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arXiv · 1412.7087

Polarized neutron diffraction and X-ray magnetic circular dichroism study of Ru doped UCoGe

Michal Valiska·Jiri Pospisil·Anne Stunault·Yukiharu Takeda·Beatrice Gillon·Yoshinori Haga·Karel Prokes·Gwilherm Nenert·Tetsuo Okane·Hiroshi Yamagami·Laurent Chapon·Arsene Goukassov·Allain Cousson·Etsuji Yamamoto·Vladimir Sechovsky
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Abstract

We report on microscopic study of the ferromagnetism enhancement in the Ru doped ferromagnetic superconductor (FM SC) UCoGe. For that purpose, two single crystals with composition UCo0.97Ru0.03Ge and UCo0.88Ru0.12Ge were prepared. Both single crystals were investigated by polarized neutron diffraction (PND) at low temperatures in magnetic fields and the latter one also by the soft X-ray magnetic circular dichroism (XMCD) method. UCo0.96Ru0.03Ge and UCo0.88Ru0.12Ge have been found ordering ferromagnetically below the Curie temperature TC = 6 K and 8.5 K, respectively, which are considerable higher than TC = 3 K of UCoGe. The increase of TC is accompanied by enhancement of the spontaneous moment to ms = 0.11 mB/f.u. and ms = 0.21 mB/f.u., respectively. The analysis of the PND results assigns the ferromagnetism enhancement mainly to the growth of the orbital part of uranium 5 f moment. In contrast to the published results of PND study of the parent UCoGe, we have found parallel orientation of the U and Co moments in both doped compounds. Evolution of magnetic characteristics with Ru concentration is discussed within a scenario considering the varying 5 f-ligand hybridization as the key mechanism.

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Michal Valiska, Jiri Pospisil, Anne Stunault, Yukiharu Takeda, Beatrice Gillon, Yoshinori Haga, Karel Prokes, Gwilherm Nenert, Tetsuo Okane, Hiroshi Yamagami, Laurent Chapon, Arsene Goukassov, Allain Cousson, Etsuji Yamamoto, Vladimir Sechovsky. 2014-12-22. Polarized neutron diffraction and X-ray magnetic circular dichroism study of Ru doped UCoGe. https://arxiv.org/abs/1412.7087

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