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C. Scheidenberger

Publications and source records attributed to C. Scheidenberger.

At least 19 recordsLinked to original sources

Ground State Decay of the Three-Proton Emitter $^{17}$Na Reveals Isospin Symmetry Breaking

The spectrum of the exotic three-proton (3p) emitter $^{17}$Na has been studied by detecting all in-flight decay products. Derived from the measured angular correlations $^{14}$O+p+p+p, a resonant peak has been discovered at the 3p-decay energy of 2.24($^{+0.17}_{-0.25}$) MeV, which likely corresponds to the $^{17}$Na ground state. This decay energy value is significantly smaller than the previous experimental upper limit. Our measured $^{14}$O-p correlations stemming from the ground state decay have been quantitatively described by a sequential 1p-2p emission from a $^{17}$Na resonance via the intermediate $^{16}$Ne ground state, which allowed to derive the upper limit of $^{17}$Na ground-state width of 0.6 MeV. A dramatic systematic decrease in the mirror energy differences of mirror nuclei pairs has been observed at almost all 3p emitters with known proton separation energy (such as $^{31}$K, $^{20}$Al, and $^{17}$Na), in sharp contrast to the behavior in less exotic nuclei. Such a lowering effect indicates a general trend in evolution of nuclear structure for light to medium mass nuclei beyond the proton drip line, which is often associated with strong isospin symmetry breaking.

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Mass measurements of $^{179-184}$Yb identify an anomalous proton-neutron interaction

Mass measurements of nuclei can identify structurally-driven trends in binding energy across isotopic chains, and can also isolate specific nucleon-nucleon interactions, such as the $\delta V_{\mathrm{pn}}$ interaction of the last two valence protons with the last two valence neutrons. Below $^{208}$Pb, investigation of the local binding energy and $\delta V_{\mathrm{pn}}$ systematics can facilitate a better understanding of the behaviour of the proton-neutron interaction in the 'hole-hole' regime (where valence interactions can be modelled in hole-space rather than particle-space) and provide insight on the potential onset of a prolate-to-oblate shape transition. However, measurement of the necessary nuclei has been exceptionally challenging. Here we present six first-time measurements of neutron-rich ytterbium, using advanced rare isotope production and mass spectrometry techniques, leading to the identification of an anomalously strong proton-neutron interaction in the 'hole-hole' quadrant below $^{208}$Pb. The scale of this interaction, at $^{186}$Hf, is comparable to that of similar signals at doubly-magic nuclei and shape transitions. The experimental results are compared with contemporary mean-field model predictions, that do not accurately reproduce the anomaly. The results are also used to benchmark predictions from several models, to facilitate more accurate descriptions towards a key r-process waiting point at $N = 126$.

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Hadron Physics Opportunities at FAIR

This White Paper outlines a coordinated, decade-spanning programme of hadron and QCD studies anchored at the GSI/FAIR accelerator complex. Profiting from intense deuteron, proton and pion beams coupled with high-rate capable detectors and an international theory effort, the initiative addresses fundamental questions related to the strong interaction featuring confinement and dynamical mass generation. This includes our understanding of hadron-hadron interactions and the composition of hadrons through mapping the baryon and meson spectra, including exotic states, and quantifying hadron structure. This interdisciplinary research connects topics in the fields of nuclear, heavy-ion, and (nuclear) astro (particle) physics, linking, for example, terrestrial data to constraints on neutron star structure. A phased roadmap with SIS100 accelerator start-up and envisaged detector upgrades will yield precision cross sections, transition form factors, in-medium spectral functions, and validated theory inputs. Synergies with external programmes at international accelerator facilities worldwide are anticipated. The programme is expected to deliver decisive advances in our understanding of non-perturbative (strong) QCD and astrophysics, and high-rate detector and data-science technology.

hep-ex

First Proton-Induced Cross Sections on a Stored Rare Ion Beam: Measurement of 118Te(p,{\gamma}) for Explosive Nucleosynthesis

We present the first nuclear cross-section measurements of (p,{\gamma}) and (p,n) reactions on 118Te at energies relevant for the {\gamma}-process nucleosynthesis. Absolute cross-section values for center-of-mass energies of 6, 7 and 10 MeV are provided, together with a theoretical extrapolation to the Gamow window. This experiment marks the first time that direct proton-induced reactions have been measured on a radioactive ion beam at the Experimental Storage Ring (ESR) at GSI, Darmstadt. This paves the way for a large variety of measurements, delivering new constraints for explosive nucleosynthesis and for physics beyond nuclear stability.

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Excitation Spectra of the ${}^{12}{\rm C}(p,d)$ Reaction near the $\eta'$-Meson Emission Threshold Measured in Coincidence with High-Momentum Protons

The missing mass of the ${}^{12}{\rm C}(p,d)$ reaction has been measured near the $\eta'$-meson emission threshold in coincidence with a high-momentum proton to selectively collect $\eta'$-${}^{11}{\rm C}$ mesic nucleus formation events at GSI, Germany. A 2.5 GeV proton excites a carbon nucleus to form an $\eta'$-mesic nucleus emitting a deuteron forward with an energy of $\sim 1.6$ GeV. The deuteron is momentum-analyzed by the Fragment Separator used as a high-resolution spectrometer to deduce the excitation energy of the residual system. The large-acceptance detector WASA surrounding the target identifies high-momentum protons emitted in the decay of the $\eta'$-mesic nucleus. The measured semi-exclusive spectrum exhibits structures below the threshold though the statistical significance is limited. The spectrum is fitted by theoretically calculated spectra varying optical-potential parameters of the $\eta'$-nucleus interaction. The analysis results indicate $\eta'$-mesic nuclei formation for the real potential depth of $\sim -61$ MeV with a local statistical significance of $3.5 \sigma$ and, taking into account the look-elsewhere effect, a global significance of $2.1 \sigma$.

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Observation of Tensor-Driven High-Momentum Neutrons in ${}^{16}$O via ($p,d$) Reactions and Zero-Degree Deuteron Momentum Spectroscopy

The $^{16}\mathrm{O}(p,d)^{15}\mathrm{O}$ reaction has been studied at $0^{\circ}$ using 403-, 604-, 907- and 1209-MeV protons, comparing cross sections populating positive- and negative-parity states in $^{15}\mathrm{O}$. Transitions to positive-parity states exhibit strong sensitivity to high-momentum neutrons, while negative-parity transitions show much smaller effects. The cross-section ratio between positive- and negative-parity states rises sharply with momentum transfer, matching theoretical predictions that include tensor interactions, particularly the peak near $2~\mathrm{fm}^{-1}$ for the $5/2^{+}$ to ground-state ratio. These results highlight $0^{\circ}$ neutron-pickup reactions as a sensitive probe for tensor-driven high-momentum components, paving the way for studies in exotic nuclei via radioactive beams.

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Performance of newly constructed plastic scintillator barrel in the WASA-FRS experiments and evaluation of radiation damage effects on multi-pixel photon counter

A barrel-shaped plastic scintillation counter with Multi-Pixel Photon Counter (MPPC) readout has been developed and operated in the first WASA-FRS experimental campaign at GSI. The detector was used to measure charged particles emitted from reactions induced by a 2.5 GeV proton beam incident on a carbon target, providing particle identification in combination with momentum reconstruction in a 1 T magnetic field. The performance of this detector, particularly its response to energy deposition and time resolution, was systematically investigated as a function of count rate and total number of irradiating protons. A time resolution of 45-75 ps ($\sigma$), depending on the energy deposition, was achieved. Stable performance was maintained under high-rate conditions up to 1.35 MHz per single counter, with no significant degradation in either signal amplitude or timing response. Radiation-induced damage to the MPPCs was observed primarily as a reduction in signal amplitude, with approximately $35\%$ decrease at an estimated 1 MeV neutron-equivalent fluence of $2.4 \times 10^{10}$ cm$^{-2}$.

physics.ins-det

Charge Pickup Reaction Cross Section for Neutron-Rich p-Shell Isotopes at 900A MeV

We report charge pickup reaction cross sections for 24 \textit{p}-shell isotopes, including $^{8,9}$Li, $^{10-12}$Be, $^{10,13-15}$B, $^{12,14-19}$C and $^{14,15,17-22}$N, measured at relativistic energies (approximately 900$A$ MeV) on both hydrogen and carbon targets. For the first time, we reveal a universal rapid increase in the charge pickup cross sections of unstable projectiles with isospin asymmetry along several isotopic chains. The cross sections can be decoupled into distinct contributions from the mass number and isospin asymmetry of the projectile, highlighting the critical role of the latter, and can be formulated empirically.

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Half-life determination of heavy ions in a storage ring considering feeding and depleting background processes

Heavy-ion storage rings have relatively large momentum acceptance which allows for multiple ion species to circulate at the same time. This needs to be considered in radioactive decay measurements of highly charged ions, where atomic charge exchange reactions can significantly alter the intensities of parent and daughter ions. In this study, we investigate this effect using the decay curves of ion numbers in the recent $^{205}$Tl$^{81+}$ bound-state beta decay experiment conducted using the Experimental Storage Ring at GSI Darmstadt. To understand the intricate dynamics of ion numbers, we present a set of differential equations that account for various atomic and nuclear reaction processes-bound-state beta decay, atomic electron recombination and capture, and electron ionization. By incorporating appropriate boundary conditions, we develop a set of differential equations that accurately simulate the decay curves of various simultaneously stored ions in the storage ring: $^{205}$Tl$^{81+}$, $^{205}$Pb$^{81+}$, $^{205}$Pb$^{82+}$, $^{200}$Hg$^{79+}$, and $^{200}$Hg$^{80+}$. Through a quantitative comparison between simulations and experimental data, we provide insights into the detailed reaction mechanisms governing stored heavy ions within the storage ring. Our approach effectively models charge-changing processes, reduces the complexity of the experimental setup, and provides a simpler method for measuring the decay half-lives of highly charged ions in storage rings.

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Bayesian and Monte Carlo approaches to estimating uncertainty for the measurement of the bound-state $\beta$ decay of $^{205}\mathrm{Tl}^{81+}$

The measurement of the bound-state $\beta$ decay of $^{205}\mathrm{Tl}^{81+}$ at the Experimental Storage Ring at GSI, Darmstadt, has recently been reported with substantial impact on the use of $^{205}\mathrm{Pb}$ as an early Solar System chronometer and the low-energy measurement of the solar neutrino spectrum via the LOREX project. Due to the technical challenges in producing a high-purity $^{205}\mathrm{Tl}^{81+}$ secondary beam, a robust statistical method needed to be developed to estimate the variation in the contaminant $^{205}\mathrm{Pb}^{81+}$ produced in the fragmentation reaction, which was subsequently transmitted and stored in the ESR. Here we show that Bayesian and Monte Carlo methods produced comparable estimates for the contaminant variation, each with unique advantages and challenges given the complex statistical problems for this experiment. We recommend the adoption of such methods in future experiments that exhibit unknown statistical fluctuations.

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Investigation of Direct Nuclear Reactions in a Storage Ring Using In-Ring Detection

\textbf{Background:} Experiments involving nuclear reactions in a storage ring offer exceptional possibilities for precise measurements in inverse kinematics. These experiments provide excellent angular and energy resolution by particle spectroscopy, in addition to high luminosities. However, the extremely low-pressure environment maintained in the storage rings poses significant difficulties for experiments employing detectors or any outgassing material in the ring. \textbf{Purpose:} To investigate nuclear reactions in inverse kinematics using the storage-ring technique. The reactions were induced by scattering of a ${}^{20}\mathrm{Ne}$ beam off a hydrogen target at an energy of 50~MeV/u. \textbf{Method:} A beam of fully stripped ${}^{20}$Ne ions was injected into the ESR storage ring at an energy of 50 MeV/u. The beam interacted with an internal hydrogen gas-jet target. An ultra-high vacuum compatible detector setup was installed around the gas jet inside the ring to measure the recoiling particles generated by nuclear reactions. \textbf{Results:} Multiple reaction channels were observed during the experiment. In particular, we present the results from studies on elastic and inelastic scattering, as well as the neutron transfer reaction ${}^{20}\mathrm{Ne}(p,d){}^{19}\mathrm{Ne}^*$. The experimental data were compared to calculations that took into account the most significant excited states, using a coupled-reaction channel approach. A very good agreement with the experimental data was achieved. \textbf{Conclusions:} The present results are the first demonstration of the investigation transfer reactions using detectors directly installed in the ring. This provides an important proof-of-principle for prospective studies with far-from-stability radioactive beams in the future.

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Exploring the Onset of Collectivity Approaching N=40 through Manganese Masses

Isotopes in the region of the nuclear chart below $^{68}\mathrm{Ni}$ have been the subject of intense experimental and theoretical effort due to the potential onset of a new ``island of inversion'' when crossing the harmonic oscillator subshell closure at $N = 40$. We have measured the masses of $^{64-68}\textrm{Mn}$ using TITAN's multiple-reflection time-of-flight mass spectrometer, resulting in the first precision mass measurements of $^{67}\mathrm{Mn}$ and $^{68}\mathrm{Mn}$. These results are compared to \textit{ab initio} calculations and modern shell model calculations and show an increase in collectivity approaching $N=40$.

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Refined topology of the N = 20 island of inversion with high precision mass measurements of $^{31-33}$Na and $^{31-35}$Mg

Mass measurements of $^{31-33}$Na and $^{31-35}$Mg using the TITAN MR-TOF-MS at TRIUMF's ISAC facility are presented, with the uncertainty of the $^{33}$Na mass reduced by over two orders of magnitude. The excellent performance of the MR-TOF-MS has also allowed the discovery of a millisecond isomer in $^{32}$Na. The precision obtained shows that the binding energy of the normally closed N = 20 neutron shell reaches a minimum for $^{32}$Mg but increases significantly for $^{31}$Na, hinting at the possibility of enhanced shell strength toward the unbound $^{28}$O. We compare the results with new ab initio predictions that raise intriguing questions of nuclear structure beyond the dripline.

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Precision mass measurements of $^{74-76}$Sr using TITAN's Multiple-Reflection Time-of-Flight Mass Spectrometer

We report precision mass measurements of $^{74-76}$Sr performed with the TITAN Multiple-Reflection Time-of-Flight Mass Spectrometer. This marks a first time mass measurement of $^{74}$Sr and gives increased mass precision to both $^{75}$Sr and $^{76}$Sr which were previously measured using storage ring and Penning trap methods, respectively. This completes the A = 74, T = 1 isospin triplet and gives increased precision to the A = 75, T = 1/2 isospin doublet which are both the heaviest experimentally evaluated triplets and doublets to date. The new data allow us to evaluate coefficients of the isobaric multiplet mass equation for the first time at A = 74, and with increased precision at A = 75. With increased precision of 75Sr, we confirm the recent measurement reported by CSRe which was used to remove a staggering anomaly in the doublets. New ab initio valence-space in-medium similarity renormalization group calculations of the T = 1 triplet are presented at A = 74. We also investigate the impact of the new mass data on the reaction flow of the rapid proton capture process in type I x-ray bursts using a single-zone model.

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Bound-State Beta Decay of $\mathbf{\mathrm{^{205}{Tl}^{81+}}}$ Ions and the LOREX Project

Stable $^{205}$Tl ions have the lowest known energy threshold for capturing electron neutrinos ($\nu_e$) of ${ E}_{\nu_e}\ge50.6$\,keV. The Lorandite Experiment (LOREX), proposed in the 1980s, aims at obtaining the longtime averaged solar neutrino flux by utilizing natural deposits of Tl-bearing lorandite ores. To determine the $\nu_e$ capture cross section, it is required to know the strength of the weak transition connecting the ground state of $^{205}$Tl and the 2.3 keV first excited state in $^{205}$Pb. The only way to experimentally address this transition is to measure the bound-state beta decay ($\beta_{b}$) of fully ionized $\mathrm{^{205}Tl^{81+}}$ ions. After three decades of meticulous preparation, the half-life of the $\beta_{b}$ decay of $\mathrm{^{205}Tl^{81+}}$ has been measured to be $291_{-27}^{+33}$ days using the Experimental Storage Ring (ESR) at GSI, Darmstadt. The longer measured half-life compared to theoretical estimates reduces the expected signal-to-noise ratio in the LOREX, thus challenging its feasibility.

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Convergence on the Proton Drip-Line in Thulium

Direct observation of proton emission for very small Q-values is often unfeasible due to the long partial half-lives of the proton emission channel associated with tunneling through the Coulomb barrier. Therefore, proton emitters with very small decay energies may require the masses of both parent and daughter nuclei in order to establish them as proton unbound. Nuclear mass models have been used to predict the proton drip-line of the thulium (Tm) isotopic chain ($Z=69$), but until now the proton separation energy has not been experimentally tested. Mass measurements were performed using a Multiple Reflection Time-Of-Flight Mass Spectrometer (MR-TOF-MS) at TRIUMF's TITAN facility to conclusively map the limit of proton-bound Tm. The masses of neutron-deficient, $^{149}$Tm and $^{150}$Tm, combined with measurements of $^{149m,g}$Er (which were found to deviate from literature by $\approx$150 keV), provide the first experimental confirmation that $^{149}$Tm is the first proton-unbound nuclide in the Tm chain. Our measurements also enable the strength of the $N=82$ neutron shell gap to be determined at the Tm proton drip-line, providing evidence supporting its continued existence.

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Mirror Symmetry Breaking Disclosed in the Decay of Three-Proton Emitter 20Al

The previously-unknown nucleus 20Al has been observed for the first time by detecting its in-flight decays. Tracking trajectories of all decay products with silicon micro-strip detectors allowed for a conclusion that 20Al is unbound with respect to three-proton (3p) emission. The 3p-decay energy of 20Al ground state has been determined to be 1.93(+0.11,-0.09) MeV through a detailed study of angular correlations of its decay products, 17Ne+p+p+p. This value is much smaller in comparison with the predictions inferred from the isospin symmetry by using the known energy of its mirror nucleus 20N, which indicates a possible mirror symmetry violation in the structure of 3p emitters. Such an isospin symmetry breaking is supported by the calculations of the continuum embedded theoretical frameworks, describing the observed 20Al ground state as an 1p s-wave state with a spin-parity of 1-, which contradicts to the spin-parity (2-) of the 20N ground state. The 20Al ground state decays by sequential 1p-2p emission via intermediate ground state of 19Mg, which is the first observed case of daughter two-proton radioactivity following 1p decay of the parent state.

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High-temperature $^{205}$Tl decay clarifies $^{205}$Pb dating in early Solar System

Radioactive nuclei with lifetimes on the order of millions of years can reveal the formation history of the Sun and active nucleosynthesis occurring at the time and place of its birth. Among such nuclei whose decay signatures are found in the oldest meteorites, $^{205}$Pb is a powerful example, as it is produced exclusively by slow neutron captures (the s process), with most being synthesized in asymptotic giant branch (AGB) stars. However, making accurate abundance predictions for $^{205}$Pb has so far been impossible because the weak decay rates of $^{205}$Pb and $^{205}$Tl are very uncertain at stellar temperatures. To constrain these decay rates, we measured for the first time the bound-state $\beta^-$ decay of fully ionized $^{205}$Tl$^{81+}$, an exotic decay mode that only occurs in highly charged ions. The measured half-life is 4.7 times longer than the previous theoretical estimate and our 10% experimental uncertainty has eliminated the main nuclear-physics limitation. With new, experimentally backed decay rates, we used AGB stellar models to calculate $^{205}$Pb yields. Propagating those yields with basic galactic chemical evolution (GCE) and comparing with the $^{205}$Pb/$^{204}$Pb ratio from meteorites, we determined the isolation time of solar material inside its parent molecular cloud. We find positive isolation times that are consistent with the other s-process short-lived radioactive nuclei found in the early Solar System. Our results reaffirm the site of the Sun's birth as a long-lived, giant molecular cloud and support the use of the $^{205}$Pb--$^{205}$Tl decay system as a chronometer in the early Solar System.

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