arXiv subjects

Zs. Fülöp

Publications and source records attributed to Zs. Fülöp.

At least 19 recordsLinked to original sources

arXiv2026

Detector characterization for a new $^{12}$C+$^{12}$C reaction study at LUNA

The $^{12}$C+$^{12}$C fusion reaction plays a crucial role in stellar evolution, including the occurrence of supernova explosions, and in the synthesis of the chemical elements. However, our understanding of its cross section remains severely deficient, particularly below $E_\textrm{cm}=2.5$\,MeV, the energy range of interest for astrophysics. To address these unresolved issues, the LUNA collaboration will conduct a dedicated study of the $^{12}$C+$^{12}$C reaction at the Bellotti Ion Beam Facility (Bellotti IBF) located deep underground within the Gran Sasso National Laboratory (LNGS) in Italy. Based on the combination of passive and active shields, this campaign aims to achieve unprecedented sensitivity in measuring the cross sections of the two key reaction channels, $^{12}$C($^{12}$C,$α$)$^{20}$Ne and $^{12}$C($^{12}$C,$p$)$^{23}$Na in the low-energy regime via $γ$-ray detection. Here, we report on a sensitivity study for the upcoming campaign with a focus on the characterization of two detectors, namely a HPGe detector and a NaI(Tl) array. Furthermore, their intrinsic contamination is thoroughly investigated since this could potentially influence the overall sensitivity. Assuming typical beam intensities of the Bellotti IBF, we will be able to investigate reaction rates significantly below 100 counts per day. In case of the $^{12}$C+$^{12}$C reaction we therefore expect to acquire experimental data well below the current limit of $E_\textrm{cm}=2.1\,$MeV. The results are supported by simulations to highlight the advantageous low-background environment, essential for high-precision nuclear astrophysics studies.

physics.ins-det↗

arXiv2025

Gas-cell development for nuclear astrophysics motivated studies on noble gas targets and the $^3$He($α$,$γ$)$^7$Be reaction

In many astrophysical scenarios, alpha induced reactions on noble gas nuclei play a crucial role. Studying these reactions in the laboratory requires the noble gas atoms to be confined in a sufficient amount to allow the reactions. At Atomki thin-windowed gas-cell targets were developed and improved for studying alpha induced reactions on noble gases. Several stages of the gas-cell design used for activation experiments and lately a version to be used for particle scattering experiments will be presented. A new experimental study of the $^3$He($α$,$γ$)$^7$Be reaction with one of the activation gas-cell targets was performed. This reaction plays an important role both in the solar pp-chains and in big bang nucleosynthesis. The reaction cross section was measured in the past in several works, however, there are still energy regions lacking experimental data, rendering the extrapolations towards the astrophysically relevant energies uncertain. New experimental total cross section of the $^3$He($α$,$γ$)$^7$Be reaction was thus determined here in the energy range of $E_\mathrm{c.m.} = 2600-3000$ keV in about 50 keV energy steps. These results confirm the overall trend, and also the absolute scale set by the only one previous measurement in this energy range. In addition, two pilot experiments with the scattering cell were performed aiming to study the $^4$He($α$,$α$)$^4$He and $^{124}$Xe($α$,$α$)$^{124}$Xe reactions at $E_α= 18$ MeV. These studies benchmark the performance of the cell and detection system both for light and heavy noble gas targets.

physics.ins-det↗

arXiv2025

Towards a comprehensive study of the 14N(p,g)15O astrophysical key reaction: Description of the experimental technique including novel target preparation

While the 14N(p,g)15O reaction plays a key role in the hydrogen-burning processes in various stellar conditions, its reaction rate is not known with sufficient precision. Therefore, the first scientific project at the recently launched Bellotti Ion Beam Facility of the Laboratori Nazionali del Gran Sasso was the measurement of the 14N(p,g)15O reaction cross section in the proton energy range between 250 and 1500 keV. In this paper, the experimental techniques are summarized with special emphasis on the description of solid state nitrogen target production and characterization. The first results of the reaction yield measured at 55 deg detection angle are also presented.

physics.ins-det↗

arXiv2025

A Comparative Analysis of R-Matrix Fitting: ${}^{12}$C$(p,γ)$${}^{13}$N as Test Case

In nuclear astrophysics, the accurate determination of nuclear reaction cross sections at astrophysical energies is critical for understanding stellar evolution and nucleosynthesis. This study focuses on the $^{12}$C($p, γ$)$^{13}$N reaction, which takes part in the CNO cycle and is significant for determining the $^{12}$C/$^{13}$C ratio in stellar interiors. Data from various studies, including recent LUNA measurements, reveal high discrepancies in cross section values, underscoring the need for robust fitting approaches. Utilizing the R-matrix theory, we compare different frequentist and Bayesian methodologies for estimating reaction cross sections and their uncertainties. The analysis evaluates the strengths and weaknesses of different statistical techniques, highlighting the importance of systematic uncertainty treatment and the estimate of covariance matrix estimation to enhance the reliability and reproducibility of uncertainty estimates in nuclear astrophysics.

nucl-ex↗

arXiv2025

Continuous high-yield fast neutron generation with few-cycle laser pulses at 10 Hz for applications

We present a laser-based neutron source that produces $1.8 \times 10^5$ neutrons/s with a conversion rate of $7.8 \times 10^5$ neutrons/J. Laser pulses of 12 fs and 23 mJ were focused onto a 430-nm-thick heavy water liquid sheet at a 10 Hz repetition rate. The resulting peak intensity of $4 \times 10^{18}$ W/cm$^2$ accelerated deuterium ions from the target rear side to a kinetic energy of 1 MeV. This deuteron beam induced $^{2}$H(d,n)$^{3}$He fusion reactions in a deuterated polyethylene target, producing fast neutrons. The neutron yield was measured using two independent detection systems: the LILITH time-of-flight spectrometer, consisting of eight plastic scintillators covering nearly $180^\circ$, and a calibrated bubble detector spectrometer. The neutron yield per laser shot is 35 times higher than that recently achieved by lasers with comparable pulse energies, while the conversion rate is the highest ever achieved by continuously operating, sub-100 fs lasers. The generated neutrons are emitted from an area of 0.65 cm$^2$ corresponding to the deuteron beam spot on the catcher. Their angular distribution is peaked in forward and backward directions in agreement with the literature data on the angular distribution of $^{2}$H(d,n)$^{3}$He reaction. The system operated continuously for several hours per day with an unprecedented stability of 5%.

physics.plasm-ph↗

arXiv2024

Measurement of the E_p = 416.9 keV resonance strength in the 29Si(p,gamma)30P reaction

Silicon isotopic ratios measured in meteoritic presolar grains can provide useful information about the nucleosynthesis origin of these isotopes if the rates of nuclear reactions responsible for their production are known. One of the key reactions determining the Si isotopic abundances is 29Si(p,gamma)30P. Its reaction rate is not known with sufficient precision due in part to some ambiguous resonance strength values. In the present work, the strength of the E_p = 416.9 keV resonance has been measured with high precision using the activation technique. The new strength of omega_gamma = 219 +- 16 meV can be used in updated reaction rate estimations and astrophysical models.

nucl-ex↗

arXiv2024

First direct measurement of the 64.5 keV resonance strength in $^{17}$O(p,$γ$)$^{18}$F reaction

The CNO cycle is one of the most important nuclear energy sources in stars. At temperatures of hydrostatic H-burning (20 MK $<$ T $<$ 80 MK) the $^{17}$O(p,$γ$)$^{18}$F reaction rate is dominated by the poorly constrained 64.5~keV resonance. Here we report on the first direct measurements of its resonance strength and of the direct capture contribution at 142 keV, performed with a new high sensitivity setup at LUNA. The present resonance strength of $ωγ_{(p, γ)}$\textsuperscript{bare} = (30 $\pm$ 6\textsubscript{stat} $\pm$ 2\textsubscript{syst})~peV is about a factor of 2 higher than the values in literature, leading to a $Γ$\textsubscript{p}\textsuperscript{bare} = (34 $\pm$ 7\textsubscript{stat} $\pm$ 3\textsubscript{syst})~neV, in agreement with LUNA result from the (p,$α$) channel. Such agreement strengthen our understanding of the oxygen isotopic ratios measured in red giant stars and in O-rich presolar grains.

nucl-ex↗

arXiv2024

Low energy alpha-nucleus optical potential studied via (a,n) cross section measurements on Te isotopes

In several processes of stellar nucleosynthesis, like the astrophysical gamma-process, nuclear reactions involving alpha particles play an important role. The description of these reactions necessitates the knowledge of the alpha-nucleus optical model potential (AOMP) which is highly ambiguous at low, astrophysical energies. This ambiguity introduces a substantial uncertainty in the stellar models for predicting elemental and isotopic abundances. The experimental study of the AOMP is thus necessary which can be implemented by measuring the cross section of alpha-induced nuclear reactions. At low energies, (a,n) reactions are suitable for such a purpose. Therefore, in the present work, the (a,n) cross sections of four Te isotopes have been measured, mostly for the first time, and compared with theoretical predictions. The (a,n) cross sections of 120,122,124,130Te have been measured in the energy range between about 10 and 17 MeV using the activation method. The detection of the gamma radiation following the decay of the radioactive reaction products were used to determine the cross sections. The measured cross sections are compared with statistical model calculations obtained from the widely used TALYS nuclear reaction simulation code. Predictions using various available AOMPs are investigated. It is found that the recently developed Atomki-V2 AOMP provides the best description for all studied reactions and this potential also reproduces well the total reaction cross sections from elastic scattering experiments, when they are available in literature. We recommend therefore to use the astrophysical reaction rates based on this potential for nucleosynthesis models of heavy elements.

nucl-ex↗

arXiv2023

First measurement of the low-energy direct capture in 20Ne(p, γ)21Na and improved energy and strength of the Ecm = 368 keV resonance

The $\mathrm{^{20}Ne(p, γ)^{21}Na}$ reaction is the slowest in the NeNa cycle and directly affects the abundances of the Ne and Na isotopes in a variety of astrophysical sites. Here we report the measurement of its direct capture contribution, for the first time below $E\rm_{cm} = 352$~keV, and of the contribution from the $E^{\rm }_{cm} = 368$~keV resonance, which dominates the reaction rate at $T=0.03-1.00$~GK. The experiment was performed deep underground at the Laboratory for Underground Nuclear Astrophysics, using a high-intensity proton beam and a windowless neon gas target. Prompt $γ$ rays from the reaction were detected with two high-purity germanium detectors. We obtain a resonance strength $ωγ~=~(0.112 \pm 0.002_{\rm stat}~\pm~0.005_{\rm sys})$~meV, with an uncertainty a factor of $3$ smaller than previous values. Our revised reaction rate is 20\% lower than previously adopted at $T < 0.1$~GK and agrees with previous estimates at temperatures $T \geq 0.1$~GK. Initial astrophysical implications are presented.

nucl-ex↗

arXiv2023

New proton-capture rates on carbon isotopes and their impact on the astrophysical $^{12}\mathrm{C}/{}^{13}\mathrm{C}$ ratio

The ${}^{12}\mathrm{C}/{}^{13}\mathrm{C}$ ratio is a significant indicator of nucleosynthesis and mixing processes during hydrogen burning in stars. Its value mainly depends on the relative rates of the ${}^{12}\mathrm{C}(p,γ){}^{13}\mathrm{N}$ and ${}^{13}\mathrm{C}(p,γ){}^{14}\mathrm{N}$ reactions. Both reactions have been studied at the Laboratory for Underground Nuclear Astrophysics (LUNA) in Italy down to the lowest energies to date ($E_\mathrm{c.m.} = 60\,\mathrm{keV}$) reaching for the first time the high energy tail of hydrogen burning in the shell of giant stars. Our cross sections, obtained with both prompt $γ$-ray detection and activation measurements, are the most precise to date with overall systematic uncertainties of $7-8\%$. Compared with most of the literature, our results are systematically lower, by $25\%$ for the ${}^{12}\mathrm{C}(p,γ){}^{13}\mathrm{N}$ reaction and by $30\%$ for ${}^{13}\mathrm{C}(p,γ){}^{14}\mathrm{N}$. We provide the most precise value up to now of $(3.6 \pm 0.4)$ in the $20-140\,\mathrm{MK}$ range for the lowest possible ${}^{12}\mathrm{C}/{}^{13}\mathrm{C}$ ratio that can be produced during H burning in giant stars.

nucl-ex↗

arXiv2023

Experimental determination of the $^3$He($α$,$γ$)$^7$Be reaction cross section above the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction plays a major role both in the BBN producing the majority of the primordial $^7$Li, and in the pp-chain, where it is the branching point. As a few-nucleon system, this reaction is often used to validate ab-initio theoretical calculations and/or test R-matrix theory and code implementations. For the latter, experimental data in an extended energy range is of crucial importance to test the fit and extrapolation capabilities of the different codes. The $^3$He($α$,$γ$)$^7$Be reaction cross section has been measured by several groups up to the first resonance ($E_{c.m.} \approx 3$ MeV) in the reaction. However, only one dataset exists above the $^7$Be proton separation threshold measured in a narrow energy range ($E_{c.m.} = 4.0-4.4$ MeV). In this work we extend the available experimental capture cross section database to the energy range of known $^7$Be levels. The activation method was used. The experiment was performed using a thin-window gas cell with two high-purity Al foils as entrance and exit windows. The activity of the $^7$Be nuclei implanted in the exit/catcher foil was measured by detecting the yield of the emitted $γ$~rays using shielded high-purity germanium detectors. New experimental $^3$He($α$,$γ$)$^7$Be reaction cross section data were obtained for the first time in the $E_{c.m.}=4.3-8.3$ MeV energy region. The new dataset with about 0.2 MeV step covers the energy range of known levels and particle separation thresholds. No prominent structures are observer around the $^7$Be levels. The reaction cross section is slowly increasing with increasing energy. Above the $^6$Li$+p_1$ threshold, a decrease starts in the cross section trend. The overall structure of the cross section suggest a broad resonance peaking around $E_x=7.5$ MeV $^7$Be excitation energy, with a width of 8 MeV.

nucl-ex↗

arXiv2023

The $γ$-process nucleosynthesis in core-collapse supernovae. I. A novel analysis of $γ$-process yields in massive stars

The $γ$-process nucleosynthesis in core-collapse supernovae is generally accepted as a feasible process for the synthesis of neutron-deficient isotopes beyond iron. However, crucial discrepancies between theory and observations still exist: the average production of $γ$-process yields from massive stars are too low to reproduce the solar distribution in galactic chemical evolution calculations, and the yields of the Mo and Ru isotopes are by a further factor of 10 lower than the yields of the other $γ$-process nuclei. We investigate the $γ$-process in 5 sets of core-collapse supernova models published in literature with initial masses 15, 20, and 25 M$_{\odot}$ at solar metallicity. We compared the $γ$-process overproduction factors from the different models. To highlight the possible effect of nuclear physics input, we also considered 23 ratios of two isotopes close to each other in mass, relative to their solar values. Further, we investigated the contribution of C-O shell mergers in the supernova progenitors as an additional site of the $γ$-process. Our analysis shows that a large scatter among the different models exists for both the $γ$-process integrated yields and the isotopic ratios. We found only 10 ratios that agree with their solar values, all the others differ by at least a factor of 3 from the solar values in all the considered sets of models. The $γ$-process within C-O shell mergers mostly influence the isotopic ratios that involve intermediate and heavy proton-rich isotopes with $\rm A>100$.

astro-ph.SR↗

arXiv2023

Cross section measurement of the 12C(p,gamma)13N reaction with activation in a wide energy range

The CNO cycle is one of the fundamental processes of hydrogen burning in stars. The first reaction of the cycle is the radiative proton capture on 12C and the rate of this 12C(p,gamma)13N reaction is related to the 12C/13C ratio observed e.g. in the Solar System. The low-energy cross section of this reaction was measured several times in the past, however, the experimental data are scarce in a wide energy range especially around the resonance at 1.7 MeV. In the present work the 12C(p,gamma)13N cross section was measured between 300 and 1900 keV using the activation method. This method was only used several decades ago in the low-energy region. As the activation method provides the total cross section and has uncertainties different from those of the in-beam gamma-spectroscopy technique, the present results provide a largely independent data set for future low-energy extrapolations and thus for astrophysical reaction rate calculations.

nucl-ex↗

arXiv2023

Cross section measurement of the 144Sm(alpha,n)147Gd reaction for studying the alpha-nucleus optical potential at astrophysical energies

Nuclear reactions involving alpha particles play an important role in various astrophysical processes such as the gamma-process of heavy element nucleosynthesis. The poorly known low-energy alpha-nucleus optical (AOMP) potential is a key parameter to estimate the rates of these reactions. The AOMP can be tested by measuring the cross section of alpha-scattering as well as alpha-induced reactions. Low energy elastic alpha-scattering on 144Sm has recently been measured with high precision. The aim of the present work was to complement that work by measuring the (a,n) cross sections on 144Sm at low energies. The experimental data shall be used to constrain the AOMP. From this potential the 144Sm(a,g)148Gd reaction rate can be derived with reduced uncertainties. The 144Sm(a,n)147Gd reaction was studied by bombarding Sm targets with alpha-beams provided by the cyclotron accelerator of Atomki. The cross section was determined using the activation method. The gamma-radiation following the decay of the 147Gd reaction product was measured with a HPGe detector. The experimental data are analyzed within the statistical model. The cross section was measured in the alpha-energy range between 13 and 20 MeV in 1 MeV steps, i.e., from close above the (a,n) threshold. The results were compared with statistical model calculations using various approaches and parametrizations for the AOMP, and excellent agreement was obtained for two recent potentials. However, these potentials cannot reproduce literature data for the 144Sm(a,g)148Gd reaction with the same accuracy. Constraints for the AOMP were derived from an analysis of the new 144Sm(a,n)147Gd data and literature data for 144Sm(a,g)148Gd. These constraints enable a determination of the reaction rate of the 144Sm(a,g)148Gd reaction with significantly reduced uncertainties of less than a factor of two.

nucl-ex↗

arXiv2022

First direct limit on the 334 keV resonance strength in the $^{22}$Ne(α,γ)$^{26}$Mg reaction

In stars, the fusion of $^{22}$Ne and $^4$He may produce either $^{25}$Mg, with the emission of a neutron, or $^{26}$Mg and a $γ$ ray. At high temperature, the ($α,n$) channel dominates, while at low temperature, it is energetically hampered. The rate of its competitor, the $^{22}$Ne($α$,$γ$)$^{26}$Mg reaction, and, hence, the minimum temperature for the ($α,n$) dominance, are controlled by many nuclear resonances. The strengths of these resonances have hitherto been studied only indirectly. The present work aims to directly measure the total strength of the resonance at $E$_{r}$\,=\,$334$\,$keV (corresponding to $E$_{x}$\,=\,$10949$\,$keV in $^{26}$Mg). The data reported here have been obtained using high intensity $^4$He$^+$ beam from the INFN LUNA 400 kV underground accelerator, a windowless, recirculating, 99.9% isotopically enriched $^{22}$Ne gas target, and a 4$π$ bismuth germanate summing $γ$-ray detector. The ultra-low background rate of less than 0.5 counts/day was determined using 67 days of no-beam data and 7 days of $^4$He$^+$ beam on an inert argon target. The new high-sensitivity setup allowed to determine the first direct upper limit of 4.0$\,\times\,$10$^{-11}$ eV (at 90% confidence level) for the resonance strength. Finally, the sensitivity of this setup paves the way to study further $^{22}$Ne($α$,$γ$)$^{26}$Mg resonances at higher energy.

nucl-ex↗

arXiv2021

Measurement of the 91Zr(p,gamma)92mNb cross section motivated by type Ia supernova nucleosynthesis

The synthesis of heavy, proton rich isotopes is a poorly understood astrophysical process. Thermonuclear (type Ia) supernova explosions are among the suggested sites and the abundance of some isotopes present in the early solar system may be used to test the models. 92Nb is such an isotope and one of the reactions playing a role in its synthesis is 91Zr(p,gamma)92Nb. As no experimental cross sections were available for this reaction so far, nucleosynthesis models had to solely rely on theoretical calculations. In the present work the cross section of 91Zr(p,gamma)92mNb has been measured at astrophysical energies by activation. The results excellently confirm the predictions of cross sections and reaction rates for 91Zr(p,gamma)92Nb, as used in astrophysical simulations.

nucl-ex↗

arXiv2020

Successful prediction of total $α$-induced reaction cross sections at astrophysically relevant sub-Coulomb energies using a novel approach

The prediction of stellar ($γ$,$α$) reaction rates for heavy nuclei is based on the calculation of ($α$,$γ$) cross sections at sub-Coulomb energies. These rates are essential for modeling the nucleosynthesis of so-called $p$-nuclei. The standard calculations in the statistical model show a dramatic sensitivity to the chosen $α$-nucleus potential. The present study explains the reason for this dramatic sensitivity which results from the tail of the imaginary $α$-nucleus potential in the underlying optical model calculation of the total reaction cross section. As an alternative to the optical model, a simple barrier transmission model is suggested. It is shown that this simple model in combination with a well-chosen $α$-nucleus potential is able to predict total $α$-induced reaction cross sections for a wide range of heavy target nuclei above $A \gtrsim 150$ with uncertainties below a factor of two. The new predictions from the simple model do not require any adjustment of parameters to experimental reaction cross sections whereas in previous statistical model calculations all predictions remained very uncertain because the parameters of the $α$-nucleus potential had to be adjusted to experimental data. The new model allows to predict the reaction rate of the astrophysically important $^{176}$W($α$,$γ$)$^{180}$Os reaction with reduced uncertainties, leading to a significantly lower reaction rate at low temperatures. The new approach could also be validated for a broad range of target nuclei from $A \approx 60$ up to $A \gtrsim 200$.

nucl-th↗

arXiv2020

Setup commissioning for an improved measurement of the D(p,gamma)3He cross section at Big Bang Nucleosynthesis energies

Among the reactions involved in the production and destruction of deuterium during Big Bang Nucleosynthesis, the deuterium-burning D(p,gamma)3He reaction has the largest uncertainty and limits the precision of theoretical estimates of primordial deuterium abundance. Here we report the results of a careful commissioning of the experimental setup used to measure the cross-section of the D(p,gamma)3He reaction at the Laboratory for Underground Nuclear Astrophysics of the Gran Sasso Laboratory (Italy). The commissioning was aimed at minimising all sources of systematic uncertainty in the measured cross sections. The overall systematic error achieved (< 3 %) will enable improved predictions of BBN deuterium abundance.

physics.ins-det↗