arXiv subjects

Zhe Sun

Publications and source records attributed to Zhe Sun.

At least 109 records · Page 6Linked to original sources

arXiv2023

Electronic band reconstruction across the insulator-metal transition in colossal magnetoresistive EuCd2P2

While colossal magnetoresistance (CMR) in Eu-based compounds is often associated with strong spin-carrier interactions, the underlying reconstruction of the electronic bands is much less understood from spectroscopic experiments. Here using angle-resolved photoemission, we directly observe an electronic band reconstruction across the insulator-metal (and magnetic) transition in the recently discovered CMR compound EuCd2P2. This transition is manifested by a large magnetic band splitting associated with the magnetic order, as well as unusual energy shifts of the valence bands: both the large ordered moment of Eu and carrier localization in the paramagnetic phase are crucial. Our results provide spectroscopic evidence for an electronic structure reconstruction underlying the enormous CMR observed in EuCd2P2, which could be important for understanding Eu-based CMR materials, as well as designing CMR materials based on large-moment rare-earth magnets.

cond-mat.mtrl-sci↗

arXiv2023

Photoemission Evidence of a Novel Charge Order in Kagome Metal FeGe

A charge order has been discovered to emerge deep into the antiferromagnetic phase of the kagome metal FeGe. To study its origin, the evolution of the low-lying electronic structure across the charge order phase transition is investigated with angle-resolved photoemission spectroscopy. We do not find signatures of nesting between Fermi surface sections or van-Hove singularities in zero-frequency joint density of states, and there are no obvious energy gaps at the Fermi level, which exclude the nesting mechanism for the charge order formation in FeGe. However, two obvious changes in the band structure have been detected, i.e., one electron-like band around the K point and another one around the A point move upward in energy position when the charge order forms. These features can be well reproduced by our density-functional theory calculations, where the charge order is primarily driven by magnetic energy saving via large dimerizations of a quarter of Ge1-sites (in the kagome plane) along the c-axis. Our results provide strong support for this novel charge order formation mechanism in FeGe, in contrast to the conventional nesting mechanism.

cond-mat.str-el↗

arXiv2023

The Goldman symplectic form on the PGL(V)-Hitchin component

This article is the second of a pair of articles about the Goldman symplectic form on the PGL(V)-Hitchin component of a closed, connected, oriented, hyperbolic surface S. We show that any ideal triangulation on S and any compatible bridge system determine a symplectic trivialization of the tangent bundle to the PGL(V)-Hitchin component of S. Using this, we prove that a large class of vector fields defined in the companion paper [SWZ20] are Hamiltonian. This is then used to prove that the explicit global coordinate system defined in the companion paper [SWZ20] is a global Darboux coordinate system for the PGL(V)-Hitchin component.

math.DG↗

arXiv2023

Quantum metric nonlinear Hall effect in a topological antiferromagnetic heterostructure

Quantum geometry - the geometry of electron Bloch wavefunctions - is central to modern condensed matter physics. Due to the quantum nature, quantum geometry has two parts, the real part quantum metric and the imaginary part Berry curvature. The studies of Berry curvature have led to countless breakthroughs, ranging from the quantum Hall effect in 2DEGs to the anomalous Hall effect (AHE) in ferromagnets. However, in contrast to Berry curvature, the quantum metric has rarely been explored. Here, we report a new nonlinear Hall effect induced by quantum metric by interfacing even-layered MnBi2Te4 (a PT-symmetric antiferromagnet (AFM)) with black phosphorus. This novel nonlinear Hall effect switches direction upon reversing the AFM spins and exhibits distinct scaling that suggests a non-dissipative nature. Like the AHE brought Berry curvature under the spotlight, our results open the door to discovering quantum metric responses. Moreover, we demonstrate that the AFM can harvest wireless electromagnetic energy via the new nonlinear Hall effect, therefore enabling intriguing applications that bridges nonlinear electronics with AFM spintronics.

cond-mat.mes-hall↗

arXiv2023

Electrical detection of the flat band dispersion in van der Waals field-effect structures

Two-dimensional flat-band systems have recently attracted considerable interest due to the rich physics unveiled by emergent phenomena and correlated electronic states at van Hove singularities. However, the difficulties in electrically detecting the flat band position in field-effect structures are slowing down the investigation of their properties. In this work, we employ Indium Selenide (InSe) as a flat-band system due to a van Hove singularity at the valence band edge in a few-layer form of the material without the requirement of a twist angle. We investigate tunneling photocurrents in gated few-layer InSe structures and relate them to ambipolar transport and photoluminescence measurements. We observe an appearance of a sharp change in tunneling mechanisms due to the presence of the van Hove singularity at the flat band. We further corroborate our findings by studying tunneling currents as a reliable probe for the flat-band position up to room temperature. Our results create an alternative approach to studying flat-band systems in heterostructures of 2D materials.

cond-mat.mes-hall↗

arXiv2023

Origin of the exotic electronic states in antiferromagnetic NdSb

Using angle resolved photoemission spectroscopy measurements and first principle calculations, we report that the possible unconventional 2q antiferromagnetic (AFM) order in NdSb can induce unusual modulation on its electronic structure. The obvious extra bands observed in the AFM phase of NdSb are well reproduced by theoretical calculations, in which the Fermi-arc-like structures and sharp extra bands are originated from the in-gap surface states. However, they are demonstrated to be topological trivial. By tuning the chemical potential, the AFM phase of NdSb would go through a topological phase transition, realizing a magnetic topological insulator phase. Hence, our study sheds new light on the rare earth monopnictides for searching unusual AFM structure and the potential of intrinsic magnetic topological materials.

cond-mat.mtrl-sci↗

arXiv2023

Spectroscopic Evidence for Dirac Nodal Surfaces and Nodal Rings in Superconductor NaAlSi

The discovery of the topological states has become a key topic in condensed matter physics with the focus evolving from the Dirac or Weyl points to high-dimension topological states of the nodal lines and nodal surfaces. For a topological material to manifest its quantum properties and become useful in applications, the topological states need to be genuine and clean so that they lie close to the Fermi level without other trivial bands existing at the Fermi level. While a number of high-dimension topological materials are predicted, only a few of them have been synthesized and confirmed and the genuine and clean ones are especially scarce. Here we report the realization of the genuine clean multiple high-dimension topological states in NaAlSi. By performing high-resolution angle-resolved photoemission measurements and band structure calculations, we have observed two sets of nodal surfaces and the formation of two homocentric nodal ring states in NaAlSi. The observed nodal rings are distinct in that the inner one is a type-{\uppercase\expandafter{\romannumeral1}} nodal ring while the outer one is a type-{\uppercase\expandafter{\romannumeral1}} nodal ring embedded with four type-{\uppercase\expandafter{\romannumeral3}} nodal points. All the bands involved in the nodal rings lie very close to the Fermi level with no other trivial bands coexisting at the Fermi level. These observations make NaAlSi a desirable topological material to explore for novel quantum states and exotic properties.

cond-mat.mtrl-sci↗

arXiv2023

Observation of spin-polarized surface states in a nodal line semimetal SnTaS$_{2}$

The superconductor SnTaS$_{2}$ is theoretically predicted to be an intriguing topological nodal line semimetal without consideration of spin-orbit coupling. By carrying out angle-resolved photoemission (ARPES) and spin-resolved ARPES measurements combined with band structure calculations, we have provided a complete picture of the electronic structure and spin polarization property for the prominent surface states of SnTaS$_{2}$. The low-energy electronic states are dominated by surface states; two of them are from the S-terminated surface, while four of them are from the Sn-terminated surface. These give rise to interesting Fermi surface topology of SnTaS$_{2}$: three pockets located at $\barΓ$, $\bar{M}$ and $\bar{K}$ for the S-terminated surface and two pockets surrounding $\barΓ$ and $\bar{K}$ for the Sn-terminated surface. We further reveal that two surface states that cross the Fermi level are spin-polarized. Since SnTaS$_{2}$ is also a superconductor, our observations indicate that it may provide a new platform to explore topological superconductivity and other exotic properties.

cond-mat.supr-con↗

arXiv2023

Electrical control of hybrid exciton transport in a van der Waals heterostructure

Interactions between out-of-plane dipoles in bosonic gases enable the long-range propagation of excitons. The lack of direct control over collective dipolar properties has hitherto limited the degrees of tunability and the microscopic understanding of exciton transport. In this work, we modulate the layer hybridization and interplay between many-body interactions of excitons in a van der Waals heterostructure with an applied vertical electric field. By performing spatiotemporally resolved measurements supported by microscopic theory, we uncover the dipole-dependent properties and transport of excitons with different degrees of hybridization. Moreover, we find constant emission quantum yields of the transporting species as a function of excitation power with dominating radiative decay mechanisms over nonradiative ones, a fundamental requirement for efficient excitonic devices. Our findings provide a complete picture of the many-body effects in the transport of dilute exciton gases and have crucial implications for the study of emerging states of matter, such as Bose-Einstein condensation, as well as for optoelectronic applications based on exciton propagation.

cond-mat.mes-hall↗

arXiv2023

Evidence of high-temperature exciton condensation in a two-dimensional semimetal

Electrons and holes can spontaneously form excitons and condense in a semimetal or semiconductor, as predicted decades ago. This type of Bose condensation can happen at much higher temperatures in comparison with dilute atomic gases. Two-dimensional (2D) materials with reduced Coulomb screening around the Fermi level are promising for realizing such a system. Here we report a change in the band structure accompanied by a phase transition at about 180 K in single-layer ZrTe2 based on angle-resolved photoemission spectroscopy (ARPES) measurements. Below the transition temperature, gap opening and development of an ultra-flat band top around the zone center are observed. This gap and the phase transition are rapidly suppressed with extra carrier densities introduced by adding more layers or dopants on the surface. The results suggest the formation of an excitonic insulating ground state in single-layer ZrTe2, and the findings are rationalized by first principles calculations and a self-consistent mean-field theory. Our study provides evidence for exciton condensation in a 2D semimetal and demonstrates strong dimensionality effects on the formation of intrinsic bound electron-hole pairs in solids.

cond-mat.mes-hall↗

arXiv2022

Enabling Temporal-Spectral Decoding in Pre-movement Detection

Non-invasive brain-computer interfaces help the subjects to control external devices by brain intentions. The multi-class classification of upper limb movements can provide external devices with more control commands. The onsets of the upper limb movements are located by the external limb trajectory to eliminate the delay and bias among the trials. However, the trajectories are not recorded due to the limitation of experiments. The delay cannot be avoided in the analysis of signals. The delay negatively influences the classification performance, which limits the further application of upper limb movements in the brain-computer interface. This work focuses on multi-channel brain signals analysis in the temporal-frequency approach. It proposes the two-stage-training temporal-spectral neural network (TTSNet) to decode patterns from brain signals. The TTSNet first divides the signals into various filter banks. In each filter bank, task-related component analysis is used to reduce the dimension and reject the noise of the brain. A convolutional neural network (CNN) is then used to optimize the temporal characteristic of signals and extract class-related features. Finally, these class-related features from all filter banks are fused by concatenation and classified by the fully connected layer of the CNN. The proposed method is evaluated in two public datasets. The results show that TTSNet has an improved accuracy of 0.7456$\pm$0.1205 compared to the EEGNet of 0.6506$\pm$0.1275 ($p<0.05$) and FBTRCA of 0.6787$\pm$0.1260 ($p<0.1$) in the movement detection task, which classifies the movement state and the resting state. The proposed method is expected to help detect limb movements and assist in the rehabilitation of stroke patients.

cs.HC↗

arXiv2022

Advantage of quantum coherence in postselected metrology

In conventional measurement, to reach the greatest accuracy of parameter estimation, all samples must be measured since each independent sample contains the same quantum Fisher information. In postselected metrology, postselection can concentrate the quantum Fisher information of the initial samples into a tiny post-selected sub-ensemble. It has been proven that this quantum advantage can not be realized in any classically commuting theory. In this work, we present that the advantage of postselection in weak value amplification (WVA) can not be achieved without quantum coherence. The quantum coherence of the initial system is closely related to the preparation costs and measurement costs in parameter estimation. With the increase of initial quantum coherence, the joint values of preparation costs and measurement costs can be optimized to smaller. Moreover, we derive an analytical tradeoff relation between the preparation, measurement and the quantum coherence. We further experimentally test the tradeoff relation in a linear optical setup. The experimental and theoretical results are in good agreement and show that the quantum coherence plays a key role in bounding the resource costs in the postselected metrology process.

quant-ph↗

arXiv2022

Towards Multi-class Pre-movement Classification

In non-invasive brain-computer interface systems, pre-movement decoding plays an important role in the detection of movement before limbs actually move. Movement-related cortical potential is a kind of brain activity associated with pre-movement decoding. In current studies, patterns decoded from movement are mainly applied to the binary classification between movement state and resting state, such as elbow flexion and rest. The classifications between two movement states and among multiple movement states are still challenging. This study proposes a new method, the star-arrangement spectral filtering (SASF), to solve the multi-class pre-movement classification problem. We first design a referenced task-related component analysis (RTRCA) framework that consists of two modules. This first module is the classification between movement state and resting state; the second module is the classification of multiple movement states. SASF is developed by optimizing the features in RTRCA. In SASF, feature selection on filter banks is used on the first module of RTRCA, and feature selection on time windows is used on the second module of RTRCA. A linear discriminant analysis classifier is used to classify the optimized features. In the binary classification between two motions, the classification accuracy of SASF achieves 0.9670$\pm$0.0522, which is significantly higher than the result provided by the deep convolutional neural network (0.6247$\pm$0.0680) and the discriminative spatial pattern method (0.4400$\pm$0.0700). In the multi-class classification of 7 states, the classification accuracy of SASF is 0.9491$\pm$0.0372. The proposed SASF greatly improves the classification between two motions and enables the classification among multiple motions. The result shows that the movement can be decoded from EEG signals before the actual limb movement.

cs.HC↗

arXiv2022

Flat-band-induced many-body interactions and exciton complexes in a layered semiconductor

Interactions among a collection of particles generate many-body effects in solids resulting in striking modifications of material properties. The heavy carrier mass that yields strong interactions and gate control of carrier density over a wide range, make two-dimensional semiconductors an exciting playground to explore many-body physics. The family of III-VI metal monochalcogenides emerges as a new platform for this purpose due to its excellent optical properties and the flat valence band dispersion with a Mexican-hat-like inversion. In this work, we present a complete study of charge-tunable excitons in few-layer InSe by photoluminescence spectroscopy. From the optical spectra, we establish that free excitons in InSe are more likely to be captured by ionized donors due to the large exciton Bohr radius, leading to the formation of bound exciton complexes. Surprisingly, a pronounced redshift of the exciton energy accompanied by a decrease of the exciton binding energy upon hole-doping reveals a significant band gap renormalization and dynamical screening induced by the presence of the Fermi reservoir. Our findings establish InSe as a reproducible and potentially manufacturable platform to explore electron correlation phenomena without the need for twist-angle engineering.

cond-mat.mes-hall↗

arXiv2022

Interfacial Charge-transfer Excitonic Insulator in a Two-dimensional Organic-inorganic Superlattice

Excitonic insulators are long-sought-after quantum materials predicted to spontaneously open a gap by the Bose condensation of bound electron-hole pairs, namely, excitons, in their ground state. Since the theoretical conjecture, extensive efforts have been devoted to pursuing excitonic insulator platforms for exploring macroscopic quantum phenomena in real materials. Reliable evidences of excitonic character have been obtained in layered chalcogenides as promising candidates. However, owing to the interference of intrinsic lattice instabilities, it is still debatable whether those features, such as charge density wave and gap opening, are primarily driven by the excitonic effect or by the lattice transition. Herein, we develop a novel charge-transfer excitonic insulator in organic-inorganic superlattice interfaces, which serves as an ideal platform to decouple the excitonic effect from the lattice effect. In this system, we observe the narrow gap opening and the formation of a charge density wave without periodic lattice distortion, providing visualized evidence of exciton condensation occurring in thermal equilibrium. Our findings identify spontaneous interfacial charge transfer as a new strategy for developing novel excitonic insulators and investigating their correlated many-body physics.

cond-mat.mtrl-sci↗

arXiv2022

Implementing quantum walks with a single qubit

Quantum walks have wide applications in quantum information, such as universal quantum computation, so it is important to explore properties of quantum walks thoroughly. We propose a novel method to implement discrete-time quantum walks (DTQWs) using only a single qubit, in which both coin and walker are encoded in the two-dimensional state space of a single qubit, operations are realized using single-qubit gates only, and high-dimensional final states of DTQWs can be obtained naturally. With this "one-qubit" approach, DTQW experiments can be realized much more easily, compared with previous methods, in most quantum systems and all properties based on quantum states of DTQWs (such as quantum correlation and coherence) can be investigated. By this approach, we experimentally implement one-particle and two-particle DTQWs with seven steps using single photons. Furthermore, we systematically investigate quantum correlations and coherence (based on the full state of the coin and walker) of the DTQW systems with different initial states of the coin, which have not been obtained and studied in DTQW experiments. As an application, we also study the assisted distillation of quantum coherence using the full state of the two-particle DTQW from the experiment. The maximal increase in distillable coherence for high-dimensional mixed states is investigated for the first time by obtaining its upper and lower bounds. Our work opens a new door to implement DTQW experiments and to better explore properties of quantum walks.

quant-ph↗

arXiv2022

A new class of bilayer kagome lattice compounds with Dirac nodal lines and pressure-induced superconductivity

Kagome lattice composed of transition-metal ions provides a great opportunity to explore the intertwining between geometry, electronic orders and band topology. The discovery of multiple competing orders that connect intimately with the underlying topological band structure in nonmagnetic kagome metals $A$V$_3$Sb$_5$ ($A$ = K, Rb, Cs) further pushes this topic to the quantum frontier. Here we report the discovery and characterization of a new class of vanadium-based compounds with kagome bilayers, namely $A$V$_6$Sb$_6$ ($A$ = K, Rb, Cs) and V$_6$Sb$_4$, which, together with $A$V$_3$Sb$_5$, compose a series of kagome compounds with a generic chemical formula ($A_{m-1}$Sb$_{2m}$)(V$_3$Sb)$_n$ (m = 1, 2; n = 1, 2). Theoretical calculations combined with angle-resolved photoemission measurements reveal that these compounds feature Dirac nodal lines in close vicinity to the Fermi level. Pressure-induced superconductivity in $A$V$_6$Sb$_6$ further suggests promising emergent phenomena in these materials. The establishment of a new family of layered kagome materials paves the way for designer of fascinating kagome systems with diverse topological nontrivialities and collective ground states.

cond-mat.mtrl-sci↗

arXiv2022

Angle-resolved photoemission spectroscopy study of the charge density wave order in layered semiconductor EuTe4

Layered tellurides have been extensively studied as a platform for investigating the Fermi surface (FS) nesting-driven charge density wave (CDW) states. EuTe4, one of quasi-two-dimensional (quasi-2D) binary rare-earth tetratellurides CDW compounds, with unconventional hysteretic transition, is currently receiving much attention. Here, the CDW modulation vector, momentum and temperature dependence of CDW gaps in EuTe4 are investigated using angle-resolved photoemission spectroscopy. Our results reveal that (i) a FS nesting vector q ~ 0.67 b* drives the formation of CDW state, (ii) a large anisotropic CDW gap is fully open in the whole FS, and maintains a considerable size even at 300 K, leading to appearance of semiconductor properties, (iii) an abnormal non-monotonic increase of CDW gap in magnitude as a function of temperature, (iv) an extra, larger gap opens at a higher binding energy due to the interaction between the different orbits of the main bands.

cond-mat.mtrl-sci↗