arXiv subjects

Yuxin Leng

Publications and source records attributed to Yuxin Leng.

At least 37 records · Page 2Linked to original sources

arXiv2024

Superluminal spacetime boundary, time reflection and quantum light generation from relativistic plasma mirrors

A plasma mirror is an optical device for high-power, ultrashort-wavelength electromagnetic fields, utilizing a sheet of relativistic oscillating electrons to generate and manipulate light. In this work, we propose that the spatiotemporally varying plasma oscillation, induced by an ultra-high-intensity laser beam, functions as a "spacetime mirror" with significant potential for exploring quantum light. We find that the spacetime mirror exhibits several exotic features: (i) a superluminal spacetime boundary, (ii) time reflection and refraction, and (iii) quantum light sources with pair generation. Our theoretical and simulation results are in excellent agreement, and experimental verification is underway. Our work demonstrates the interplay with emerging fields such as time varying media, suggesting the plasma mirror as an ideal platform to study strong-field quantum optics at extremes.

physics.optics↗

arXiv2024

Multi-watt long-wavelength infrared femtosecond lasers and resonant enamel ablation

High-power broadband tunable long-wavelength infrared (LWIR) femtosecond lasers operating at fingerprint wavelengths of 7-14 μm hold significant promise across a range of applications, including molecular hyperspectral imaging, strong-field light-matter interaction, and resonant tissue ablation. Here we present 6-12 μm broadband tunable parametric amplifier based on LiGaS2 or BaGa4S7, generating new record output power of 2.4 W at 7.5 μm, and 1.5 W at 9.5 μm, pumped by a simple and effective thin-square-rod Yb:YAG amplifier producing 110 W 274 fs output pulses. As a proof of concept, we showcase efficient resonant ablation and microstructure fabrication on enamel at the hydroxyapatite resonant wavelength of 9.5 μm, with a laser intensity two orders-of-magnitude lower than that required by non-resonant femtosecond lasers, which could foster more precision surgical applications with superior biosafety.

physics.optics↗

arXiv2024

Octave-wide broadening of ultraviolet dispersive wave driven by soliton-splitting dynamics

Coherent dispersive wave emission, as an important phenomenon of soliton dynamics, manifests itself in multiple platforms of nonlinear optics from fibre waveguides to integrated photonics. Limited by its resonance nature, efficient generation of coherent dispersive wave with ultra-broad bandwidth has, however, proved difficult to realize. Here, we unveil a new regime of soliton dynamics in which the dispersive wave emission process strongly couples with the splitting dynamics of the driving pulse. High-order dispersion and self-steepening effects, accumulated over soliton self-compression, break the system symmetry, giving rise to high-efficiency generation of coherent dispersive wave in the ultraviolet region. Simultaneously, asymmetric soliton splitting results in the appearance of a temporally-delayed ultrashort pulse with high intensity, overlapping and copropagating with the dispersive wave pulse. Intense cross-phase modulations lead to octave-wide broadening of the dispersive wave spectrum, covering 200 to 400 nm wavelengths. The highly-coherent, octave-wide ultraviolet spectrum, generated from the simple capillary fibre set-up, is in great demand for time-resolved spectroscopy, ultrafast electron microscopy and frequency metrology applications, and the critical role of the secondary pulse in this process reveals some new opportunities for all-optical control of versatile soliton dynamics.

physics.optics↗

arXiv2023

Broadband Dispersive-Wave Emission Coupled with Two-Stage Soliton Self-Compression in Gas-Filled Anti-Resonant Hollow-Core Fibers

We studied the underlying mechanism of broadband dispersive-wave emission within a resonance band of gas-filled anti-resonant hollow-core fiber. Both theoretical and experimental results unveiled that the high-order soliton, launched into the hollow-core fiber, experienced two stages of pulse compression, resulting in a multi-peak structure of the dispersive-wave spectrum. Over the first-stage pulse compression, a sharp increase of the pulse peak power triggered the first time of dispersion-wave emission, and simultaneously caused ionization of the noble gas filled in the fiber core. Strong soliton-plasma interactions led to blue shifting of the pump pulse, and the blue-shifted pulse experienced a decreasing dispersion value in the fiber waveguide, resulting in an increase of its soliton order. Then, the second-stage pulse compression due to the high-order soliton effect triggered the second time of dispersive-wave emission at a phase-matched frequency slightly lower than that in the first stage. Multi-peak spectra of the output dispersive-waves and their formation dynamics were clearly observed in our experiments, which can be understood using a delicate coupling mechanism among three nonlinear effects including high-order-soliton compression, soliton-plasma interaction and phase-matched dispersive-wave emission. The output broadband dispersive-wave could be potentially compressed to sub-30 fs duration using precise chirp-compensation technique.

physics.optics↗

arXiv2023

A novel small-scale self-focusing suppression method for ultrahigh peak power lasers

We proposed a novel method, using an asymmetric four grating compressor (AFGC) to improve the spatial uniformity of laser beams, to suppress the small-scale self-focusing (SSSF) during the post-compression of ultrahigh peak power lasers. The spatial uniformity is an important factor in performing post-compression, due to the spatial intensity nonuniformity will be enhanced while going through a nonlinear process. And what's more, the strong intensity spikes induced during nonlinear process can seriously damage the subsequent optical components. Moreover, the three-dimensional numerical simulations of the post-compression are implemented based on a petawatt (PW) class laser with a standard compressor and an AFGC. The results show that the post-compression with AFGC can shorten the laser pulses from 30fs to sub-10fs and meanwhile efficiently suppress SSSF. This work provides a promising scheme for the post-compression scaling to PW and even 10PW lasers.

physics.optics↗

arXiv2023

Spectroscopic Evidence for Interfacial Charge Separation and Recombination in Graphene-MoS2 Vertical Heterostructures

Vertical van der Waals (vdW) heterostructures consisting of graphene (Gr) and transition metal dichalcogenides (TMDs) have created a fascinating platform for exploring optical and electronic properties in the two-dimensional limit. Previous study has revealed the ultrafast formation of interfacial excitons and the exciton dynamics in the Gr/MoS2 heterostructure. However, a fully understanding of interfacial charge separation and the subsequent dynamics in graphene-based heterostructures remains elusive. Here, we investigate the carrier dynamics of Gr-MoS2 (including Gr/MoS2 and MoS2/Gr stacking sequences) heterostructures under different photoexcitation energies and stacking sequences by comprehensive ultrafast means, including time-resolved terahertz spectroscopy (TRTS), terahertz emission spectroscopy (TES) and transient absorption spectroscopy (TAS). We demonstrate that the Gr/MoS2 heterostructure generates hot electron injection from graphene into the MoS2 layer with photoexcitation of sub-A-exciton of MoS2, while the interfacial charge separation in the MoS2/Gr could be partially blocked by the electric field of substrate. Charge transfer (CT) occurs in same directions for the Gr-MoS2 heterostructures with opposite stacking order, resulting in the opposite orientations of the interfacial photocurrent, as directly demonstrated by the terahertz (THz) emission. Moreover, we demonstrate that the recombination time of interfacial charges after CT is on a timescale of 18 ps to 1 ns, depending on the density of defect states in MoS2 layer. This work provides a comprehensive and unambiguous picture of the interfacial charge dynamics of graphene-based heterostructures, which is essential for developing Gr/TMDs based optoelectronic devices.

physics.optics↗

arXiv2023

Highly-stable, flexible delivery of microjoule-level ultrafast pulses in vacuumized anti-resonant hollow-core fibers for active synchronization

We demonstrate the stable and flexible light delivery of multi-μJ, sub-200-fs pulses over a ~10-m-long vacuumized anti-resonant hollow-core fiber (AR-HCF), which was successfully used for high-performance pulse synchronization. Compared with the pulse train launched into the AR-HCF, the transmitted pulse train out of the fiber exhibits excellent stabilities in pulse power and spectrum, with pointing stability largely improved. The walk-off between the fiber-delivery and the other free-space-propagation pulse trains, in an open loop, was measured to be <6 fs root-mean-square (RMS) over 90 minutes, corresponding to a relative optical-path variation of <2x10-7. This walk-off can be further suppressed to ~2 fs RMS simply using an active control loop, highlighting the great application potentials of this AR-HCF set-up in large-scale laser and accelerator facilities.

physics.optics↗

arXiv2022

Self-referencing 3D characterization of ultrafast optical-vortex beams using tilted interference TERMITES technique

Femtosecond light pulses carrying optical angular momentums (OAMs), possessing intriguing properties of helical phase fronts and ultrafast temporal profiles, enable many applications in nonlinear optics, strong-field physics and laser micro-machining. While generation of OAM-carrying ultrafast pulses and their interactions with matters have been intensively studied in experiments, three-dimensional characterization of ultrafast OAM-carrying light beams in spatio-temporal domain has, however, proved difficult to achieve. Conventional measurement schemes rely on the use of a reference pulsed light beam which needs to be well-characterized in its phase front and to have sufficient overlap and coherence with the beam under test, largely limiting practical applications of these schemes. Here we demonstrate a self-referencing set-up based on a tilted interferometer that can be used to measure complete spatio-temporal information of OAM-carrying femtosecond pulses with different topological charges. Through scanning one interferometer arm, the spectral phase over the pulse spatial profile can be obtained using the tilted interference signal, and the temporal envelope of the light field at one particular position around its phase singularity can be retrieved simultaneously, enabling three-dimensional beam reconstruction. This self-referencing technique, capable of measuring spatio-temporal ultrafast optical-vortex beams, may find many applications in fields of nonlinear optics and light-matter interactions.

physics.optics↗

arXiv2022

Measurements of microjoule-level, few-femtosecond ultraviolet dispersive-wave pulses generated in gas-filled hollow capillary fibers

High-energy ultraviolet pulse generation in gas-filled hollow capillary fibers (HCFs) through dispersive-wave-emission process, has attracted considerable attentions in recent several years due to its great application potentials in ultraviolet spectroscopy and photochemistry. While the ability of this technique to deliver high-energy, ultrafast ultraviolet pulses is widely recognized, few-fs duration of μJ-level dispersive-wave (DW) pulses has, however, escaped direct measurements. In this letter, we demonstrate that using several chirped mirrors, few-fs ultraviolet DW pulses can be obtained in atmosphere environment without the use of vacuum chambers. The pulse temporal profiles, measured using a self-diffraction frequency-resolved optical gating set-up, exhibit full-width-half-maximum pulse widths of 9.6 fs at 384 nm and 9.4 fs at 430 nm, close to the Fourier-transform limits. Moreover, theoretical and experimental studies reveal the strong influences of driving pulse energy and HCF length on temporal width and shape of the measured DW pulses. The ultraviolet pulses obtained in atmosphere environment with μJ-level pulse energy, few-fs pulse width and broadband wavelength tunability are ready to be used in many applications.

physics.optics↗

arXiv2022

High-quality femtosecond laser surface micro/nano-structuring assisted by a thin frost layer

Femtosecond laser ablation has been demonstrated to be a versatile tool to produce micro/nanoscale features with high precision and accuracy. However, the use of high laser fluence to increase the ablation efficiency usually results in unwanted effects, such as redeposition of debris, formation of recast layer and heat-affected zone in or around the ablation craters. Here we circumvent this limitation by exploiting a thin frost layer with a thickness of tens of microns, which can be directly formed by the condensation of water vapor from the air onto the exposed surface whose temperature is below the freezing point. When femtosecond laser beam is focused onto the target surface covered with a thin frost layer, only the local frost layer around the laser-irradiated spot melts into water, helping to boost ablation efficiency, suppress the recast layer and reduce the heat-affect zone, while the remaining frost layer can prevent ablation debris from adhering to the target surface. By this frost-assisted strategy, high-quality surface micro/nano-structures are successfully achieved on both plane and curved surfaces at high laser fluences, and the mechanism behind the formation of high-spatial-frequency (HSF) laser induced periodic surface structures (LIPSSs) on silicon is discussed.

physics.optics↗

arXiv2022

High-order harmonic generation in X-ray range from laser induced noble gas multivalent ions

Sub-femtosecond x-ray burst is powerful tool for probing and imaging electronic and concomitant atomic motion in attosecond physics. For years, x-ray source (above 2 keV) had mainly been obtained from X-ray free electron laser (XFEL) or synchrotron radiation, which are high energy consumption, high cost and huge volume. Here we propose a low-cost and small-size method to generate X-ray source. We experimentally obtained high photon energy spectrum (~ 5.2 keV) through both atom and multiple valence state ions using a near-infrared 1.45 μm driving laser interacting with krypton gas, according to our knowledge, which is the highest photon energy generated through high-order harmonic generation up to now. In our scheme, multi-keV photon energy can be achieved with a relaxed requirement on experimental conditions, and make time-resolved studies more accessible to many laboratories that are capable of producing high energy photon extending to hard x-ray region. Furthermore, our scheme minimizes the influence of X-ray fluorescence process on detection, and can also be utilized to study the quantum-optical nature of high-order harmonic generation.

physics.optics↗

arXiv2022

Observation of Ultrafast Interfacial Exciton Formation and Recombination in Graphene/MoS2 Heterostructure

In this study,we combined time-resolved terahertz spectroscopy along with transient absorption spectroscopy to revisit the interlayer non-equilibrium carrier dynamics in largely lateral size Gr/MoS2 heterostructure fabricated with chemical vapor deposition method. Our experimental results reveal that, with photon-energy below the A-exciton of MoS2 monolayer, hot electrons transfer from graphene to MoS2 takes place in time scale of less than 0.5 ps, resulting in ultrafast formation of interfacial exciton in the heterostructure, subsequently, recombination relaxation of the interfacial exciton occurs in time scale of ~18 ps. A new model considering carrier heating and photogating effect in graphene is proposed to estimate the amount of carrier transfer in the heterostructure, which shows a good agreement with experimental result. Moreover, when the photon-energy is on-resonance with the A-exciton of MoS2, photogenerated holes in MoS2 are transferred to graphene layer within 0.5 ps, leading to the formation of interfacial exciton, the subsequent photoconductivity (PC) relaxation of graphene and bleaching recovery of A-exciton in MoS2 take place around ~10 ps time scale, ascribing to the interfacial exciton recombination. The faster recombination time of interfacial exciton with on-resonance excitation could come from the reduced interface barrier caused by bandgap renormalization effect. Our study provides deep insight into the understanding of interfacial charge transfer as well as the relaxation dynamics in graphene-based heterostructures, which are promising for the applications of graphene-based optoelectronic devices.

physics.optics↗

arXiv2021

Intense harmonics with time-varying orbital angular momentum from relativistic plasma mirrors

In this work using three-dimensional particle-in-cell simulations and analytical considerations we demonstrate intense high-order plasma surface harmonics carrying a time-varying orbital angular momentum (OAM) -- the self-torque. We show that by using two laser beams with different OAMs $l_1$ and $l_2$ and a certain delay between each other and shooting them obliquely on an overdense plasma target, one can generate harmonics with OAM spanning $nl_1$ to $nl_2$, where $n$ is the order of the harmonic. Such intense self-torqued harmonics can offer new possibilities in ultrafast spectroscopy.

physics.plasm-ph↗

arXiv2021

Disorder-assisted Robustness of Ultrafast Cooling in High Doped CVD-Graphene

Dirac Fermion, which is the low energy collective excitation near the Dirac cone in monolayer graphene, have gained great attention by low energy Terahertz probe. In the case of undoped graphene, it has been generally understood that the ultrafast terahertz thermal relaxation is mostly driven by the electron-phonon coupling (EOP), which can be prolonged to tens and hundreds of picoseconds. However, for the high doped graphene, which manifests the negative photoinduced terahertz conductivity, there is still no consensus on the dominant aspects of the cooling process on a time scale of a few picoseconds. Here, the competition between the disorders assisted defect scattering and the electron-phonon coupling process in the cooling process of the graphene terahertz dynamics is systematically studied and disentangled. We verify experimentally that the ultrafast disorder assisted lattice-phonon interaction, rather than the electron-phonon coupling process, would play the key role in the ultrafast thermal relaxation of the terahertz dynamics. Furthermore, the cooling process features robustness which is independent on the pump wavelength and external temperature. Our finding is expected to propose a considerable possible cooling channel in CVD-graphene and to increase the hot electron extracting efficiency for the design of graphene-based photoconversion devices.

cond-mat.mes-hall↗

arXiv2021

Photoionization-induced broadband dispersive wave generated in an Ar-filled hollow-core photonic crystal fiber

The resonance band in hollow-core photonic crystal fiber (HC-PCF), while leading to high-loss region in the fiber transmission spectrum, has been successfully used for generating phase-matched dispersive wave (DW). Here, we report that the spectral width of the resonance-induced DW can be largely broadened due to plasma-driven blueshifting soliton. In the experiment, we observed that in a short length of Ar-filled single-ring HC-PCF the soliton self-compression and photoionization effects caused a strong spectral blueshift of the pump pulse, changing the phase-matching condition of the DW emission process. Therefore, broadening of DW spectrum to the longer-wavelength side was obtained with several spectral peaks, which correspond to the generation of DW at different positions along the fiber. In the simulation, we used super-Gauss windows with different central wavelengths to filter out these DW spectral peaks, and studied the time-domain characteristics of these peaks respectively using Fourier transform method. The simulation results verified that these multiple-peaks on the DW spectrum have different delays in the time domain, agreeing well with our theoretical prediction. Remarkably, we found that the whole time-domain DW trace can be compressed to ~29 fs using proper chirp compensation. The experimental and numerical results reported here provide some insight into the resonance-induced DW generation process in gas-filled HC-PCFs, they could also pave the way to ultrafast pulse generation using DW-emission mechanism.

physics.optics↗

arXiv2020

Single-scan, dual-functional interferometer for fast spatiotemporal characterization of few-cycle pulses

Accurate and fast characterization of spatiotemporal information of high-intensity, ultrashort pulses is crucial in the field of strong-field laser science and technology. While conventional self-referenced interferometers were widely used to retrieve the spatial profile of the relative spectral phase of pulses, additional measurements of temporal and spectral information at a particular position of the laser beam were, however, necessary to remove the indeterminacy, which increases the system complexity. Here we report an advanced, dual-functional interferometer that is able to reconstruct the complete spatiotemporal information of ultrashort pulses with a single scan of the interferometer arm. The set-up integrates an interferometric frequency-resolved optical gating (FROG) with a radial shearing Michelson interferometer. Trough scanning one arm of the interferometer, both cross-correlated FROG trace at the central part of the laser beam and delay-dependent interferograms of the entire laser profile are simultaneously obtained, allowing a fast 3-dimensional reconstruction of few-cycle laser pulses.

physics.optics↗

arXiv2020

Stable intense 1 kHz supercontinuum light generation in air

Supercontinuum (SC) light source has advanced ultrafast laser spectroscopy in condensed matter science, biology, physics, and chemistry. Compared to the frequently used photonic crystal fibers and bulk materials, femtosecond laser filamentation in gases is damage-immune for supercontinuum generation. A bottleneck problem is the strong jitters from filament induced self-heating at kHz repetition rate level. We demonstrate stable kHz supercontinuum generation directly in air with multiple mJ level pulse energy. This is achieved by applying an external DC electric field to the air plasma filament through the effects of plasma wave guiding and Coulomb interaction. Both pointing and intensity jitters of 1 kHz air filament induced SC light are reduced by more than 2 fold. This offers the opportunities for stable intense SC generation and other laser filament based applications in air.

physics.optics↗

arXiv2020

In-house beam-splitting pulse compressor with compensated spatiotemporal coupling for high-energy petawatt lasers

One of the most serious bottleneck on achieving kilojoule-level high-energy petawatt (PW) to hundreds-petawatt (100PW) lasers with ps to fs pulse duration is the requirement of as large as meter-sized gratings in the compressor so as to avoid the laser-induced damage to the gratings. However, this kind of meter-sized grating with high quality is hard to manufacture so far. Here, we propose a new in-house beam-splitting compressor based on the property that the damage threshold of gratings depend on the pulse duration. The new scheme will simultaneously improve the stability, save expensive gratings, and simplify the size of compressor because the split beams share the first two parallel gratings. Furthermore, based on the fact that the transmitted wavefront of a glass plate can be much better and more precisely controlled than that of the diffraction wavefront of a large grating, then glass plates with designed transmitted wavefront are proposed to compensate the wavefront distortion introduced by the second, the third gratings, and other optics in-house such as the beam splitter. This simple and economical method can compensate the space-time distortion in the compressor and then improve the focal intensity, which otherwise cannot be compensated by the deformable mirror outside the compressor due to angular chirp. Together with multi-beams tiled-aperture combining scheme, the novel compressor provides a new scheme to achieve high-energy PW-100PW lasers or even exawatt lasers with relatively small gratings in the future.

physics.optics↗