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arXiv · 2111.07710

Inducing and tuning Kondo screening in a narrow-electronic-band system

Shiwei Shen·Chenhaoping Wen·Pengfei Kong·Jingjing Gao·Jianguo Si·Xuan Luo·Wenjian Lu·Yu-Ping Sun·Gang Chen·Shichao Yan
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Abstract

Although the single-impurity Kondo physics has already been well understood, the understanding of the Kondo lattice problem where a dense array of local moments couples to the conduction electrons is still far from complete. The ability of creating and tuning the Kondo lattice in non-f-electron systems will be great helpful for further understanding the Kondo lattice behavior. Here we show that the Pb intercalation in the charge-density-wave-driven narrow-electronic-band system 1T-TaS2 induces a transition from the insulating gap to a sharp Kondo resonance in the scanning tunneling microscopy measurements. It results from the Kondo screening of the localized moment in the 13-site Star-of-David clusters of 1T-TaS2, and thus confirms the cluster Mott localization of the unpaired electrons and local moment formation in the 1T-TaS2 layer. As increasing the Pb concentration, the narrow electronic band derived from the localized electrons shifts away from the Fermi level and the Kondo resonance peak is gradually suppressed. Our results pave a way for creating and tuning many-body electronic states in layered narrow-electronic-band materials.

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Shiwei Shen, Chenhaoping Wen, Pengfei Kong, Jingjing Gao, Jianguo Si, Xuan Luo, Wenjian Lu, Yu-Ping Sun, Gang Chen, Shichao Yan. 2021-11-15. Inducing and tuning Kondo screening in a narrow-electronic-band system. https://doi.org/10.1038/s41467-022-29891-4

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