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Yoon Seok Oh

Publications and source records attributed to Yoon Seok Oh.

28 records · Page 2Linked to original sources

Electric field control of nonvolatile four-state magnetization at room temperature

We find the realization of large converse magnetoelectric (ME) effects at room temperature in a multiferroic hexaferrite Ba$_{0.52}$Sr$_{2.48}$Co$_{2}$Fe$_{24}$O$_{41}$ single crystal, in which rapid change of electric polarization in low magnetic fields (about 5 mT) is coined to a large ME susceptibility of 3200 ps/m. The modulation of magnetization then reaches up to 0.62 $μ$$_{B}$/f.u. in an electric field of 1.14 MV/m. We find further that four ME states induced by different ME poling exhibit unique, nonvolatile magnetization versus electric field curves, which can be approximately described by an effective free energy with a distinct set of ME coefficients.

cond-mat.mtrl-sci↗

Strong magnetoelastic effect on the magnetoelectric phenomena of TbMn$_{2}$O$_{5}$

Comparative studies of magnetoelectric susceptibility ($α$), magnetization ($M$), and magnetostriction ($u$) in TbMn$_{2}$O$_{5}$ reveal that the increment of $M$ owing to the field-induced Tb$^{3+}$ spin alignment coins a field-asymmetric line shape in the $α(H)$ curve, being conspicuous in a low temperature incommensurate phase but persistently subsisting in the entire ferroelectric phase. Correlations among electric polarization, $u$, and $M^{2}$ variation represent linear relationships, unambiguously showing the significant role of Tb magnetoelastic effects on the low field magnetoelectric phenomena of TbMn$_{2}$O$_{5}$. An effective free energy capturing the observed experimental features is also suggested.

cond-mat.str-el↗

Quantitative determination of anisotropic magnetoelectric coupling in BiFeO$_{3}$-CoFe$_{2}$O$_{4}$ nanostructures

The transverse and longitudinal magnetoelectric susceptibilities (MES) were quantitatively determined for (001) heteroepitaxial BiFeO$_{3}$-CoFe$_{2}$O$_{4}$ nanostructures. Both of these MES values were sharply enhanced at magnetic fields below 6 kOe and revealed asymmetric lineshapes with respect to the dc magnetic field, demonstrating the strain-induced magnetoelectric effect. The maximum transverse MES, which reached as high as $\sim$60 mV/cm Oe, was about five times larger than the longitudinal MES. This observation signifies that transverse magnetostriction of the CoFe$_{2}$O$_{4}$ nanopillars is enhanced more than the bulk value due to preferred magnetic domain alignment along the [001] direction coming from compressive, heteroepitaxial strain.

cond-mat.str-el↗

Evidence of a universal and isotropic 2Δ/kBTC ratio in 122-type iron pnictide superconductors over a wide doping range

We have systematically investigated the doping and the directional dependence of the gap structure in the 122-type iron pnictide superconductors by point contact Andreev reflection spectroscopy. The studies were performed on single crystals of Ba1-xKxFe2As2 (x = 0.29, 0.49, and 0.77) and SrFe1.74Co0.26As2 with a sharp tip of Pb or Au pressed along the c-axis or the ab-plane direction. The conductance spectra obtained on highly transparent contacts clearly show evidence of a robust superconducting gap. The normalized curves can be well described by the Blonder-Tinkham-Klapwijk model with a lifetime broadening. The determined gap value scales very well with the transition temperature, giving the 2Δ/kBTC value of ~ 3.1. The results suggest the presence of a universal coupling behavior in this class of iron pnictides over a broad doping range and independent of the sign of the doping. Moreover, conductance spectra obtained on c-axis junctions and ab-plane junctions indicate that the observed gap is isotropic in these superconductors.

cond-mat.supr-con↗

NMR study on the stability of the magnetic ground state in MnCr${}_2$O${}_4$

The canting angles and fluctuation of the magnetic ion spins of spinel oxide MnCr${}_2$O${}_4$ were studied by nuclear magnetic resonance (NMR) at low temperatures, which has a collinear ferrimagnetic order below $T_C$ and a ferrimagnetic spiral order below $T_s < T_C$. Contrary to previous reports, only one spin canting angle of Cr ions was observed. The spin canting angles of Mn and Cr ions in the ferrimagnetic spiral obtained at a liquid-He temperature were $43\,^{\circ}$ and $110\,^{\circ}$, respectively. The nuclear spin-spin relaxation was determined by the Suhl-Nakamura interaction at low temperatures but the relaxation rate $T_2^{-1}$ increases rapidly as the temperature approaches $T_s$. This indicates that the fluctuation of the spiral component becomes faster as the temperature increases but not fast enough to leave an averaged hyperfine field to nuclei in the time scale of nuclear spin precession in the ferrimagnetic phase, which is on the order of $10^{-8}$ s. The spiral volume fraction measured for various temperatures reveals that the collinear and the spiral ferrimagnetic phases are mixed below the transition temperature of the spiral order. The temperature hysteresis in the volume fraction implies that this transition has first-order characteristics.

cond-mat.str-el↗

Realization of giant magnetoelectricity in helimagnets

We show that low field magnetoelectric (ME) properties of helimagnets Ba0.5Sr1.5Zn2(Fe1-xAlx)12O22 can be efficiently tailored by Al-substitution level. As x increases, the critical magnetic field for switching electric polarization is systematically reduced from ~1 T down to ~1 mT, and the ME susceptibility is greatly enhanced to reach a giant value of 2.0 x 10^4 ps/m at an optimum x = 0.08. We find that control of nontrivial orbital moment in the octahedral Fe sites through the Al-substitution is crucial for fine tuning of magnetic anisotropy and obtaining the conspicuously improved ME characteristics.

cond-mat.mtrl-sci↗

Josephson effect between electron-doped and hole-doped iron pnictide single crystals

We have observed the Josephson effect in junctions formed between single crystals of SrFe1.74Co0.26As2 and Ba0.23K0.77Fe2As2. I-V curves showed resistively-shunted junction characteristics, and the ac Josephson effect was observed under microwave irradiation. By applying an in-plane magnetic field, the critical current is completely modulated and shows a relatively symmetric diffraction pattern, consistent with the intermediate junction limit. The observation of the Josephson effect in the p-n bicrystal structure not only has significant implications for designing phase-sensitive junctions to probe the pairing symmetry of iron pnictide superconductors, but also represents an important step in developing all iron pnictide devices for applications.

cond-mat.supr-con↗

Observation of the Josephson effect in Pb/(Ba,K)Fe2As2 single crystal junctions

We have fabricated c-axis Josephson junctions on single crystals of (Ba,K)Fe2As2 by using Pb as the counter electrode in two geometries, planar and point contact. Junctions in both geometries show resistively shunted junction I-V curves below the Tc of the counter electrode. Microwave induced steps were observed in the I-V curves, and the critical currents are suppressed with an in-plane magnetic field in a manner consistent with the small junction limit. ICRN products of up to 0.3 mV have been observed in these junctions at 4.2 K. The observation of Josephson coupling along the c-axis between (Ba,K)Fe2As2 and a conventional superconductor suggests the existence of a s-wave superconducting order parameter in this class of iron pnictide superconductors.

cond-mat.supr-con↗

Vortex-glass phase transition and superconductivity in an under- doped (Ba,K)Fe2As2 single crystal

Measurements of magnetotransport and current-voltage (I-V) characteristics up to 9 T were used to investigate the vortex phase diagram of an under-doped Measurements of magnetotransport and current-voltage (I-V) characteristics up to 9 T were used to investigate the vortex phase diagram of an under-doped (Ba,K)Fe2As2 single crystal with Tc=26.2 K. It is found that the anisotropy ratio of the upper critical field Hc2 decreases from 4 to 2.8 with decreasing temperature from Tc to 24.8 K. Consistent with the vortex-glass theory, the I-V curves measured at H=9 T can be well scaled with the vortex-glass transition temperature of Tg=20.7 K and critical exponents z=4.1 and v=1. Analyses in different magnetic fields produced almost identical critical exponent values, with some variation in Tg, corroborating the existence of the vortex-glass transition in this under-doped (Ba,K)Fe2As2 single crystal up to 9 T. A vortex phase diagram is presented, based on the evolution of Tg and Hc2 with magnetic field.

cond-mat.supr-con↗

Magnetoelectric effects of nanoparticulate Pb(Zr0.52Ti0.48)O3-NiFe2O4 composite films

We fabricated Pb(Zr0.52Ti0.48)O3-NiFe2O4 composite films consisting of randomly dispersed NiFe2O4 nanoparticles in the Pb(Zr0.52Ti0.48)O3 matrix. The structural analysis revealed that the crystal axes of the NiFe2O4 nanoparticles are aligned with those of the ferroelectric matrix. The composite has good ferroelectric and magnetic properties. We measured the transverse and longitudinal components of the magnetoelectric voltage coefficient, which supports the postulate that the magnetoelectric effect comes from direct stress coupling between magnetostrictive NiFe2O4 and piezoelectric Pb(Zr0.52Ti0.48)O3 grains.

cond-mat.mtrl-sci↗