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Zhouyang Ge

Publications and source records attributed to Zhouyang Ge.

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Dissipation and microstructure in sheared active suspensions of squirmers

We study the energy expenditure and structural correlations in semi-dilute to concentrated suspensions of squirmers using active fast Stokesian dynamics simulations. Specifically, we simulate apolar active suspensions of squirmers, or 'shakers,' and show that shear enhances the total dissipation but reduces the relative viscosity for both puller- and pusher-type shakers. At low shear rates where activity dominates, pushers dissipate more energy than pullers, and more so at higher volume fractions, in contrast to bacterial suspensions displaying a 'superfluid' transition. At high shear rates where shear dominates, pullers and pushers behave effectively as passive spheres, generating negative normal stress differences due to shear-induced collision. Remarkably, the rate-dependent rheological responses are accompanied by unusual microstructural signatures of an enhanced nematic order and anisotropic pair correlation, both of which contribute to a higher viscosity under shear. Further simulations of self-propelled, neutral squirmers exhibit similar but weaker shear-thinning, highlighting the importance of activity over motility, underpinned by hydrodynamic interactions. Overall, our results elucidate the interplay of internal activity and external flow on the dissipation and microstructure in sheared active suspensions of squirmers.

cond-mat.soft

Nonmonotonic diffusion in sheared active suspensions of squirmers

We investigate how shear influences the dynamics of active particles in dilute to concentrated suspensions. Using apolar active suspensions of squirmers as model systems, we show how their long-time diffusive dynamics can surprisingly slow down and vary nonmonotonically with the shear rate arising from an interplay between the activity-induced persistent motion and shear-induced reorientation and diffusion. Further simulations of self-propelled particles with tunable persistence exhibit richer dynamics and confirm the observed coupling, suggesting that nonmonotonic diffusion may be a general feature of fluids endowed with an underlying microstructure and large persistence. Our results reveal a nonlinear effect of shear on diffusion in active suspensions, elucidate how internal and external forcing interact, and provide new possibilities to modulate transport in active fluids.

cond-mat.soft

Dense Suspensions in Rotary Shear

We introduce a novel unsteady shear protocol, which we name Rotary Shear (RS), where the flow and vorticity directions are continuously rotated around the velocity gradient direction by imposing two out-of-phase oscillatory shear (OS) in orthogonal directions. We perform numerical simulations of dense suspensions of rigid non-Brownian spherical particles at volume fractions ($\phi$) between 0.40 and 0.55 subject to this new RS protocol and compare to the classical OS protocol. We find that the suspension viscosity displays a similar non-monotonic response as the strain amplitude ($\gamma_0$) is increased: a minimum viscosity is found at an intermediate, volume-fraction dependent strain amplitude. However, the suspension dynamics is different in the new protocol. Unlike the OS protocol, suspensions under RS do not show self-adsorbing states at any $\gamma_0$ and do not undergo the reversible-irreversible transition: the stroboscropic particle dynamics are always diffusive, which we attribute to the fact that the RS protocol is irreversible. To validate this hypothesis, we introduce a reversible-RS (RRS) protocol, a combination of RS and OS, where we rotate the shear direction (as in RS) until it is instantaneously reversed (as in OS), and find the resulting rheology and dynamics to be closer to OS. Detailed microstructure analysis shows that both the OS and RRS protocols result in a contact-free, isotropic to an in-contact, anisotropic microstructure at the dynamically reversible-to-irreversible transition. The RS protocol does not render such a transition, and the dynamics remain diffusive with an in-contact, anisotropic microstructure for all strain amplitudes.

cond-mat.soft

Hydrodynamic diffusion in apolar active suspensions

Active suspensions encompass a wide range of complex fluids containing microscale energy-injecting particles, such as cells, bacteria or artificially powered active colloids. Because they are intrinsically non-equilibrium, active suspensions can display a number of fascinating phenomena, including turbulent-like large-scale coherent motion and enhanced diffusion. Here, using a recently developed active Fast Stokesian Dynamics method, we present a detailed numerical study on the hydrodynamic diffusion in apolar active suspensions. Specifically, we simulate suspensions of active but non-self-propelling spherical squirmers, of either puller- or pusher-type, at volume fractions from 0.5% to 55%. Our results show little difference between pullers and pushers in their instantaneous and long-time dynamics, where the translational dynamics vary non-monotonically with the volume fraction, with a peak diffusivity at around 10% to 20%, in stark contrast to suspensions of self-propelling particles. On the other hand, the rotational dynamics tend to increase with the volume fraction as is the case for self-propelling particles. To explain these dynamics, we provide detailed scaling and statistical analyses based on the activity-induced hydrodynamic interactions and the observed microstructural correlations, which display a weak local order. Overall, these results elucidate and highlight the different effects of particle activity on the collective dynamics and transport phenomena in active fluids.

cond-mat.soft

Rheology of periodically sheared suspensions undergoing reversible-irreversible transition

The rheology of non-colloidal suspensions under cyclic shear is studied numerically. The main findings are a strain amplitude ($\gamma_0$) dependent response in the shear stress and second normal stress difference ($N_2$). Specifically, we find a reduced viscosity, an enhanced intracycle shear thinning, the onset of a finite $N_2$ and its frequency doubling, all near a critical strain amplitude $\gamma_c$ that scales with the volume fraction $\phi$ as $\gamma_c \sim \phi^{-2}$. These rheological changes also signify a reversible-irreversible transition (RIT), dividing stroboscopic particle dynamics into a reversible absorbing phase (for $\gamma_0<\gamma_c$) and a persistently diffusing phase (for $\gamma_0>\gamma_c$). We explain the results based on two flow-induced mechanisms and elucidate their connection in the context of RIT through the underlying microstructure, which tends towards hyperuniformity near $\gamma_0=\gamma_c$. Overall, we expect this correspondence between rheology and emergent dynamics to hold in a wide range of settings where structural organizations are dominated by volume exclusions.

cond-mat.soft

Irreversibility and rate dependence in sheared adhesive suspensions

Recent experiments report that slowly-sheared noncolloidal particle suspensions can exhibit unexpected rate($\omega$)-dependent complex viscosities in oscillatory shear, despite a constant relative viscosity in steady shear. Using a minimal hydrodynamic model, we show that a weak interparticle attraction reproduces this behavior. At volume fractions $\phi=20\sim50$%, the complex viscosities in both experiments and simulations display power-law reductions in shear, with a $\phi$-dependent exponent maximum at $\phi=40$%, resulting from the interplay between hydrodynamic, collision and adhesive interactions. Furthermore, this rate dependence is accompanied by diverging particle diffusivities and pronounced cluster formations even at small oscillation amplitudes $\gamma_0$. Previous studies established that suspensions transition from reversible absorbing states to irreversible diffusing states when $\gamma_0$ exceeds a $\phi$-dependent critical value $\gamma_{0,\phi}^c$. Here, we show that a second transition to irreversibility occurs below an $\omega$-dependent critical amplitude, $\gamma_{0,\omega}^c \leq \gamma_{0,\phi}^c$, in the presence of weak attractions.

cond-mat.soft

Weakly adhesive suspension shows rate-dependence in oscillatory but not steady shear flows

We report rheological measurements of a noncolloidal particle suspension in a Newtonian solvent at 40% solid volume fraction. An anomalous, frequency-dependent complex viscosity is found under oscillatory shear (OS) flow, whereas a constant dynamic viscosity is found under the same shear rates in steady shear (SS) flow. We show that this contradiction arises from the underlying microstructural difference between OS and SS, mediated by weak interparticle forces. Discrete element simulations of proxy particle suspensions confirm this hypothesis and reveal an adhesion-induced, shear thinning mechanism with a -1/5 slope, only in OS, in agreement with experiments.

cond-mat.soft

Implementation note on a minimal hybrid lubrication/granular dynamics model for dense suspensions

We describe and summarize a class of minimal numerical models emerged from recent development of simulation methods for dense particle suspensions in overdamped linear flows. The main ingredients include (i) a frame-invariant, short-range lubrication model for spherical particles, and (ii) a soft-core, stick/slide frictional contact model activated when particles overlap. We implement a version of the model using a modified velocity-Verlet algorithm that explicitly solves the $N$-body dynamical system in $\mathcal{O}(cN)$ operations, where $c$ is a kernel constant depending on the cutoff of particle interactions. The implementation is validated against literature results on jamming transition and shear thickening suspensions from 40% to 64% volume fractions. Potential strategies to extend the present methodology to non-spherical particles are also suggested for very concentrated suspensions.

cond-mat.soft

The effect of a wall on the interaction of two spheres in shear flow: Batchelor-Green theory revisited

The seminal Batchelor-Green's (BG) theory on the hydrodynamic interaction of two spherical particles of radii a suspended in a viscous shear flow neglects the effect of the boundaries. In the present paper we study how a plane wall modifies this interaction. Using an integral equation for the surface traction we derive the expression for the particles' relative velocity as a sum of the BG's velocity and the term due to the presence of a wall at finite distance, z_0. Our calculation is not the perturbation theory of the BG solution, so the contribution due to the wall is not necessarily small. The distance at which the wall significantly alters the particles interaction scales as z_0^{3/5}. The phase portrait of the particles' relative motion is different from the BG theory, where there are two singly-connected regions of open and closed trajectories both of infinite volume. For finite z_0, there is a new domain of closed (dancing) and open (swapping) trajectories. The width of this region behaves as 1/z_0. Along the swapping trajectories, that have been previously observed numerically, the incoming particle is turning back after the encounter with the reference particle, rather than passing it by, as in the BG theory. The region of dancing trajectories has infinite volume. We found a one-parameter family of equilibrium states, overlooked previously, whereas the pair of spheres flows as a whole without changing its configuration. These states are marginally stable and their perturbation yields a two-parameter family of the dancing trajectories, where the particle is orbiting around a fixed point in a frame co-moving with the reference particle. We suggest that the phase portrait obtained at z_0>>a is topologically stable and can be extended down to rather small z_0 of several particle diameters. We confirm this by direct numerical simulations of the Navier-Stokes equations with z_0=5a.

physics.flu-dyn

Droplets in homogeneous shear turbulence

We simulate the flow of two immiscible and incompressible fluids separated by an interface in a homogeneous turbulent shear flow at a shear Reynolds number equal to 15200. The viscosity and density of the two fluids are equal, and various surface tensions and initial droplet diameters are considered in the present study. We show that the two-phase flow reaches a statistically stationary turbulent state sustained by a non-zero mean turbulent production rate due to the presence of the mean shear. Compared to single-phase flow, we find that the resulting steady state conditions exhibit reduced Taylor microscale Reynolds numbers owing to the presence of the dispersed phase, which acts as a sink of turbulent kinetic energy for the carrier fluid. At steady state, the mean power of surface tension is zero and the turbulent production rate is in balance with the turbulent dissipation rate, with their values being larger than in the reference single-phase case. The interface modifies the energy spectrum by introducing energy at small-scales, with the difference from the single-phase case reducing as the Weber number increases. This is caused by both the number of droplets in the domain and the total surface area increasing monotonically with the Weber number. This reflects also in the droplets size distribution which changes with the Weber number, with the peak of the distribution moving to smaller sizes as the Weber number increases. We show that the Hinze estimate for the maximum droplet size, obtained considering breakup in homogeneous isotropic turbulence, provides an excellent estimate notwithstanding the action of significant coalescence and the presence of a mean shear.

physics.flu-dyn

Effective slip over partially filled microcavities and its possible failure

Motivated by the emerging applications of liquid-infused surfaces (LIS), we study the drag reduction and robustness of transverse flows over two-dimensional microcavities partially filled with an oily lubricant. Using separate simulations at different scales, characteristic contact line velocities at the fluid-solid intersection are first extracted from nano-scale phase field simulations and then applied to micron-scale two-phase flows, thus introducing a multiscale numerical framework to model the interface displacement and deformation within the cavities. As we explore the various effects of the lubricant-to-outer-fluid viscosity ratio $\tilde{\mu}_2/\tilde{\mu}_1$, the capillary number Ca, the static contact angle $\theta_s$, and the filling fraction of the cavity $\delta$, we find that the effective slip is most sensitive to the parameter $\delta$. The effects of $\tilde{\mu}_2/\tilde{\mu}_1$ and $\theta_s$ are generally intertwined, but weakened if $\delta < 1$. Moreover, for an initial filling fraction $\delta =0.94$, our results show that the effective slip is nearly independent of the capillary number, when it is small. Further increasing Ca to about $0.01 \tilde{\mu}_1/\tilde{\mu}_2$, we identify a possible failure mode, associated with lubricants draining from the LIS, for $\tilde{\mu}_2/\tilde{\mu}_1 \lesssim 0.1$. Very viscous lubricants (\eg $\tilde{\mu}_2/\tilde{\mu}_1 >1$), on the other hand, are immune to such failure due to their generally larger contact line velocity.

physics.flu-dyn

Integral representation of channel flow with interacting particles

We construct a boundary integral representation for the low-Reynolds-number flow in a channel in the presence of freely-suspended particles (or droplets) of arbitrary size and shape. We demonstrate that lubrication theory holds away from the particles at horizontal distances exceeding the channel height and derive a multipole expansion of the flow which is dipolar to the leading approximation. We show that the dipole moment of an arbitrary particle is a weighted integral of the stress and the flow at the particle surface, which can be determined numerically. We introduce the equation of motion that describes hydrodynamic interactions between arbitrary, possibly different, distant particles, with interactions determined by the product of the mobility matrix and the dipole moment. Further, the problem of three identical interacting spheres initially aligned in the streamwise direction is considered and the experimentally observed "pair exchange" phenomenon is derived analytically and confirmed numerically. For non-aligned particles, we demonstrate the formation of a configuration with one particle separating from a stable pair. Our results suggest that in a dilute initially homogeneous particulate suspension flowing in a channel the particles will eventually separate into singlets and pairs.

physics.flu-dyn

An efficient mass-preserving interface-correction level set/ghost fluid method for droplet suspensions under depletion forces

Aiming for the simulation of colloidal droplets in microfluidic devices, we present here a numerical method for two-fluid systems subject to surface tension and depletion forces among the suspended droplets. The algorithm is based on an efficient solver for the incompressible two-phase Navier-Stokes equations, and uses a mass-conserving level set method to capture the fluid interface. The four novel ingredients proposed here are, firstly, an interface-correction level set (ICLS) method; global mass conservation is achieved by performing an additional advection near the interface, with a correction velocity obtained by locally solving an algebraic equation, which is easy to implement in both 2D and 3D. Secondly, we report a second-order accurate geometric estimation of the curvature at the interface and, thirdly, the combination of the ghost fluid method with the fast pressure-correction approach enabling an accurate and fast computation even for large density contrasts. Finally, we derive a hydrodynamic model for the interaction forces induced by depletion of surfactant micelles and combine it with a multiple level set approach to study short-range interactions among droplets in the presence of attracting forces.

physics.flu-dyn