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Christian Lisdat

Publications and source records attributed to Christian Lisdat.

At least 19 recordsLinked to original sources

International Optical Clock Comparison Using the European Optical Fiber Network

Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying the international consistency of optical clocks remains critical as efforts intensify toward redefining the SI second based on an optical transition or transitions. We report on a two-month international clock comparison campaign involving seven optical clocks in four national metrology institutes (INRIM, LNE-OP, NPL, and PTB) connected via the optical fiber network established in Europe. The campaign resulted in optical frequency ratios with uncertainties ranging from $7.7\times10^{-18}$ to $6.1\times10^{-17}$. Among the results, the $^{171}$Yb$^+$(E3) clocks at NPL and PTB demonstrated agreement within an uncertainty of $7.7\times10^{-18}$, marking the first international verification of two independently developed optical clocks below one part in $10^{17}$. The operation of the $^{199}$Hg clock at LNE-OP (formerly LNE-SYRTE) resulted in frequency ratios with improved uncertainties with $^{171}$Yb$^+$(E3), $^{171}$Yb, and $^{87}$Sr optical clocks. These results provide input for the redefinition of the second and underscore how fiber-linked clock networks can advance metrology and scientific applications.

physics.atom-ph

The QTF-Backbone: Proposal for a Nationwide Optical Fibre Backbone in Germany for Quantum Technology and Time and Frequency Metrology

The recent breakthroughs in the distribution of quantum information and high-precision time and frequency (T&F) signals over long-haul optical fibre networks have transformative potential for physically secure communications, resilience of timing infrastructure (such as that supporting Global Navigation Satellite Systems (GNSS)) and fundamental physics. To date, these capabilities remain confined to isolated testbeds, with quantum and T&F signals accessible, for example in Germany, to only a few institutions. In this white paper we propose the QTF Backbone: a dedicated national fibre-optic infrastructure in Germany for the networked distribution of Quantum and T&F signals using dark fibres and specialised hardware. The QTF Backbone is planned as a four-phase deployment over ten years to ensure scalable, sustainable access for research institutions and industry. The concept builds on successful demonstrations of time and frequency distribution at high Technology Readiness Levels (TRLs) across Europe, including PTB-MPQ links in Germany, REFIMEVE in France, and the Italian LIFT network. The QTF Backbone will enable transformative Research and Development (R&D), support a nationwide QTF ecosystem, and ensure the transition from innovation to deployment. As a national and European hub, it will position Germany and Europe at the forefront of quantum networking, as well as T&F transfer.

physics.ins-det

Interspecies clock comparison below $5 \times 10^{-18}$ uncertainty with a transportable clock

We report a measurement of the optical frequency ratio between the $^2\mathrm{S}_{1/2}(F=0)$--${^2\mathrm{F}_{7/2}(F=3)}$ electric-octupole (E3) transition of $^{171}$Yb$^{+}$ and the $^1\mathrm{S}_0$--${^3\mathrm{P}_0}$ transition of $^{87}$Sr, $ν_{\mathrm{Yb}^{+}}/ν_\mathrm{Sr} = 1.495\,991\,618\,544\,900\,588\,1(65)$. Reaching a fractional uncertainty of $4.3 \times 10^{-18}$, this result improves upon the previous best by more than a factor of three and is among the few that meet the requirements for interspecies clock comparisons specified by the roadmap towards the redefinition of the SI second. The comparison is between a transportable optical lattice clock and a stationary single-ion clock. It spans a period of nearly two years, during which the transportable clock was intermittently operated off-campus. The ratio was reproducibly measured during four separate campaigns, which are consistent within their statistical uncertainties. The results demonstrate reproducible $10^{-18}$ level operation of the transportable clock and thus validate its application for chronometric geodesy and as a transfer standard for inter-institute clock comparisons, e.g., in the absence of optical fiber links.

physics.atom-ph

An Al$^+$ clock with $1.6\times10^{-18}$ systematic uncertainty and its frequency ratios

Advances in optical clocks motivate a redefinition of the second, requiring rigorous evaluations of systematic uncertainties and robust consistency among the clocks. Here, we report the full evaluation of the systematic frequency shifts of an $^{27}\mathrm{Al}^+$ single-ion clock, and the measurement of its absolute frequency and frequency ratio with a $^{87}$Sr optical lattice clock at PTB. The evaluated total systematic fractional frequency uncertainty is $1.6\times10^{-18}$, mainly limited by the accuracy of the relevant atomic coefficients and by background gas collisions. The absolute frequency of the clock has been measured to be $ν_{\mathrm{Al}^+}=1 121 015 393 207 859.19(24)\,$Hz, obtained by comparison with two primary caesium fountain clocks at PTB. The frequency ratio between the Al and Sr optical clocks has been determined to be $ν_{\mathrm{Al}^+}/ν_{^{87}\mathrm{Sr}}=2.611 701 431 781 462 668(36)$, limited by the accuracy of the Sr clock. This ratio differs by $8.6σ$ and $1.2σ$ from the 2021 and 2025 frequency ratio published by the BACON collaboration, respectively. These results represent an important contribution toward a future redefinition of the second using optical clocks, and underscore the importance of independent measurements of clock-candidate frequency ratios across different institutions.

physics.atom-ph

Ultra-stable transportable ultraviolet clock laser using cancellation between photo-thermal and photo-birefringence noise

Optical clocks require an ultra-stable laser to probe and precisely measure the frequency of the narrow-linewidth clock transition. We introduce a portable ultraviolet (UV) laser system for use in an aluminum quantum logic clock, demonstrating a fractional frequency instability of approximately $\mathrm{mod}\,σ_\mathrm{y} = 2 \times 10^{-16}$. The system is based on an ultra-stable cavity with crystalline AlGaAs/GaAs mirror coatings, alongside with a frequency quadrupling system employing two single-pass second harmonic generation (SHG) stages. Its acceleration sensitivity, measured in all three axes, does not exceed $4(2) \times 10^{-12}$/(ms$^{-2}$) and is among the lowest recorded for transportable systems to date. Additionally, partial cancellation between photo-thermal noise and photo-birefringence noise is used to effectively mitigate noise induced by intra-cavity optical power fluctuation at lower Fourier frequencies.

physics.optics

A high-stability optical clock based on a continuously ground-state cooled Al$^+$ ion without compromising its accuracy

Single ion optical clocks have shown systematic frequency uncertainties below $10^{-18}$, but typically require more than one week of averaging to achieve a corresponding statistical uncertainty. This time can be reduced with longer probe times, but comes at the cost of a higher time-dilation shift due to motional heating of the ions in the trap. We show that sympathetic ground-state cooling using electromagnetically-induced transparency (EIT) of an \Al clock ion via a co-trapped \Ca ion during clock interrogation suppresses the heating of the ions. \Al can be kept close to the motional ground state, independent from the chosen interrogation time, at a relative time dilation shift of $(-1.69\pm0.20)\times10^{-18}$. The \Ca cooling light introduces an additional light shift on the \Al clock transition of $(-9.27\pm 1.03)\times10^{-18}$. We project that the uncertainty of this light shift can be further reduced by nearly an order of magnitude. This sympathetic cooling enables seconds of interrogation time with $10^{-19}$ motional and cooling laser-induced uncertainties for \Al and can be employed in other ion clocks as well.

physics.atom-ph

Realization of a clock-based global height system: A simulation study for Europe and Brazil

Chronometric levelling is a novel technique for the realisation of the International Height Reference System (IHRS). A detailed study of this technique is carried out through closed-loop simulations, aiming to unify regional/local height systems (LHS) in Europe and Brazil. Focusing on a unification accuracy of 1 cm, realistic scenarios with various error parameters/vertical datum parameters in LHS and clock observation uncertainties were analysed. The errors associated with local heights raised from datum offsets, local vertical datum alignment discrepancies in latitude and longitude, accumulated tilts depending on the distance from the reference tide gauge and levelling point elevation-dependent offsets were introduced. Clocks achieving a fractional uncertainty of 10^-18 and 10^-17 were assumed in the simulations, considering temporal correlations of clock intrinsic uncertainties, external effects on clock observations such as tidal effects, propagation delay in terms of link uncertainties and presence of outliers. We determine the preferred distributions of clocks in a network for the best estimation of error parameters. The estimation of the error parameters is related to the spatial distribution of the clocks, hence, an optimal setup of placing clocks at the most distant levelling points, reference tide gauges and elevated points is implemented. Further, a configuration of clock distribution is proposed with master clocks and local clocks with reduced links. Taking into consideration all these realistic constraints, a unification accuracy of 1 cm can be obtained. The unified European and Brazilian height systems are further related to the global geoid such that all geoid-related heights achieve an accuracy of 3 cm.

physics.geo-ph

Entanglement-enhanced optical ion clock

Entangled states hold the promise of improving the precision and accuracy of quantum sensors. We experimentally demonstrate that spectroscopy of an optical clock transition using entangled states can outperform its classical counterpart. Two ^{40}\text{Ca}^{+} ions are entangled in a quantum state with vanishing first-order magnetic field sensitivity, extending the coherence time of the atoms and enabling near lifetime-limited probe times of up to 550 ms. In our protocol, entangled ions reach the same instability as uncorrelated ions, but at half the probe time, enabling faster cycle times of the clock. We run two entangled ^{40}\text{Ca}^{+} ions as an optical clock and compare its frequency instability with a ^{87}\text{Sr} lattice clock. The instability of the entangled ion clock is below a clock operated with classically correlated states for all probe times. We observe instabilities below the theoretically expected quantum projection noise limit of two uncorrelated ions for interrogation times below 100 ms. The lowest fractional frequency instability of 7e-16 / sqrt(tau / 1 s) is reached for 250 ms probe time, limited by residual phase noise of the probe laser. This represents the lowest instability reported to date for a ^{40}\text{Ca}^{+} ion clock.

physics.atom-ph

Coordinated international comparisons between optical clocks connected via fiber and satellite links

Optical clocks provide ultra-precise frequency references that are vital for international metrology as well as for tests of fundamental physics. To investigate the level of agreement between different clocks, we simultaneously measured the frequency ratios between ten optical clocks in six different countries, using fiber and satellite links. This is the largest coordinated comparison to date, from which we present a subset of 38 optical frequency ratios and an evaluation of the correlations between them. Four ratios were measured directly for the first time, while others had significantly lower uncertainties than previously achieved, supporting the advance towards a redefinition of the second and the use of optical standards for international time scales.

physics.atom-ph

International comparison of optical frequencies with transportable optical lattice clocks

Optical clocks have improved their frequency stability and estimated accuracy by more than two orders of magnitude over the best caesium microwave clocks that realise the SI second. Accordingly, an optical redefinition of the second has been widely discussed, prompting a need for the consistency of optical clocks to be verified worldwide. While satellite frequency links are sufficient to compare microwave clocks, a suitable method for comparing high-performance optical clocks over intercontinental distances is missing. Furthermore, remote comparisons over frequency links face fractional uncertainties of a few $10^{-18}$ due to imprecise knowledge of each clock's relativistic redshift, which stems from uncertainty in the geopotential determined at each distant location. Here, we report a landmark campaign towards the era of optical clocks, where, for the first time, state-of-the-art transportable optical clocks from Japan and Europe are brought together to demonstrate international comparisons that require neither a high-performance frequency link nor information on the geopotential difference between remote sites. Conversely, the reproducibility of the clocks after being transported between countries was sufficient to determine geopotential height offsets at the level of 4 cm. Our campaign paves the way for redefining the SI second and has a significant impact on various applications, including tests of general relativity, geodetic sensing for geosciences, precise navigation, and future timing networks.

physics.atom-ph

Compact structures for single-beam magneto-optical trapping of ytterbium

Today's best optical lattice clocks are based on the spectroscopy of trapped alkaline-earth-like atoms such as ytterbium and strontium atoms. The development towards mobile or even space-borne clocks necessitates concepts for the compact laser-cooling and trapping of these atoms with reduced laser requirements. Here we present two compact and robust achromatic mirror structures for single-beam magneto-optical trapping of alkaline-earth-like atoms using two widely separated optical cooling frequencies. We have compared the trapping and cooling performance of a monolithic aluminium structure that generates a conventional trap geometry to a quasi-planar platform based on a periodic mirror structure for different isotopes of Yb. Compared to prior work with strontium in non-conventional traps, where only bosons were trapped on a narrow line transition, we demonstrate two-stage cooling and trapping of a fermionic alkaline-earth-like isotope in a single-beam quasi-planar structure.

physics.atom-ph

Achromatic, planar Fresnel-Reflector for a Single-beam Magneto-optical Trap

We present a novel achromatic, planar, periodic mirror structure for single-beam magneto-optical trapping and demonstrate its use in first- and second-stage cooling and trapping for different isotopes of strontium. We refer to it as Fresnel MOT as the structure is inspired by Fresnel lenses. By design, it avoids many of the problems that arise for multi-color cooling using planar structures based on diffraction gratings, which have been the dominant planar structures to be used for single-beam trapping thus far. In addition to a complex design process and cost-intensive fabrication, diffraction gratings suffer from their inherent chromaticity, which causes different axial displacements of trap volumes for the different wavelengths and necessitates tradeoffs in their diffraction properties and achievable trap depths. In contrast, the Fresnel reflector structure presented here is a versatile, easy-to-manufacture device that combines achromatic beam steering with the advantages of a planar architecture. It enables miniaturizing trapping systems for alkaline-earth-like atoms with multiple cooling transitions as well as multi-species trapping in the ideal tetrahedral configuration and within the same volume above the structure. Our design presents a novel approach for the miniaturization of cold-atom systems based on single-beam MOTs and enables the widespread adoption of these systems.

physics.atom-ph

Experimental determination of the E2-M1 polarizability of the strontium clock transition

To operate an optical lattice clock at a fractional uncertainty below $10^{-17}$, one must typically consider not only electric-dipole (E1) interaction between an atom and the lattice light field when characterizing the resulting lattice light shift of the clock transition but also higher-order multipole contributions, such as electric-quadrupole (E2) and magnetic-dipole (M1) interactions. However, strongly incompatible values have been reported for the E2-M1 polarizability difference of the clock states $(5s5p)\,{}^{3}\mathrm{P}_{0}$ and $(5s^2)\,{}^{1}\mathrm{S}_{0}$ of strontium [Ushijima et al., Phys. Rev. Lett. 121 263202 (2018); Porsev et al., Phys. Rev. Lett. 120, 063204 (2018)]. This largely precludes operating strontium clocks with uncertainties of few $10^{-18}$, as the resulting lattice light shift corrections deviate by up to $1 \times 10^{-17}$ from each other at typical trap depths. We have measured the E2-M1 polarizability difference using our ${}^{87}\mathrm{Sr}$ lattice clock and find a value of $Δα_{\mathrm{qm}} = -987^{+174}_{-223} \; \mathrm{μHz}$. This result is in very good agreement with the value reported by Ushijima et al.

physics.atom-ph

A transportable clock laser system with an instability of $1.6 \times 10^{-16}$

We present a transportable ultra-stable clock laser system based on a Fabry-Pérot cavity with crystalline Al$_{0.92}$Ga$_{0.08}$As/GaAs mirror coatings, fused silica (FS) mirror substrates and a 20~cm-long ultra-low expansion (ULE\textsuperscript{\textregistered}) glass spacer with a predicted thermal noise floor of $\mathrm{mod}\,σ_\mathrm{y} = 7 \times 10^{-17}$ in modified Allan deviation at one second averaging time. The cavity has a cylindrical shape and is mounted at ten points. Its measured sensitivity of the fractional frequency to acceleration for the three Cartesian directions are $2(1) \times 10^{-12}$/(ms$^{-2}$), $3(3) \times 10^{-12}$/(ms$^{-2}$) and $3(1) \times 10^{-12}$/(ms$^{-2}$), which belong to the lowest acceleration sensitivities published for transportable systems. The laser system's instability reaches down to $\mathrm{mod}\,σ_\mathrm{y} = 1.6 \times 10^{-16}$

physics.optics

Two-color grating magneto-optical trap for narrow-line laser cooling

We demonstrate for the first time the two-color cooling and trapping of alkaline-earth atoms in a grating magneto-optical trap (gMOT). The trap is formed by a single incident laser beam together with four secondary beams that are generated via diffraction from a nanostructured wafer. A grating structure for a gMOT operating with strontium atoms is optimized and fabricated. We trap $10^6$ $^{88}$Sr atoms on the $^1$S$_0$ $\rightarrow$ $^1$P$_1$ transition at $461\;\mathrm{nm}$ and transfer $25\;\%$ of these atoms to the second cooling stage on the narrower $^1$S$_0$ $\rightarrow$ $^3$P$_1$ intercombination transition at $689\;\mathrm{nm}$, preparing a sample of $2.5\times 10^5$ atoms at $5\;μ$K. These results demonstrate for the first time the applicability of the gMOT technology in conjunction with two widely differing wavelengths and enable the continued miniaturization of alkaline-earth based quantum technologies like optical atomic clocks.

physics.atom-ph

Optical frequency ratio of a ${}^{171}\mathrm{Yb}^+$ single-ion clock and a ${}^{87}\mathrm{Sr}$ lattice clock

We report direct measurements of the frequency ratio of the 642 THz ${}^2S_{1/2} (F=0)$--${}^2F_{7/2} (F=3)$ electric octupole transition in ${}^{171}\mathrm{Yb}^+$ and the 429 THz ${}^1S_0$--${}^3P_0$ transition in ${}^{87}\mathrm{Sr}$. A series of 107 measurements has been performed at the Physikalisch-Technische Bundesanstalt between December 2012 and October 2019. Long-term variations of the ratio are larger than expected from the individual measurement uncertainties of few $10^{-17}$. The cause of these variations remains unknown. Even taking these into account, we find a fractional uncertainty of the frequency ratio of $2.5 \times 10^{-17}$, which improves upon previous knowledge by one order of magnitude. The average frequency ratio is $ν_{\mathrm{Yb}^+} / ν_{\mathrm{Sr}} = 1.495\,991\,618\,544\,900\,537(38)$. This represents one of the most accurate measurements between two different atomic species to date.

physics.atom-ph

Prospects and challenges for squeezing-enhanced optical atomic clocks

We have investigated the benefits of spin squeezed states for clocks operated with typical Brownian frequency noise-limited laser sources. Based on an analytic model of the closed servo-loop of an optical atomic clock, we can give quantitative predictions on the optimal clock stability for a given dead time and laser noise. Our analytic predictions are in very good agreement with numerical simulations of the closed servo-loop. We find that for usual cyclic Ramsey interrogation of single atomic ensembles with dead time, even with the current most stable lasers spin squeezing can only improve the clock stability for ensembles below a critical atom number of about one thousand in an optical Sr lattice clock. Even with a future improvement of the laser performance by one order of magnitude the critical atom number still remains below 100,000. In contrast, clocks based on smaller, non-scalable ensembles, such as ion clocks, can already benefit from squeezed states with current clock lasers.

quant-ph

A transportable interrogation laser system with an instability of $\mathrm{mod}\,σ_{\rm y} = 3\times10^{-16}$

We present an interrogation laser system for a transportable strontium lattice clock operating at 698 nm, which is based on an ultra-low-expansion glass reference cavity. Transportability is achieved by implementing a rigid, compact, and vibration insensitive mounting of the 12 cm-long reference cavity, sustaining shocks of up to 50 g. The cavity is mounted at optimized support points that independently constrain all degrees of freedom. This mounting concept is especially beneficial for cavities with a ratio of length $L$ over diameter $D$ $L/D>1$. Generally large $L$ helps to reduce thermal noise-induced laser frequency instability while small $D$ leads to small cavity volume. The frequency instability was evaluated, reaching its thermal noise floor of $\mathrm{mod}\,σ_{\rm y} \approx 3 \times 10^{-16}$ for averaging times between 0.5 s and 10 s. The laser system was successfully operated during several field studies.

physics.ins-det