arXiv subjects

Zhaogang Dong

Publications and source records attributed to Zhaogang Dong.

At least 19 recordsLinked to original sources

arXiv2026

Observation of the Inherent Chiral Smith-Purcell Effect via Symmetry Breaking

The Smith-Purcell effect arises when charged particles move near a periodic structure, emitting radiation. Conventional approaches for generating chiral Smith-Purcell radiation rely on metasurface phase engineering or resonant mode interference, typically producing narrow-band, weakly chiral emission. Here, we introduce a resonance-interference-free mechanism that leverages the properties of the charged particles themselves. Using a non-chiral, non-resonant silicon grating, we demonstrate broadband, tunable Smith-Purcell radiation with high chirality, achieving a record-high degree of polarization of 0.87. This is enabled by converting the transverse spin angular momentum of electron-induced evanescent waves into a longitudinal form, producing opposite chirality at different azimuthal angles. Beam twisting or displacement offers precise control over chirality, paving the way for compact chiral light sources, advanced X-ray imaging, and integrated particle diagnostics platforms.

physics.optics↗

arXiv2026

Engineering Hybrid Resonances in Nanophotonics

Hybridization of resonances is known to overcome inherent limitations of individual systems, enabling advanced functionalities and applications. Here we discuss hybrid plasmonic-Mie resonators that emerged recently as a promising direction in advancing nanophotonic structures by synergistically combining the strong near-field enhancement of plasmonic components with the low-loss, multipolar resonances of dielectric Mie elements. We review the recent progress in the field, encompassing the fundamental physical principles, structural design strategies, material platforms, computational optimization approaches, and representative device implementations. Our discussion starts by evaluating the complementary characteristics of plasmonic and Mie resonances followed by a description of the coupling between these resonances in order to boost light-matter interactions. Afterward, we explore the performance of efficient hybrid resonators for different application areas. Apart from the conventional metal-dielectric systems, we consider the recent class of epsilon-near-zero (ENZ) materials, which can provide unique advantages in terms of field localization, phase engineering, and energy flow management in the vicinity of zero-permittivity conditions, offering more flexibility in designing hybrid nano-optical devices. Lastly, we point out potential research avenues aiming to improve functional and efficient nanophotonic devices, especially those involving emerging topological material systems, such as Sb2Te3, Bi2Te3, Bi2Se3, combining plasmonic amplification, dielectric confinement, and spin-dependent optical behavior.

physics.optics↗

arXiv2026

In-Line Fiber-Integrated Photon-Pair Generation from van der Waals Crystals

Miniaturized quantum light sources that operate directly in optical fibers are an attractive platform for optical quantum technologies. However, most miniaturized spontaneous parametric down- conversion (SPDC) sources still rely on objective-lens-based free-space pumping and collection, which limits compactness, robustness, and direct compatibility with fiber-based systems. Here we demonstrate a lens-free in-line SPDC photon-pair source by integrating a van der Waals NbOI2 flake directly onto the end facet of an optical fiber. In this configuration, the generated photon- pairs are efficiently collected into optical fibers, eliminating the need for bulk free-space collection optics. Despite the limited numerical aperture of the single-mode fiber, efficient photon-pair collection with high purity, characterized by a coincidence-to-accidental ratio of up to ~4600, is achieved in an ultracompact configuration. These results establish van der Waals ferroelectric materials as a promising platform for fiber-integrated quantum light sources and provide a pathway toward compact, alignment-free quantum photonic devices.

quant-ph↗

arXiv2026

Quantum Dots as Solid-State Sources of Entangled Photon Pairs

Semiconductor quantum dots (QDs) have emerged as a premier solid-state platform for the deterministic generation of nonclassical light, offering a compelling pathway toward scalable quantum photonic systems. While single-photon emission from QDs has reached a high level of maturity, the realization of high-fidelity entangled photon-pair sources remains an active and rapidly evolving frontier. In this review, we survey the recent progress in QD-based entangled photon sources, highlighting the conceptual evolution from the established biexciton-exciton cascade to the emerging paradigm of spontaneous two-photon emission. We further examine how advances in nanophotonic architectures and coherent control strategies are redefining fundamental performance limits, enabling concurrent improvements in source brightness, coherence, and entanglement fidelity. Finally, we discuss the key physical and technological challenges that must be addressed to bridge the gap between laboratory demonstrations and large-scale deployment. We conclude by outlining the future opportunities for integrating QD-based entangled photon sources into practical quantum communication, computation, and sensing platforms.

physics.optics↗

arXiv2025

Weyl Semimetals: from Principles, Materials to Applications

Weyl semimetals have attracted significant interest in condensed matter physics and materials science, due to their unique electronic and topological properties. These characteristics not only deepen our understanding of fundamental quantum phenomena, but also make Weyl semimetals promising candidates for advanced applications in electronics, photonics, and spintronics. This review provides a systematic overview of the field, covering theoretical foundations, material synthesis, engineering strategies, and emerging device applications. We first outline the key theoretical principles and distinctive properties of Weyl semimetals, followed by an examination of recent advancements that enhance their functional versatility. Finally, we discuss the critical challenges hindering their practical implementation and explore future development directions, along with the potential for expanding and enhancing their existing range of applications. By integrating discussions of both opportunities and obstacles, this review offers a balanced perspective on current progress and future directions in Weyl semimetal research.

cond-mat.mtrl-sci↗

arXiv2025

Reality-Infused Deep Learning for Angle-resolved Quasi-optical Fourier Surfaces

Optical Fourier surfaces (OFSs), featuring sinusoidally profiled diffractive elements, manipulate light through patterned nanostructures and incident angle modulation. Compared to altering structural parameters, tuning elevation and azimuth angles offers greater design flexibility for light field control. However, angle-resolved responses of OFSs are often complex due to diverse mode excitations and couplings, complicating the alignment between simulations and practical fabrication. Here, we present a reality-infused deep learning framework, empowered by angle-resolved measurements, to enable real-time and accurate predictions of angular dispersion in quasi-OFSs. This approach captures critical features, including nanofabrication and measurement imperfections, which conventional simulation-based methods typically overlook. Our framework significantly accelerates the design process while achieving predictive performance highly consistent with experimental observations across broad angular and spectral ranges. Our study supports valuable insights into the development of OFS-based devices, and represents a paradigm shift from simulation-driven to reality-infused methods, paving the way for advancements in optical design applications.

physics.optics↗

arXiv2025

Valley optoelectronics based on meta-waveguide photodetectors

In transition metal dichalcogenides, the valley degree of freedom directly couples valley-polarised excitons - excited by circularly polarised light - to valley-dependent chiral photons, enabling ultrafast light-driven valleytronics. However, achieving fully integrated valley optoelectronics - incorporating on-chip generation, selective routing, and electrical readout of valley-dependent chiral photons - remains an unresolved challenge. We present a valley-driven hybrid nanophotonic-optoelectronic circuit that integrates chirality-selective meta-waveguide photodetectors with transition metal dichalcogenides. At room temperature, our purposely designed meta-waveguide device generates near-unity valley-dependent chiral photons in the second harmonic generation from an encapsulated tungsten disulfide monolayer and selectively couples them to unidirectional waveguide modes, achieving an exceptional polarisation selectivity of 0.97. These valley-dependent waveguide modes were subsequently detected by atomically thin few-layer tungsten diselenide photodetectors, exclusively responsive to the above-bandgap upconverted photons, thereby enabling all-on-chip processing of valley-multiplexed images. Our demonstration bridges a critical gap in lightwave valleytronics, paving the way for compact, scalable valley information processing and fostering the development of light-based valleytronic quantum technologies.

physics.optics↗

arXiv2025

Enabling Highly Efficient Infrared Silicon Photodetectors via Disordered Metasurfaces with Upconversion Nanoparticles

Silicon photodetectors are highly desirable for their CMOS compatibility, low cost, and fast response speed. However, their application the infrared (IR) is limited by silicon's intrinsic bandgap, which restricts its detection to photons with wavelengths shorter than 1100 nm. Although several methods have been developed to extend silicon photodetectors further in the IR range, these approaches often introduce additional challenges, such as increased fabrication complexity and compatibility issues with standard CMOS processes. Here, we present an approach to overcome these limitations by integrating disordered metasurfaces with upconversion nanoparticles (UCNPs), enabling IR detection by silicon photodetectors. The disordered design consists of hybrid Mie-plasmonic cavities, which can enhance both the near-field localization and wide-band light absorption from visible to IR, improving photocurrent conversion. Compared to ordered structures, the infrared absorption and near field of the highly disordered configuration are increased by 2.6-folds and 3.9-folds, respectively. UCNPs not only convert near-infrared photons into visible light but also enhance absorption in the mid-infrared range, thereby improving hot electron generation. The measured responsivity of the disordered element for 1550 nm laser is up to 0.22 A/W at room temperature, corresponding to an external quantum efficiency of 17.6%. Our design not only enhances the photocurrent performance significantly, but also extends the working wavelength of silicon photodetectors to IR wavelength, making them suitable for broad spectrum applications.

physics.optics↗

arXiv2024

Chalcogenide Metasurfaces Enabling Ultra-Wideband Detectors from Visible to Mid-infrared

Thermoelectric materials can be designed to support optical resonances across multiple spectral ranges to enable ultra-wide band photodetection. For instance, antimony telluride (Sb2Te3) chalcogenide exhibits interband plasmonic resonances in the visible range and Mie resonances in the mid-infrared (mid-IR) range, while simultaneously possessing large thermoelectric Seebeck coefficients. In this paper, we designed and fabricated Sb2Te3 metasurface devices to achieve resonant absorption for enabling photodetectors operating across an ultra-wideband spectrum, from visible to mid-IR. Furthermore, relying on asymmetric Sb2Te3 metasurface, we demonstrated the thermoelectric photodetectors with polarization-selectivity. This work provides a potential platform towards the portable ultrawide band spectrometers at room temperature, for environmental sensing applications.

physics.optics↗

arXiv2024

Room-temperature Optically Detected Magnetic Resonance of Telecom Single Photon Emitters in GaN

Solid-state defects susceptible of spin manipulation hold great promise for scalable quantum technology. To broaden their utility, operating at room temperature and emitting in the telecom wavelength range are desired, eliminating cryogenic requirements and leveraging existing optical fiber infrastructure for transmitting the quantum information. To that end, we report that telecom single photon emitters (SPEs) in gallium nitride (GaN) exhibit optically detected magnetic resonance (ODMR) at room temperature. The analysis of ODMR as a function of magnetic field orientation enables the determination of the orientation of the spin quantization axis with respect to the GaN crystalline lattice. The optical transitions dynamics are analyzed to gain further insight into the transition rates dominating ODMR. Our findings, coupled with GaN's mature fabrication technology, could facilitate the realization of scalable quantum technology.

cond-mat.mtrl-sci↗

arXiv2024

Dielectric Fano Nanoantennas for Enabling Sub-Nanosecond Lifetimes in NV-based Single Photon Emitters

Solid-state quantum emitters are essential sources of single photons, and enhancing their emission rates is of paramount importance for applications in quantum communications, computing, and metrology. One approach is to couple quantum emitters with resonant photonic nanostructures, where the emission rate is enhanced due to the Purcell effect. Dielectric nanoantennas are promising as they provide strong emission enhancement compared to plasmonic ones, which suffer from high Ohmic loss. Here, we designed and fabricated a dielectric Fano resonator based on a pair of silicon (Si) ellipses and a disk, which supports the mode hybridization between quasi-bound-states-in-the-continuum (quasi-BIC) and Mie resonance. We demonstrated the performance of the developed resonant system by interfacing it with single photon emitters (SPEs) based on nitrogen-vacancy (NV-) centers in nanodiamonds (NDs). We observed that the interfaced emitters have a Purcell enhancement factor of ~10, with sub-ns emission lifetime and a polarization contrast of 9. Our results indicate a promising method for developing efficient and compact single-photon sources for integrated quantum photonics applications.

physics.optics↗

arXiv2024

Unidirectional Chiral Emission via Twisted Bi-layer Metasurfaces

Controlling and channelling light emissions from unpolarized quantum dots into specific directions with chiral polarization remains a key challenge in modern photonics. Stacked metasurface designs offer a potential compact solution for chirality and directionality engineering. However, experimental observations of directional chiral radiation from resonant metasurfaces with quantum emitters remain obscure. In this paper, we present experimental observations of unidirectional chiral emission from a twisted bi-layer metasurface via multi-dimensional control, including twist angle, interlayer distance, and lateral displacement between the top and bottom layers, as enabled by doublet alignment lithography (DAL). First, maintaining alignment, the metasurface demonstrates a resonant intrinsic optical chirality with near-unity circular dichroism of 0.94 and reflectance difference of 74%, where a high circular dichroism greater than 0.9 persists across a wide range of angles from -11 to 11 degrees. Second, engineered lateral displacement induces a unidirectional chiral resonance, resulting in unidirectional chiral emission from the quantum dots deposited onto the metasurface. Our bi-layer metasurfaces offer a universal compact platform for efficient radiation manipulation over a wide angular range, promising potential applications in miniaturized lasers, grating couplers, and chiral nanoantennas.

physics.optics↗

arXiv2023

Silicon Nanoantenna Mix Arrays for a Trifecta of Quantum Emitter Enhancements

Dielectric nanostructures have demonstrated optical antenna effects due to Mie resonances. Preliminary investigations on dielectric nanoantennas have been carried out for a trifecta of enhancements, i.e., simultaneous enhancements in absorption, emission directionality and radiative decay rates of quantum emitters. However, these investigations are limited by fragile substrates or low Purcell factor, which is extremely important for exciting quantum emitters electrically. In this paper, we present a Si mix antenna array to achieve the trifecta enhancement of ~1200 fold with a Purcell factor of ~47. The antenna design incorporates ~10 nm gaps within which fluorescent molecules strongly absorb the pump laser energy through a resonant mode. In the emission process, the antenna array increases the radiative decay rates of the fluorescence molecules via Purcell effect and provides directional emission through a separate mode. This work could lead to novel CMOS compatible platforms for enhancing fluorescence for biological and chemical applications.

physics.optics↗

arXiv2023

Reply to: Mobility overestimation in MoS$_2$ transistors due to invasive voltage probes

In this reply, we include new experimental results and verify that the observed non-linearity in rippled-MoS$_2$ (leading to mobility kink) is an intrinsic property of a disordered system, rather than contact effects (invasive probes) or other device issues. Noting that Peng Wu's hypothesis is based on a highly ordered ideal system, transfer curves are expected to be linear, and the carrier density is assumed be constant. Wu's model is therefore oversimplified for disordered systems and neglects carrier-density dependent scattering physics. Thus, it is fundamentally incompatible with our rippled-MoS$_2$, and leads to the wrong conclusion.

cond-mat.mtrl-sci↗

arXiv2023

Engineering Perovskite Emissions via Optical Quasi-Bound-States-in-the-Continuum

Metal halide perovskite quantum dots (PQDs) have emerged as promising materials due to their exceptional photoluminescence (PL) properties. A wide range of applications could benefit from adjustable luminescence properties, while preserving the physical and chemical properties of the PQDs. Therefore, post-synthesis engineering has gained attention recently, involving the use of ion-exchange or external stimuli, such as extreme pressure, magnetic and electric fields. Nevertheless, these methods typically suffer from spectrum broadening, intensity quenching or yield multiple bands. Alternatively, photonic antennas can modify the radiative decay channel of perovskites via the Purcell effect, with the largest wavelength shift being 8 nm to date, at an expense of 5-fold intensity loss. Here, we present an optical nanoantenna array with polarization-controlled quasi-bound-states-in-the-continuum (q-BIC) resonances, which can engineer and shift the photoluminescence wavelength over a ~39 nm range and confers a 21-fold emission enhancement of FAPbI3 perovskite QDs. The spectrum is engineered in a non-invasive manner via lithographically defined antennas and the pump laser polarization at ambient conditions. Our research provides a path towards advanced optoelectronic devices, such as spectrally tailored quantum emitters and lasers.

physics.optics↗

arXiv2022

Asymmetric parametric generation of images with nonlinear dielectric metasurfaces

Subwavelength dielectric resonators assembled into metasurfaces have become a versatile tool for miniaturising optical components approaching the nanoscale. An important class of metasurface functionalities is associated with asymmetry in both generation and transmission of light with respect to reversals of the positions of emitters and receivers. Nonlinear light-matter interaction in metasurfaces offers a promising pathway towards miniaturisation of the asymmetric control of light. Here we demonstrate asymmetric parametric generation of light in nonlinear metasurfaces. We assemble dissimilar nonlinear dielectric resonators into translucent metasurfaces that produce images in the visible spectral range being illuminated by infrared radiation. By design, the metasurfaces produce different and completely independent images for the reversed direction of illumination, that is when the positions of the infrared emitter and the visible light receiver are exchanged. Nonlinearity-enabled asymmetric control of light by subwavelength resonators paves the way towards novel nanophotonic components via dense integration of large quantities of nonlinear resonators into compact metasurface designs.

physics.optics↗

arXiv2022

Tri-Functional Metasurface for Phase, Amplitude, and Luminescence Control

In optical anti-counterfeiting, several distinct optically variable devices (OVDs) are often concurrently employed to compensate for the insufficient security level of constituent OVDs. Alternatively, metasurfaces that exhibit multiple optical responses effectively combine multiple OVDs into one, thus significantly enhancing their security and hindering fraudulent replication. This work demonstrates the simultaneous control of three separate optical responses, i.e., phase, amplitude, and luminescence, using anisotropic gap-plasmon metasurfaces. Due to the incorporated geometric anisotropy, the designed structure exhibits distinct responses under x- and y-polarized light, revealing either a color image, or a holographic projection in the far field. Furthermore, inserting upconversion nanoparticles (UCNPs) into the dielectric gaps of the structures, the designed metasurface is able to generate a third luminescent image upon illumination with the near-infrared light. The stochastic distribution of the UCNPs constitutes a unique fingerprint, achieving a physically unclonable function (PUF) layer. Crucially, our triple-mode metasurface requires only readily attainable equipment such as a macro-lens/camera and a laser pointer to read most of the channels, thus paving the way towards highly secure and easy-to-authenticate metasurface-driven OVDs (mOVDs).

physics.optics↗

arXiv2022

Miniaturizing Color-Sensitive Photodetectors via Hybrid Nanoantennas towards Sub-micron Dimensions

Digital camera sensors utilize color filters on photodiodes to achieve color selectivity. As color filters and photosensitive silicon layers are separate elements, these sensors suffer from optical cross-talk, which sets limits to the minimum pixel size. In this paper, we report hybrid silicon-aluminum nanostructures in the extreme limit of zero distance between color filters and sensors. This design could essentially achieve sub micron pixel dimensions and minimize the optical cross-talk originated from tilt illuminations. The designed hybrid silicon-aluminum nanostructure has dual functionalities. Crucially, it supports a hybrid Mie-plasmon resonance of magnetic dipole to achieve the color-selective light absorption, generating electron hole pairs. Simultaneously, the silicon-aluminum interface forms a Schottky barrier for charge separation and photodetection. This design could potentially replace the traditional dye based filters for camera sensors at ultra-high pixel densities with advanced functionalities in sensing polarization and directionality, as well as UV selectivity via interband plasmons of silicon.

physics.optics↗