Searcharxiv⌕ Search

arXiv subjects

Bhaskaran Muralidharan

Publications and source records attributed to Bhaskaran Muralidharan.

At least 91 records · Page 5Linked to original sources

Landauer-Büttiker approach for hyperfine mediated electronic transport in the integer quantum Hall regime

The interplay of spin-polarized electronic edge states with the dynamics of the host nuclei in quantum Hall systems presents rich and non-trivial transport physics. Here, we develop a Landauer-Büttiker approach to understand various experimental features observed in the integer quantum Hall set ups featuring quantum point contacts. The approach developed here entails a phenomenological description of spin resolved inter-edge scattering induced via hyperfine assisted electron-nuclear spin flip-flop processes. A self-consistent simulation framework between the nuclear spin dynamics and edge state electronic transport is presented in order to gain crucial insights into the dynamic nuclear polarization effects on electronic transport and in turn the electron-spin polarization effects on the nuclear spin dynamics. In particular, we show that the hysteresis noted experimentally in the conductance-voltage trace as well as in the resistively detected NMR lineshape results from a lack of quasi-equilibrium between electronic transport and nuclear polarization evolution. In addition, we present circuit models to emulate such hyperfine mediated transport effects to further facilitate a clear understanding of the electronic transport processes occurring around the quantum point contact. Finally, we extend our model to account for the effects of quadrupolar splitting of nuclear levels and also depict the electronic transport signatures that arise from single and multi-photon processes.

cond-mat.mes-hall↗

Eliminating reservoir density-of-states fingerprints in Coulomb blockade spectroscopy

The differential conductance map of a single electron transistor (SET) provides information about a variety of parameters related to (quantum) dots, relevant for semiconductor-based quantum computing schemes. However, in ultra-scaled device architectures, identification of excited-state resonances of the quantum dot in the conductance map is often complicated by the appearance of features due to non-uniform density-of-states (DOS) of the source and drain reservoirs of the SET. Here, we demonstrate theoretically that the pump-probe spectroscopic technique, originally introduced by Fujisawa et al., allows the fingerprint of the reservoir-DOS to be completely suppressed while preserving the visibility of the excited state resonances. We also propose a specific approach for performing DC Coulomb blockade spectroscopy, which can effectively eliminate the DOS-related features. The advantages and limitations of the two approaches are investigated in detail. The results demonstrated here may provide an important optimization capability for emerging proposals of computer-automated control of large arrays of coupled but independently controlled charge and spin qubits.

cond-mat.mes-hall↗

Classical information driven quantum dot thermal machines

We analyze the transient response of quantum dot thermal machines that can be driven by hyperfine interaction acting as a source of classical information. Our setup comprises a quantum dot coupled to two contacts that drive heat flow while coupled to a nuclear spin bath. The quantum dot thermal machines operate both as batteries and as engines, depending on the parameter range. The electrons in the quantum dot interact with the nuclear spins via hyperfine spin-flip processes as typically seen in solid state systems such as GaAs quantum dots. The hyperfine interaction in such systems, which is often treated as a deterrent for quantum information processing, can favorably be regarded as a driving agent for classical information flow into a heat engine setup. We relate this information flow to Landauer's erasure of the nuclear spin bath, leading to a battery operation. We further demonstrate that the setup can perform as a transient power source even under a voltage bias across the dot. Focusing on the transient thermoelectric operation, our analysis clearly indicates the role of Landauer's erasure to deliver a higher output power than a conventional quantum dot thermoelectric setup and an efficiency greater than that of an identical Carnot cycle in steady state, which is consistent with recently proposed bounds on efficiency for systems subject to a feedback controller. The role of nuclear spin relaxation processes on these aspects is also studied. Finally, we introduce the Coulomb interaction in the dot and analyze the transient thermoelectric response of the system. Our results elaborate on the effective use of somewhat undesirable scattering processes as a non-equilibrium source of Shannon information flow in thermal machines and the possibilities that may arise from the use of a quantum information source.

cond-mat.mes-hall↗

Scaling Projections on Spin Transfer Torque Magnetic Tunnel Junctions

We investigate scaling of technologically relevant magnetic tunnel junction devices in the trilayer and pentalayer configurations by varying the cross-sectional area along the transverse direction using the non-equilibrium Green's function spin transport formalism. We study the geometry dependence by considering square and circular cross-sections. As the transverse dimension in each case reduces, we demonstrate that the transverse mode energy profile plays a major role in the resistance-area product. Both types of devices show constant tunnel magnetoresistance at larger cross-sectional areas but achieve ultra-high magnetoresistance at small cross-sectional areas, while maintaining low resistance-area products. We notice that although the critical switching voltage for switching the magnetization of the free layer nanomagnet in the trilayer case remains constant at larger areas, it needs more energy to switch at smaller areas. In the pentalayer case, we observe an oscillatory behavior at smaller areas as a result of double barrier tunneling. We also describe how switching characteristics of both kinds of devices are affected by the scaling.

cond-mat.mes-hall↗

Speeding up Thermalisation via Open Quantum System Variational Optimisation

Optimizing open quantum system evolution is an important step on the way to achieving quantum computing and quantum thermodynamic tasks. In this article, we approach optimisation via variational principles and derive an open quantum system variational algorithm explicitly for Lindblad evolution in Liouville space. As an example of such control over open system evolution, we control the thermalisation of a qubit attached to a thermal Lindbladian bath with a damping rate $γ$. Since thermalisation is an asymptotic process and the variational algorithm we consider is for fixed time, we present a way to discuss the potential speedup of thermalisation that can be expected from such variational algorithms.

quant-ph↗

Incoherent scattering can favorably influence energy filtering in nanostructured thermoelectrics

Investigating in detail the physics of energy filtering through a single planar energy barrier in nanostructured thermoelectric generators, we reinforce the non-trivial result that the anticipated enhancement in generated power at a given efficiency via energy filtering is a characteristic of systems dominated by incoherent scattering and is absent in ballistic devices. In such cases, assuming an energy dependent relaxation time $τ(E)=kE^r$, we show that there exists a minimum value $r_{min}$ beyond which generation can be enhanced by embedding nanobarriers. For bulk generators with embedded nanobarriers, we delve into the details of inter sub-band scattering and show that it has finite contribution to the enhancement in generation. We subsequently discuss the realistic aspects, such as the effect of smooth transmission cut-off and show that for $r>r_{min}$, the optimized energy barrier is just sufficiently wide enough to scatter off low energy electrons, a very wide barrier being detrimental to the performance. Analysis of the obtained results should provide general design guidelines for enhancement in thermoelectric generation via energy filtering. Our non-equilibrium approach is typically valid in the absence of local quasi-equilibrium and hence sets the stage for future advancements in thermoelectric device analysis, for example, Peltier cooling near a barrier interface.

cond-mat.mes-hall↗

Thermoelectric cooling and thermal switching via the non-linear phonon Peltier effect

Investigating the non-linear transport regime in a quantum dot heat engine described by the Anderson-Holstein model, it is shown that a finite electron-phonon interaction leads to a charge induced phonon generation that stimulates a phonon current even in the absence of a thermal gradient. This gives rise to the non-linear phonon Peltier effect which shows a non-trivial dependence on varying the electron-phonon interaction. Utilizing the reversal of phonon currents via charge induced phonon accumulation, we demonstrate that the heat engine surprisingly can be cooled when coupled to a hot reservoir. In further exploring possibilities that can arise from this effect, we propose a charge-induced phonon switching mechanism.

cond-mat.mes-hall↗

Superior thermoelectric performance via "anti-reflection" enabled double-barrier structures

We demonstrate theoretically using the atomistic non-equilibrium Green's function formalism with the inclusion of self-consistent charging, the design of a superior thermoelectric generator based on an "anti-reflection" coated double barrier resonant tunnelling diode. Unlike a typical double barrier device, we show that enabling the anti-reflection design facilitates a "boxcar" type feature in its transmission spectrum, which significantly enhances the thermoelectric performance. It is demonstrated that the best operating regime of this device offers a maximum power in the range of $0.7$ to $0.9 MW/m^{2}$ at efficiencies ranging from $46$ to $54\%$ of Carnot efficiency. The physics of charge and heat transport in the ballistic regime of operation helps us gain additional insights on how a large number of transverse current carrying modes boost the output power and simultaneously how the diminishing effects of high-energy parasitic currents aid the efficiency. Finally, a comparative study with a conventional double barrier thermoelectric is presented in terms of standard performance parameters which clearly reveals the performance benefits of enabling an anti-reflection coating.

physics.app-ph↗

A Bayesian view of Single-Qubit Clocks, and an Energy versus Accuracy tradeoff

We bring a Bayesian approach to the analysis of clocks. Using exponential distributions as priors for clocks, we analyze how well one can keep time with a single qubit freely precessing under a magnetic field. We find that, at least with a single qubit, quantum mechanics does not allow exact timekeeping, in contrast to classical mechanics which does. We find the design of the single-qubit clock that leads to maximum accuracy. Further, we find an energy versus accuracy tradeoff --- the energy cost is at least $k_BT$ times the improvement in accuracy as measured by the entropy reduction in going from the prior distribution to the posterior distribution. We propose a physical realization of the single qubit clock using charge transport across a capacitively-coupled quantum dot.

cond-mat.stat-mech↗

Resonant spin transfer torque nano-oscillators

Spin transfer torque nano-oscillators are potential candidates for replacing the traditional inductor based voltage controlled oscillators in modern communication devices. Typical oscillator designs are based on trilayer magnetic tunnel junctions which are disadvantaged by low power outputs and poor conversion efficiencies. In this letter, we theoretically propose to use resonant spin filtering in pentalayer magnetic tunnel junctions as a possible route to alleviate these issues and present device designs geared toward a high microwave output power and an efficient conversion of the d.c. input power. We attribute these robust qualities to the resulting non-trivial spin current profiles and the ultra high tunnel magnetoresistance, both arising from resonant spin filtering. The device designs are based on the nonequilibrium Green's function spin transport formalism self-consistently coupled with the stochastic Landau-Lifshitz-Gilbert-Slonczewski's equation and the Poisson's equation. We demonstrate that the proposed structures facilitate oscillator designs featuring a large enhancement in microwave power of around $775\%$ and an efficiency enhancement of over $1300\%$ in comparison with typical trilayer designs. We also rationalize the optimum operating regions via an analysis of the dynamic and static device resistances. This work sets stage for pentalyer spin transfer torque nano-oscillator device designs that extenuate most of the issues faced by the typical trilayer designs.

cond-mat.mes-hall↗

Thermoelectric study of dissipative quantum dot heat engines

This paper examines the thermoelectric response of a dissipative quantum dot heat engine based on the Anderson-Holstein model in two relevant operating limits: (i) when the dot phonon modes are out of equilibrium, and (ii) when the dot phonon modes are strongly coupled to a heat bath. In the first case, a detailed analysis of the physics related to the interplay between the quantum dot level quantization, the on-site Coulomb interaction and the electron-phonon coupling on the thermoelectric performance reveals that an n-type heat engine performs better than a p-type heat engine. In the second case, with the aid of the dot temperature estimated by incorporating a {\it{thermometer bath}}, it is shown that the dot temperature deviates from the bath temperature as electron-phonon interaction becomes stronger. Consequently, it is demonstrated that the dot temperature controls the direction of phonon heat currents, thereby influencing the thermoelectric performance. Finally, the conditions on the maximum efficiency with varying phonon couplings between the dot and all the other macroscopic bodies are analyzed in order to reveal the nature of the optimum junction.

cond-mat.mes-hall↗

Role of incoherent scattering on energy filtering in nanostructured thermoelectric generators

The physics of energy filtering in electronic transport through nanoscale barriers is a fundamental aspect in the context of electronic engineering of nanostructured thermoelectrics. In the context of thermoelectric generators, it aims to engineer the Seebeck coefficient to favorably increase the power factor and ultimately the power generated. In this work, we employ the incoherent non-equilibrium Green's function formalism to investigate in detail the physics of energy filtering and how it leads to a direct enhancement in power generation across nanostructured thermoelectrics featuring a single planar energy barrier. In particular, we reinforce that the enhancement in the generated power via energy filtering at a particular operating efficiency is a characteristic of incoherent scattering and is absent in ballistic devices. In such cases, by assuming an energy dependent relaxation time, $τ(E)=kE^r$, we show that there exists a minimum value $r_{min}$ for which the thermoelectric power generation is enhanced and thereby leading to a degradation in power generation for $r<r_{min}$. For bulk generators, we delve into the details of intermode scattering and show that such scattering processes between electrons in higher energy modes and lower energy modes have a finite contribution to the enhancement in the generated power. We also discuss realistic aspects such as finite width of energy barriers and imperfect energy filtering due to partial reflections. In particular, we show that such imperfect filtering and partial transmission of electrons near the top of the barrier affects the enhancement in the generated power drastically in the high efficiency regime of operation. Analysis of the results obtained in this work should provide general design guidelines for nanostructured enhancement in power generation via energy filtering.

cond-mat.mes-hall↗

Resonant enhancement in nanostructured thermoelectric performance via electronic thermal conductivity engineering

The use of an asymmetric broadening in the transport distribution, a characteristic of resonant structures, is proposed as a route to engineer a decrease in electronic thermal conductivity thereby enhancing the electronic figure of merit in nanostructured thermoelectrics. Using toy models, we first demonstrate that a decrease in thermal conductivity resulting from such an asymmetric broadening may indeed lead to an electronic figure of merit well in excess of 1000 in an idealized situation and in excess of 10 in a realistic situation. We then substantiate with realistic resonant structures designed using graphene nano-ribbons by employing a tight binding framework with edge correction that match density functional theory calculations under the local density approximation. The calculated figure of merit exceeding 10 in such realistic structures further reinforces the concept and sets a promising direction to use nano-ribbon structures to engineer a favorable decrease in the electronic thermal conductivity.

cond-mat.mes-hall↗

Ultra-sensitive nanoscale magnetic field sensors based on resonant spin filtering

Solid state magnetic field sensors based on magneto-resistance modulation find direct applications in communication devices, specifically in proximity detection, rotational reference detection and current sensing. In this work, we propose sensor structures based on the magneto-resistance physics of resonant spin-filtering and present device designs catered toward exceptional magnetic field sensing capabilities. Using the non-equilibrium Green's function spin transport formalism self consistently coupled to the Poisson's equation, we present highly-tunable pentalayer magnetic tunnel junction structures that are capable of exhibiting an ultra-high peak tunnel magneto resistance $(\approx 2500 \%$). We show how this translates to device designs featuring an ultra-high current sensitivity enhancement of over 300\% in comparison with typical trilayer MTJ sensors, and a wider tunable range of field sensitivity. We also demonstrate that a dynamic variation in sensor functionalities with the structural landscape enables a superior design flexibility over typical trilayer sensors. An optimal design exhibiting close to a 700\% sensitivity increase as a result of angle dependent spin filtering is then presented.This work sets a stage to engineer spintronic building blocks via the design of functional structures tailored to exhibit ultra-sensitive spin filtering.

cond-mat.mes-hall↗

Programming current reduction via enhanced asymmetry-induced thermoelectric effects in vertical nanopillar phase change memory cells

Thermoelectric effects are envisioned to reduce programming currents in nanopillar phase change memory cells. However, due to the inherent symmetry in such a structure, the contribution due to thermoelectric effects on programming currents is minimal. In this work, we propose a hybrid phase change memory structure which incorporates a two-fold asymmetry specifically aimed to favorably enhance thermoelectric effects. The first asymmetry is introduced via an interface layer of low thermal conductivity and high negative Seebeck coefficient, such as, polycrystalline SiGe, between the bottom electrode contact and the active region comprising the phase change material. This results in an enhanced Peltier heating of the active material. The second one is introduced structurally via a taper that results in an angle dependent Thomson heating within the active region. Various device geometries are analyzed using 2D-axis-symmetric simulations to predict the effect on programming currents as well as for different thicknesses of the interface layer. A programming current reduction of up to $60\%$ is predicted for specific cell geometries. Remarkably, we find that due to an interplay of Thomson cooling in the electrode and the asymmetric heating profile inside the active region, the predicted programming current reduction is resilient to fabrication variability.

cond-mat.mes-hall↗

Optimal Single Quantum Dot Heat-to-pure-spin-current Converters

We delve into the conditions under which a quantum dot thermoelectric setup may be tuned to realize an optimal heat-to-pure-spin-current converter. It is well known that a heat-to-pure-spin-current converter may be realized using a non-interacting quantum dot with a spin-split energy spectrum under particle hole symmetry conditions. However, with the inclusion of Coulomb interaction $U$, ubiquitous in typical quantum dot systems, the relevant transport physics is expected to be altered. In this work, we provide a detailed picture of thermoelectric pure spin currents at various Coulomb interaction parameters $U$ and describe the conditions necessary for an exact cancellation of charge transport between energy levels $ε$ and their Coulomb-charged partner levels $ε+U$, so as to yield the largest terminal pure spin currents. A non-trivial aspect pointed out here is that at sufficiently large values of $U$ ($\ge U_0$), pure spin currents tend to optimize at points other than where the particle-hole symmetry occurs. It is also ascertained that a global maximum of pure spin current is generated at a typical value of the interaction parameter $U$. These optimum conditions may be easily realized using a typical gated quantum dot thermoelectric transport setup

cond-mat.mes-hall↗

Proposal for a Domain Wall Nano-Oscillator driven by Non-uniform Spin Currents

We propose a new mechanism and a related device concept for a robust, magnetic field tunable radio-frequency (rf) oscillator using the self oscillation of a magnetic domain wall subject to a uniform static magnetic field and a spatially non-uniform vertical dc spin current. The self oscillation of the domain wall is created as it translates periodically between two unstable positions, one being in the region where both the dc spin current and the magnetic field are present, and the other, being where only the magnetic field is present. The vertical dc spin current pushes it away from one unstable position while the magnetic field pushes it away from the other. We show that such oscillations are stable under noise and can exhibit a quality factor of over 1000. A domain wall under dynamic translation, not only being a source for rich physics, is also a promising candidate for advancements in nanoelectronics with the actively researched racetrack memory architecture, digital and analog switching paradigms as candidate examples. Devising a stable rf oscillator using a domain wall is hence another step towards the realization of an all domain wall logic scheme.

cond-mat.mes-hall↗

Exploring Packaging Strategies of Nano-embedded Thermoelectric Generators

Embedding nanostructures within a bulk matrix is an important practical approach towards the electronic engineering of high performance thermoelectric systems. For power generation applications, it ideally combines the efficiency benefit offered by low dimensional systems along with the high power output advantage offered by bulk systems. In this work, we uncover a few crucial details about how to embed nanowires and nanoflakes in a bulk matrix so that an overall advantage over pure bulk may be achieved. First and foremost, we point out that a performance degradation with respect to bulk is inevitable as the nanostructure transitions to being multi moded. It is then shown that a nano embedded system of suitable cross-section offers a power density advantage over a wide range of efficiencies at higher packing fractions, and this range gradually narrows down to the high efficiency regime, as the packing fraction is reduced. Finally, we introduce a metric - \emph{the advantage factor}, to elucidate quantitatively, the enhancement in the power density offered via nano-embedding at a given efficiency. In the end, we explore the maximum effective width of nano-embedding which serves as a reference in designing generators in the efficiency range of interest.

cond-mat.mes-hall↗