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arXiv · 1503.01197

Tunable negative thermal expansion related with the gradual evolution of antiferromagnetic ordering in antiperovskite manganese nitrides Ag1-xNMn3+x (0<x<0.6)

J. C. Lin·P. Tong·W. Tong·S. Lin·B. S. Wang·W. H. Song·Y. M. Zou·Y. P. Sun
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Abstract

The thermal expansion and magnetic properties of antiperovskite manganese nitrides Ag1-xNMn3+x were reported. The substitution of Mn for Ag effectively broadens the temperature range of negative thermal expansion and drives it to cryogenic temperatures. As x increases, the paramagnetic (PM) to antiferromagnetic (AFM) phase transition temperature (TN) decreases. At x~0.2, the PM-AFM transition overlaps with the AFM to glass-like state transition. Above x=0.2, two new distinct magnetic transitions were observed: one occurs above room temperature from PM to ferromagnetic (FM), and the other one evolves at a lower temperature (T*) below which both AFM and FM orderings are involved. Further electron spin resonance measurement suggests that the broadened volume change near T* is closely related with the evolution of Γ5g AFM ordering.

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J. C. Lin, P. Tong, W. Tong, S. Lin, B. S. Wang, W. H. Song, Y. M. Zou, Y. P. Sun. 2015-03-04. Tunable negative thermal expansion related with the gradual evolution of antiferromagnetic ordering in antiperovskite manganese nitrides Ag1-xNMn3+x (0<x<0.6). https://doi.org/10.1063/1.4913663

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