arXiv subjects

Zhaopin Chen

Publications and source records attributed to Zhaopin Chen.

At least 19 recordsLinked to original sources

arXiv2026

Multidimensional attosecond clocking near Dirac cones in graphite

Two-color high-harmonic spectroscopy is widely used to access sub-cycle electron dynamics and to retrieve harmonic timing information, including harmonic phases and attochirp across gases, solids, and liquids. However, the dependence of such timing observables on additional laser-control parameters remains largely unexplored. Here, we introduce driving intensity as an additional dimension of two-color harmonic spectroscopy in highly oriented pyrolytic graphite (HOPG). The retrieved attosecond two-color delays maximizing the 4th and 5th harmonic yields evolve systematically and differently with driving intensity. Semiconductor Bloch-equation calculations reproduce these trends and reveal a pronounced sensitivity of the intensity-dependent delays to the electronic band dispersion. Our results demonstrate multidimensional attosecond clocking near Dirac cones and establish intensity-dependent two-color delays as a sensitive observable for band-dispersion in quantum materials.

physics.optics↗

arXiv2026

Stable three-dimensional solitons in spin-orbit-coupled atomic-molecular condensates

We elaborate a mechanism for the creation of stable three-dimensional (3D) solitons in spin-orbit-coupled (SOC) atomic-molecular Bose-Einstein condensate, modeled by the mean-field equations with the quadratic three-wave interaction, characterized by mismatch $α$. The planar (effectively two-dimensional) SOC is applied to the soliton's atomic component, structuring it as a mixed mode (MM) or semi-vortex (SV). The molecular component of the SV soliton is shaped as a 3D vortex, while the molecular component in the MM soliton is an MM too. The solitons exist up to a critical value of $α$. The system demonstrates a relatively large norm share of the vortex components, exceeding $50\%$ of the total norm, which is an essential feature of SOC-supported solitons. This is scheme for realizing stable vortex solitons in free space with the quadratic nonlinearity.

quant-ph↗

arXiv2026

Clocking and controlling attosecond currents in a scanning tunnelling microscope

Quantum tunnelling of electrons can be confined to the sub-cycle time scale of strong light fields, contributing decisively to the extreme time resolution of attosecond science. Because tunnelling also enables atomic-scale spatial resolution in scanning tunnelling microscopy (STM), integrating STM with light pulses has long been a key objective in ultrafast microscopy, spanning the picosecond and femtosecond domains, with first signatures of attosecond dynamics. However, while sub-cycle dynamics on the attosecond time scale are routinely controlled and determined with high precision, controlling the direction of attosecond currents and determining their duration have remained elusive in STM. Here, we induce STM tunnelling currents using two-colour laser pulses and dynamically control their direction, relying solely on the sub-cycle waveform of the pulses. Projecting our measurement data onto one-electron and many-body theory descriptions reveals a three-step transport process in the non-adiabatic tunnelling regime as the physical mechanism, with a theory-derived current burst duration of 860 as. Despite working under ambient conditions but free of thermal artifacts, we achieve sub-angström topographic sensitivity and a lateral spatial resolution of 2 nm. This unprecedented capability to directionally control attosecond bursts will enable triggering and imaging ultrafast charge dynamics at the spatio-temporal microscopy frontier of lightwave electronics.

quant-ph↗

arXiv2026

Formation and dynamics of self-bound droplets in dipolar molecular condensate

Recent advances in the work with ultracold condensates of polar molecules have enabled the realization of highly tunable self-bound quantum droplets (QDs), with the help of dual microwave fields dressig the dipole-dipole interactions (DDIs) It has been reported that symmetry properties and the equilibrium phase diagram of such QDs can be controlled by parameters of the two microwave fields. However, the effect of these fields on the formation and dynamics of the QD has not yet been systematically explored. Here we address self-bound QDs in a regime dominated by non-axisymmetric DDIs and governed by the extended Gross-Pitaevskii equation with the Lee-Huang-Yang corrections. Within this framework, we identify the existence region of the self-bound QDs and characterize their chemical potential, total energy, effective volume, peak density, and geometric anisotropy. The results reveal a pronounced nonmonotonous dependence on the non-axisymmetric DDI strength, whereas the increase of the number of particles in the condensate leads to tighter bound and more anisotropic QDs. Furthermore, reducing the s-wave scattering length drives a transition from stable self-bound states to the collapse. Collisions between QDs moving along different directions reveal a strong directional dependence, with outcomes ranging from quasi-elastic rebound and merger to fragmentation.

cond-mat.quant-gas↗

arXiv2026

The bulk modulus of three-dimensional quantum droplets

Quantum droplets (QDs), formed by ultradilute quantum fluids under the action of the Lee-Huang-Yang (LHY) effect, provide a unique platform for investigating a wide range of macroscopic quantum effects. Recent studies of QDs' breathing modes and collisional dynamics have revealed their compressibility and extensibility, which suggests that their elasticity parameters can be identified. In this work we derive the elastic bulk modulus (BM) of QDs by means of theoretical analysis and numerical simulations and establish a relation between the BM and the eigenfrequency of the QD's intrinsic vibrations. The analysis reveals the dependence of the QD's elasticity on the particle number and the strength of interparticle interactions. We additionally provide a realistic estimate of the bulk modulus for the system, yielding a concrete physical value that may serve as a reference for future experimental measurements. Taken together, these results also point to possibilities for realizing elastic media governed by the LHY effect.

cond-mat.quant-gas↗

arXiv2026

Two-color harmonic spectroscopy of ultrafast Dirac electron dynamics

High-harmonic generation (HHG), the hallmark effect of attosecond science, is a nonperturbative nonlinear process leading to the emission of high-harmonic light from gases and solids. In gases, extreme driving laser pulse intensities can deplete the ground state, suppressing harmonic emission during the trailing edge of the pulse. Here, we report a similar effect, pronounced ultrafast carrier saturation dynamics and harmonic emission suppression during nonperturbative harmonic generation (NPHG) in a gapless Dirac semimetal -- highly oriented pyrolytic graphite (HOPG). Remarkably, HOPG supports NPHG at laser intensities as low as $\sim 10^{10}$ W cm$^{-2}$, facilitated by its vanishing bandgap. Ultrafast carrier saturation strongly modulates the interplay between interband and intraband currents, a key characteristic of NPHG in Dirac materials. Using two-color spectroscopy, we reveal the excitation dynamics of Dirac electron-hole pairs as it affects the emission of harmonics during the presence of the driving laser pulse. The excitation of out-of-equilibrium hot carriers and the concomitant saturation near the Dirac points leads to a marked suppression of interband harmonics and induces measurable temporal shifts. These observations are supported by simulations based on semiconductor Bloch equations. Our finding reveal that field-driven carrier saturation plays a critical role in gapless solid NPHG. We demonstrate the potential of NPHG and HHG as a sensitive, all-optical probe of ultrafast carrier dynamics, offering novel opportunities for ultrafast optoelectronics in Dirac materials.

physics.optics↗

arXiv2025

Single-shot pulse retrieval of femtosecond bright squeezed vacuum

Bright squeezed vacuum (BSV) is an intense quantum state of light with zero mean electric field and huge photon number fluctuations, sufficiently intense to drive extreme nonlinear processes and imprint nonclassical statistics. However, the temporal structure of single BSV shots has not been fully characterized. Here, we retrieve the spectral and temporal pulse characteristics of a set of single-peak BSV shots. It is obtained by realizing a femtosecond BSV source at 1040 nm with a single spatial mode and perform single-shot spectral interferometry with a fully characterized coherent-state reference pulse. Our approach reveals that the group delay is consistent between the various shots, resulting in an average pulse duration of 27.2 fs, much shorter than the pump pulse, and a variation of 5.5 fs (standard deviation). We also observe a characteristic nodal structure in the spectral interferograms, demonstrating the BSV's random phase ambiguity of $π$ rad. Our approach demonstrates that BSV is a viable source of femtosecond light pulses for attosecond sub-cycle metrology of ultrafast electron dynamics.

physics.optics↗

arXiv2025

Chiral solitons in quadratic quasi-phase-matched photonic crystals

We introduce a quasi-phase-matched technique in quadratic nonlinear crystals, constructing an artificial gauge field by changing the inclination angle of stripes, which is realized by the positive and negative polarization directions of nonlinear susceptibility along the crystal. Unlike the artificial gauge field constructed through linear coupling in other settings, the gauge field in this system is realized by nonlinear coupling. We demonstrate that this gauge field can generate stable chiral solitons with chiral energy flow rotating around the solitons. In contrast to conventional chiral currents generated with the same specie or frequency, the chiral currents in the present system are formed by mutual coupling between fundamental frequency and second harmonic components. We derive the semi-analytical solution for the chiral energy flow in this system. It is found that there exists an optimal inclination angle that can maximize the chiral energy flow under different parameters, and this optimal inclination shows a positive correlation with the power and detuning. The mobility and collisions of the chiral solitons are also discussed. The results show that chiral solitons move in response to kicking and undergo fully elastic collisions with each other. In addition, the possibility of experimentally generating chiral solitons and chiral currents is outlined.

physics.optics↗

arXiv2025

Elongated vortex quantum droplets in binary Bose-Einstein condensates

Stability of elongated (``slender") quantum droplets (QDs) with embedded unitary and multiple vorticity is a problem that was not solved previously. In this work, we propose a solution which relies upon the use of the spatial modulation of the inter-species scattering length in the binary Bose-Einstein condensates, in the form of a two-dimensional axisymmetric Gaussian, shaped by means of the optical Feshbach resonance. The corresponding effective nonlinear trapping potential supports completely stable elongated QDs with vorticity $S=0$ and partly stable families of elongated QDs with $S=1,2,3,4$ (other nonlinear systems do not maintain stability of vortex droplets with $\geq 2$). We systematically analyze effects of the amplitude and width of the Gaussian modulation, as well as the total number of atoms, on the shape and stability of the QDs, some effects being explained analytically. Collisions between identical QDs with $% S=1$ moving in opposite directions along the central axis leads to their merger into still more elongated breathing QDs with the same vorticity, while collisions between QDs with $S=\pm 1$ are quasi-elastic. Moving modulation profiles are able to adiabatically rotate the trapped elongated QDs. Application of a torque to the vector QD sets in the gyroscopic regime of robust precession, which realizes a macroscopic spin-orbit-coupling effect.

cond-mat.quant-gas↗

arXiv2025

Amplifying solid-state high harmonic generations with momentum k-gaps in band structure engineering

We propose a novel amplification mechanism for high harmonic generation (HHG) in solids by leveraging bandgap engineering with momentum k-gaps. By constructing a simple diatomic lattice featuring balanced, alternating gain and loss profiles, facilitated by an array of four-level systems, we explore the physics of k-gap-amplified Bloch oscillations in the intraband channel of solid-state HHG. Through numerical simulations, we elucidate the coexistence of amplification and harmonic radiation processes in a solid. Our finding reveals that advanced bandgap engineering can define k-space optical devices - such as Brillouin cavity, Bloch-Zener oscillator and k-gap amplifier - thereby enabling the coherent manipulation of semiconductor radiation and high harmonic generation in both semiconductor superlattices and artificial materials. Furthermore, we analyze the spectrogram and material realizations required for amplifying solid-state HHG. These results underscore the potential of k-gap band structure engineering to advance coherent light sources at extremely short wavelengths.

physics.optics↗

arXiv2024

Attosecond pulses from a solid driven by a synthesized two-color field at megahertz repetition rate

Probing coherent quantum dynamics in light-matter interactions at the microscopic level requires high-repetition-rate isolated attosecond pulses (IAPs) in pump-probe experiments. To date, the generation of IAPs has been mainly limited to the kilohertz regime. In this work, we experimentally achieve attosecond control of extreme-ultraviolet (XUV) high harmonics in the wide-bandgap dielectric MgO, driven by a synthesized field of two femtosecond pulses at 800nm and 2000nm with relative phase stability. The resulting quasi-continuous harmonic plateau with ~ 9 eV spectral width centered around 16.5 eV photon energy can be tuned by the two-color phase and supports the generation of an IAP (~ 730 attoseconds), confirmed by numerical simulation based on three-band semiconductor Bloch equations. Leveraging the high-repetition-rate driver laser and the moderate intensity requirements of solid-state high-harmonic generation, we achieve IAP production at an unprecedented megahertz repetition rate, paving the way for all-solid compact XUV sources for IAP generation.

physics.optics↗

arXiv2024

Strongly anisotropic vortices in dipolar quantum droplets

We construct strongly anisotropic quantum droplets with embedded vorticity in the 3D space, with mutually perpendicular vortex axis and polarization of atomic magnetic moments. Stability of these anisotropic vortex quantum droplets (AVQDs) is verified by means of systematic simulations. Their stability area is identified in the parametric plane of the total atom number and scattering length of the contact interactions. We also construct vortex-antivortex-vortex bound states and find their stability region in the parameter space. The application of a torque perpendicular to the vorticity axis gives rise to robust intrinsic oscillations or rotation of the AVQDs. The effect of three-body losses on the AVQD stability is considered too. The results show that the AVQDs can retain the topological structure (vorticity) for a sufficiently long time if the scattering length exceeds a critical value.

cond-mat.quant-gas↗

arXiv2024

Semi-vortex solitons and their excited states in spin-orbit-coupled binary bosonic condensates

It is known that two-dimensional two-component fundamental solitons of the semi-vortex (SV) type, with vorticities $(s_{+},s_{-})=(0,1)$ in their components, are stable ground states (GSs) in the spin-orbit-coupled (SOC) binary Bose-Einstein condensate with the contact self-attraction acting in both components, in spite of the possibility of the critical collapse in the system. However, excited states(ESs) of the SV solitons, with the vorticity set $(s_{+},s_{-})=( S_{+},S_{+}+1)$ and $S_{+}=1,2,3,...$, are unstable in the same system. We construct ESs of SV solitons in the SOC system with opposite signs of the self-interaction in the two components. The main finding is stability of the ES-SV solitons, with the extra vorticity (at least) up to $S_{+}=6$. The threshold value of the norm for the onset of the critical collapse, $N_{\mathrm{thr}}$, in these excited states is higher than the commonly known critical value, $N_{c}\approx 5.85$,associated with the single-component Townes solitons, $N_{\mathrm{thr}}$ increasing with the growth of $S_{+}$. A velocity interval for stable motion of the GS-SV solitons is found too. The results suggest a solution for the challenging problem of the creation of stable vortex solitons with high topological charges.

cond-mat.quant-gas↗

arXiv2024

High Harmonic Generation by Bright Squeezed Vacuum

We observe non-perturbative high harmonic generation in solids driven by a macroscopic quantum state of light, bright squeezed vacuum (BSV), which we generate in a single spatiotemporal mode. The BSV-driven process is considerably more efficient in the generation of high harmonics than classical light of the same mean intensity. Due to its broad photon-number distribution, covering states from $0$ to $2 \times 10^{13}$ photons per pulse, and sub-cycle electric field fluctuations over $\pm1\hbox{V}/\hbox{Å}$, BSV provides access to free carrier dynamics within a much broader range of peak intensities than accessible with classical light. Our findings contribute to recent developments of quantum optics with extreme intensities, moving beyond its traditional focus on low photon numbers, and providing a new method for exploring extreme nonlinearities in solids.

quant-ph↗

arXiv2023

Self-trapping of slow electrons in the energy domain

The interaction of light and swift electrons has enabled phase-coherent manipulation and acceleration of electron wavepackets. Here we investigate this interaction in a new regime where low-energy electrons (~20-200 eV) interact with a phase-matched light field. Our analytical and one-dimensional numerical study shows that slow electrons are subject to strong confinement in the energy domain due to the non-vanishing curvature of the electron dispersion. The spectral trap is tunable and an appropriate choice of light field parameters can reduce the interaction dynamics to only two energy states. The capacity to trap electrons expands the scope of electron beam physics, free-electron quantum optics and quantum simulators.

quant-ph↗

arXiv2023

Semidiscrete optical vortex droplets in quasi-phase-matched photonic crystals

A new scheme for producing semidiscrete self-trapped vortices (\textquotedblleft swirling photon droplets\textquotedblright ) in photonic crystals with competing quadratic ($χ^{(2)}$) and self-defocusing cubic ($χ^{(3)}$) nonlinearities is proposed. The photonic crystal is designed with a striped structure, in the form of spatially periodic modulation of the $χ^{(2)}$ susceptibility, which is imposed by the quasi-phase-matching technique. Unlike previous realizations of semidiscrete optical modes in composite media, built as combinations of continuous and arrayed discrete waveguides, the semidiscrete vortex droplets are produced here in the fully continuous medium. This work reveals that the system supports two types of semidiscrete vortex droplets, \textit{viz}., onsite- and intersite-centered ones, which feature, respectively, odd and even numbers of stripes, $\mathcal{N}$. Stability areas for the states with different values of $\mathcal{N}$ are identified in the system's parameter space. Some stability areas overlap with each others, giving rise to multistability of states with different $\mathcal{N}$. The coexisting states are mutually degenerate, featuring equal values of the Hamiltonian and propagation constant. An experimental scheme to realize the droplets is outlined, suggesting new possibilities for the long-distance transmission of structured light carrying orbital angular momentum in nonlinear media.

physics.optics↗

arXiv2023

Two-dimensional anisotropic vortex quantum droplets in dipolar Bose-Einstein condensates

Creation of stable intrinsically anisotropic self-bound states with embedded vorticity is a challenging issue. Previously, no such states in Bose-Einstein condensates (BECs) or other physical settings were known. Dipolar BEC suggests a unique possibility to predict stable anisotropic vortex quantum droplets (AVQDs). We demonstrate that they can be created with the vortex' axis oriented \emph{perpendicular} to the polarization of dipoles. The stability area and characteristics of the AVQDs in the parameter space are revealed by means of analytical and numerical methods. Further, the rotation of the polarizing magnetic field is considered, and the largest angular velocities, up to which spinning AVQDs can follow the rotation in clockwise and anti-clockwise directions, are found. Collisions between moving AVQDs are studied too, demonstrating formation of bound states with a vortex-antivortex-vortex structure. A stability domain for such stationary bound states is identified. Unstable dipolar states, that can be readily implemented by means of phase imprinting, quickly transform into robust AVQDs, which suggests a straightforward possibility for the creation of these states in the experiment.

cond-mat.quant-gas↗

arXiv2023

Vortex solitons in quasi-phase-matched photonic crystals

We report solutions for stable compound solitons in a three-dimensional quasi-phase-matched photonic crystal with the quadratic ($χ^{(2)}$) nonlinearity. The photonic crystal is introduced with a checkerboard structure, which can be realized by means of the available technology. The solitons are built as four-peak vortex modes of two types, rhombuses and squares (intersite- and onsite-centered self-trapped states, respectively). Their stability areas are identified in the system's parametric space (rhombuses occupy an essentially broader stability domain), while all bright vortex solitons are subject to strong azimuthal instability in uniform $χ^{(2)}$ media. Possibilities for experimental realization of the solitons are outlined.

physics.optics↗