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Youguang Zhang

Publications and source records attributed to Youguang Zhang.

At least 19 recordsLinked to original sources

Single femtosecond laser pulse-driven ferromagnetic switching

Light pulses offer a faster, more energy-efficient, and direct route to magnetic bit writing, pointing toward a hybrid memory and computing paradigm based on photon transmission and spin retention. Yet progress remains hindered, as deterministic, single-pulse optical toggle switching has so far been achieved only with ferrimagnetic materials, which require too specific a rare-earth composition and temperature conditions for technological use. In mainstream ferromagnet--central to spintronic memory and storage--such bistable switching is considered fundamentally difficult, as laser-induced heating does not inherently break time-reversal symmetry. Here, we report coherent magnetization switching in ferromagnets, driven by thermal anisotropy torque with single laser pulses. The toggle switching behavior is robust over a broad range of pulse durations, from femtoseconds to picoseconds, a prerequisite for practical applications. Furthermore, the phenomenon exhibits reproducibility in CoFeB/MgO-based magnetic tunnel junctions with a high magnetoresistance exceeding 110%, as well as the scalability down to nanoscales with remarkable energy efficiency (17 fJ per 100-nm-sized bit). These results mark a notable step toward integrating opto-spintronics into next-generation memory and storage technologies.

cond-mat.mes-hall

Single-shot optical precessional magnetization switching of Pt/Co/Pt ferromagnetic trilayers

Ultra-fast magnetization switching triggered by a single femtosecond laser pulse has gained significant attention over the last decade for its potential in low-power consumption, high-speed memory applications. However, this phenomenon has been primarily observed in Gd-based ferrimagnetic materials, which are unsuitable for storage due to their weak perpendicular magnetic anisotropy (PMA). In this work, we demonstrated that applying a single laser pulse and an in-plane magnetic field can facilitate magnetic switching in a Pt/Co/Pt ferromagnetic trilayers stack within a specific laser power window. To further understand this phenomenon, we introduce a Cu layer to accelerates the re-establishment time of the anisotropy field of Pt/Co/Pt trilayers, which leads to bullseye-patterned magnetic switching. We have mapped state diagrams for these phenomena, and through micromagnetic simulations, we have determined that these switchings are influenced by thermal anisotropy torque, which can be modulated through PMA. These findings indicate that single-shot optical precessional magnetization reversal is feasible in a broader range of materials, opening avenues for the development of optical-magnetic memory devices.

cond-mat.mtrl-sci

Triple-Q state in magnetic breathing kagome lattice

Magnetic frustration in two-dimensional spin lattices with triangular motifs underpins a series of exotic states, ranging from multi-Q configurations to disordered spin-glasses. The antiferromagnetic kagome lattice, characterized by its network of corner-sharing triangles, represents a paradigmatic frustrated system exhibiting macroscopic degeneracy. Expanding upon the kagomerization mechanism, we focus on the magnetic breathing kagome lattice formed by a Mn monolayer deposited on a heavy metal substrate and capped with h-BN. The Mn kagome arrangement induces pronounced magnetic frustration, as evidenced by the nearly flat bands derived from spin spiral energy calculations. Including further-neighbor interactions reveals a spin spiral energy minimum along the $Γ$-K line and an intriguing triple-Q state with nonzero topological charge, potentially leading to highly nonlinear Hall effects. Furthermore, the flat band properties can further give rise to an even more complex spin configuration, marked by several Q-pockets in the spin structure factor. These results present a fertile ground for advancing the study of multi-Q states and exploring emergent topological phenomena.

cond-mat.mtrl-sci

Kagomerization of transition metal monolayers induced by two-dimensional hexagonal boron nitride

The kagome lattice is an exciting solid state physics platform for the emergence of nontrivial quantum states driven by electronic correlations: topological effects, unconventional superconductivity, charge and spin density waves, and unusual magnetic states such as quantum spin liquids. While kagome lattices have been realized in complex multi-atomic bulk compounds, here we demonstrate from first-principles a process that we dub kagomerization, in which we fabricate a two-dimensional kagome lattice in monolayers of transition metals utilizing a hexagonal boron nitride (h-BN) overlayer. Surprisingly, h-BN induces a large rearrangement of the transition metal atoms supported on a fcc(111) heavy-metal surface. This reconstruction is found to be rather generic for this type of heterostructures and has a profound impact on the underlying magnetic properties, ultimately stabilizing various topological magnetic solitons such as skyrmions and bimerons. Our findings call for a reconsideration of h-BN as merely a passive capping layer, showing its potential for not only reconstructing the atomic structure of the underlying material, e.g. through the kagomerization of magnetic films, but also enabling electronic and magnetic phases that are highly sought for the next generation of device technologies.

cond-mat.mtrl-sci

NAND-SPIN-Based Processing-in-MRAM Architecture for Convolutional Neural Network Acceleration

The performance and efficiency of running large-scale datasets on traditional computing systems exhibit critical bottlenecks due to the existing "power wall" and "memory wall" problems. To resolve those problems, processing-in-memory (PIM) architectures are developed to bring computation logic in or near memory to alleviate the bandwidth limitations during data transmission. NAND-like spintronics memory (NAND-SPIN) is one kind of promising magnetoresistive random-access memory (MRAM) with low write energy and high integration density, and it can be employed to perform efficient in-memory computation operations. In this work, we propose a NAND-SPIN-based PIM architecture for efficient convolutional neural network (CNN) acceleration. A straightforward data mapping scheme is exploited to improve the parallelism while reducing data movements. Benefiting from the excellent characteristics of NAND-SPIN and in-memory processing architecture, experimental results show that the proposed approach can achieve $\sim$2.6$\times$ speedup and $\sim$1.4$\times$ improvement in energy efficiency over state-of-the-art PIM solutions.

cs.AR

Field-free spin-orbit torque-induced switching of perpendicular magnetization in a ferrimagnetic layer with vertical composition gradient

Current-induced spin-orbit torques (SOTs) are of interest for fast and energy-efficient manipulation of magnetic order in spintronic devices. To be deterministic, however, switching of perpendicularly magnetized materials by SOT requires a mechanism for in-plane symmetry breaking. Existing methods to do so involve the application of an in-plane bias magnetic field, or incorporation of in-plane structural asymmetry in the device, both of which can be difficult to implement in practical applications. Here, we reported bias-field-free SOT switching in a single perpendicular CoTb layer with an engineered vertical composition gradient. The vertical structural inversion asymmetry induces strong intrinsic SOTs and a gradient-driven Dzyaloshinskii-Moriya interaction (g-DMI), which breaks the in-plane symmetry during the switching process. Micromagnetic simulations are in agreement with experimental results, and elucidate the role of g-DMI in the deterministic switching. This bias-field-free switching scheme for perpendicular ferrimagnets with g-DMI provides a strategy for efficient and compact SOT device design.

cond-mat.mes-hall

Stochastic Computing Implemented by Skyrmionic Logic Devices

Magnetic skyrmion, topologically non-trivial spin texture, has been considered as promising information carrier in future electronic devices because of its nanoscale size, low depinning current density and high motion velocity. Despite the broad interests in skyrmion racetrack memory, researchers have been recently exploiting logic functions enabled by using the particle-like behaviors of skyrmions. These functions can be applied to unconventional computing, such as stochastic computing (SC), which treats data as probabilities and is superior to binary computing due to its simplicity of logic operation. In this work, we demonstrate SC implemented by skyrmionic logic devices. We propose a skyrmionic AND-OR logic device as a multiplier in the stochastic domain and two skyrmionic multiplexer (MUX) logic devices as stochastic adders. With the assist of voltage controlled magnetic anisotropy (VCMA), the precise control of skyrmions collision is not required in the skyrmionic AND-OR logic device, thus improving the operation robustness. In the two MUX logic devices, skyrmions can be driven by Zhang-Li torque or spin orbit torque (SOT). Particularly, we can flexibly regulate the skyrmion motion by VCMA or voltage controlled Dzyaloshinskii-Moriya Interaction (VCDMI) in the SOT case. Furthermore, 3-bit stochastic multiplier and adder are demonstrated by micromagnetic simulations. In addition, simulations in synthetic antiferromagnets (SAF) show that the performance of our skyrmionic logic gates can be optimized through advanced materials. Our work opens up perspective to implement SC using skyrmionic logic devices.

physics.app-ph

Thermal Brownian Motion of Skyrmion for True Random Number Generation

The true random number generators (TRNGs) have received extensive attention because of their wide applications in information transmission and encryption. The true random numbers generated by TRNG are typically applied to the encryption algorithm or security protocol of the information security core. Recently, TRNGs have also been employed in emerging stochastic computing paradigm for reducing power consumption. Roughly speaking, TRNG can be divided into circuits-based, e.g., oscillator sampling or directly noise amplifying; and quantum physics-based, e.g., photoelectric effect. The former generally requires a large area and has a large power consumption, whereas the latter is intrinsic random but is more difficult to implement and usually requires additional post-processing circuitry. Very recently, magnetic skyrmion has become a promising candidate for implementing TRNG because of their nanometer size, high stability, and intrinsic thermal Brownian motion dynamics. In this work, we propose a TRNG based on continuous skyrmion thermal Brownian motion in a confined geometry at room temperature. True random bitstream can be easily obtained by periodically detecting the relative position of the skyrmion without the need for additional current pulses. More importantly, we implement a probability-adjustable TRNG, in which a desired ratio of 0 and 1 can be acquired by adding an anisotropy gradient through voltage-controlled magnetic anisotropy (VCMA) effect. The behaviors of the skyrmion-based TRNG are verified by using micromagnetic simulations. The National Institute of Standards and Technology (NIST) test results demonstrate that our proposed random number generator is TRNG with good randomness. Our research provides a new perspective for efficient TRNG realization.

physics.app-ph

Universal transfer and stacking technique of van der Waals heterostructures for spintronics

The key to achieving high-quality van der Waals heterostructure devices made from various two-dimensional (2D) materials lies in the control over clean and flexible interfaces. However, existing transfer methods based on different mediators possess insufficiencies including the presence of residues, the unavailability of flexible interface engineering, and the selectivity towards materials and substrates since their adhesions differ considerably with the various preparation conditions, from chemical vapor deposition (CVD) growth to mechanical exfoliation. In this paper, we introduce a more universal method using a prefabricated polyvinyl alcohol (PVA) film to transfer and stack 2D materials, whether they are prepared by CVD or exfoliation. This peel-off and drop-off technique promises an ideal interface of the materials without introducing contamination. In addition, the method exhibits a micron-scale spatial transfer accuracy and meets special experimental conditions such as the preparation of twisted graphene and the 2D/metal heterostructure construction. We illustrate the superiority of this method with a WSe2 vertical spin valve device, whose performance verifies the applicability and advantages of such a method for spintronics. Our PVA-assisted transfer process will promote the development of high-performance 2D-material-based devices.

physics.app-ph

Frequency Modulation and Voltage Locking of the Voltage Controlled Spin Oscillators (VCSOs)

The oscillating frequency of typical Spin Torque Nano Oscillators (STNOs) can be modulated by injected DC current or bias magnetic field. And phase locking of STNOs to an external Radio Frequency (RF) signal can be imposed by AC current or RF bias magnetic field. However, in this study, we have proposed a Voltage Controlled Spin Oscillators (VCSOs) by introducing Voltage Controlled Magnetic Anisotropy (VCMA) effect. The oscillating frequency of VCSOs can be modulated by VCMA voltage as well as injected DC current. Furthermore, we have shown a novel locking mechanism caused by AC VCMA voltage. Both the frequency modulation and voltage locking mechanism are analyzed theoretically by Nonlinear Auto-oscillator theory and verified by numerical simulation. At last, we proposed that by utilizing negative capacitance material to enhance VCMA effect, the locking range for voltage locking can be expanded thus may lead to easy mutual synchronization of multiple VCSOs.

cond-mat.mes-hall

Magnetic skyrmion spectrum under voltage excitation and its linear modulation

Magnetic skyrmions are topological quasiparticles with great potential for applications in future information storage and processing devices because of their nanoscale size, high stability, and large velocity. Recently, the high-frequency properties of skyrmions have been explored for magnon nanodevices. Here we systematically study the dynamics of an isolated skyrmion under voltage excitation through the voltage-controlled magnetic anisotropy effect in a circular thin film. A theoretical model considering the demagnetization energy, which has often been neglected or treated superficially in previous skyrmion research but is demonstrated to have importance in determining the skyrmion dynamic state, is developed. With our model, the periodic oscillation of the skyrmion radius can be solved numerically with similar precision compared to micromgnetic simulations, and the characteristic frequency of the skyrmion breathing can be determined analytically with greater precision than previous studies. Furthermore, we find that the breathing skyrmion can be analogized as a modulator by investigating its linear modulation functionality under sinusoidal-form voltage excitation. Different from the conventional modulation system with complex CMOS circuits, this skyrmion modulator device integrates with both the modulation and carrier wave generation functionality, thus showing greater convenience and efficiency in applications. Our findings can provide useful guidance for both theoretical and experimental skyrmions research as well as the development of skyrmion-based magnonic devices with significant potential applicability in future communication system.

physics.app-ph

Field-free switching of perpendicular magnetic tunnel junction by the interplay of spin orbit and spin transfer torques

Spin-orbit torque and spin-transfer torque are leading the pathway to the future of spintronic memories. However, both of the mechanisms are suffering from intrinsic limitations. In particular, an external magnetic field is required for spin-orbit torque to execute deterministic switching in perpendicular magnetic tunnel junctions; the demand for reduced spin-transfer torque switching current to realize ultralow power is still remaining. Thus, a more advanced switching mechanism is urgently needed to move forward spintronics for wide applications. Here, we experimentally demonstrate the field-free switching of three-terminal perpendicular-anisotropy nanopillar devices through the interaction between spin-orbit and spin-transfer torques. The threshold current density of spin-transfer torque switching is reduced to 0.94 MA.cm-2, which is a significant decrease compared to that in other current-induced magnetization switching mechanisms. In addition, thanks to the interplay of spin-orbit and spin-transfer torques, lower current-induced switching in the conventional two-terminal perpendicular magnetic tunnel junctions is also achieved.

physics.app-ph

Field-Free Switching of Perpendicular Magnetic Tunnel Junction via Voltage-Gated Spin Hall Effect for Low-Power Spintronic Memory

Spin Hall effect (SHE) and voltage-controlled magnetic anisotropy (VCMA) are two promising methods for low-power electrical manipulation of magnetization. Recently, magnetic field-free switching of perpendicular magnetization through SHE has been reported with the aid of an exchange bias from an antiferromagnetic IrMn layer. In this letter, we experimentally demonstrate that the IrMn/CoFeB/MgO structure exhibits a VCMA effect of 39 fJ/Vm, which is comparable to that of the Ta/CoFeB/MgO structure. Magnetization dynamics under a combination of the SHE and VCMA are modeled and simulated. It is found that, by applying a voltage of 1.5 V, the critical SHE switching current can be decreased by 10 times owing to the VCMA effect, leading to low-power operations. Furthermore, a high-density spintronic memory structure can be built with multiple magnetic tunnel junctions (MTJs) located on a single IrMn strip. Through hybrid CMOS/MTJ simulations, we demonstrate that fast-speed write operations can be achieved with power consumption of only 8.5 fJ/bit. These findings reveal the possibility to realize high-density and low-power spintronic memory manipulated by voltage-gated SHE.

physics.app-ph

Heterogeneous Memristive Devices Enabled by Magnetic Tunnel Junction Nanopillars Surrounded by Resistive Silicon Switches

Emerging non-volatile memories (NVMs) have currently attracted great interest for their potential applications in advanced low-power information storage and processing technologies. Conventional NVMs, such as magnetic random access memory (MRAM) and resistive random access memory (RRAM) suffer from limitations of low tunnel magnetoresistance (TMR), low access speed or finite endurance. NVMs with synergetic advantages are still highly desired for future computer architectures. Here, we report a heterogeneous memristive device composed of a magnetic tunnel junction (MTJ) nanopillar surrounded by resistive silicon switches, named resistively enhanced MTJ (Re-MTJ), that may be utilized for novel memristive memories, enabling new functionalities that are inaccessible for conventional NVMs. The Re-MTJ device features a high ON/OFF ratio of >1000% and multilevel resistance behaviour by combining magnetic switching together with resistive switching mechanisms. The magnetic switching originates from the MTJ, while the resistive switching is induced by a point-switching filament process that is related to the mobile oxygen ions. Microscopic evidence of silicon aggregated as nanocrystals along the edges of the nanopillars verifies the synergetic mechanism of the heterogeneous memristive device. This device may provide new possibilities for advanced memristive memory and computing architectures, e.g., in-memory computing and neuromorphics.

physics.app-ph

Voltage-Driven High-Speed Skyrmion Motion in a Skyrmion Shift Device

Magnetic skyrmions are promising information carriers for building future high-density and high-speed spintronic devices. However, to achieve a current-driven high-speed skyrmion motion, the required driving current density is usually very large, which could be energy inefficient and even destroy the device due to Joule heating. Here, we propose a voltage-driven skyrmion motion approach in a skyrmion shift device made of magnetic nanowires. The high-speed skyrmion motion is realized by utilizing the voltage shift, and the average skyrmion velocity reaches up to 259 m/s under 0.45 V applied voltage. In comparison with the widely studied vertical current-driven model, the energy dissipation is three orders of magnitude lower in our voltage-driven model, for the same speed motion of skyrmions. Our approach uncovers valuable opportunities for building skyrmion racetrack memories and logic devices with both ultra-low power consumption and ultra-high processing speed, which are appealing features for future spintronic applications.

physics.app-ph

Ultra-Fast Ferrimagnetic All Spin Logic Device

All spin logic device (ASLD) blazes an alternative path for realizing ultra-low power computing in the Post-Moore era. However, initial device structure relying on ferromagnetic input/output and spin transfer torque (STT) driven magnetization switching degrades its performance and even hinders its realization. In this paper, we propose an ASLD based on rare-earth (RE)-transition-metal (TM) ferromagnetic alloy that can achieve an ultra-high frequency up to terahertz. The spin orbit torque (SOT) induced fast precession near the spin angular momentum compensated point is investigated through the macrospin model. Combining the non-local spin current diffusing from the input to the output, a deterministic picosecond switching can be realized without any external magnetic field. Our results show that ASLD has the potential to exceed the performance of mainstream computing.

physics.app-ph

Intelligent Identification of Two-Dimensional Structure by Machine-Learning Optical Microscopy

Two-dimensional (2D) materials and their heterostructures, with wafer-scale synthesis methods and fascinating properties, have attracted numerous interest and triggered revolutions of corresponding device applications. However, facile methods to realize accurate, intelligent and large-area characterizations of these 2D structures are still highly desired. Here, we report a successful application of machine-learning strategy in the optical identification of 2D structure. The machine-learning optical identification method (MOI method) endows optical microscopy with intelligent insight into the characteristic colour information in the optical photograph. Experimental results indicate that the MOI method enables accurate, intelligent and large-area characterizations of graphene, molybdenum disulphide (MoS2) and their heterostructures, including identifications of the thickness, the existence of impurities, and even the stacking order. Thanks to the convergence of artificial intelligence and nanoscience, this intelligent identification method can certainly promote the fundamental research and wafer-scale device application of 2D structures.

cond-mat.mtrl-sci

First-principles investigation of magnetocrystalline anisotropy oscillations in Co$_{2}$FeAl/Ta heterostructures

We report first-principles investigations of magnetocrystalline anisotropy energy (MCAE) oscillations as a function of capping layer thickness in Heusler alloy Co\textsubscript{2}FeAl/Ta heterostructures. Substantial oscillation is observed in FeAl-interface structure. According to $k$-space and band-decomposed charge density analyses, this oscillation is mainly attributed to the Fermi-energy-vicinal quantum well states (QWS) which are confined between Co\textsubscript{2}FeAl/Ta interface and Ta/vacuum surface. The smaller oscillation magnitude in the Co-interface structure can be explained by the smooth potential transition at the interface. These findings clarify that MCAE in Co\textsubscript{2}FeAl/Ta is not a local property of the interface and that the quantum well effect plays a dominant role in MCAE oscillations of the heterostructures. This work presents the possibility of tuning MCAE by QWS in capping layers, and paves the way for artificially controlling magnetic anisotropy energy in magnetic tunnel junctions.

cond-mat.mtrl-sci