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arXiv · 2507.11494

Nuclear Spin-Mediated Relaxation Mechanisms of the V$_{B}^-$ Center in hBN

Chanaprom Cholsuk·Tobias Vogl·Viktor Ivády
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Abstract

The negatively charged boron vacancy $V_B^-$ defect in hexagonal boron nitride (hBN) has recently emerged as a promising spin qubit for sensing due to its high-temperature spin control and versatile integration into van der Waals structures. While extensive experiments have explored their coherence properties, much less is known about the spin relaxation time $T_1$ and its control-parameter dependence. In this work, we develop a parameter-free spin dynamics model based on the cluster-expansion technique to investigate $T_1$ relaxation mechanisms at low temperature. Our results reveal that the $V_B^-$ center constitutes a strongly coupled electron spin-nuclear spin core, which necessitates the inclusion of the coherent dynamics and derived memory effects of the three nearest-neighbor nitrogen nuclear spins. Using this framework, this work closely reproduces the experimentally observed $T_1$ time at $B = 90\,\mathrm{G}$ and further predicts the $T_1$ dependence on external magnetic field in the $0 \le B \le 2000\,\mathrm{G}$ interval, when the spin relaxation is predominantly driven by electron-nuclear and nuclear-nuclear flip-flop processes mediated by hyperfine and dipolar interactions. This study establishes a reliable and scalable approach for describing $T_1$ relaxation in $V_B^-$ centers and offers microscopic insights to support future developments in nuclear-spin-based quantum technologies.

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Chanaprom Cholsuk, Tobias Vogl, Viktor Ivády. 2025-07-15. Nuclear Spin-Mediated Relaxation Mechanisms of the V$_{B}^-$ Center in hBN. https://doi.org/10.1038/s41524-025-01859-0

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