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Z. Hussain

Publications and source records attributed to Z. Hussain.

At least 73 records · Page 4Linked to original sources

Doping Evolution of the Underlying Fermi Surface in La2-xSrxCuO4

We have performed a systematic doping dependent study of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) (0.03$\leq x \leq$0.3) by angle-resolved photoemission spectroscopy. In the entire doping range, the underlying ``Fermi surface" determined from the low energy spectral weight approximately satisfies Luttinger's theorem, even down to the lightly-doped region. This is in strong contrast to the result on Ca$_{2-x}$Na$_x$CuO$_2$Cl$_2$ (Na-CCOC), which shows a strong deviation from Luttinger's theorem. The differences between LSCO and Na-CCOC are correlated with the different behaviors of the chemical potential shift and spectral weight transfer induced by hole doping.

cond-mat.str-el↗

Nodal quasiparticle in pseudogapped colossal magnetoresistive manganites

A characteristic feature of the copper oxide high-temperature superconductors is the dichotomy between the electronic excitations along the nodal (diagonal) and antinodal (parallel to the Cu-O bonds) directions in momentum space, generally assumed to be linked to the "d-wave" symmetry of the superconducting state. Angle-resolved photoemission measurements in the superconducting state have revealed a quasiparticle spectrum with a d-wave gap structure that exhibits a maximum along the antinodal direction and vanishes along the nodal direction. Subsequent measurements have shown that, at low doping levels, this gap structure persists even in the high-temperature metallic state, although the nodal points of the superconducting state spread out in finite "Fermi arcs". This is the so-called pseudogap phase, and it has been assumed that it is closely linked to the superconducting state, either by assigning it to fluctuating superconductivity or by invoking orders which are natural competitors of d-wave superconductors. Here we report experimental evidence that a very similar pseudogap state with a nodal-antinodal dichotomous character exists in a system that is markedly different from a superconductor: the ferromagnetic metallic groundstate of the colossal magnetoresistive bilayer manganite La1.2Sr1.8Mn2O7. Our findings therefore cast doubt on the assumption that the pseudogap state in the copper oxides and the nodal-antinodal dichotomy are hallmarks of the superconductivity state.

cond-mat.str-el↗

Multiple Bosonic Mode Coupling in Electron Self-Energy of (La_2-xSr_x)CuO_4

High resolution angle-resolved photoemission spectroscopy data along the (0,0)-($π$,$π$) nodal direction with significantly improved statistics reveal fine structure in the electron self-energy of the underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ samples in the normal state. Fine structure at energies of (40$\sim$46) meV and (58$\sim$63)meV, and possible fine structure at energies of (23$\sim$29)meV and (75$\sim$85)meV, have been identified. These observations indicate that, in LSCO, more than one bosonic modes are involved in the coupling with electrons.

cond-mat.str-el↗

Mapping the spin-dependent electron reflectivity of Fe and Co ferromagnetic thin films

Spin Polarized Low Energy Electron Microscopy is used as a spin dependent spectroscopic probe to study the spin dependent specular reflection of a polarized electron beam from two different magnetic thin film systems: Fe/W(110) and Co/W(110). The reflectivity and spin-dependent exchange-scattering asymmetry are studied as a function of electron kinetic energy and film thickness, as well as the time dependence. The largest value of the figure of merit for spin polarimetry is observed for a 5 monolayer thick film of Co/W(110) at an electron kinetic energy of 2eV. This value is 2 orders of magnitude higher than previously obtained with state of the art Mini-Mott polarimeter. We discuss implications of our results for the development of an electron-spin-polarimeter using the exchange-interaction at low energy.

cond-mat.mtrl-sci↗

Polaronic behavior of undoped high-Tc cuprates

We present angle-resolved photoemission spectroscopy (ARPES) data on undoped La2CuO4, indicating polaronic coupling between bosons and charge carriers. Using a shell model, we calculate the electron-phonon coupling and find that it is strong enough to give polarons. We develop an efficient method for calculating ARPES spectra in undoped systems. Using the calculated couplings, we find the width of the phonon side band in good agreement with experiment. We analyze reasons for the observed dependence of the width on the binding energy.

cond-mat.str-el↗

Normal State Spectral Lineshapes of Nodal Quasiparticles in Single Layer Bi2201 Superconductor

A detailed study of the normal state photoemission lineshapes and quasiparticle dispersion for the single layer Bi$_2$Sr$_{2-x}$La$_x$CuO$_{6+δ}$ (Bi2201) superconductor is presented. We report the first experimental evidence of a double peak structure and a dip of spectral intensity in the energy distribution curves (EDCs) along the nodal direction. The double peak structure is well identified in the normal state, up to ten times the critical temperature. As a result of the same self-energy effect, a strong mass renormalization of the quasiparticle dispersion, i.e. kink, and an increase of the quasiparticle lifetime in the normal state are also observed. Our results provide unambiguous evidence on the existence of bosonic excitation in the normal state, and support a picture where nodal quasiparticles are strongly coupled to the lattice.

cond-mat.supr-con↗

Orientation-dependent C60 electronic structures revealed by photoemission

We observe, with angle-resolved photoemission, a dramatic change in the electronic structure of two C60 monolayers, deposited respectively on Ag (111) and (100) substrates, and similarly doped with potassium to half-filling of the C60 lowest unoccupied molecular orbital. The Fermi surface symmetry, the bandwidth, and the curvature of the dispersion at Gamma point are different. Orientations of the C60 molecules on the two substrates are known to be the main structural difference between the two monolayers, and we present new band-structure calculations for some of these orientations. We conclude that orientations play a key role in the electronic structure of fullerides.

cond-mat.str-el↗

Space Charge Effect and Mirror Charge Effect in Photoemission Spectroscopy

We report the observation and systematic investigation of the space charge effect and mirror charge effect in photoemission spectroscopy. When pulsed light is incident on a sample, the photoemitted electrons experience energy redistribution after escaping from the surface because of the Coulomb interaction between them (space charge effect) and between photoemitted electrons and the distribution of mirror charges in the sample (mirror charge effect). These combined Coulomb interaction effects give rise to an energy shift and a broadening which can be on the order of 10 meV for a typical third-generation synchrotron light source. This value is comparable to many fundamental physical parameters actively studied by photoemission spectroscopy and should be taken seriously in interpreting photoemission data and in designing next generation experiments.

cond-mat.str-el↗

Coupling Of The B1g Phonon To The Anti-Nodal Electronic States of Bi2Sr2Ca0.92Y0.08Cu2O(8+delta)

Angle-resolved photoemission spectroscopy (ARPES) on optimally doped Bi2Sr2Ca0.92Y0.08Cu2O(8+delta) uncovers a coupling of the electronic bands to a 40 meV mode in an extended k-space region away from the nodal direction, leading to a new interpretation of the strong renormalization of the electronic structure seen in Bi2212. Phenomenological agreements with neutron and Raman experiments suggest that this mode is the B1g oxygen bond-buckling phonon. A theoretical calculation based on this assignment reproduces the electronic renormalization seen in the data.

cond-mat.supr-con↗

Fermi Surface reconstruction in the CDW state of CeTe3 observed by photoemission

CeTe3 is a layered compound where an incommensurate Charge Density Wave (CDW) opens a large gap (400 meV) in optimally nested regions of the Fermi Surface (FS), whereas other sections with poorer nesting remain ungapped. Through Angle-Resolved Photoemission, we identify bands backfolded according to the CDW periodicity. They define FS pockets formed by the intersection of the original FS and its CDW replica. Such pockets illustrate very directly the role of nesting in the CDW formation but they could not be detected so far in a CDW system. We address the reasons for the weak intensity of the folded bands, by comparing different foldings coexisting in CeTe3.

cond-mat.str-el↗

The Dichotomy between Nodal and Antinodal Quasiparticles in Underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ Superconductors

High resolution angle-resolved photoemission measurements on underdoped (La$_{2-x}$Sr$_x$)CuO$_4$ system show that, at energies below 70 meV, the quasiparticle peak is well defined around the ($π$/2,$π$/2) nodal region and disappears rather abruptly when the momentum is changed from the nodal point to the ($π$,0) antinodal point along the underlying ``Fermi surface''. It indicates that there is an extra low energy scattering mechanism acting upon the antinodal quasiparticles. We propose that this mechanism is the scattering of quasiparticles across the nearly parallel segments of the Fermi surface near the antinodes.

cond-mat.str-el↗

Direct extraction of the Eliashberg function for electron-phonon coupling: A case study of Be(1010)

We propose a systematic procedure to directly extract the Eliashberg function for electron-phonon coupling from high-resolution angle-resolved photoemission data. The procedure is successfully applied to the Be(1010) surface, providing new insights to electron-phonon coupling at this surface. The method is shown to be robust against imperfections in experimental data and suitable for wider applications.

cond-mat.str-el↗

Thermodynamic and transport properties of underdoped cuprates from ARPES data

he relationship between photoemission spectra of high-$T_{\textrm{c}}$ cuprates and their thermodynamic and transport properties are discussed. The doping dependence of the expected quasi-particle density at the Fermi level ($E_\mathrm{F}$) are compared with the electronic specific heat coefficient $γ$ and that of the spectral weight at $E_\mathrm{F}$ with the in-plane and out-of-plane superfluid density. We have estimated the electrical resistivity of underdoped cuprates from the momentum distribution curve (MDC) at $E_\mathrm{F}$ in the nodal direction. The temperature dependence of the MDC width is also consistent with that of the electrical resistivity.

cond-mat.str-el↗

Effects of next-nearest-neighbor hopping $t^{\prime}$ on the electronic structure of cuprates

Photoemission spectra of underdoped and lightly-doped Bi$_{2-z}$Pb$_z$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ($R=$ Pr, Er) (BSCCO) have been measured and compared with those of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO). The lower-Hubbard band of the insulating BSCCO, like Ca$_2$CuO$_2$Cl$_2$, shows a stronger dispersion than La$_2$CuO$_4$ from ${\bf k}\sim$($π/2,π/2$) to $\sim$($π,0$). The flat band at ${\bf k}\sim$($π,0$) is found generally deeper in BSCCO. These observations together with the Fermi-surface shapes and the chemical potential shifts indicate that the next-nearest-neighbor hopping $|t^{\prime}|$ of the single-band model is larger in BSCCO than in LSCO and that $|t^{\prime}|$ rather than the super-exchange $J$ influences the pseudogap energy scale.

cond-mat.supr-con↗

Fermi surface and quasiparticle dynamics of Na(x)CoO2 {x=0.7} investigated by Angle-Resolved Photoemission Spectroscopy

We present an angle-resolved photoemission study of Na0.7CoO2, the host cobaltate of the NaxCoO2.yH2O series. Our results show a large hexagonal-like hole-type Fermi surface, an extremely narrow strongly renormalized quasiparticle band and a small Fermi velocity. Along the Gamma to M high symmetry line, the quasiparticle band crosses the Fermi level from M toward Gamma consistent with a negative sign of effective single-particle hopping (t ): t is estimated to be about 8 meV which is on the order of exchange coupling J in this system. This suggests that t ~ J ~ 10 meV is an important energy scale in the system. Quasiparticles are well defined only in the T-linear resistivity regime. Small single particle hopping and unconventional quasiparticle dynamics may have implications for understanding the unusual behavior of this new class of compounds.

cond-mat.str-el↗

An angle-resolved photoemission spectral function analysis of the electron doped cuprate Nd_1.85Ce_0.15CuO_4

Using methods made possible by recent advances in photoemission technology, we perform an indepth line-shape analysis of the angle-resolved photoemission spectra of the electron doped (n-type) cuprate superconductor Nd_1.85Ce_0.15CuO_4. Unlike for the p-type materials, we only observe weak mass renormalizations near 50-70 meV. This may be indicative of smaller electron-phonon coupling or due to the masking effects of other interactions that make the electron-phonon coupling harder to detect. This latter scenario may suggest limitations of the spectral function analysis in extracting electronic self-energies when some of the interactions are highly momentum dependent.

cond-mat.supr-con↗

Nodal metallic behavior of lightly-doped La$_{2-x}$Sr$_x$CuO$_4$

Lightly-doped La$_{2-x}$Sr$_x$CuO$_4$ in the so-called "insulating" spin-glass/diagonal-stripe phase has been studied by angle-resolved photoemission spectroscopy. A quasi-particle (QP) peak crossing the Fermi level has been observed in the node direction of the d-wave superconducting gap, forming an "arc" of Fermi surface consistent with the recently observed metallic transport behavior at high temperatures of lightly-doped materials. The spectral weight of the nodal QP smoothly increases with hole doping, corresponding to the $n \sim x$ behavior of the carrier number in the underdoped and lightly-doped regions.

cond-mat.str-el↗