arXiv subjects

Arun Paramekanti

Publications and source records attributed to Arun Paramekanti.

At least 37 records · Page 2Linked to original sources

arXiv2024

Probing octupolar hidden order via Janus impurities

Quantum materials with non-Kramers doublets are a fascinating venue to realize multipolar hidden orders. Impurity probes which break point group symmetries, such as implanted muons or substitutional impurities, split the non-Kramers degeneracy and exhibit a Janus-faced influence in such systems: they can destroy the very order they seek to probe. Here, we explore this duality in cubic osmate double perovskites which are candidates for exotic $d$-orbital octupolar order competing with quadrupolar states. Using {\it ab initio} computations, Landau theory, and Monte Carlo simulations, we show that Janus impurities induce local strain fields, nucleating quadrupolar puddles and suppressing the octupolar $T_c$. At the same time, strains mix the non-Kramers doublet with an excited magnetic triplet, creating parasitic dipole moments which directly expose the hidden octupolar order parameter. Our work unravels this Janus duality in recent impurity nuclear magnetic resonance (NMR) experiments, with important implications for uncovering hidden order in diverse multipolar materials.

cond-mat.str-el↗

arXiv2023

Nematic order in topological SYK models

We study a class of multi-orbital models based on those proposed by Venderbos, Hu, and Kane which exhibit an interplay of topology, interactions, and fermion incoherence. In the non-interacting limit, these models exhibit trivial and Chern insulator phases with Chern number $C \geq 1$ bands as determined by the relative angular momentum of the participating orbitals. These quantum anomalous Hall insulator phases are separated by topological transitions protected by crystalline rotation symmetry, featuring Dirac or quadratic band-touching points. Here we study the impact of Sachdev-Ye-Kitaev (SYK) type interactions on these lattice models. Given the random interactions, these models display `average symmetries' upon disorder averaging, including a charge conjugation symmetry, so they behave as interacting models in topological class $\mathbf{D}$ enriched by crystalline rotation symmetry. The phase diagram of this model features a non-Fermi liquid at high temperature and an `exciton condensate' with nematic transport at low temperature. We present results from the free-energy, spectral functions, and the anomalous Hall resistivity as a function of temperature and tuning parameters. Our results are broadly relevant to correlated topological matter in multiorbital systems, and may also be viewed, with a suitable particle hole transformation, as an exploration of strong interaction effects on mean-field topological superconductors.

cond-mat.str-el↗

arXiv2023

Proximate Dirac spin liquid in honeycomb lattice $J_1$-$J_3$ XXZ model: Numerical study and application to cobaltates

Recent theoretical and experimental work suggest that the honeycomb cobaltates, initially proposed as candidate Kitaev quantum magnets, are in fact described by a pseudospin-$1/2$ easy-plane spin Hamiltonian with nearest neighbor ferromagnetic (FM) exchange $J_1$ being frustrated by antiferromagnetic third-neighbor exchange $J_3$ and weaker compass anisotropies. Using exact diagonalization and density-matrix renormalization group (DMRG) calculations, we show that this model exhibits FM order at small $J_3/J_1$ and zig-zag (ZZ) order at large $J_3/J_1$, separated by an intermediate phase, which we label as $\widetilde{\mathrm{SL}}$. This $\widetilde{\mathrm{SL}}$ phase is shown to exhibit spin-liquid-like correlations in DMRG, although we cannot preclude weak broken symmetries, e.g. weak Ising type Néel order, given the limits on our explored system sizes. Using a modified parton mean field theory and variational Monte Carlo on Gutzwiller projected wavefunctions, we show that the optimal FM and ZZ orders as well as the intermediate $\widetilde{\mathrm{SL}}$ state are proximate to a `parent' Dirac spin liquid (SL). This Dirac SL is shown to capture the broad continuum in the temperature and magnetic field dependent terahertz spectroscopy of BaCo$_2$(AsO$_4$)$_2$, and the reported low temperature metallic thermal conductivity in Na$_2$Co$_2$TeO$_6$ and BaCo$_2$(AsO$_4$)$_2$ upon incorporating disorder induced broadening.

cond-mat.str-el↗

arXiv2023

Nematic phases and elastoresistivity from a multiorbital non-Fermi liquid

We propose and study a two-orbital lattice extension of the Sachdev-Ye-Kitaev model in the large-$N$ limit. The phase diagram of this model features a high temperature isotropic strange metal which undergoes a first-order thermal transition into a nematic insulator or a continuous thermal transition into nematic metal phase, separated by a tunable tricritical point. These phases arise from spontaneous partial orbital polarization of the multiorbital non-Fermi liquid. We explore the spectral and transport properties of this model, including the d.c. elastoresistivity, which exhibits a peak near the nematic transition, as well as the nonzero frequency elastoconductivity. Our work offers a useful perspective on nematic phases and transport in correlated multiorbital systems.

cond-mat.str-el↗

arXiv2023

Impact of gapped spin-orbit excitons on low energy pseudospin exchange interactions

The quest for exotic quantum magnetic ground states, including the Kitaev spin liquid and quantum spin-ices, has led to the discovery of several quantum materials where low energy pseudospin-$1/2$ doublets arise from the splitting of spin-orbit entangled multiplets with higher degeneracy. Such systems include $d$-orbital and $f$-orbital Mott insulators. When the gap between the low energy pseudospin-$1/2$ levels and the excited levels of the multiplet or `excitons' is not large, the effective low-energy exchange interactions between the low energy pseudospin-$1/2$ moments can acquire significant corrections from coupling to the excitons. We extract these corrections using higher order perturbation theory as well as an exact Schrieffer-Wolff transformation. Such corrections can impact the exchange matrix for the low energy pseudospin-$1/2$ levels by renormalizing the strength and the sign of Heisenberg exchange or Ising anisotropies, and potentially even inducing bond-anisotropic couplings such as Kitaev-$Γ$ exchange interactions. We discuss recent experiments on various cobaltate and osmate materials which hint at the ubiquity and importance of this physics.

cond-mat.str-el↗

arXiv2022

Krein-unitary Schrieffer-Wolff transformation and band touchings in bosonic Bogoliubov-de Gennes and other Krein-Hermitian Hamiltonians

Krein-Hermitian Hamiltonians, i.e., Hamiltonians Hermitian with respect to an indefinite inner product, have emerged as an important class of non-Hermitian Hamiltonians in physics, encompassing both single-particle bosonic Bogoliubov-de Gennes (BdG) Hamiltonians and so-called "$PT$-symmetric" non-Hermitian Hamiltonians. In particular, they have attracted considerable scrutiny owing to the recent surge in interest for boson topology. Motivated by these developments, we formulate a perturbative Krein-unitary Schrieffer-Wolff transformation for finite-size dynamically stable Krein-Hermitian Hamiltonians, yielding an effective Hamiltonian for a subspace of interest. The effective Hamiltonian is Krein Hermitian and, for sufficiently small perturbations, also dynamically stable. As an application, we use this transformation to justify codimension-based analyses of band touchings in bosonic BdG Hamiltonians, which complement topological characterization. We use this simple approach based on symmetry and codimension to revisit known topological magnon band touchings in several materials of recent interest.

cond-mat.str-el↗

arXiv2022

Chiral Broken Symmetry Descendants of the Kagomé Lattice Chiral Spin Liquid

The breaking of chiral and time-reversal symmetries provides a pathway to exotic quantum phenomena and topological phases. In particular, the breaking of chiral (mirror) symmetry in quantum materials has been shown to have important technological applications. Recent work has extensively explored the resulting emergence of chiral charge orders and chiral spin liquids on the kagomé lattice. Such chiral spin liquids are closely tied to bosonic fractional quantum Hall states and host anyonic quasiparticles; however, their connection to nearby magnetically ordered states has remained a mystery. Here, we show that two distinct non-coplanar magnetic orders with uniform spin chirality, the XYZ umbrella state and the Octahedral spin crystal, emerge as competing orders in close proximity to the kagomé chiral spin liquid. Our results highlight the intimate link between a many-body topologically ordered liquid and broken symmetry states with nontrivial real-space topology.

cond-mat.str-el↗

arXiv2022

Exchange interactions and spin dynamics in the layered honeycomb ferromagnet CrI$_3$

We derive the microscopic spin Hamiltonian for rhombohedral CrI$_3$ using extensive first-principles density functional theory (DFT) calculations which incorporate spin-orbit coupling and Hubbard U. Our calculations indicate a dominant nearest-neighbor ferromagnetic Heisenberg exchange with weaker further-neighbor Heisenberg terms. In addition, we find a Dzyaloshinskii-Moriya interaction which primarily drives a topological gap in the spin-wave spectrum at the Dirac point, and uncover a non-negligible antiferromagnetic Kitaev coupling between the S=3/2 Cr moments. The out-of-plane magnetic moment is stabilized by weak symmetric bond-dependent terms and a local single-ion anisotropy. Using linear spin wave theory, we find that our exchange parameters are in reasonably good agreement with inelastic neutron scattering (INS) experiments. Employing classical Monte Carlo simulations, we study the magnetic phase transition temperature $T_c$ and its evolution with an applied in-plane magnetic field. We further demonstrate how future high-resolution INS experiments on the magnon dispersion of single crystals in an in-plane magnetic field may be used to quantitatively extract the strength of the antiferromagnetic Kitaev exchange coupling.

cond-mat.str-el↗

arXiv2022

Magnetic skyrmion crystal at a topological insulator surface

We consider a magnetic skyrmion crystal formed at the surface of a topological insulator. Incorporating the exchange interaction between the helical Dirac surface states and the periodic Néel or Bloch skyrmion texture, we obtain the resulting electronic band structure and discuss the constraints that symmetries impose on the energies and Berry curvature. We find substantive qualitative differences between the Néel and Bloch cases, with the latter generically permitting a multiband low energy tight-binding representation whose parameters are tightly constrained by symmetries. We explicitly compute the associated Wannier orbitals, which resemble the ringlike chiral bound states of helical Dirac fermions coupled to a single skyrmion in a ferromagnetic background. We construct a two-band tight-binding model with real nearest-neighbor hoppings which captures the salient topological features of the low-energy bands. Our results are relevant to magnetic topological insulators (TIs), as well as to TI-magnetic thin film heterostructures, in which skyrmion crystals may be stabilized.

cond-mat.mes-hall↗

arXiv2021

XY magnetism, Kitaev exchange, and long-range frustration in the $J_{\rm eff}=1/2$ honeycomb cobaltates

The quest for Kitaev quantum spin liquids has led to great interest in honeycomb quantum magnets with strong spin-orbit coupling. It has been recently proposed that even Mott insulators with $3d$ transition metal ions, having nominally weak spin-orbit coupling, can realize such exotic physics. Motivated by this, we study the rhombohedral honeycomb cobaltates CoTiO$_3$, BaCo$_2$(PO$_4$)$_2$, and BaCo$_2$(AsO$_4$)$_2$, using $\textit{ab initio}$ density functional theory, which takes into account realistic crystal field distortions and chemical information, in conjunction with exact diagonalization numerics. We show that these Co$^{2+}$ magnets host $j_\text{eff}=1/2$ local moments with highly anisotropic $g$-factors, and we extract their full spin Hamiltonians including longer-range and anisotropic exchange couplings. For CoTiO$_3$, we find a nearest-neighbor easy-plane ferromagnetic $XXZ$ model with additional bond-dependent anisotropies and interlayer exchange, which supports three-dimensional (3D) Dirac nodal line magnons. In contrast, for BaCo$_2$(PO$_4$)$_2$ and BaCo$_2$(AsO$_4$)$_2$, we find a strongly suppressed interlayer coupling, and significant frustration from additional third-neighbor antiferromagnetic exchange mediated by P/As. Such bond-anisotropic $J_1$-$J_3$ spin models can support collinear zig-zag or coplanar spiral ground states; we discuss their dynamical spin correlations which reveal a gapped Goldstone mode, and argue that the effective parameters of these pseudospin-$1/2$ models may be strongly renormalized by coupling to a low energy spin-exciton. Our results call for re-examining proposals for realizing Kitaev spin liquids in the honeycomb cobaltates.

cond-mat.str-el↗

arXiv2021

Octupolar order and Ising quantum criticality tuned by strain and dimensionality: Application to $d$-orbital Mott insulators

Recent experiments have discovered multipolar orders in a variety of $d$-orbital Mott insulators. Motivated by uncovering the exchange interactions which underlie octupolar order proposed in the osmate double perovskites, we study a two-site model using exact diagonalization on a five-orbital Hamiltonian, incorporating spin-orbit coupling (SOC) and interactions, and including both intra-orbital and inter-orbital hopping. Using an exact Schrieffer-Wolff transformation, we then extract an effective pseudospin Hamiltonian for the non-Kramers doublets, uncovering dominant ferrooctupolar coupling driven by the interplay of two distinct intra-orbital hopping terms. Using classical Monte Carlo simulations on the face-centered cubic lattice, we obtain a ferrooctupolar transition temperature which is in good agreement with experiments on the osmate double perovskites. We also explore the impact of uniaxial strain and dimensional tuning via ultrathin films, which are shown to induce a transverse field on the Ising octupolar order. This suppresses $T_c$ and potentially allows one to access octupolar Ising quantum critical points. We discuss possible implications of our results for a broader class of materials which may host such non-Kramers doublet ions.

cond-mat.str-el↗

arXiv2021

Higher-order topology and corner triplon excitations in two-dimensional quantum spin-dimer models

The concept of free fermion topology has been generalized to $d$-dimensional phases that exhibit $(d-n)$-dimensional boundary modes, such as zero-dimensional (0D) corner excitations. Motivated by recent extensions of these ideas to magnetic systems, we consider 2D quantum paramagnets formed by interacting spin dimers with dispersive triplet excitations. We propose two examples of such dimer models, where the spin-gapped bosonic triplon excitations are shown to host bands with nontrivial higher-order topology. We demonstrate this using real-space Bogoliubov--de Gennes calculations that reveal the existence of mid-bandgap corner triplon modes as a signature of higher-order bulk topology. We provide an understanding of the higher-order topology in these systems via a computation of bulk topological invariants as well as the construction of edge theories, and study their phase transitions as we tune parameters in the model Hamiltonians. We also discuss possible experimental approaches for detecting the emergent corner triplon modes.

cond-mat.str-el↗

arXiv2021

Tuning the nontrivial topological properties of the Weyl semimetal CeAlSi

In the ferromagnetic Weyl semimetal CeAlSi both space-inversion and time-reversal symmetries are broken. We use external pressure as an effective tuning parameter and relate three observations to the presence of a nontrivial topology in its ferromagnetic regime: an exceptional temperature response of the quantum oscillations amplitude, the presence of an anomalous Hall effect (AHE), and the existence of an unusual loop Hall effect (LHE). We find a suppression of the AHE and the LHE with increasing pressure, while the Curie temperature is enhanced. The magnetic structure and the electronic bands exhibit only a negligible pressure effect suggesting the importance of the domain wall landscape for the topological behavior in CeAlSi.

cond-mat.mtrl-sci↗

arXiv2021

Resonant optical topological Hall conductivity from skyrmions

We study the high frequency Hall conductivity in a two-dimensional (2D) model of conduction electrons coupled to a background magnetic skyrmion texture via an effective Hund's coupling term. For an ordered skyrmion crystal, a Kubo formula calculation using the basis of skyrmion crystal Chern bands reveals a resonant Hall response at a frequency set by the Hund's coupling: $\hbarω_{\text{res}} \approx J_H$. A complementary real-space Kubo formula calculation for an isolated skyrmion in a box reveals a similar resonant Hall response. A linear relation between the area under the Hall resonant curve and the skyrmion density is discovered numerically and is further elucidated using a gradient expansion which is valid for smooth textures and a local approximation based on a spin-trimer calculation. We point out the issue of distinguishing this skyrmion contribution from a similar feature arising from spin-orbit interactions, as demonstrated in a model for Rashba spin-orbit coupled electrons in a collinear ferromagnet, which is analogous to the difficulty of unambiguously separating the d.c. topological Hall effect from the anomalous Hall effect. The resonant feature in the high frequency topological Hall effect is proposed to provide a potentially useful local optical signature of skyrmions via probes such as scanning magneto-optical Kerr microscopy.

cond-mat.mes-hall↗

arXiv2021

Tunable skyrmion crystals and topological quantum oscillations in magnetic metals

Skyrmions are spatially localized magnetic swirls which carry a nonzero integer topological charge. We study crystals of skyrmions in a two-dimensional ferromagnet model with chiral interactions induced by the presence of broken inversion symmetry. We show that non-linear quartic mode-coupling terms allowed by symmetry enhances the Zeeman-field range over which the skyrmion-crystal phase remains stable. Furthermore, it leads to a significant dependence of the lattice constant of this spin crystal over this wide field range. Conduction electrons coupled to such a tunable spin crystal are shown to experience a Berry-flux density which varies with the Zeeman field. Such tunable skyrmion crystals provide a distinct realization of a Berry-Hofstadter butterfly, resulting in a phenomenon we term "topological quantum oscillations" in the electronic density of states and associated observables.

cond-mat.str-el↗

arXiv2021

Molecular dipoles in designer honeycomb lattices

Recent advances in ultracold atoms in optical lattices and developments in surface science have allowed for the creation of artificial lattices as well as the control of many-body interactions. Such systems provide new settings to investigate interaction-driven instabilities and non-trivial topology. In this paper, we explore the interplay between molecular electric dipoles on a two-dimensional triangular lattice with fermions hopping on the dual decorated honeycomb lattice which hosts Dirac and flat band states. We show that short-range dipole-dipole interaction can lead to ordering into various stripe and vortex crystal ground states. We study these ordered states and their thermal transitions as a function of the interaction range using simulated annealing and Monte Carlo methods. For the special case of zero wave vector ferrodipolar order, incorporating dipole-electron interactions and integrating out the electrons leads to a six-state clock model for the dipole ordering. Finally, we discuss the impact of the various dipole orders on the electronic band structure and the local tunneling density of states. Our work may be relevant to studies of "molecular graphene" -- CO molecules arranged on the Cu(111) surface -- which have been explored using scanning tunneling spectroscopy, as well as ultracold molecule-fermion mixtures in optical lattices.

cond-mat.str-el↗

arXiv2021

Nematic order driven by superconducting correlations

The interplay of nematicity and superconductivity has been observed in a wide variety of quantum materials. To explore this interplay, we consider a two-dimensional (2D) array of nematogens, local droplets with $Z_3$ nematicity, coupled to a network of Josephson junction wires. Using finite temperature classical Monte Carlo simulations, we elucidate the phase diagram of this model and show that the development of superconducting correlations and the directional delocalization of Cooper pairs can promote nematogen ordering, resulting in long-range nematic order. We obtain the transport properties of our model within an effective resistor network picture. We discuss these ideas in the context of the 2D electron gas at the (111) KTaO$_3$ interface and the doped topological insulators Nb$_x$Bi$_2$Se$_3$ and Cu$_x$Bi$_2$Se$_3$. Our work makes contact with Phil Anderson's numerous contributions to broken symmetries driven by the saving of kinetic energy, including double exchange ferromagnetism and the interlayer tunneling theory of high $T_c$ superconductivity.

cond-mat.supr-con↗

arXiv2021

Domain wall skew scattering in ferromagnetic Weyl metals

We study transport in the presence of magnetic domain walls (DWs) in a lattice model of ferromagnetic type-I Weyl metals. We compute the diagonal and Hall conductivities in the presence of a DW, using both Kubo and Landauer formalisms, and uncover the effect of DW scattering. When the Fermi level lies near Weyl points, we find a strong skew scattering at the DW which leads to a significant additional Hall effect. We estimate the average Hall resistivity for multi-domain configurations and identify the limit where the DW scattering contribution becomes significant. We show that a continuum model obtained by linearizing the lattice dispersion around the Weyl points does not correctly capture this DW physics. Going beyond the linearized theory, and incorporating leading curvature terms, leads to a semi-quantitative agreement with our lattice model results. Our results are relevant for experiments on the Hall resistivity of spin-orbit coupled ferromagnets, which can have Weyl points near the Fermi energy.

cond-mat.mes-hall↗