Searcharxiv⌕ Search

arXiv subjects

Zs. Fülöp

Publications and source records attributed to Zs. Fülöp.

At least 37 records · Page 2Linked to original sources

Setup commissioning for an improved measurement of the D(p,gamma)3He cross section at Big Bang Nucleosynthesis energies

Among the reactions involved in the production and destruction of deuterium during Big Bang Nucleosynthesis, the deuterium-burning D(p,gamma)3He reaction has the largest uncertainty and limits the precision of theoretical estimates of primordial deuterium abundance. Here we report the results of a careful commissioning of the experimental setup used to measure the cross-section of the D(p,gamma)3He reaction at the Laboratory for Underground Nuclear Astrophysics of the Gran Sasso Laboratory (Italy). The commissioning was aimed at minimising all sources of systematic uncertainty in the measured cross sections. The overall systematic error achieved (< 3 %) will enable improved predictions of BBN deuterium abundance.

physics.ins-det↗

Cross section of $α$-induced reactions on $^{197}$Au at sub-Coulomb energies

Statistical model calculations have to be used for the determination of reaction rates in large-scale reaction networks for heavy-element nucleosynthesis. A basic ingredient of such a calculation is the a-nucleus optical model potential. Several different parameter sets are available in literature, but their predictions of a-induced reaction rates vary widely, sometimes even exceeding one order of magnitude. This paper presents the result of a-induced reaction cross-section measurements on gold which could be carried out for the first time very close to the astrophysically relevant energy region. The new experimental data are used to test statistical model predictions and to constrain the a-nucleus optical model potential. For the measurements the activation technique was used. The cross section of the (a,n) and (a,2n) reactions was determined from g-ray counting, while that of the radiative capture was determined via X-ray counting. The cross section of the reactions was measured below E$_a=20.0$~MeV. In the case of the $^{197}$Au(a,2n)$^{199}$Tl reaction down to 17.5~MeV with 0.5-MeV steps, reaching closer to the reaction threshold than ever before. The cross section of $^{197}$Au(a,n)$^{200}$Tl and $^{197}$Au(a,g)$^{201}$Tl was measured down to E$_a=13.6$ and 14.0~MeV, respectively, with 0.5-MeV steps above the (a,2n) reaction threshold and with 1.0-MeV steps below that. The new dataset is in agreement with the available values from the literature, but is more precise and extends towards lower energies. Two orders of magnitude lower cross sections were successfully measured than in previous experiments which used g-ray counting only, thus providing experimental data at lower energies than ever before. The new precision dataset allows us to find the best-fit a-nucleus optical model potential and to predict cross sections in the Gamow window with smaller uncertainties.

nucl-ex↗

Resonance strengths in the 14N(p,gamma)15O astrophysical key reaction measured with activation

The 14N(p,gamma)15O reaction plays a vital role in various astrophysical scenarios. Its reaction rate must be accurately known in the present era of high precision astrophysics. The cross section of the reaction is often measured relative to a low energy resonance, the strength of which must therefore be determined precisely. The activation method, based on the measurement of 15O decay, has not been used in modern measurements of the 14N(p,gamma)15O reaction. The aim of the present work is to provide strength data for two resonances in the 14N(p,gamma)15O reaction using the activation method. The obtained values are largely independent from previous data measured by in-beam gamma-spectroscopy and are free from some of their systematic uncertainties. Solid state TiN targets were irradiated with a proton beam provided by the Tandetron accelerator of Atomki using a cyclic activation. The decay of the produced 15O isotopes was measured by detecting the 511 keV positron annihilation gamma-rays. The strength of the Ep = 278 keV resonance was measured to be 13.4 +- 0.8 meV while for the Ep = 1058 keV resonance the strength is 442 +- 27 meV. The obtained Ep = 278 keV resonance strength is in fair agreement with the values recommended by two recent works. On the other hand, the Ep = 1058 keV resonance strength is about 20% higher than the previous value. The discrepancy may be caused in part by a previously neglected finite target thickness correction. As only the low energy resonance is used as a normalization point for cross section measurements, the calculated astrophysical reaction rate of the 14N(p,gamma)15O reaction and therefore the astrophysical consequences are not changed by the present results.

nucl-ex↗

Cross section of $^3$He($α$,$γ$)$^7$Be around the $^7$Be proton separation threshold

The $^3$He($α$,$γ$)$^7$Be reaction is a widely studied nuclear reaction; however, it is still not understood with the required precision. It has a great importance both in Big Bang nucleosynthesis and in solar hydrogen burning. The low mass number of the reaction partners makes it also suitable for testing microscopic calculations. Despite the high number of experimental studies, none of them addresses the $^3$He($α$,$γ$)$^7$Be reaction cross sections above 3.1-MeV center-of-mass energy. Recently, a previously unobserved resonance in the $^6$Li(p,$γ$)$^7$Be reaction suggested a new level in $^7$Be, which would also have an impact on the $^3$He($α$,$γ$)$^7$Be reaction in the energy range above 4.0 MeV. The aim of the present experiment is to measure the $^3$He($α$,$γ$)$^7$Be reaction cross section in the energy range of the proposed level. For this investigation the activation technique was used. A thin window gas-cell target confining $^3$He gas was irradiated using an $α$ beam. The $^7$Be produced was implanted into the exit foil. The $^7$Be activity was determined by counting the $γ$ rays following its decay by a well-shielded high-purity germanium detector. Reaction cross sections have been determined between $E_{cm} = 4.0 - 4.4$ MeV with 0.04-MeV steps covering the energy range of the proposed nuclear level. One lower-energy cross-section point was also determined to be able to compare the results with previous studies. A constant cross section of around 10.5 $μ$barn was observed around the $^7$Be proton separation energy. An upper limit of 45 neV for the strength of a $^3$He($α$,$γ$)$^7$Be resonance is derived.

nucl-ex↗

High precision half-life measurement of $^{125}$Cs and $^{125}$Xe with γ-spectroscopy

In order to provide data for the simulation of the astrophysical $γ$-process, the cross section measurement of the $^{124}$Xe(p,$γ$)$^{125}$Cs reaction is in progress at MTA Atomki using the activation technique. Precise information on the decay characteristics of the reaction products is of crucial importance for measurements carried out using this method. The half-lives of the produced $^{125}$Cs and its daughter $^{125}$Xe are published in previous works, but with large uncertainties and ambiguous values. To make these nuclear parameters more precise, the half-lives have been re-measured with high precision using $γ$-spectroscopy. The obtained new half-life values are t$_{1/2}$ = 44.35 $\pm$ 0.29 minutes for $^{125}$Cs and t$_{1/2}$ = 16.87 $\pm$ 0.08 hours for $^{125}$Xe.

nucl-ex↗

Half-life measurement of 65Ga with gamma-spectroscopy

The literature half-life value of 65Ga is based on only one experiment carried out more than 60 years ago and it has a relatively large uncertainty. In the present work this half-life is determined based on the counting of the gamma-rays following the beta-decay of 65Ga. Our new recommended half-life is 15.133 +- 0.028 min which is in agreement with the literature value but almost one order of magnitude more precise.

nucl-ex↗

The activation method for cross section measurements in nuclear astrophysics

The primary aim of experimental nuclear astrophysics is to determine the rates of nuclear reactions taking place in stars in various astrophysical conditions. These reaction rates are important ingredient for understanding the elemental abundance distribution in our solar system and the galaxy. The reaction rates are determined from the cross sections which need to be measured at energies as close to the astrophysically relevant ones as possible. In many cases the final nucleus of an astrophysically important reaction is radioactive which allows the cross section to be determined based on the off-line measurement of the number of produced isotopes. In general, this technique is referred to as the activation method, which often has substantial advantages over in-beam particle- or gamma-detection measurements. In this paper the activation method is reviewed from the viewpoint of nuclear astrophysics. Important aspects of the activation method are given through several reaction studies for charged particle, neutron and gamma-induced reactions. Various techniques for the measurement of the produced activity are detailed. As a special case of activation, the technique of Accelerator Mass Spectrometry in cross section measurements is also reviewed.

nucl-ex↗

Direct capture cross section and the $E_p$ = 71 and 105 keV resonances in the $^{22}$Ne($p,γ$)$^{23}$Na reaction

The $^{22}$Ne($p,γ$)$^{23}$Na reaction, part of the neon-sodium cycle of hydrogen burning, may explain the observed anticorrelation between sodium and oxygen abundances in globular cluster stars. Its rate is controlled by a number of low-energy resonances and a slowly varying non-resonant component. Three new resonances at $E_p$ = 156.2, 189.5, and 259.7 keV have recently been observed and confirmed. However, significant uncertainty on the reaction rate remains due to the non-resonant process and to two suggested resonances at $E_p$ = 71 and 105 keV. Here, new $^{22}$Ne($p,γ$)$^{23}$Na data with high statistics and low background are reported. Stringent upper limits of 6$\times$10$^{-11}$ and 7$\times$10$^{-11}$\,eV (90\% confidence level), respectively, are placed on the two suggested resonances. In addition, the off-resonant S-factor has been measured at unprecedented low energy, constraining the contributions from a subthreshold resonance and the direct capture process. As a result, at a temperature of 0.1 GK the error bar of the $^{22}$Ne($p,γ$)$^{23}$Na rate is now reduced by three orders of magnitude.

nucl-ex↗

Effect of beam energy straggling on resonant yield in thin gas targets: The cases $^{22}$Ne(p,γ)$^{23}$Na and $^{14}$N(p,γ)$^{15}$O

When deriving resonance strengths using the thick-target yield approximation, for very narrow resonances it may be necessary to take beam energy straggling into account. This applies to gas targets of a few keV width, especially if there is some additional structure in target stoichiometry or detection efficiency. The correction for this effect is shown and tested on recent studies of narrow resonances in the $^{22}$Ne(p,γ)$^{23}$Na and $^{14}$N(p,γ)$^{15}$O reactions.

nucl-ex↗

Investigation of $α$-induced reactions on Sb isotopes relevant to the astrophysical $γ$-process

The aim of the present work is to measure the $^{121}$Sb($α,γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reaction cross sections. The $α$-induced reactions on natural and enriched antimony targets were investigated using the activation technique. The ($α$,$γ$) cross sections of $^{121}$Sb were measured and are reported for first time. To determine the cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I, and $^{123}$Sb($α$,n)$^{126}$I reactions, the yields of $γ$-rays following the $β$-decay of the reaction products were measured. For the measurement of the lowest cross sections, the characteristic X-rays were counted with a LEPS (Low Energy Photon Spectrometer) detector. The cross section of the $^{121}$Sb($α$,$γ$)$^{125}$I, $^{121}$Sb($α$,n)$^{124}$I and $^{123}$Sb($α$,n)$^{126}$I reactions were measured with high precision in an energy range between 9.74 MeV to 15.48 MeV, close to the astrophysically relevant energy window. The results are compared with the predictions of statistical model calculations. The ($α$,n) data show that the $α$ widths are predicted well for these reactions. The ($α$,$γ$) results are overestimated by the calculations but this is due to the applied neutron- and $γ$ widths. Relevant for the astrophysical reaction rate is the $α$ width used in the calculations.While for other reactions the $α$ widths seem to have been overestimated and their energy dependence was not described well in the measured energy range, this is not the case for the reactions studied here. The result is consistent with the proposal that additional reaction channels, such as Coulomb excitation, may have led to the discrepancies found in other reactions.

nucl-ex↗

A high-efficiency gas target setup for underground experiments, and redetermination of the branching ratio of the 189.5 keV $\mathbf{^{22}Ne(p,γ)^{23}Na}$ resonance

The experimental study of nuclear reactions of astrophysical interest is greatly facilitated by a low-background, high-luminosity setup. The Laboratory for Underground Nuclear Astrophysics (LUNA) 400 kV accelerator offers ultra-low cosmic-ray induced background due to its location deep underground in the Gran Sasso National Laboratory (INFN-LNGS), Italy, and high intensity, 250-500 $μ$A, proton and $α$ ion beams. In order to fully exploit these features, a high-purity, recirculating gas target system for isotopically enriched gases is coupled to a high-efficiency, six-fold optically segmented bismuth germanate (BGO) $γ$-ray detector. The beam intensity is measured with a beam calorimeter with constant temperature gradient. Pressure and temperature measurements have been carried out at several positions along the beam path, and the resultant gas density profile has been determined. Calibrated $γ$-intensity standards and the well-known $E_p$ = 278 keV $\mathrm{^{14}N(p,γ)^{15}O}$ resonance were used to determine the $γ$-ray detection efficiency and to validate the simulation of the target and detector setup. As an example, the recently measured resonance at $E_p$ = 189.5 keV in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction has been investigated with high statistics, and the $γ$-decay branching ratios of the resonance have been determined.

nucl-ex↗

Nuclear physics uncertainties of the astrophysical gamma-process studied through the 64Zn(p,alpha)61Cu and 64Zn(p,gamma)65Ga reactions

In a recent work, the cross section measurement of the 64Zn(p,alpha)61Cu reaction was used to prove that the standard alpha-nucleus optical potentials used in astrophysical network calculation fail to reproduce the experimental data at energies relevant for heavy element nucleosynthesis. In the present paper the analysis of the obtained experimental data is continued by comparing the results with the predictions using different parameters. It is shown that the recently suggested modification of the standard optical potential leads to a better description of the data.

nucl-ex↗

Cross section of $α$-induced reactions on iridium isotopes obtained from thick target yield measurement for the astrophysical $γ$ process

The stellar reaction rates of radiative $α$-capture reactions on heavy isotopes are of crucial importance for the $γ$ process network calculations. These rates are usually derived from statistical model calculations, which need to be validated, but the experimental database is very scarce. This paper presents the results of $α$-induced reaction cross section measurements on iridium isotopes carried out at first close to the astrophysically relevant energy region. Thick target yields of $^{191}$Ir($α$,$γ$)$^{195}$Au, $^{191}$Ir($α$,n)$^{194}$Au, $^{193}$Ir($α$,n)$^{196m}$Au, $^{193}$Ir($α$,n)$^{196}$Au reactions have been measured with the activation technique between E$_α= 13.4$ MeV and 17 MeV. For the first time the thick target yield was determined with X-ray counting. This led to a previously unprecedented sensitivity. From the measured thick target yields, reaction cross sections are derived and compared with statistical model calculations. The recently suggested energy-dependent modification of the $α$+nucleus optical potential gives a good description of the experimental data.

nucl-ex↗

Cross section measurement of the astrophysically important 17O(p,gamma)18F reaction in a wide energy range

The 17O(p,g)18F reaction plays an important role in hydrogen burning processes in different stages of stellar evolution. The rate of this reaction must therefore be known with high accuracy in order to provide the necessary input for astrophysical models. The cross section of 17O(p,g)18F is characterized by a complicated resonance structure at low energies. Experimental data, however, is scarce in a wide energy range which increases the uncertainty of the low energy extrapolations. The purpose of the present work is therefore to provide consistent and precise cross section values in a wide energy range. The cross section is measured using the activation method which provides directly the total cross section. With this technique some typical systematic uncertainties encountered in in-beam gamma-spectroscopy experiments can be avoided. The cross section was measured between 500 keV and 1.8 MeV proton energies with a total uncertainty of typically 10%. The results are compared with earlier measurements and it is found that the gross features of the 17O(p,g)18F excitation function is relatively well reproduced by the present data. Deviation of roughly a factor of 1.5 is found in the case of the total cross section when compared with the only one high energy dataset. At the lowest measured energy our result is in agreement with two recent datasets within one standard deviation and deviates by roughly two standard deviations from a third one. An R-matrix analysis of the present and previous data strengthen the reliability of the extrapolated zero energy astrophysical S-factor. Using an independent experimental technique, the literature cross section data of 17O(p,g)18F is confirmed in the energy region of the resonances while lower direct capture cross section is recommended at higher energies. The present dataset provides a constraint for the theoretical cross sections.

nucl-ex↗

Origin of meteoritic stardust unveiled by a revised proton-capture rate of $^{17}$O

Stardust grains recovered from meteorites provide high-precision snapshots of the isotopic composition of the stellar environment in which they formed. Attributing their origin to specific types of stars, however, often proves difficult. Intermediate-mass stars of 4-8 solar masses are expected to contribute a large fraction of meteoritic stardust. However, no grains have been found with characteristic isotopic compositions expected from such stars. This is a long-standing puzzle, which points to serious gaps in our understanding of the lifecycle of stars and dust in our Galaxy. Here we show that the increased proton-capture rate of $^{17}$O reported by a recent underground experiment leads to $^{17}$O/$^{16}$O isotopic ratios that match those observed in a population of stardust grains, for proton-burning temperatures of 60-80 million K. These temperatures are indeed achieved at the base of the convective envelope during the late evolution of intermediate-mass stars of 4-8 solar masses, which reveals them as the most likely site of origin of the grains. This result provides the first direct evidence that these stars contributed to the dust inventory from which the Solar System formed.

astro-ph.SR↗

Statistical model analysis of $α$-induced reaction cross sections of $^{64}$Zn at low energies

Background $α$-nucleus potentials play an essential role for the calculation of $α$-induced reaction cross sections at low energies in the statistical model. Uncertainties of these calculations are related to ambiguities in the adjustment of the potential parameters to experimental elastic scattering angular distributions (typically at higher energies) and to the energy dependence of the effective $α$-nucleus potentials. Purpose The present work studies cross sections of $α$-induced reactions for $^{64}$Zn at low energies and their dependence on the chosen input parameters of the statistical model calculations. The new experimental data from the recent Atomki experiments allow for a $χ^2$-based estimate of the uncertainties of calculated cross sections at very low energies. Method The recent data for the ($α$,$γ$), ($α$,$n$), and ($α$,$p$) reactions on $^{64}$Zn are compared to calculations in the statistical model. A survey of the parameter space of the widely used computer code TALYS is given, and the properties of the obtained $χ^2$ landscape are discussed. Results The best fit to the experimental data at low energies shows $χ^2/F \approx 7.7$ per data point which corresponds to an average deviation of about 30% between the best fit and the experimental data. Several combinations of the various ingredients of the statistical model are able to reach a reasonably small $χ^2/F$, not exceeding the best-fit result by more than a factor of 2. Conclusions The present experimental data for $^{64}$Zn in combination with the statistical model calculations allow to constrain the astrophysical reaction rate within about a factor of 2. However, the significant excess of $χ^2/F$ of the best-fit from unity asks for further improvement of the statistical model calculations and in particular the $α$-nucleus potential.

nucl-th↗

$α$-scattering and $α$-induced reaction cross sections of $^{64}$Zn at low energies

Background: alpha-nucleus potentials play an essential role for the calculation of alpha-induced reaction cross sections at low energies in the statistical model... Purpose: The present work studies the total reaction cross section sigma_reac of alpha-induced reactions at low energies which can be determined from the elastic scattering angular distribution or from the sum over the cross sections of all open non-elastic channels. Method: Elastic and inelastic 64Zn(a,a)64Zn angular distributions were measured at two energies around the Coulomb barrier at 12.1 MeV and 16.1 MeV. Reaction cross sections of the (a,g), (a,n), and (a,p) reactions were measured at the same energies using the activation technique. The contributions of missing non-elastic channels were estimated from statistical model calculations. Results: The total reaction cross sections from elastic scattering and from the sum of the cross sections over all open non-elastic channels agree well within the uncertainties. This finding confirms the consistency of the experimental data. At the higher energy of 16.1 MeV, the predicted significant contribution of compound-inelastic scattering to the total reaction cross section is confirmed experimentally. As a by-product it is found that most recent global alpha-nucleus potentials are able to describe the reaction cross sections for 64Zn around the Coulomb barrier. Conclusions: Total reaction cross sections of alpha-induced reactions can be well determined from elastic scattering angular distributions. The present study proves experimentally that the total cross section from elastic scattering is identical to the sum of non-elastic reaction cross sections. Thus, the statistical model can reliably be used to distribute the total reaction cross section among the different open channels.

nucl-ex↗

The impact of the revised $^{17}$O$(p,α)^{14}$N reaction rate on $^{17}$O stellar abundances and yields

Context. Material processed by the CNO cycle in stellar interiors is enriched in 17O. When mixing processes from the stellar surface reach these layers, as occurs when stars become red giants and undergo the first dredge up, the abundance of 17O increases. Such an occurrence explains the drop of the 16O/17O observed in RGB stars with mass larger than 1.5 M_\solar. As a consequence, the interstellar medium is continuously polluted by the wind of evolved stars enriched in 17O . Aims. Recently, the Laboratory for Underground Nuclear Astrophysics (LUNA) collaboration released an improved rate of the 17O(p,alpha)14N reaction. In this paper we discuss the impact that the revised rate has on the 16O/17O ratio at the stellar surface and on 17O stellar yields. Methods. We computed stellar models of initial mass between 1 and 20 M_\solar and compared the results obtained by adopting the revised rate of the 17O(p,alpha)14N to those obtained using previous rates. Results. The post-first dredge up 16O/17O ratios are about 20% larger than previously obtained. Negligible variations are found in the case of the second and the third dredge up. In spite of the larger 17O(p,alpha)14N rate, we confirm previous claims that an extra-mixing process on the red giant branch, commonly invoked to explain the low carbon isotopic ratio observed in bright low-mass giant stars, marginally affects the 16O/17O ratio. Possible effects on AGB extra-mixing episodes are also discussed. As a whole, a substantial reduction of 17O stellar yields is found. In particular, the net yield of stars with mass ranging between 2 and 20 M_\solar is 15 to 40% smaller than previously estimated. Conclusions. The revision of the 17O(p,alpha)14N rate has a major impact on the interpretation of the 16O/17O observed in evolved giants, in stardust grains and on the 17O stellar yields.

astro-ph.SR↗