in a 2D magnet via nonlocal photovoltaic effect

The quantum geometry of Bloch wavefunctions underpins a wealth of emergent phenomena in quantum materials. Its imaginary part, the Berry curvature, has long been recognized as a key source for hallmark effects such as quantum Hall and topological phenomena, etc. The real part of quantum geometry, the quantum metric, has recently garnered considerable attention due to predictions of a range of unconventional nonlinear and nonequilibrium responses. Such responses usually vanish in centrosymmetric systems, largely restricting relevant studies to non-centrosymmetric materials. Here we challenge this convention by revealing that the vanished quantum metric response can survive in a hidden form. Using a non-local photovoltaic scheme in a layered magnetic semiconductor, we spatially separate mutually compensating photocurrents and thereby detect such hidden quantum metric response. We demonstrate this effect across distinct magnetic states and down to the ultrathin limit. Moreover, we realize reconfigurable, nonvolatile and probabilistic photodetection enabled by the quantum metric response. These results not only fundamentally expand the material landscape for quantum geometric physics, but also open new gateway to harvest the quantum geometric contributions for state-of-the-art nonvolatile reprogrammable sensing and computing applications.

cond-mat.mes-hall

Epitaxial growth and magneto-transport properties of kagome metal FeGe thin films

Antiferromagnetic kagome metal FeGe has attracted tremendous attention in condensed matter physics due to the charge density wave (CDW) being well below its magnetic transition temperature. Up to now, numerous works on kagome FeGe have been based on single crystal bulk, but its thin film form has still not been reported. Here, we achieved epitaxial growth of FeGe thin films on Al2O3 substrates using molecular beam epitaxy. Structural characterization with x-ray diffraction, atomic force microscopy, and high-resolution scanning transmission electron microscopy reveals single phase with flat surface of kagome FeGe thin films. Moreover, a Néel temperature of 397 K and a rapid variation of Hall coefficient and magnetoresistance around 100 K, which might be related to the CDW, were revealed via transport measurements. The high quality kagome FeGe thin films are expected to provide a versatile platform to study the mechanism of CDW and explore the application of FeGe in antiferromagnetic spintronics.

cond-mat.mtrl-sci

Two-dimensional magnetic tunnel p-n junctions for low-power electronics

For decades, semiconductors and their heterostructures have underpinned both fundamental and applied research across all areas of electronics. Two-dimensional, 2D (atomically thin) semiconductors have now the potential to push further the miniaturization of electronic components, enabling the development of more efficient electronics. Here, we report on a giant anomalous zero-bias spin voltage in magnetic tunnel junctions based on 2D materials. The generation, manipulation and detection of electron spin across a nanometer-thick magnetic tunnel junction do not require any applied bias. It is achieved by exploiting high-quality ferromagnetic/semiconductor interfaces and the asymmetric diffusion of spin-up/spin-down electrons across a semiconductor p-n junction. The large spin-voltage signal exceeds 30,000% and is far greater than the highest magnetoresistance signals reported to date. Our findings reveal unexplored opportunities to transform and amplify spin information for low-power electronics.

cond-mat.mes-hall

Anomalous magnetoresistance in an antiferromagnetic Kagome semimetal heterostructures

Antiferromagnetic Kagome semimetals have attracted tremendous attentions for their potential application in antiferromagnetic topological spintronics. Effectively manipulating Kagome antiferromagnetic states could reveal abundant physical phenomena induced from quantum interactions between topology, spin, and correlation. Here, we achieved tunable spin textures of FeSn thin films via introducing interfacial Dzyaloshinskii Moriya interaction from heavy-metal Pt overlayer. With increasing FeSn thickness, the variable spin textures result in gradual change in Hall resistivity and magnetoresistance. Importantly, an unconventional damped oscillatory-like behavior of magnetoresistance at relatively low magnetic field can be observed in thin FeSn-Pt samples. This oscillatory like magnetoresistance feature was confirmed to be related to the special topological spin textures revealed by magnetic force microscopy measurements. The formation of rich variety of topological spin textures in association with exotic magneto-transport properties in antiferromagnetic Kagome FeSn heterostructures offers new perspectives for understanding the novel emergent phenomena in Kagome antiferromagnets.

cond-mat.mtrl-sci

Orbital Hall Effect Enables Field-Free Magnetization Reversal in Ferrimagnets without Additional Conversion Layer

The spin Hall effect (SHE) enables efficient electrical manipulation of magnetization through the spin Hall current \left(\mathbit{J}_{\mathbit{SHE}}\right), advancing energy-efficient spintronics. In parallel, the orbital Hall effect (OHE) offers an alternative pathway to SHE for converting charge current into an angular momentum flow. In this study, we demonstrate field-free current-induced perpendicular ferrimagnetic deterministic switching within a Mo/CoGd device without an additional orbital-to-spin conversion layer. This is achieved by harnessing localized orbital Hall currents \left(\mathbit{J}_{\mathbit{OHE}}\right) generated in the Mo layer. The in-plane symmetry breaking at the Mo/CoGd surface-interface layer, validated by a pronounced planar Hall effect, gives rise to a substantial unconventional z-polarized damping-like torque. The CoGd serves a dual role: not only as a converter that transforms the significant \mathbit{J}_{\mathbit{OHE}} into \mathbit{J}_{\mathbit{SHE}} but also as a ferrimagnetic self-switching mechanism. This dual functionality enables highly efficient field-free current-induced magnetization switching with a critical current density as low as \mathbf{2}.\mathbf{51}\ \times{\mathbf{10}}^\mathbf{6} A cm-2. Our work highlights the potential of orbital Hall currents for energy-efficient magnetization switching, making a notable contribution to the burgeoning field of orbitronics.

cond-mat.mtrl-sci

Room-temperature van der Waals 2D ferromagnet switching by spin-orbit torques

Emerging wide varieties of the two-dimensional (2D) van der Waals (vdW) magnets with atomically thin and smooth interfaces holds great promise for next-generation spintronic devices. However, due to the lower Curie temperature of the vdW 2D ferromagnets than room temperature, electrically manipulating its magnetization at room temperature has not been realized. In this work, we demonstrate the perpendicular magnetization of 2D vdW ferromagnet Fe3GaTe2 can be effectively switched at room temperature in Fe3GaTe2/Pt bilayer by spin-orbit torques (SOTs) with a relatively low current density of 1.3 10^7A/cm2. Moreover, the high SOT efficiency of ξ_{DL}~0.22 is quantitatively determined by harmonic measurements, which is higher than those in Pt-based heavy metal/conventional ferromagnet devices. Our findings of room-temperature vdW 2D ferromagnet switching by SOTs provide a significant basis for the development of vdW-ferromagnet-based spintronic applications.

physics.app-ph

Large and tunable magnetoresistance in van der Waals Ferromagnet/Semiconductor junctions

Magnetic tunnel junctions (MTJs) with conventional bulk ferromagnets separated by a nonmagnetic insulating layer are key building blocks in spintronics for magnetic sensors and memory. A radically different approach of using atomically-thin van der Waals (vdW) materials in MTJs is expected to boost their figure of merit, the tunneling magnetoresistance (TMR), while relaxing the lattice-matching requirements from the epitaxial growth and supporting high-quality integration of dissimilar materials with atomically-sharp interfaces. We report TMR up to 192% at 10 K in all-vdW Fe3GeTe2/GaSe/Fe3GeTe2 MTJs. Remarkably, instead of the usual insulating spacer, this large TMR is realized with a vdW semiconductor GaSe. Integration of two-dimensional ferromagnets in semiconductor-based vdW junctions offers gate-tunability, bias dependence, magnetic proximity effects, and spin-dependent optical-selection rules. We demonstrate that not just the magnitude, but also the TMR sign is tuned by the applied bias or the semiconductor thickness, enabling modulation of highly spin-polarized carriers in vdW semiconductors.

cond-mat.mtrl-sci

Tunable Rapid Electron Transport in Titanium Oxide Thin Films

Rapid electron transport in the quantum well triggers many novel physical phenomena and becomes a critical point for the high-speed electronics. Here, we found electrical properties of the titanium oxide changed from semiconducting to metallic as the degree of oxidation decreased and Schottky quantum well was formed at the interface. We take the asymmetry interface electron scattering effect into consideration when studying the electrical transport properties of the multilayer thin films. A novel physical conductivity model for the multilayer thin films was developed. We found electron would be transferred from the low-mobility semiconducting and metallic conductive channels to the high-mobility Schottky quantum well conductive channel with an in-plane applied electric field. Electron concentration and mobility of the forming 2DEG in the Schottky quantum well could be tuned thus the nano-devices exhibited non-linear voltage-current curves. The differential resistivity of the nano-devices could decrease by two orders with increasing electric field at room temperature. Weak electron localization of electrons has been experimentally observed in our nano-devices at low temperature, which further demonstrated the existence of 2DEG in the Schottky quantum well. Our work will provide us new physics about the rapid electron transport in the multilayer thin films, and bring novel functional devices for the modern microelectronic industry.

physics.app-ph

Electrically function switchable magnetic domain-wall memory

More-versatile memory is strongly desired for end-users to protect their information in the information era. In particular, bit-level switchable memory, from rewritable to read-only function, allows end-users to prevent any important data from being tampered with. However, no such switchable memory has been reported. We demonstrated the rewritable function can be converted into a read-only function by a sufficiently large current pulse in a U-shaped domain-wall memory composed of an asymmetric Pt/Co/Ru/AlOx heterostructure with strong Dzyaloshinskii-Moriya interaction. Wafer-scale switchable magnetic domain-wall memory arrays on 4-inch Si/SiO2 substrate were designed and fabricated. Furthermore, we confirmed the information can be stored in rewritable or read-only state at bit-level according to the security-needs of end-users. Our work not only provides a solution for personal confidential data, but also paves the way for developing multi-functional spintronic devices.

physics.app-ph

All-electrical switching of a topological non-collinear antiferromagnet at room temperature

Non-collinear antiferromagnetic Weyl semimetals, combining the advantages of a zero stray field and ultrafast spin dynamics as well as a large anomalous Hall effect and the chiral anomaly of Weyl fermions, have attracted extensive interests. However, the all-electrical control of such systems at room temperature, a crucial step toward practical applications, has not been reported. Here using a small writing current of around 5*10^{6} A/cm^{2}, we realize the all-electrical current-induced deterministic switching of the non-collinear antiferromagnet Mn3Sn with a strong readout signal at room temperature in the Si/SiO2/Mn3Sn/AlOx structure, without external magnetic field and injected spin current. Our simulations reveal that the switching is originated from the current-induced intrinsic non-collinear spin-orbit torques in Mn3Sn itself. Our findings pave the way for the development of topological antiferromagnetic spintronics.

cond-mat.mes-hall

All-Linear Multistate Magnetic Switching Induced by Electrical Current

We present an alternative mechanism to control the domain wall motion, whose directions are manipulated by the amplitude of electrical currents when modulating the ratio of D/A (constants of Dzyaloshinskii-Moriya interaction over exchange interaction). To confirm this mechanism, we observe this type of domain wall motion and demonstrate linear magnetic switching without hysteresis effect via adjusting the D/A of Ta/Pt/Co/Ta multilayer device with ion implantations. We further find field-free biased and chirally controllable multistate switching at the lateral interface of ion exposed and unexposed area, which is due to the current induced Neel wall motion and a strong exchange coupling at this interface.

physics.app-ph

Spin Logic Devices via Electric Field Controlled Magnetization Reversal by Spin-Orbit Torque

We describe a spin logic device with controllable magnetization switching of perpendicularly magnetized ferromagnet / heavy metal structures on a ferroelectric (1-x)[Pb(Mg1/3Nb2/3)O3]-x[PbTiO3] (PMN-PT) substrate using current-induced spin-orbit torque. The devices were operated without an external magnetic field and controlled by voltages as low as 10 V applied across the PMN-PT substrate, which is much lower compared to previous reports (500 V). The deterministic switching with smaller voltage was realized from the virgin state of the PMN-PT. Ferroelectric simulation shows the unsaturated minor loop exhibits obvious asymmetries in the polarizations. Larger polarization can be induced from the initial ferroelectric state, while it is difficult for opposite polarization. The XNOR, AND, NAND and NOT logic functions were demonstrated by the deterministic magnetization switching from the interaction between the spin-orbit torque and electric field at the PMN-PT/Pt interface. The nonvolatile spin logic scheme in this work is simple, scalable, programmable, which are favorable in the logic-in-memory design with low energy consumption.

physics.app-ph