Electrical, Thermal and Spectroscopic Characterization of Bulk Bi2Se3 Topological Insulator

Rabia Sultana; Geet Awana; Banabir Pal; P. K. Maheshwari; Monu Mishra; Govind Gupta; Anurag Gupta; S. Thirupathaiah; V. P. S. Awana

arXiv · 1703.05492

Electrical, Thermal and Spectroscopic Characterization of Bulk Bi2Se3 Topological Insulator

Rabia Sultana·Geet Awana·Banabir Pal·P. K. Maheshwari·Monu Mishra·Govind Gupta·Anurag Gupta·S. Thirupathaiah·V. P. S. Awana

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Abstract

We report electrical (angular magneto-resistance, and Hall), thermal (heat capacity) and spectroscopic (Raman, x-ray photo electron, angle resolved photo electron) characterization of bulk Bi2Se3 topological insulator, which is being is grown by self flux method through solid state reaction from high temperature (950C) melt and slow cooling (2C/hour) of constituent elements. Bi2Se3 exhibited metallic behaviour down to 5K. Magneto transport measurements revealed linear up to 400% and 30% MR at 5K under 14 Tesla field in perpendicular and parallel field direction respectively. We noticed that the magneto-resistance (MR) of Bi2Se3 is very sensitive to the angle of applied field. MR is maximum when the field is normal to the sample surface, while it is minimum when the field is parallel. Hall coefficient (RH) is seen nearly invariant with negative carrier sign down to 5K albeit having near periodic oscillations above 100K. Heat capacity (Cp) versus temperature plot is seen without any phase transitions down to 5K and is well fitted (Cp = gammaT + betaT3) at low temperature with calculated Debye temperature (ThetaD) value of 105.5K. Clear Raman peaks are seen at 72, 131 and 177 cm-1 corresponding to A1g1, Eg2 and A1g2 respectively. Though, two distinct asymmetric characteristic peak shapes are seen for Bi 4f7/2 and Bi 4f5/2, the Se 3d region is found to be broad displaying the overlapping of spin - orbit components of the same. Angle-resolved photoemission spectroscopy (ARPES) data of Bi2Se3 revealed distinctly the bulk conduction bands (BCB), surface state (SS), Dirac point (DP) and bulk valence bands (BVB) and 3D bulk conduction signatures are clearly seen. Summarily, host of physical properties for as grown Bi2Se3 crystal are reported here.

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Rabia Sultana, Geet Awana, Banabir Pal, P. K. Maheshwari, Monu Mishra, Govind Gupta, Anurag Gupta, S. Thirupathaiah, V. P. S. Awana. 2017-03-18. Electrical, Thermal and Spectroscopic Characterization of Bulk Bi2Se3 Topological Insulator. https://arxiv.org/abs/1703.05492

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