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Zhengtai Liu

Publications and source records attributed to Zhengtai Liu.

63 records · Page 4Linked to original sources

Tunable intrinsic ferromagnetic topological phases in bulk van der Waals crystal MnSb6Te10

Intrinsic ferromagnetism is a crucial ingredient to realize quantum anomalous Hall effect in quasi two dimensional materials, thus the search of intrinsic ferromagnetic topological materials is one of the most concerned issues in the field of topological phases of matter. In this work, combining magnetotransport measurements, first principles calculations, and angle-resolved photoemission spectroscopy studies, we find that in MnSb6Te10, the n = 2 member of the MnSb2Te4/(Sb2Te3)n family, the strong magnetic competition realizes a fragile ferromagnetic ground state, which whereas easily enters into ferrimagnetic and the Z_2 antiferromagnetic topological insulator phase with warming to higher temperature. Interestingly, the system stays in an inversion-symmetry-protected axion insulator phase in the ferromagnetic ground state as well as in the external magnetic field driven spin-polarized FM phase and can be converted into a Weyl semimetal with multiple Weyl nodes in the valence bands with hole doping, which are manifested by the measured notable intrinsic anomalous Hall effect. Our work thus provides an intrinsic magnetic topological material which is highly tunable into versatile topological phases by temperature, magnetic field, as well as carrier doping.

cond-mat.mtrl-sci↗

Dirac Nodal Lines and Nodal Loops in a Topological Kagome Superconductor CsV$_3$Sb$_5$

The intertwining of charge order, superconductivity and band topology has promoted the AV$_3$Sb$_5$ (A=K, Rb, Cs) family of materials to the center of attention in condensed matter physics. Underlying those mysterious macroscopic properties such as giant anomalous Hall conductivity (AHC) and chiral charge density wave is their nontrivial band topology. While there have been numerous experimental and theoretical works investigating the nontrivial band structure and especially the van Hove singularities, the exact topological phase of this family remains to be clarified. In this work, we identify CsV$_3$Sb$_5$ as a Dirac nodal line semimetal based on the observation of multiple Dirac nodal lines and loops close to the Fermi level. Combining photoemission spectroscopy and density functional theory, we identify two groups of Dirac nodal lines along $k_z$ direction and one group of Dirac nodal loops in the A-H-L plane. These nodal loops are located at the Fermi level within the instrumental resolution limit. Importantly, our first-principle analyses indicate that these nodal loops may be a crucial source of the mysterious giant AHC observed. Our results not only provide a clear picture to categorize the band structure topology of this family of materials, but also suggest the dominant role of topological nodal loops in shaping their transport behavior.

cond-mat.str-el↗

Emergence of Quantum Confinement in Topological Kagome Superconductor CsV$_3$Sb$_5$ family

Quantum confinement is a restriction on the motion of electrons in a material to specific region, resulting in discrete energy levels rather than continuous energy bands. In certain materials quantum confinement could dramatically reshape the electronic structure and properties of the surface with respect to the bulk. Here, in the recently discovered kagome superconductor CsV$_3$Sb$_5$ (A=K, Rb, Cs) family of materials, we unveil the dominant role of quantum confinement in determining their surface electronic structure. Combining angle-resolved photoemission spectroscopy (ARPES) measurement and density-functional theory simulation, we report the observations of two-dimensional quantum well states due to the confinement of bulk electron pocket and Dirac cone to the nearly isolated surface layer. The theoretical calculations on the slab model also suggest that the ARPES observed spectra are almost entirely contributed by the top two layers. Our results not only explain the disagreement of band structures between the recent experiments and calculations, but also suggest an equally important role played by quantum confinement, together with strong correlation and band topology, in shaping the electronic properties of this family of materials.

cond-mat.str-el↗

Charge-density-wave-induced bands renormalization and energy gaps in a kagome superconductor RbV3Sb5

Recently discovered Z2 topological kagome metals AV3Sb5 (A = K, Rb, and Cs) exhibit charge density wave (CDW) phases and novel superconducting paring states, providing a versatile platform for studying the interplay between electron correlation and quantum orders. Here we directly visualize CDW-induced bands renormalization and energy gaps in RbV3Sb5 using angle-resolved photoemission spectroscopy, pointing to the key role of tuning van Hove singularities to the Fermi energy in mechanisms of ordering phases. Near the CDW transition temperature, the bands around the Brillouin zone (BZ) boundary are shifted to high-binding energy, forming an "M"-shape band with singularities near the Fermi energy. The Fermi surfaces are partially gapped and the electronic states on the residual ones should be possibly dedicated to the superconductivity. Our findings are significant in understanding CDW formation and its associated superconductivity.

cond-mat.supr-con↗

Emergence of new van Hove singularities in the charge density wave state of a topological kagome metal RbV3Sb5

Quantum materials with layered kagome structures have drawn considerable attention due to their unique lattice geometry, which gives rise to flat bands co-existing with Dirac-like dispersions. The interplay between strong Coulomb correlations and nontrivial band topology in these systems results in various exotic phenomena. Recently, vanadium-based materials with layered kagome structures are discovered to be topological metals, which exhibit charge density wave (CDW) properties, significant anomalous Hall effect, and unusual superconductivity at low temperatures. Here we exploit high-resolution angle-resolved photoemission spectroscopy to investigate the electronic structure evolution induced by the CDW transition in a vanadium-based kagome material RbV3Sb5. A remarkable band renormalization in the CDW state is observed, which is consistent with first principles calculations based on an inverse star-of-David superstructure. The CDW phase transition gives rise to a partial energy gap opening at the Fermi level, a shift in the band dispersion, and most importantly, the emergence of new van Hove singularities associated with large density of states, which are absent in the normal phase and may be related to superconductivity observed at lower temperatures. Our work would shed light on the microscopic mechanisms for the formation of the CDW and superconducting states in these topological kagome metals.

cond-mat.supr-con↗

Multiple Symmetry-Protected Dirac Nodal Lines in A Quasi-One-Dimensional Semimetal

Nodal-line semimetals (NLSMs) contains Dirac/Weyl type band-crossing nodes extending into shapes of line, loop and chain in the reciprocal space, leading to novel band topology and transport responses. Robust NLSMs against spin-orbit coupling typically occur in three-dimensional materials with more symmetry operations to protect the line nodes of band crossing, while the possibilities in lower-dimensional materials are rarely discussed. Here we demonstrate robust NLSM phase in a quasi-one-dimensional nonmagnetic semimetal TaNiTe5. Combining angle-resolved photoemission spectroscopy measurements and first-principles calculations, we reveal how reduced dimension can interact with nonsymmorphic symmetry and result into multiple Dirac-type nodal lines with four-fold degeneracy. Our findings suggest rich physics and application in (quasi-)one-dimensional topological materials and call for further investigation on the interplay between the quantum confinement and nontrivial band topology.

cond-mat.other↗

Electron-plasmon interaction induced plasmonic-polaron band replication in epitaxial perovskite SrIrO$_3$ films

Electron-boson interaction is fundamental to a thorough understanding of various exotic properties emerging in many-body physics. In photoemission spectroscopy, photoelectron emission due to photon absorption would trigger diverse collective excitations in solids, including the emergence of phonons, magnons, electron-hole pairs, and plasmons, which naturally provides a reliable pathway to study electron-boson couplings. While fingerprints of electron-phonon/-magnon interactions in this state-of-the-art technique have been well investigated, much less is known about electron-plasmon coupling, and direct observation of the band renormalization solely due to electron-plasmon interactions is extremely challenging. Here by utilizing integrated oxide molecular-beam epitaxy and angle-resolved photoemission spectroscopy, we discover the long sought-after pure electron-plasmon coupling-induced low-lying plasmonic-polaron replica bands in epitaxial semimetallic SrIrO$_3$ films, in which the characteristic low carrier concentration and narrow bandwidth combine to provide a unique platform where the electron-plasmon interaction can be investigated kinematically in photoemission spectroscopy. This finding enriches the forms of electron band normalization on collective modes in solids and demonstrates that, to obtain a complete understanding of the quasiparticle dynamics in 5d electron systems, the electron-plasmon interaction should be considered on equal footing with the acknowledged electron-electron interaction and spin-orbit coupling.

cond-mat.str-el↗

Multiple magnetic topological phases in bulk van der Waals crystal MnSb4Te7

The magnetic van der Waals crystals MnBi2Te4/(Bi2Te3)n have drawn significant attention due to their rich topological properties and the tunability by external magnetic field. Although the MnBi2Te4/(Bi2Te3)n family have been intensively studied in the past few years, their close relatives, the MnSb2Te4/(Sb2Te3)n family, remain much less explored. In this work, combining magnetotransport measurements, angle-resolved photoemission spectroscopy, and first principles calculations, we find that MnSb4Te7, the n = 1 member of the MnSb2Te4/(Sb2Te3)n family, is a magnetic topological system with versatile topological phases which can be manipulated by both carrier doping and magnetic field. Our calculations unveil that its A-type antiferromagnetic (AFM) ground state stays in a Z_2 AFM topological insulator phase, which can be converted to an inversion-symmetry-protected axion insulator phase when in the ferromagnetic (FM) state. Moreover, when this system in the FM phase is slightly carrier doped on either the electron or hole side, it becomes a Weyl semimetal with multiple Weyl nodes in the highest valence bands and lowest conduction bands, which are manifested by the measured notable anomalous Hall effect. Our work thus introduces a new magnetic topological material with different topological phases which are highly tunable by carrier doping or magnetic field.

cond-mat.str-el↗

Evidence of topological nodal lines and surface states in the centrosymmetric superconductor SnTaS2

The discovery of signatures of topological superconductivity in superconducting bulk materials with topological surface states has attracted intensive research interests recently. Utilizing angle-resolved photoemission spectroscopy and first-principles calculations, here, we demonstrate the existence of topological nodal-line states and drumheadlike surface states in centrosymmetric superconductor SnTaS2, which is a type-II superconductor with a critical transition temperature of about 3 K. The valence bands from Ta 5d orbitals and the conduction bands from Sn 5p orbitals cross each other, forming two nodal lines in the vicinity of the Fermi energy without the inclusion of spin-orbit coupling (SOC), protected by the spatial-inversion symmetry and time-reversal symmetry. The nodal lines are gapped out by SOC. The drumheadlike surface states, the typical characteristics in nodal-line semimetals, are quite visible near the Fermi level. Our findings indicate that SnTaS2 offers a promising platform for exploring the exotic properties of the topological nodal-line fermions and gives a help to study topological superconductivity.

cond-mat.supr-con↗