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arXiv · 1609.08883

Frustrated magnetism in the Heisenberg pyrochlore antiferromagnets $A$Yb$_2$$X$$_4$ ($A$ = Cd, Mg, $X$ = S, Se)

Tomoya Higo·Kensuke Iritani·Mario Halim·Wataru Higemoto·Takashi U. Ito·Kentaro Kuga·Kenta Kimura·Satoru Nakatsuji
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Abstract

Our polycrystalline sample study on the Yb-based chalcogenide spinels $A$Yb$_2$$X_4$ ($A =$ Cd, Mg, $X =$ S, Se) has revealed frustrated magnetism due to the antiferromagnetically coupled Heisenberg spin on the pyrochlore lattice. Our crystal electric field analysis indicates the Yb ground state has nearly Heisenberg spins with a strong quantum character of the ground doublet. All the materials exhibit an antiferromagnetic order at 1.4-1.8 K, much lower temperature than the antiferromagnetic exchange coupling scale of $\sim 10$ K. The magnetic specific heat $C_{\rm M}$ shows a $T^{3}$ dependence, indicating the gapless feature in the Yb-based chalcogenide spinels. The magnetic entropy change much smaller than $R$ ln 2 below the N\'{e}el temperature and the small local magnetic field estimated from the $\mu$SR measurements strongly suggest the significantly reduced size of the ordered moment in comparison with the bare moment size 1.33 $\mu_{\rm B}$/Yb supporting strong fluctuations in the commensurate and incommensurate ordered states in CdYb$_2$S$_4$ and MgYb$_2$S$_4$, respectively.

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Tomoya Higo, Kensuke Iritani, Mario Halim, Wataru Higemoto, Takashi U. Ito, Kentaro Kuga, Kenta Kimura, Satoru Nakatsuji. 2016-09-28. Frustrated magnetism in the Heisenberg pyrochlore antiferromagnets $A$Yb$_2$$X$$_4$ ($A$ = Cd, Mg, $X$ = S, Se). https://doi.org/10.1103/physrevb.95.174443

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