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Zs. Fülöp

Publications and source records attributed to Zs. Fülöp.

At least 55 records · Page 3Linked to original sources

Direct measurement of low-energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction is the most uncertain process in the neon-sodium cycle of hydrogen burning. At temperatures relevant for nucleosynthesis in asymptotic giant branch stars and classical novae, its uncertainty is mainly due to a large number of predicted but hitherto unobserved resonances at low energy. Purpose: A new direct study of low energy $^{22}$Ne(p,$γ$)$^{23}$Na resonances has been performed at the Laboratory for Underground Nuclear Astrophysics (LUNA), in the Gran Sasso National Laboratory, Italy. Method: The proton capture on $^{22}$Ne was investigated in direct kinematics, delivering an intense proton beam to a $^{22}$Ne gas target. $γ$ rays were detected with two high-purity germanium detectors enclosed in a copper and lead shielding suppressing environmental radioactivity. Results: Three resonances at 156.2 keV ($ωγ$ = (1.48\,$\pm$\,0.10)\,$\cdot$\,10$^{-7}$ eV), 189.5 keV ($ωγ$ = (1.87\,$\pm$\,0.06)\,$\cdot$\,10$^{-6}$ eV) and 259.7 keV ($ωγ$ = (6.89\,$\pm$\,0.16)\,$\cdot$\,10$^{-6}$ eV) proton beam energy, respectively, have been observed for the first time. For the levels at 8943.5, 8975.3, and 9042.4 keV excitation energy corresponding to the new resonances, the $γ$-decay branching ratios have been precisely measured. Three additional, tentative resonances at 71, 105 and 215 keV proton beam energy, respectively, were not observed here. For the strengths of these resonances, experimental upper limits have been derived that are significantly more stringent than the upper limits reported in the literature. Conclusions: Based on the present experimental data and also previous literature data, an updated thermonuclear reaction rate is provided in tabular and parametric form. The new reaction rate is significantly higher than previous evaluations at temperatures of 0.08-0.3 GK.

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Experimental study of the astrophysical gamma-process reaction 124Xe(alpha,gamma)128Ba

The synthesis of heavy, proton rich isotopes in the astrophysical gamma-process proceeds through photodisintegration reactions. For the improved understanding of the process, the rates of the involved nuclear reactions must be known. The reaction 128Ba(g,a)124Xe was found to affect the abundance of the p nucleus 124Xe. Since the stellar rate for this reaction cannot be determined by a measurement directly, the aim of the present work was to measure the cross section of the inverse 124Xe(a,g)128Ba reaction and to compare the results with statistical model predictions. Of great importance is the fact that data below the (a,n) threshold was obtained. Studying simultaneously the 124Xe(a,n)127Ba reaction channel at higher energy allowed to further identify the source of a discrepancy between data and prediction. The 124Xe + alpha cross sections were measured with the activation method using a thin window 124Xe gas cell. The studied energy range was between E = 11 and 15 MeV close above the astrophysically relevant energy range. The obtained cross sections are compared with statistical model calculations. The experimental cross sections are smaller than standard predictions previously used in astrophysical calculations. As dominating source of the difference, the theoretical alpha width was identified. The experimental data suggest an alpha width lower by at least a factor of 0.125 in the astrophysical energy range. An upper limit for the 128Ba(g,a)124Xe stellar rate was inferred from our measurement. The impact of this rate was studied in two different models for core-collapse supernova explosions of 25 solar mass stars. A significant contribution to the 124Xe abundance via this reaction path would only be possible when the rate was increased above the previous standard value. Since the experimental data rule this out, they also demonstrate the closure of this production path.

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Underground nuclear astrophysics: why and how

The goal of nuclear astrophysics is to measure cross sections of nuclear physics reactions of interest in astrophysics. At stars temperatures, these cross sections are very low due to the suppression of the Coulomb barrier. Cosmic ray induced background can seriously limit the determination of reaction cross sections at energies relevant to astrophysical processes and experimental setups should be arranged in order to improve the signal-to-noise ratio. Placing experiments in underground sites, however, reduces this background opening the way towards ultra low cross section determination. LUNA (Laboratory for Underground Nuclear Astrophysics) was pioneer in this sense. Two accelerators were mounted at the INFN National Laboratories of Gran Sasso (LNGS) allowing to study nuclear reactions close to stellar energies. A summary of the relevant technology used, including accelerators, target production and characterisation, and background treatment is given.

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Three new low-energy resonances in the $^{22}$Ne(p,$γ$)$^{23}$Na reaction

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle affects the synthesis of the elements between $^{20}$Ne and $^{27}$Al in asymptotic giant branch stars and novae. The $^{22}$Ne(p,$γ$)$^{23}$Na reaction rate is very uncertain because of a large number of unobserved resonances lying in the Gamow window. At proton energies below 400\,keV, only upper limits exist in the literature for the resonance strengths. Previous reaction rate evaluations differ by large factors. In the present work, the first direct observations of the $^{22}$Ne(p,$γ$)$^{23}$Na resonances at 156.2, 189.5, and 259.7\,keV are reported. Their resonance strengths have been derived with 2-7\% uncertainty. In addition, upper limits for three other resonances have been greatly reduced. Data were taken using a windowless $^{22}$Ne gas target and high-purity germanium detectors at the Laboratory for Underground Nuclear Astrophysics in the Gran Sasso laboratory of the National Institute for Nuclear Physics, Italy, taking advantage of the ultra-low background observed deep underground. The new reaction rate is a factor of 5 higher than the recent evaluation at temperatures relevant to novae and asymptotic giant branch stars nucleosynthesis.

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Determination of gamma-ray widths in $^{15}$N using nuclear resonance fluorescence

The stable nucleus $^{15}$N is the mirror of $^{15}$O, the bottleneck in the hydrogen burning CNO cycle. Most of the $^{15}$N level widths below the proton emission threshold are known from just one nuclear resonance fluorescence (NRF) measurement, with limited precision in some cases. A recent experiment with the AGATA demonstrator array determined level lifetimes using the Doppler Shift Attenuation Method (DSAM) in $^{15}$O. As a reference and for testing the method, level lifetimes in $^{15}$N have also been determined in the same experiment. The latest compilation of $^{15}$N level properties dates back to 1991. The limited precision in some cases in the compilation calls for a new measurement in order to enable a comparison to the AGATA demonstrator data. The widths of several $^{15}$N levels have been studied with the NRF method. The solid nitrogen compounds enriched in $^{15}$N have been irradiated with bremsstrahlung. The $γ$-rays following the deexcitation of the excited nuclear levels were detected with four HPGe detectors. Integrated photon-scattering cross sections of ten levels below the proton emission threshold have been measured. Partial gamma-ray widths of ground-state transitions were deduced and compared to the literature. The photon scattering cross sections of two levels above the proton emission threshold, but still below other particle emission energies have also been measured, and proton resonance strengths and proton widths were deduced. Gamma and proton widths consistent with the literature values were obtained, but with greatly improved precision.

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Measurements of $^{152}$Gd(p,$γ$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reaction cross sections for the astrophysical $γ$ process

The total cross sections for the $^{152}$Gd(p,$γ$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reactions have been measured by the activation method at effective center-of-mass energies \mbox{$3.47 \leq E_\mathrm{c.m.}^\mathrm{eff}\leq 7.94$ MeV} and \mbox{$4.96 \leq E_\mathrm{c.m.}^\mathrm{eff} \leq 7.94$ MeV}, respectively. The targets were prepared by evaporation of 30.6\% isotopically enriched $^{152}$Gd oxide on aluminum backing foils, and bombarded with proton beams provided by a cyclotron accelerator. The cross sections were deduced from the observed $γ$-ray activity, which was detected off-line by a HPGe detector in a low background environment. The results are presented and compared with predictions of statistical model calculations. This comparison supports a modified optical proton+$^{152}$Gd potential suggested earlier.

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The 106Cd(alpha,alpha)106Cd elastic scattering in a wide energy range for gamma-process studies

Alpha elastic scattering angular distributions of the 106Cd(alpha,alpha)106Cd reaction were measured at three energies around the Coulomb barrier to provide a sensitive test for the alpha + nucleus optical potential parameter sets. Furthermore, the new high precision angular distributions, together with the data available from the literature were used to study the energy dependence of the locally optimized α+nucleus optical potential in a wide energy region ranging from E_Lab = 27.0 MeV down to 16.1 MeV. The potentials under study are a basic prerequisite for the prediction of alpha-induced reaction cross sections and thus, for the calculation of stellar reaction rates used for the astrophysical gamma process. Therefore, statistical model predictions using as input the optical potentials discussed in the present work are compared to the available 106Cd + alpha cross section data.

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$γ$ ray spectroscopy of $^{19}$C via single neutron knock-out reaction

The one neutron knock-out reaction $^1$H($^{20}$C,$^{19}$C$γ$) was studied at RIKEN using the DALI2 array. A $γ$ ray transition was observed at 198(10) keV. Based on the comparison between the experimental production cross section and theoretical predictions, the transition was assigned to the decay of the 3/2$_1^+$ state to the ground state.

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Test of statistical model cross section calculations for $α$-induced reactions on $^{107}$Ag at energies of astrophysical interest

Astrophysical reaction rates, which are mostly derived from theoretical cross sections, are necessary input to nuclear reaction network simulations for studying the origin of $p$ nuclei. Past experiments have found a considerable difference between theoretical and experimental cross sections in some cases, especially for ($α$,$γ$) reactions at low energy. Therefore, it is important to experimentally test theoretical cross section predictions at low, astrophysically relevant energies. The aim is to measure reaction cross sections of $^{107}$Ag($α$,$γ$)$^{111}$In and $^{107}$Ag($α$,n)$^{110}$In at low energies in order to extend the experimental database for astrophysical reactions involving $α$ particles towards lower mass numbers. Reaction rate predictions are very sensitive to the optical model parameters and this introduces a large uncertainty into theoretical rates involving $α$ particles at low energy. We have also used Hauser-Feshbach statistical model calculations to study the origin of possible discrepancies between prediction and data. An activation technique has been used to measure the reaction cross sections at effective center of mass energies between 7.79 MeV and 12.50 MeV. Isomeric and ground state cross sections of the ($α$,n) reaction were determined separately. The measured cross sections were found to be lower than theoretical predictions for the ($α$,$γ$) reaction. Varying the calculated averaged widths in the Hauser-Feshbach model, it became evident that the data for the ($α$,$γ$) and ($α$,n) reactions can only be simultaneously reproduced when rescaling the ratio of $γ$- to neutron width and using an energy-dependent imaginary part in the optical $α$+$^{107}$Ag potential.......

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KADoNiS-$p$: The astrophysical $p$-process database

The KADoNiS-$p$ project is an online database for cross sections relevant to the $p$-process. All existing experimental data was collected and reviewed. With this contribution a user-friendly database using the KADoNiS (Karlsruhe Astrophysical Database of Nucleosynthesis in Stars) framework is launched, including all available experimental data from (p,$γ$), (p,n), (p,$α$), ($α$,$γ$), ($α$,n) and ($α$,p) reactions in or close to the respective Gamow window with cut-off date of August 2012 (www.kadonis.org/pprocess).

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Nuclear structure studies of $^{24}$F

The structure of the $^{24}$F nucleus has been studied at GANIL using the $β$ decay of $^{24}$O and the in-beam $γ$-ray spectroscopy from the fragmentation of projectile nuclei. Combining these complementary experimental techniques, the level scheme of $^{24}$F has been constructed up to 3.6 Mev by means of particle-$γ$ and particle-$γγ$ coincidence relations. Experimental results are compared to shell-model calculations using the standard USDA and USDB interactions as well as ab-initio valence-space Hamiltonians calculated from the in-medium similarity renormalization group based on chiral two- and three-nucleon forces. Both methods reproduce the measured level spacings well, and this close agreement allows unidentified spins and parities to be consistently assigned.

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A new study of the $^{22}$Ne(p,$γ$)$^{23}$Na reaction deep underground: Feasibility, setup, and first observation of the 186 keV resonance

The $^{22}$Ne(p,$γ$)$^{23}$Na reaction takes part in the neon-sodium cycle of hydrogen burning. This cycle is active in asymptotic giant branch stars as well as in novae and contributes to the nucleosythesis of neon and sodium isotopes. In order to reduce the uncertainties in the predicted nucleosynthesis yields, new experimental efforts to measure the $^{22}$Ne(p,$γ$)$^{23}$Na cross section directly at the astrophysically relevant energies are needed. In the present work, a feasibility study for a $^{22}$Ne(p,$γ$)$^{23}$Na experiment at the Laboratory for Underground Nuclear Astrophysics (LUNA) 400\,kV accelerator deep underground in the Gran Sasso laboratory, Italy, is reported. The ion beam induced $γ$-ray background has been studied. The feasibility study led to the first observation of the $E_{\rm p}$ = 186\,keV resonance in a direct experiment. An experimental lower limit of 0.12\,$\times$\,10$^{-6}$\,eV has been obtained for the resonance strength. Informed by the feasibility study, a dedicated experimental setup for the $^{22}$Ne(p,$γ$)$^{23}$Na experiment has been developed. The new setup has been characterized by a study of the temperature and pressure profiles. The beam heating effect that reduces the effective neon gas density due to the heating by the incident proton beam has been studied using the resonance scan technique, and the size of this effect has been determined for a neon gas target.

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Direct study of the alpha-nucleus optical potential at astrophysical energies using the 64Zn(p,alpha)61Cu reaction

In the model calculations of heavy element nucleosynthesis processes the nuclear reaction rates are taken from statistical model calculations which utilize various nuclear input parameters. It is found that in the case of reactions involving alpha particles the calculations bear a high uncertainty owing to the largely unknown low energy alpha-nucleus optical potential. Experiments are typically restricted to higher energies and therefore no direct astrophysical consequences can be drawn. In the present work a (p,alpha) reaction is used for the first time to study the alpha-nucleus optical potential. The measured 64Zn(p,alpha)61Cu cross section is uniquely sensitive to the alpha-nucleus potential and the measurement covers the whole astrophysically relevant energy range. By the comparison to model calculations, direct evidence is provided for the incorrectness of global optical potentials used in astrophysical models.

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Alpha induced reaction cross section measurements on 162Er for the astrophysical gamma process

The cross sections of the 162Er(a,g,)166Yb and 162Er(a,n)165Yb reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m. = 16.09 down to Ec.m. = 11.21 MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The 162Er(a,n)165Yb reaction was studied above the reaction threshold between Ec.m. = 12.19 and 16.09 MeV. The fact that the 162Er(a,g)166Yb cross sections were measured below the (a,n) threshold at first time in this mass region opens the opportunity to study directly the a-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted.

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Cross section and reaction rate of 92Mo(p,gamma)93Tc determined from thick target yield measurements

For the better understanding of the astrophysical gamma-process the experimental determination of low energy proton- and alpha-capture cross sections on heavy isotopes is required. The existing data for the 92Mo(p,gamma)93Tc reaction are contradictory and strong fluctuation of the cross section is observed which cannot be explained by the statistical model. In this paper a new determination of the 92Mo(p,gamma)93Tc and 98Mo(p,gamma)99mTc cross sections based on thick target yield measurements are presented and the results are compared with existing data and model calculations. Reaction rates of 92Mo(p,gamma)93Tc at temperatures relevant for the gamma-process are derived directly from the measured thick target yields. The obtained rates are a factor of 2 lower than the ones used in astrophysical network calculations. It is argued that in the case of fluctuating cross sections the thick target yield measurement can be more suited for a reliable reaction rate determination.

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$^{110,116}$Cd($α,α$)$^{110,116}$Cd elastic scattering and systematic investigation of elastic $α$ scattering cross sections along the $Z$ = 48 isotopic and $N$ = 62 isotonic chains

The elastic scattering cross sections for the reactions $^{110,116}$Cd($α,α$)$^{110,116}$Cd at energies above and below the Coulomb barrier are presented to provide a sensitive test for the alpha-nucleus optical potential parameter sets. Additional constraints for the optical potential are taken from the analysis of elastic scattering excitation functions at backward angles which are available in literature. Moreover, the variation of the elastic alpha scattering cross sections along the $Z = 48$ isotopic and $N = 62$ isotonic chain is investigated by the study of the ratios of the of $^{106,110,116}$Cd($α,α$)$^{106,110,116}$Cd scattering cross sections at E$_{c.m.} \approx$ 15.6 and 18.8 MeV and the ratio of the $^{110}$Cd($α,α$)$^{110}$Cd and $^{112}$Sn($α,α$)$^{112}$Sn reaction cross sections at E$_{c.m.} \approx$ 18.8 MeV, respectively. These ratios are sensitive probes for the alpha-nucleus optical potential parameterizations. The potentials under study are a basic prerequisite for the prediction of $α$-induced reaction cross sections, e.g.\ for the calculation of stellar reaction rates in the astrophysical $p$- or $γ$-process.

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High precision $^{113}$In($α,α$)$^{113}$In elastic scattering at energies around the Coulomb barrier for the astrophysical $γ$ process

The $γ$ process in supernova explosions is thought to explain the origin of proton-rich isotopes between Se and Hg, the so-called $p$ nuclei. The majority of the reaction rates for $γ$ process reaction network studies has to be predicted in Hauser-Feshbach statistical model calculations using global optical potential parameterizations. While the nucleon+nucleus optical potential is fairly known, for the $α$+nucleus optical potential several different parameterizations exist and large deviations are found between the predictions calculated using different parameter sets. By the measurement of elastic $α$-scattering angular distributions at energies around the Coulomb barrier a comprehensive test for the different global $α$+nucleus optical potential parameter sets is provided. Between 20$^{\circ}$ and 175$^{\circ}$ complete elastic alpha scattering angular distributions were measured on the $^{113}$In \textit{p} nucleus with high precision at E$_{c.m.}$ = 15.59 and 18.82 MeV. The elastic scattering cross sections of the $^{113}$In($α$,$α$)$^{113}$In reaction were measured for the first time at energies close to the astrophysically relevant energy region. The high precision experimental data were used to evaluate the predictions of the recent global and regional $α$+nucleus optical potentials. Parameters for a local $α$+nucleus optical potential were derived from the measured angular distributions. Predictions for the reaction cross sections of $^{113}$In($α,γ$)$^{117}$Sb and $^{113}$In($α$,n)$^{116}$Sb at astrophysically relevant energies were given using the global and local optical potential parameterizations.

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Constraining the astrophysical origin of the p-nuclei through nuclear physics and meteoritic data

A small number of naturally occurring, proton-rich nuclides (the p-nuclei) cannot be made in the s- and r-process. Their origin is not well understood. Massive stars can produce p-nuclei through photodisintegration of pre-existing intermediate and heavy nuclei. This so-called gamma-process requires high stellar plasma temperatures and occurs mainly in explosive O/Ne burning during a core-collapse supernova. Although the gamma-process in massive stars has been successful in producing a large range of p-nuclei, significant deficiences remain. An increasing number of processes and sites has been studied in recent years in search of viable alternatives replacing or supplementing the massive star models. A large number of unstable nuclei, however, with only theoretically predicted reaction rates are included in the reaction network and thus the nuclear input may also bear considerable uncertainties. The current status of astrophysical models, nuclear input, and observational constraints is reviewed. After an overview of currently discussed models, the focus is on the possibility to better constrain those models through different means. Meteoritic data not only provide the actual isotopic abundances of the p-nuclei but can also put constraints on the possible contribution of proton-rich nucleosynthesis. The main part of the review focusses on the nuclear uncertainties involved in the determination of the astrophysical reaction rates required for the extended reaction networks used in nucleosynthesis studies. Experimental approaches are discussed together with their necessary connection to theory, which is especially pronounced for reactions with intermediate and heavy nuclei in explosive nuclear burning, even close to stability.

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