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Quantum Theory of Spontaneous Emission from Exciton-Electron-Phonon Complex in Solid: Quantum Interference and Many-Body Effect

Shi-Jie Xiong·S. J. Xu
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Abstract

A full quantum mechanical theory for the spontaneous emission from excitons simultaneously coupled to electronic excitations and anharmonic phonons in solid is developed. Origin of detailed structures, such as zero-phonon line splitting, Fano lineshape near one phonon sideband, strong second-order phonon Stokes line, asymmetric phonon anti-Stokes lines, and two-electron satellites as well as their phonon replicas recently revealed in the low-temperature photoluminescence of ZnO, has been identified by quantitative calculations from the theory.

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Shi-Jie Xiong, S. J. Xu. 2007-02-24. Quantum Theory of Spontaneous Emission from Exciton-Electron-Phonon Complex in Solid: Quantum Interference and Many-Body Effect. https://arxiv.org/abs/cond-mat/0702544

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