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A. Pocar

Publications and source records attributed to A. Pocar.

At least 19 recordsLinked to original sources

Search for two-neutrino double electron capture in $^{36}$Ar with the DarkSide-50 detector

Two-neutrino double electron capture is a rare nuclear decay where two electrons are simultaneously captured from the atomic shells and two neutrinos are emitted. We report on the first search for two-neutrino double electron capture in the $\textit{KK}$- and $\textit{KL}$-shells of $^{36}$Ar using the low-radioactivity liquid argon target from underground sources in the DarkSide-50 experiment. No statistically significant excess was observed with approximately 12 ton-day exposure of underground argon (UAr) and, taking into account the $^{36}$Ar isotopic abundance in UAr (0.007%), we set a limit on the half-life of the two-electron capture process in $^{36}$Ar of $T_{1/2} > 9.2 \times 10^{19}$ yr at 90% C.L. The sensitivity of the DarkSide-20k experiment, which will become operational in the next few years, was also evaluated and is expected to increase by a factor $\sim$100 with 10 years of expected operation and assuming the same $^{36}$Ar abundance as in the DarkSide-50 underground argon target.

nucl-ex

New limits on the Pauli forbidden transitions in 12C nuclei obtained with the complete Borexino dataset

The Pauli exclusion principle (PEP) was tested for nucleons in $\rm{^{12}C}$ nuclei using the Borexino dataset from 2007 to 2021. %the complete Borexino detector data. The approach consists of searching for $\gamma$-quanta, neutrons, protons, as well as electrons and positrons emitted in non-Paulian transitions of nucleons from the $1P_{3/2}$ shell to the filled $1S_{1/2}$ shell. Due to the uniquely low background level, the large mass, and long measurement time of the Borexino detector, the most stringent experimental constraints to date on the lifetime of the $\rm{^{12}C}$ nucleus with respect to PEP-forbidden transitions were obtained: $\tau({^{12}\rm{C}}\rightarrow{^{12}\widetilde{\rm{C}}}+\gamma) \geq {1.1\times10^{32}}$ y, $\tau({^{12}\rm{C}}\rightarrow{^{11}\widetilde{\rm{B}}}+ p) \geq {1.0\times10^{31}}$ y, $\tau({^{12}\rm{C}}\rightarrow{^{11}\widetilde{\rm{C}}}+ n) \geq 2.0 \times 10^{31}$ y, $\tau({^{12}\rm{C}}\rightarrow{^{12}\widetilde{\rm{N}}}+ e^- + \widetilde{\nu_e}) \geq 6.4 \times 10^{30}$ y and $\tau({^{12}\rm{C}}\rightarrow{^{12}\widetilde{\rm{B}}}+ e^+ + \nu_e) \geq 6.6 \times 10^{30}$ y (90\% C.L.). The upper limits on the relative strengths for the non-Paulian electromagnetic, strong, and weak transitions have been obtained: $\delta^2_{\gamma}\leq 1.0\times 10^{-57}$, $\delta^2_{N}\leq 7.0\times 10^{-61}$ and $\delta^2_{\beta}\leq 9.6\times 10^{-36}$, all at 90\% C.L..

nucl-ex

Design of a high voltage delivery system for noble liquid time projection chambers

Noble liquid time projection chambers (TPCs) are a leading technology in the detection of ionizing radiation, particularly in applications such as accelerator neutrino physics, dark matter detection, and neutrinoless double beta decay. This paper addresses the design considerations for implementing stable high voltage (HV) systems within large noble liquid TPCs, with a focus on the nEXO experiment. Utilizing insights from prior HV research and experimental investigations, we outline factors influencing HV stability and discuss design choices to improve stability and prevent electrical discharges. A novel HV delivery system concept is presented, tailored for the nEXO TPC, which incorporates these design considerations while also meeting the stringent radiopurity requirements of the nEXO neutrinoless double beta decay search. These design considerations and their specific implementation towards a HV delivery system offer guidance to future experiments applying high voltage in noble liquid environments.

physics.ins-det

First Nuclear Ultra-Heavy Dark Matter Search in Argon Time Projection Chambers with the DarkSide-50 Experiment

We report the first search for nuclear ultra-heavy dark matter (UHDM) in a dual-phase liquid argon time projection chamber using the DarkSide-50 experiment. Unlike conventional weakly interacting massive particles (WIMPs), nuclear UHDM candidates may be composed of many dark nucleons and scatter numerous times while passing through the detector. Accounting for energy loss through the Earth's overburden, we apply selection criteria optimized for multi-scatter event topologies using the 532-day low-radiation campaign of the DarkSide-50 detector. Excluded limits on the UHDM-nucleon scattering cross section for dark nucleon masses of $m_\chi = 10, 50, 100, 500 \, \mathrm{GeV/c^2}$ are presented.

hep-ex

Constraints on non-standard neutrino interactions from Borexino extended data-set

Neutrino non-standard interactions (NSI) constitute an active research field, as they are closely related to potential new physics associated with dark matter searches and exotic interactions arising from fundamental symmetry violations. The Borexino's unprecedented sensitivity to solar neutrinos, derived from its low background and precision spectral measurements, enables stringent constraints on potential deviations from the standard three-flavor neutrino oscillation paradigm. This work presents an update on the analysis of flavor-diagonal NSI using the full Borexino Phase-III data set, extending the study previously reported in Constraints on flavor-diagonal non-standard neutrino interactions from Borexino Phase-II (JHEP 2020, 38). The updated analysis incorporates the extended temporal and statistical coverage of Phase-III. The results indicate improved sensitivity to the diagonal NSI parameters, with constraints exceeding those obtained in Phase-II. Furthermore, a more general analysis that includes all possible off-diagonal NSI terms is presented for the first time, providing a comprehensive exploration of the NSI parameter space associated with the flavors of the incoming and outgoing neutrinos. This work once again underlines Borexino's critical role in probing new physics scenarios and reinforces its legacy in neutrino research. Detailed comparisons with Phase-II results are discussed, along with implications for theoretical models of NSI.

hep-ex

Novel High-Radiopurity Doped Amorphous Silicon Resistors for Low-Background Detectors

We present the results of a study of lightly doped amorphous silicon used as a resistive medium for high-radiopurity resistors in nuclear and particle physics research instrumentation. Prototypes are produced for a Time Projection Chamber design for the nEXO neutrinoless double-beta decay search experiment that meet requirements for ultra-high radiopurity, good mechanical, cryogenic and high voltage performance, as well as useful vacuum ultraviolet (VUV) reflectivity. Further study is warranted to refine production methods and to confirm that the technology used here is useful for more general applications.

physics.ins-det

Characterization of CRYO ASIC for charge readout in the nEXO experiment

nEXO is a proposed next-generation experiment searching for the neutrinoless double beta decay of $^{136}$Xe using a tonne-scale liquid xenon (LXe) time projection chamber (TPC). To image the ionization signals from events in the liquid xenon, the detector will employ metallized fused-silica charge collection tiles instrumented with cryogenic application-specific integrated circuits (ASICs), referred to as CRYO ASIC, which are designed to operate directly in LXe to minimize input capacitance and pick-up noise. Here we present the performance of the CRYO ASIC mounted on an auxiliary printed circuit board and evaluated both in a cryogenic environmental chamber and in a dedicated LXe test stand. We demonstrate that the ASICs achieve the desired performance at liquid xenon temperatures, showing a gain stability better than 0.2% over 24-hour operation and reliable in-situ calibration using an on-chip pulser. In the LXe test stand, we show that boiling caused by the chip heat dissipation can be mitigated by operating the system above ~0.1 MPa. The in-LXe noise measured agrees with simulation, which indicates it the $150~e^-$ design requirement can be satisfied. These results establish CRYO ASIC as a viable low-noise in-LXe charge readout solution for nEXO.

physics.ins-det

Search for Double Beta Decays of $^{134}$Xe with EXO-200 Phase II

EXO-200 was a leading double beta decay experiment consisting of a single-phase, enriched liquid xenon time projection chamber filled with an admixture of 80.672% $^{136}$Xe and 19.098% $^{134}$Xe. The detector operated at WIPP between 2010 and 2018 and was designed to search for double beta decay of $^{136}$Xe. Data was acquired in two phases separated by a period of detector upgrades. We report on the search for $0\nu\beta\beta$ and $2\nu\beta\beta$ decay of $^{134}$Xe with Phase II EXO-200 data, with median 90% C.L. exclusion sensitivity $T_{1/2}^{0\nu} \geq 3.7\times 10^{23}$ yr and $T_{1/2}^{2\nu} \geq 2.6 \times 10^{21}$ yr, respectively. No statistically significant signal is observed for either decay mode. We set a world-leading lower limit on the half-life of the neutrinoless decay mode of $^{134}$Xe of $T_{1/2}^{0\nu} \geq 8.7\times10^{23}$ (90% C.L.) and the second strongest constraint on the two-neutrino decay of $T_{1/2}^{2\nu} \geq 2.9\times10^{21}$ (90% C.L.), a 3-fold improvement over the EXO-200 Phase I measurement. New constraints are also set for the $2\nu\beta\beta$ and $0\nu\beta\beta$ decays of $^{134}$Xe to the lowest excited state of $^{134}$Ba.

nucl-ex

Ultra-pure Nickel for Structural Components of Low-Radioactivity Instruments

The next generation of rare-event search experiments in nuclear and particle physics demand structural materials combining exceptional mechanical strength with ultra-low levels of radioactive contamination. This study evaluates chemical vapor deposition (CVD) nickel as a candidate structural material for such applications. Manufacturer-supplied CVD Ni grown on aluminum substrates underwent tensile testing before and after welding alongside standard Ni samples. CVD Ni exhibited a planar tensile strength of ~600 MPa, significantly surpassing standard nickel. However, welding and heat treatment were found to reduce the tensile strength to levels comparable to standard Ni, with observed porosity in the welds likely contributing to this reduction. Material assay via inductively coupled plasma mass spectrometry (ICP-MS) employing isotope-dilution produced measured bulk concentration of 232-Th, 238-U, and nat-K at the levels of ~70 ppq, <100 ppq, and ~900 ppt, respectively, which is the lowest reported in nickel. Surface-etch profiling uncovered higher concentrations of these contaminants extending ~10 micrometer beneath the surface, likely associated with the aluminum growth substrate. The results reported are compared to the one other well documented usage of CVD Ni in a low radioactive background physics research experiment and a discussion is provided on how the currently reported results may arise from changes in CVD fabrication or testing process. These results establish CVD Ni as a promising low-radioactivity structural material, while outlining the need for further development in welding and surface cleaning techniques to fully realize its potential in large-scale, low radioactive background rare-event search experiments.

nucl-ex

Enhanced sensitivity to trace $^{238}$U impurity of sapphire via coincidence neutron activation analysis

Sapphire has mechanical and electrical properties that are advantageous for the construction of internal components of radiation detectors such as time projection chambers and bolometers. However, it has proved difficult to assess its $\rm ^{232}Th$ and $\rm ^{238}U$ content down to the picogram per gram level. This work reports an experimental verification of a computational study that demonstrates $\gamma\gamma$ coincidence counting, coupled with neutron activation analysis (NAA), can reach ppt sensitivities. Combining results from $\gamma\gamma$ coincidence counting with those of earlier single-$\gamma$ counting based NAA shows that a sample of Saint Gobain sapphire has $\rm ^{232}Th$ and $\rm ^{238}U$ concentrations of $<0.26$ ppt and $<2.3$ ppt, respectively; the best constraints on the radiopurity of sapphire.

nucl-ex

Sensitivity of nEXO to $^{136}$Xe Charged-Current Interactions: Background-free Searches for Solar Neutrinos and Fermionic Dark Matter

We study the sensitivity of nEXO to solar neutrino charged-current interactions, $\nu_e + ^{136}$Xe$\rightarrow ^{136}$Cs$^* + e^-$, as well as analogous interactions predicted by models of fermionic dark matter. Due to the recently observed low-lying isomeric states of $^{136}$Cs, these interactions will create a time-delayed coincident signal observable in the scintillation channel. Here we develop a detailed Monte Carlo of scintillation emission, propagation, and detection in the nEXO detector to model these signals under different assumptions about the timing resolution of the photosensor readout. We show this correlated signal can be used to achieve background discrimination on the order of $10^{-9}$, enabling nEXO to make background-free measurements of solar neutrinos above the reaction threshold of 0.668 MeV. We project that nEXO could measure the flux of CNO solar neutrinos with a statistical uncertainty of 25%, thus contributing a novel and competitive measurement towards addressing the solar metallicity problem. Additionally, nEXO could measure the mean energy of the $^7$Be neutrinos with a precision of $\sigma \leq 1.5$ keV and could determine the survival probability of $^{7}$Be and $pep$ solar $\nu_e$ with precision comparable to state-of-the-art. These quantities are sensitive to the Sun's core temperature and to non-standard neutrino interactions, respectively. Furthermore, the strong background suppression would allow nEXO to search for for charged-current interactions of fermionic dark matter in the mass range $m_\chi$ = $0.668$-$7$ MeV with a sensitivity up to three orders of magnitude better than current limits.

nucl-ex

Fermionic sub-GeV Dark Matter from evaporating Primordial Black Holes at DarkSide-50

We present a search for boosted dark matter from Primordial Black Holes (PBH) evaporation using the DarkSide-50 ionization-signal-only dataset corresponding to the experiment's ($12202\pm180$) ${\rm kg\: d}$ exposure. We focus on evaporation of PBHs with masses in the range [$10^{14},\,10^{16}$] g producing Dirac fermionic dark matter particles with sub-GeV kinetic energy. These relativistic particles, with energies up to hundreds of MeV, can generate detectable signals for masses below $\mathcal{O}(100)$ MeV. The absence of a signal enables setting complementary limits to those derived from cosmological observations and direct detection searches for cosmic ray-boosted dark matter.

hep-ph

Ultra-sensitive radon assay using an electrostatic chamber in a recirculating system

Rare event searches such as neutrinoless double beta decay and Weakly Interacting Massive Particle detection require ultra-low background detectors. Radon contamination is a significant challenge for these experiments, which employ highly sensitive radon assay techniques to identify and select low-emission materials. This work presents the development of ultra-sensitive electrostatic chamber (ESC) instruments designed to measure radon emanation in a recirculating gas loop, for future lower background experiments. Unlike traditional methods that separate emanation and detection steps, this system allows continuous radon transport and detection. This is made possible with a custom-built recirculation pump. A Python-based analysis framework, PyDAn, was developed to process and fit time-dependent radon decay data. Radon emanation rates are given for various materials measured with this instrument. A radon source of known activity provides an absolute calibration, enabling statistically-limited minimal detectable activities of 20 $\mu$Bq. These devices are powerful tools for screening materials in the development of low-background particle physics experiments.

physics.ins-det

Imaging of single barium atoms in a second matrix site in solid xenon for barium tagging in a $^{136}$Xe double beta decay experiment

Neutrinoless double beta decay is one of the most sensitive probes for new physics beyond the Standard Model of particle physics. One of the isotopes under investigation is $^{136}$Xe, which would double beta decay into $^{136}$Ba. Detecting the single $^{136}$Ba daughter provides a sort of ultimate tool in the discrimination against backgrounds. Previous work demonstrated the ability to perform single atom imaging of Ba atoms in a single-vacancy site of a solid xenon matrix. In this paper, the effort to identify signal from individual barium atoms is extended to Ba atoms in a hexa-vacancy site in the matrix and is achieved despite increased photobleaching in this site. Abrupt fluorescence turn-off of a single Ba atom is also observed. Significant recovery of fluorescence signal lost through photobleaching is demonstrated upon annealing of Ba deposits in the Xe ice. Following annealing, it is observed that Ba atoms in the hexa-vacancy site exhibit antibleaching while Ba atoms in the tetra-vacancy site exhibit bleaching. This may be evidence for a matrix site transfer upon laser excitation. Our findings offer a path of continued research toward tagging of Ba daughters in all significant sites in solid xenon.

physics.atom-ph

Review of Neutron Yield from (${\alpha}$, n) Reactions: Data, Methods, and Prospects

Understanding the radiogenic neutron production rate through the (${\alpha}$, n) reaction is crucial in many areas of physics, including dark matter searches, neutrino studies, and nuclear astrophysics. In addition to its relevance for fundamental research, the (${\alpha}$, n) reaction also plays a significant role in nuclear energy technologies, for example by contributing to neutron production in subcritical systems using UO$_{2}$, as well as in applications such as medical physics. This review examines the current state of (${\alpha}$, n) yield calculations and neutron spectra, describes the computational tools used for their estimation, and discusses the available cross-section data. We explore the uncertainties affecting (${\alpha}$, n) yield estimations and propose a strategy to enhance their accuracy. Furthermore, this paper discusses and emphasizes the need for new measurements of (${\alpha}$, n) cross-sections for a variety of relevant materials. Such measurements are essential for improving neutron flux predictions, which are crucial for reducing uncertainties in sensitivity estimates for next-generation physics experiments operating in the keV--MeV range.

nucl-ex

Report from the Workshop on Xenon Detector $0\nu\beta\beta$ Searches: Steps Towards the Kilotonne Scale

These proceedings summarize the program and discussions of the ``Workshop on Xenon Detector $0\nu\beta\beta$ Searches: Steps Towards the Kilotonne Scale'' held on October 25-27 2023 at SLAC National Accelerator Laboratory. This workshop brought together experts from the communities of neutrinoless double-beta decay and dark matter detection, to discuss paths forward for the realization of monolithic experiments with xenon approaching the kilotonne scale.

nucl-ex

Novel techniques for alpha/beta pulse shape discrimination in Borexino

Borexino could efficiently distinguish between alpha and beta radiation in its liquid scintillator by the characteristic time profile of their scintillation pulse. This alpha/beta discrimination, first demonstrated at the tonne scale in the Counting Test Facility prototype, was used throughout the lifetime of the experiment between 2007 and 2021. With this method, alpha events are identified and subtracted from the beta-like solar neutrino events. This is particularly important in liquid scintillator as alpha scintillation is quenched many-fold. In Borexino, the prominent Po-210 decay peak was a background in the energy range of electrons scattered from Be-7 solar neutrinos. Optimal alpha-beta discrimination was achieved with a "multi-layer perceptron neural network", which its higher ability to leverage the timing information of the scintillation photons detected by the photomultiplier tubes. An event-by-event, high efficiency, stable, and uniform pulse shape discrimination was essential in characterising the spatial distribution of background in the detector. This benefited most Borexino measurements, including solar neutrinos in the \pp chain and the first direct observation of the CNO cycle in the Sun. This paper presents the key milestones in alpha/beta discrimination in Borexino as a term of comparison for current and future large liquid scintillator detectors

hep-ex

Final results of Borexino on CNO solar neutrinos

We report the first measurement of CNO solar neutrinos by Borexino that uses the Correlated Integrated Directionality (CID) method, exploiting the sub-dominant Cherenkov light in the liquid scintillator detector. The directional information of the solar origin of the neutrinos is preserved by the fast Cherenkov photons from the neutrino scattered electrons, and is used to discriminate between signal and background. The directional information is independent from the spectral information on which the previous CNO solar neutrino measurements by Borexino were based. While the CNO spectral analysis could only be applied on the Phase-III dataset, the directional analysis can use the complete Borexino data taking period from 2007 to 2021. The absence of CNO neutrinos has been rejected with >5{\sigma} credible level using the Bayesian statistics. The directional CNO measurement is obtained without an external constraint on the $^{210}$Bi contamination of the liquid scintillator, which was applied in the spectral analysis approach. The final and the most precise CNO measurement of Borexino is then obtained by combining the new CID-based CNO result with an improved spectral fit of the Phase-III dataset. Including the statistical and the systematic errors, the extracted CNO interaction rate is $R(\mathrm{CNO})=6.7^{+1.2}_{-0.8} \, \mathrm{cpd/100 \, tonnes}$. Taking into account the neutrino flavor conversion, the resulting CNO neutrino flux at Earth is $\Phi_\mathrm{CNO}=6.7 ^{+1.2}_{-0.8} \times 10^8 \, \mathrm{cm^{-2} s^{-1}}$, in agreement with the high metallicity Standard Solar Models. The results described in this work reinforce the role of the event directional information in large-scale liquid scintillator detectors and open up new avenues for the next-generation liquid scintillator or hybrid neutrino experiments.

hep-ex