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Ciprian Padurariu

Publications and source records attributed to Ciprian Padurariu.

At least 19 recordsLinked to original sources

Diode Effect in Nonlinear High-Kinetic-Inductance Transmission Line Resonators

High-kinetic-inductance (HKI) transmission lines provide a promising platform for compact nonlinear superconducting microwave devices. Existing theoretical descriptions are typically based on the slowly varying envelope approximation, which becomes inadequate for strongly nonlinear resonant structures with pronounced spatial field variations. Here, we develop a theoretical framework for single-frequency nonlinear wave propagation in HKI transmission lines by formulating the problem as a boundary value problem that retains the full spatial dependence of the electromagnetic fields. Applying the method to resonant transmission-line geometries, we demonstrate power-dependent resonance shifts, bistable transmission solutions, and strongly direction-dependent transport arising from asymmetric impedance barriers, yielding transmission contrasts of up to $93\%$ without magnetic bias fields. The framework is further extended to a three-port stub geometry, where nonlinear interference produces shifted anti-resonances and Duffing-like spectral distortions. Our approach provides a versatile tool for the analysis and design of strongly nonlinear superconducting microwave devices.

cond-mat.mes-hall

Stroboscopic detection of itinerant microwave photons

We present a novel scheme to detect itinerant microwave radiation at the single photon level. Using existing Josephson-photonics devices, where two microwave cavities are coupled by a dc-voltage biased superconducting junction, we theoretically show how to implement a stroboscopically repeated, near-projective measurement of a photon impinging on one of the cavities. Optimizing rate, duration, and strength of the measurement by flux control of the junction and developing a threshold protocol to detect the photon from a homodyne measurement of the radiation output of the other cavity, we achieve highly efficient detection with low dark counts. By cascading the detector with a preamplifier, where a similar two-cavity Josephson-photonics device acts as a photon multiplier, we can further improve the device to reach a detection efficiency of $88.5 \%$ with a dark count rate of $\sim10^{-4} γ_a$, set by the resonance width $γ_a$ of the absorbing cavity. These results for a multiplication factor of two suggest that near-unity efficiencies may be reached for higher multiplication factors.

quant-ph

Dressed-State Optomechanics in the Few-Photon Regime

Efficient optomechanical cooling typically requires high photon occupancy to maximize cooling power, a constraint that generally limits the degree of coherent quantum control available in the few-photon regime. Here, we investigate this trade-off by considering a strongly nonlinear cavity operated as a discrete quantum system. In the weak-coupling limit, we derive a general connection between the optomechanical damping rate and the cavity's dressed-state manifold. This framework reveals that the damping rate (determined by the population imbalance across dressed states) is directly tunable via the coherent manipulation tools which are standard in circuit quantum electrodynamics. We illustrate this framework using a Josephson photonics architecture, where a dc-biased junction induces a photon blockade that truncates the cavity to an $N$-level system. By sacrificing raw cooling (or heating) power, this platform enables full quantum mechanical control over optomechanical properties, offering a versatile avenue for the quantum manipulation of mechanical modes.

quant-ph

Signatures of Dynes superconductivity in the THz response of ALD-grown NbN thin films

The frequency-dependent complex optical conductivity reflects key properties of superconductors, such as the energy gap in the density of states (DOS) and the superfluid density. For disordered superconductors, the optical conductivity often can be described within Bardeen-Cooper-Schrieffer (BCS) theory, while in corresponding tunneling experiments, deviations in the observed DOS typically require modelling by the phenomenological Dynes formula. The implications of such Dynes DOS for optics were rarely discussed so far. Here we probe the terahertz conductivity of superconducting NbN thin films with thicknesses ranging from 4.5 to 20nm, which were grown by atomic layer deposition (ALD). Our frequency range from 0.3 to 2.1 THz covers energies below and above the spectral gap. For 20nm thick NbN, we find in the optical conductivity distinct deviations from the BCS model, including a step-like characteristic in the absorption at half the zero-temperature spectral gap. These observations can be fully captured by Dynes electrodynamics with a small and temperature-independent pair-breaking rate. For the other films, we also observe signs of Dynes electrodynamics, and we discuss the evolution of the energy gap, the superfluid density, and the pair-breaking rate as function of film thickness.

cond-mat.supr-con

Optomechanical Cooling without Residual Heating

Resolved-sideband cooling is a standard technique in cavity optomechanics enabling quantum control of mechanical motion, but its performance is ultimately limited by quantum backaction heating. This fundamental effect imposes a limit on the minimum achievable mechanical phonon number, establishing a finite-temperature floor regardless of the applied cooling strength. We generalize the semi-classical model for optomechanical cooling to describe universal cavity Hamiltonians incorporating both passive and active nonlinearities. As a concrete demonstration, we analyze the simplest circuit optomechanical system that implements a nonlinear drive via a Josephson junction. Our analysis reveals that this active nonlinear drive can eliminate the residual heating backaction, thereby comparing favorably with alternative optomechanical cooling schemes based on passive nonlinearities arXiv:2202.13228. By successfully overcoming the finite-temperature floor that limits conventional schemes, our method paves the way for unprecedented quantum control over mechanical systems and establishes the experimental viability of zero-heating optomechanical cooling.

quant-ph

Fast initialization of Bell states with Schrödinger cats in multi-mode systems

Schrödinger cat states play an important role for applications in continuous variable quantum information technologies. As macroscopic superpositions they are inherently protected against certain types of noise making cat qubits a promising candidate for quantum computing. It has been shown recently that cat states occur naturally in driven Kerr parametric oscillators (KPOs) as degenerate ground states with even and odd parity that are adiabatically connected to the respective lowest two Fock states by switching off the drive. To perform operations with several cat qubits one crucial task is to create entanglement between them. Here, we demonstrate efficient transformations of multi-mode cat states through adiabatic and diabatic switching between Kerr-type Hamiltonians with degenerate ground state manifolds. These transformations can be used to directly initialize the cats as entangled Bell states in contrast to initializing them from entangled Fock states.

quant-ph

Quantum Coherence in Superconducting Vortex States

Abrikosov vortices, where the superconducting gap is completely suppressed in the core, are dissipative, semi-classical entities that impact applications from high-current-density wires to superconducting quantum devices. In contrast, we present evidence that vortices trapped in granular superconducting films can behave as two-level systems, exhibiting microsecond-range quantum coherence and energy relaxation times that reach fractions of a millisecond. These findings support recent theoretical modeling of superconductors with granularity on the scale of the coherence length as tunnel junction networks, resulting in gapped vortices. Using the tools of circuit quantum electrodynamics, we perform coherent manipulation and quantum non-demolition readout of vortex states in granular aluminum microwave resonators, heralding new directions for quantum information processing, materials characterization, and sensing.

quant-ph

Amplification and Detection of Single Itinerant Microwave Photons

Single-photon detectors are an essential part of the toolbox of modern quantum optics for implementing quantum technologies and enabling tests of fundamental physics. The low energy of microwave photons, the natural signal path for superconducting quantum devices, makes their detection much harder than for visible light. Despite impressive progress in recent years and the proposal and realization of a number of different detector architectures, the reliable detection of a single itinerant microwave photon remains an open topic. Here, we investigate and simulate a detailed protocol for single-photon multiplication and subsequent amplification and detection. At its heart lies a Josephson-photonics device which uses inelastic Cooper-pair tunneling driven by a dc bias in combination with the energy of an incoming photon to create multiple photons, thus compensating for the low-energy problem. Our analysis provides clear design guidelines for utilizing such devices, which have previously been operated in an amplifier mode with a continuous wave input, for counting photons. Combining a formalism recently developed by Mølmer to describe the full quantum state of in- and outgoing photon pulses with stochastic Schrödinger equations, we can describe the full multiplication and detection protocol and calculate performance parameters, such as detection probabilities and dark count rates. With optimized parameters, a high population of a single output mode can be achieved that can then be easily distinguished from vacuum noise in heterodyne measurements of quadratures with a conventional linear amplifier. Realistic devices with two multiplication stages with multiplication of $16$ reach for an impinging Gaussian pulse of length $T$ a detection probability of $84.5\%$ with a dark count rate of $10^{-3}/T$, and promise to outperform competing schemes.

cond-mat.mes-hall

Quantum microwaves: stabilizing squeezed light by phase locking

Bright sources of quantum microwave light are an important building block for various quantum technological applications. Josephson junctions coupled to microwave cavities are a particularly versatile and simple source for microwaves with quantum characteristics, such as different types of squeezing. Due to the inherent nonlinearity of the system, a pure dc-voltage bias can lead to the emission of correlated pairs of photons into a stripline resonator. However, a drawback of this method is that it suffers from bias voltage noise, which disturbs the phase of the junction and consequently destroys the coherence of the photons, severely limiting its applications. Here we describe how adding a small ac reference signal either to the dc-bias or directly into the cavity can stabilize the system and counteract the sensitivity to noise. We first consider the injection locking of a single-mode device, before turning to the more technologically relevant locking of two-mode squeezed states, where phase locking preserves the entanglement between photons. Finally, we describe locking by directly injecting a microwave into the cavity, which breaks the symmetry of the squeezing ellipse. In all cases, locking can mitigate the effects of voltage noise, and enable the use of squeezed states in quantum technological applications.

cond-mat.mes-hall

Quantum Synchronization in Presence of Shot Noise

Synchronization is a widespread phenomenon encountered in many natural and engineered systems with nonlinear classical dynamics. How synchronization concepts and mechanisms transfer to the quantum realm and whether features are universal or platform specific are timely questions of fundamental interest. Here, we present a new approach to model incoherently driven dissipative quantum systems susceptible to synchronization within the framework of Josephson photonics devices, where a dc-biased Josephson junction creates (non-classical) light in a microwave cavity. The combined quantum compound constitutes a self-sustained oscillator with a neutrally stable phase. Linking current noise to the full counting statistics of photon emission allows us to capture phase diffusion, but moreover permits phase locking to an ac-signal and mutual synchronization of two such devices. Thereby one can observe phase stabilization leading to a sharp emission spectrum as well as unique photon emission statistics revealing shot noise induced phase slips. Two-time perturbation theory is used to obtain a reduced description of the oscillators phase dynamics in form of a Fokker-Planck equation in generalization of classical synchronization theories.

cond-mat.mes-hall

Tracking a Spin-Polarized Superconducting Bound State across a Quantum Phase Transition

The magnetic exchange coupling between magnetic impurities and a superconductor induce so-called Yu-Shiba-Rusinov (YSR) states which undergo a quantum phase transition (QPT) upon increasing the exchange interaction beyond a critical value. While the evolution through the QPT is readily observable, in particular if the YSR state features an electron-hole asymmetry, the concomitant change in the ground state is more difficult to identify. We use ultralow temperature scanning tunneling microscopy to demonstrate how the change in the YSR ground state across the QPT can be directly observed for a spin-1/2 impurity in a magnetic field. We observe a change in the excitation spectrum from the doublet ground state in the free spin regime (two spectral features) to the singlet ground state in the screened spin regime (four spectral features). We also identify a transition regime, where the YSR excitation energy is smaller than the Zeeman energy. We thus provide a straightforward way for unambiguously identifying the ground state of a spin-1/2 YSR state.

cond-mat.supr-con

Microwave Excitation of Atomic Scale Superconducting Bound States

Magnetic impurities on superconductors lead to bound states within the superconducting gap, so called Yu-Shiba-Rusinov (YSR) states. They are parity protected, which enhances their lifetime, but makes it more difficult to excite them. Here, we realize the excitation of YSR states by microwaves facilitated by the tunnel coupling to another superconducting electrode in a scanning tunneling microscope (STM). We identify the excitation process through a family of anomalous microwave-assisted tunneling peaks originating from a second-order resonant Andreev process, in which the microwave excites the YSR state triggering a tunneling event transferring a total of two charges. We vary the amplitude and the frequency of the microwave to identify the energy threshold and the evolution of this excitation process. Our work sets an experimental basis and proof-of-principle for the manipulation of YSR states using microwaves with an outlook towards YSR qubits.

cond-mat.supr-con

Universal scaling of tunable Yu-Shiba-Rusinov states across the quantum phase transition

Quantum magnetic impurities give rise to a wealth of phenomena attracting tremendous research interest in recent years. On a normal metal, magnetic impurities generate the correlation-driven Kondo effect. On a superconductor, bound states emerge inside the superconducting gap called the Yu-Shiba-Rusinov (YSR) states. Theoretically, quantum impurity problems have been successfully tackled by numerical renormalization group (NRG) theory, where the Kondo and YSR physics are shown to be unified and the normalized YSR energy scales universally with the Kondo temperature divided by the superconducting gap. However, experimentally the Kondo temperature is usually extracted from phenomenological approaches, which gives rise to significant uncertainties and cannot account for magnetic fields properly. Using scanning tunneling microscopy at 10mK, we apply a magnetic field to several YSR impurities on a vanadium tip to reveal the Kondo effect and employ the microscopic single impurity Anderson model with NRG to fit the Kondo spectra in magnetic fields accurately and extract the corresponding Kondo temperature unambiguously. Some YSR states move across the quantum phase transition (QPT) due to the changes in atomic forces during tip approach, yielding a continuous universal scaling with quantitative precision for quantum spin-1/2 impurities.

cond-mat.supr-con

Compact Itinerant Microwave Photonics with Superconducting High-Kinetic Inductance Microstrips

Microwave photonics is a remarkably powerful system for quantum simulation and technologies, but its integration in superconducting circuits, superior in many aspects, is constrained by the long wavelengths and impedance mismatches in this platform. We introduce a solution to these difficulties via compact networks of high-kinetic inductance microstrip waveguides and coupling wires with strongly reduced phase velocities. We demonstrate broadband capabilities for superconducting microwave photonics in terms of routing, emulation and generalized linear and nonlinear networks.

physics.app-ph

Injection locking and synchronization in Josephson photonics devices

Injection locking can stabilize a source of radiation, leading to an efficient suppression of noise-induced spectral broadening and therefore, to a narrow spectrum. The technique is well established in laser physics, where a phenomenological description due to Adler is usually sufficient. Recently, locking experiments were performed in Josephson photonics devices, where microwave radiation is created by inelastic Cooper pair tunneling across a dc-biased Josephson junction connected in-series with a microwave resonator. An in-depth theory of locking for such devices, accounting for the Josephson non-linearity and the specific engineered environments, is lacking. Here, we study injection locking in a typical Josephson photonics device where the environment consists of a single mode cavity, operated in the classical regime. We show that an in-series resistance, however small, is an important ingredient in describing self-sustained Josephson oscillations and enables the locking region. We derive a dynamical equation describing locking, similar to an Adler equation, from the specific circuit equations. The effect of noise on the locked Josephson phase is described in terms of phase slips in a modified washboard potential. For weak noise, the spectral broadening is reduced exponentially with the injection signal. When this signal is provided from a second Josephson device, the two devices synchronize. In the linearized limit, we recover the Kuramoto model of synchronized oscillators. The picture of classical phase slips established here suggests a natural extension towards a theory of locking in the quantum regime.

cond-mat.mes-hall

Spin-dependent tunneling between individual superconducting bound states

Magnetic impurities on superconductors induce discrete bound levels inside the superconducting gap, known as Yu-Shiba-Rusinov (YSR) states. YSR levels are fully spin-polarized such that the tunneling between YSR states depends on their relative spin orientation. Here, we use scanning tunneling spectroscopy to resolve the spin dynamics in the tunneling process between two YSR states by experimentally extracting the angle between the spins. To this end, we exploit the ratio of thermally activated and direct spectral features in the measurement to directly extract the relative spin orientation between the two YSR states. We find freely rotating spins down to 7mK, indicating a purely paramagnetic nature of the impurities. Such a non-collinear spin alignment is essential not only for producing Majorana bound states but also as an outlook manipulating and moving the Majorana state onto the tip.

cond-mat.supr-con

Noise and full counting statistics of a Cooper pair splitter

We investigate theoretically the noise and the full counting statistics of electrons that are emitted from a superconductor into two spatially separated quantum dots by the splitting of Cooper pairs and further on collected in two normal-state electrodes. With negatively-biased drain electrodes and a large superconducting gap, the dynamics of the Cooper pair splitter can be described by a Markovian quantum master equation. Using techniques from full counting statistics, we evaluate the electrical currents, their noise power spectra, and the power-power correlations in the output leads. The current fluctuations can be attributed to the competition between Cooper pair splitting and elastic cotunneling between the quantum dots via the superconductor. In one regime, these processes can be clearly distinguished in the cross-correlation spectrum with peaks and dips appearing at characteristic frequencies associated with elastic cotunneling and Cooper pair splitting, respectively. We corroborate this interpretation by analyzing the charge transport fluctuations in the time domain, specifically by investigating the $g^{(2)}$-function of the output currents. Our work identifies several experimental signatures of the fundamental transport processes involved in Cooper pair splitting and provides specific means to quantify their relative strengths. As such, our results may help guide and interpret future experiments on current fluctuations in Cooper pair splitters.

cond-mat.mes-hall

Tunneling dynamics between superconducting bound states at the atomic limit

Despite plenty of room at the bottom, there is a limit to the miniaturization of every process. For charge transport this is realized by the coupling of single discrete energy levels at the atomic scale. Here, we demonstrate sequential tunneling between parity protected Yu-Shiba-Rusinov (YSR) states bound to magnetic impurities located on the superconducting tip and sample of a scanning tunneling microscope at 10 mK. We reduce the relaxation of the excited YSR state to the bare minimum and find an enhanced lifetime for single quasiparticle levels. Our work offers a way to characterize and to manipulate coupled superconducting bound states, such as Andreev levels, YSR states, or Majorana bound states.

cond-mat.supr-con