arXiv subjects

Z. X. Shen

Publications and source records attributed to Z. X. Shen.

At least 55 records · Page 3Linked to original sources

arXiv2009

A momentum-dependent perspective on quasiparticle interference in Bi_{2}Sr_{2}CaCu_{2}O_{8+δ}

Angle Resolved Photoemission Spectroscopy (ARPES) probes the momentum-space electronic structure of materials, and provides invaluable information about the high-temperature superconducting cuprates. Likewise, the cuprate real-space, inhomogeneous electronic structure is elucidated by Scanning Tunneling Spectroscopy (STS). Recently, STS has exploited quasiparticle interference (QPI) - wave-like electrons scattering off impurities to produce periodic interference patterns - to infer properties of the QP in momentum-space. Surprisingly, some interference peaks in Bi_{2}Sr_{2}CaCu_{2}O_{8+δ} (Bi-2212) are absent beyond the antiferromagnetic (AF) zone boundary, implying the dominance of particular scattering process. Here, we show that ARPES sees no evidence of quasiparticle (QP) extinction: QP-like peaks are measured everywhere on the Fermi surface, evolving smoothly across the AF zone boundary. This apparent contradiction stems from different natures of single-particle (ARPES) and two-particle (STS) processes underlying these probes. Using a simple model, we demonstrate extinction of QPI without implying the loss of QP beyond the AF zone boundary.

cond-mat.supr-con↗

arXiv2009

Dependence of Band Renormalization Effect on the Number of Copper-oxide Layers in Tl-based Copper-oxide Superconductor using Angle-resolved Photoemission Spectroscopy

Here we report the first angle-resolved photoemission measurement on nearly optimally-doped multi-layer Tl-based superconducting cuprates (Tl-2212 and Tl-1223) and a comparison study to single layer (Tl-2201) compound. A "kink" in the band dispersion is found in all three compounds but exhibits different momentum dependence for the single layer and multi-layer compounds, reminiscent to that of Bi-based cuprates. This layer number dependent renormalization effect strongly implies that the spin resonance mode is unlikely responsible for the dramatic renormalization effect near the antinodal region.

cond-mat.supr-con↗

arXiv2009

Large Gap Topological Insulator Bi2Te3 with a Single Dirac Cone on the Surface

We investigate the surface state of Bi$_2$Te$_3$ using angle resolved photoemission spectroscopy (ARPES) and transport measurements. By scanning over the entire Brillouin zone (BZ), we demonstrate that the surface state consists of a single non-degenerate Dirac cone centered at the $Γ$ point. Furthermore, with appropriate hole (Sn) doping to counteract intrinsic n-type doping from vacancy and anti-site defects, the Fermi level can be tuned to intersect only the surface states, indicating a full energy gap for the bulk states, consistent with a carrier sign change near this doping in transport properties. Our experimental results establish for the first time that Bi$_2$Te$_3$ is a three dimensional topological insulator with a single Dirac cone on the surface, as predicted by a recent theory.

cond-mat.mtrl-sci↗

arXiv2008

Fabrication of graphene nanodisk arrays using nanosphere lithography

Ordered graphene nanodisk arrays have been successfully fabricated by combining nanosphere lithography (NSL) and reactive ion etching (RIE) processes. The dimension of graphene nanodisks can be effectively tuned by varying the size of polystyrene spheres, which function as masks during RIE. Low voltage scanning electron microscopy shows that the graphene sheet could be readily patterned into periodic disk-like nanostructures by oxygen RIE. Raman mapping and spectroscopy further visualize such nanodisk arrays and reveal the nature of disks are crystalline single layer graphene. This work demonstrates an efficient and manageable way to pattern graphene. Considering the periodicity, nanometer dimension and large edge to body ratio, the graphene nanodisk arrays, such two dimensional assembly of carbon atoms offer intrisic advantages in various electronic and spintronic fabrications.

cond-mat.mtrl-sci↗

arXiv2008

Calibration of shielded microwave probes using bulk dielectrics

A stripline-type near-field microwave probe is microfabricated for microwave impedance microscopy. Unlike the poorly shielded coplanar probe that senses the sample tens of microns away, the stripline structure removes the stray fields from the cantilever body and localizes the interaction only around the focused-ion beam deposited Pt tip. The approaching curve of an oscillating tip toward bulk dielectrics can be quantitatively simulated and fitted to the finite-element analysis result. The peak signal of the approaching curve is a measure of the sample dielectric constant and can be used to study unknown bulk materials.

cond-mat.mtrl-sci↗

arXiv2008

Observation of a robust peak in the glue function of the high-Tc cuprates in the 50-60 meV range

We take advantage of the connection between the free carrier optical conductivity and the glue function in the normal state, to reconstruct from the infrared optical conductivity the glue-spectrum of ten different high-Tc cuprates revealing a robust peak in the 50-60 meV range and a broad continuum at higher energies for all measured charge carrier concentrations and temperatures up to 290 K. We observe an intriguing correlation between the doping trend of the experimental glue spectra and the critical temperature.

cond-mat.supr-con↗

arXiv2008

Doping dependent charge transfer gap and realistic electronic model of n-type cuprate superconductors

Based on the analysis of the measurement data of angle-resolved photoemission spectroscopy (ARPES) and optics, we show that the charge transfer gap is significantly smaller than the optical one and is reduced by doping in electron doped cuprate superconductors. This leads to a strong charge fluctuation between the Zhang-Rice singlet and the upper Hubbard bands. The basic model for describing this system is a hybridized two-band $t$-$J$ model. In the symmetric limit where the corresponding intra- and inter-band hopping integrals are equal to each other, this two-band model is equivalent to the Hubbard model with an antiferromagnetic exchange interaction (i.e. the $t$-$U$-$J$ model). The mean-field result of the $t$-$U$-$J$ model gives a good account for the doping evolution of the Fermi surface and the staggered magnetization.

cond-mat.supr-con↗

arXiv2008

Bogoliubov Angle, Particle-Hole Mixture and Angular Resolved Photoemission Spectroscopy in Superconductors

Superconducting excitations -- Bogoliubov quasiparticles -- are the quantum mechanical mixture of negatively charged electron (-e) and positively charged hole (+e). We propose a new observable for Angular Resolved Photoemission Spectroscopy (ARPES) studies that is the manifestation of the particle-hole entanglement of the superconducting quasiparticles. We call this observable a {\em Bogoliubov angle}. This angle measures the relative weight of particle and hole amplitude in the superconducting (Bogoliubov) quasiparticle. We show how this quantity can be measured by comparing the ratio of spectral intensities at positive and negative energies.

cond-mat.supr-con↗

arXiv2008

Superconductivity-Induced Self-Energy Evolution of the Nodal Electron of Optimally-Doped Bi2212

The temperature dependent evolution of the renormalization effect in optimally-doped Bi2212 along the nodal direction has been studied via angle-resolved photoemission spectroscopy. Fine structure is observed in the real part of the self-energy (Re$Σ$), including a subkink and maximum, suggesting that electrons couple to a spectrum of bosonic modes, instead of just one mode. Upon cooling through the superconducting phase transition, the fine structures of the extracted Re$Σ$ exhibit a two-processes evolution demonstrating an interplay between kink renormalization and superconductivity. We show that this two-process evolution can be qualitatively explained by a simple Holstein model in which a spectrum of bosonic modes is considered.

cond-mat.supr-con↗

arXiv2008

Raman spectroscopy of epitaxial graphene on a SiC substrate

The fabrication of epitaxial graphene (EG) on SiC substrate by annealing has attracted a lot of interest as it may speed up the application of graphene for future electronic devices. The interaction of EG and the SiC substrate is critical to its electronic and physical properties. In this work, Raman spectroscopy was used to study the structure of EG and its interaction with SiC substrate. All the Raman bands of EG blue shift from that of bulk graphite and graphene made by micromechanical cleavage, which was attributed to the compressive strain induced by the substrate. A model containing 13 x 13 honeycomb lattice cells of graphene on carbon nanomesh was constructed to explain the origin of strain. The lattice mismatch between graphene layer and substrate causes the compressive stress of 2.27 GPa on graphene. We also demonstrate that the electronic structures of EG grown on Si and C terminated SiC substrates are quite different. Our experimental results shed light on the interaction between graphene and SiC substrate that are critical to the future applications of EG.

cond-mat.mtrl-sci↗

arXiv2008

ARPES Study of the Evolution of Band Structure and Charge Density Wave Properties in RTe3 for R = Y, La, Ce, Sm, Gd, Tb and Dy

We present a detailed ARPES investigation of the RTe3 family, which sets this system as an ideal "textbook" example for the formation of a nesting driven Charge Density Wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDW instabilities, from the opening of large gaps on the best nested parts of Fermi Surface (FS) (up to 0.4eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k-space. An additional advantage of RTe3 is that the band structure can be very accurately described by a simple 2D tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure, by comparing our ARPES measurements with Linear Muffin-Tin Orbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and, for the first time, of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k-space, the evolution of the CDW wave vector with R and the shape of the residual metallic pockets. Finally, we give an estimation of the CDW interaction parameters and find that the change in the electronic density of states n(Ef), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.

cond-mat.str-el↗

arXiv2008

Modeling of a Cantilever-Based Near-Field Scanning Microwave Microscope

We present a detailed modeling and characterization of our scalable microwave nanoprobe, which is a micro-fabricated cantilever-based scanning microwave probe with separated excitation and sensing electrodes. Using finite-element analysis, the tip-sample interaction is modeled as small impedance changes between the tip electrode and the ground at our working frequencies near 1GHz. The equivalent lumped elements of the cantilever can be determined by transmission line simulation of the matching network, which routes the cantilever signals to 50 Ohm feed lines. In the microwave electronics, the background common-mode signal is cancelled before the amplifier stage so that high sensitivity (below 1 atto-Farad capacitance changes) is obtained. Experimental characterization of the microwave probes was performed on ion-implanted Si wafers and patterned semiconductor samples. Pure electrical or topographical signals can be realized using different reflection modes of the probe.

cond-mat.other↗

arXiv2007

AFM-compatible near-field scanning microwave microscope with separated excitation and sensing probes

We present the design and experimental results of a near-field scanning microwave microscope (NSMM) working at a frequency of 1GHz. Our microscope is unique in that the sensing probe is separated from the excitation electrode to significantly suppress the common-mode signal. Coplanar waveguides were patterned onto a silicon nitride cantilever interchangeable with atomic force microscope (AFM) tips, which are robust for high speed scanning. In the contact mode that we are currently using, the numerical analysis shows that contrast comes from both the variation in local dielectric properties and the sample topography. Our microscope demonstrates the ability to achieve high resolution microwave images on buried structures, as well as nano-particles, nano-wires, and biological samples.

cond-mat.mtrl-sci↗

arXiv2007

Angle-resolved photoemission studies of lattice polaron formation in the cuprate Ca2CuO2Cl2

To elucidate the nature of the single-particle excitations in the undoped parent cuprates, we have performed a detailed study of Ca2CuO2Cl2 using photoemission spectroscopy. The photoemission lineshapes of the lower Hubbard band are found to be well-described by a polaron model. By comparing the lineshape and temperature dependence of the lower Hubbard band with additional O 2p and Ca 3p states, we conclude that the dominant broadening mechanism arises from the interaction between the photohole and the lattice. The strength of this interaction was observed to be strongly anisotropic and may have important implications for the momentum dependence of the first doped hole states.

cond-mat.str-el↗

arXiv2005

Quantitative analysis of Sr2RuO4 ARPES spectra: Many-body interactions in a model Fermi liquid

ARPES spectra hold a wealth of information about the many-body interactions in a correlated material. However, the quantitative analysis of ARPES spectra to extract the various coupling parameters in a consistent manner is extremely challenging, even for a model Fermi liquid system. We propose a fitting procedure which allows quantitative access to the intrinsic lineshape, deconvolved of energy and momentum resolution effects, of the correlated 2-dimensional material Sr2RuO4. For the first time in correlated 2-dimensional materials, we find an ARPES linewidth that is narrower than its binding energy, a key property of quasiparticles within Fermi liquid theory. We also find that when the electron-electron scattering component is separated from the electron-phonon and impurity scattering terms it decreases with a functional form compatible with Fermi liquid theory as the Fermi energy is approached. In combination with the previously determined Fermi surface, these results give the first complete picture of a Fermi liquid system via ARPES. Furthermore, we show that the magnitude of the extracted imaginary part of the self-energy is in remarkable agreement with DC transport measurements.

cond-mat.str-el↗

arXiv2005

Two-dimensional structures of ferroelectric domain inversion in LiNbO3 by direct electron beam lithography

We report on the fabrication of domain-reversed structures in LiNbO3 by means of direct electron beam lithography at room temperature without any static bias. The LiNbO3 crystals were chemically etched after the exposure of electron beam and then, the patterns of domain inversion were characterized by atomic force microscopy (AFM). In our experiment, an interesting phenomenon occurred when the electron beam wrote a one-dimensional (1-D) grating on the negative c-face: a two-dimensional (2-D) dotted array was observed on the positive c- face, which is significant for its potential to produce 2-D and three-dimensional photonic crystals. Furthermore, we also obtained 2-D ferroelectric domain inversion in the whole LiNbO3 crystal by writing the 2-D square pattern on the negative c-face. Such a structure may be utilized to fabricate 2-D nonlinear photonic crystal. AFM demonstrates that a 2-D domain-reversed structure has been achieved not only on the negative c-face of the crystal, but also across the whole thickness of the crystal.

cond-mat.mtrl-sci↗

arXiv2004

Orientation-dependent C60 electronic structures revealed by photoemission

We observe, with angle-resolved photoemission, a dramatic change in the electronic structure of two C60 monolayers, deposited respectively on Ag (111) and (100) substrates, and similarly doped with potassium to half-filling of the C60 lowest unoccupied molecular orbital. The Fermi surface symmetry, the bandwidth, and the curvature of the dispersion at Gamma point are different. Orientations of the C60 molecules on the two substrates are known to be the main structural difference between the two monolayers, and we present new band-structure calculations for some of these orientations. We conclude that orientations play a key role in the electronic structure of fullerides.

cond-mat.str-el↗

arXiv2004

Fermi Surface reconstruction in the CDW state of CeTe3 observed by photoemission

CeTe3 is a layered compound where an incommensurate Charge Density Wave (CDW) opens a large gap (400 meV) in optimally nested regions of the Fermi Surface (FS), whereas other sections with poorer nesting remain ungapped. Through Angle-Resolved Photoemission, we identify bands backfolded according to the CDW periodicity. They define FS pockets formed by the intersection of the original FS and its CDW replica. Such pockets illustrate very directly the role of nesting in the CDW formation but they could not be detected so far in a CDW system. We address the reasons for the weak intensity of the folded bands, by comparing different foldings coexisting in CeTe3.

cond-mat.str-el↗