Atomic clock frequency ratios with fractional uncertainty $\leq 3.2 \times 10^{-18}$

Abstract

We report high-precision frequency ratio measurements between optical atomic clocks based on $^{27}$Al$^+$, $^{171}$Yb, and $^{87}$Sr. With total fractional uncertainties at or below $3.2 \times 10^{-18}$, these measurements meet an important milestone criterion for redefinition of the second in the International System of Units. Discrepancies in $^{87}$Sr ratios at approximately $1\times10^{-16}$ and the Al$^+$/Yb ratio at $1.6\times10^{-17}$ in fractional units compared to our previous measurements underscore the importance of repeated, high-precision comparisons by different laboratories. A key innovation in this work is the use of a common ultrastable reference delivered to all clocks via a 3.6 km phase-stabilized fiber link between two institutions. Derived from a cryogenic single-crystal silicon cavity, this reference improves comparison stability by a factor of 2 to 3 over previous systems, with an optical lattice clock ratio achieving a fractional instability of $1.3 \times 10^{-16}$ at 1 second. By enabling faster comparisons, this stability will improve sensitivity to non-white noise processes and other underlying limits of state-of-the-art optical frequency standards.