arXiv subjects

Cyrus F. Hirjibehedin

Publications and source records attributed to Cyrus F. Hirjibehedin.

16 recordsLinked to original sources

arXiv2026

Characterization of Aluminum Microwave SQUID Multiplexers for CE$ν$NS Detection

We present the design, fabrication, and characterization of an aluminum-based six-channel microwave SQUID multiplexer ($μ$MUX) prototype for transition-edge sensor (TES) readout in the RICOCHET experiment. The device consists of aluminum coplanar-waveguide resonators and RF SQUIDs with Dolan-style Al/AlO$_x$/Al Josephson junctions. By measuring the resonator scattering parameters at a range of probe tone frequencies, powers, and flux bias points, we demonstrate agreement between the device response and existing multiplexer models. We also characterize the noise performance in both open-loop and flux-ramping modes. With a high electron mobility transistor (HEMT) amplifier, open-loop measurements yield a flux sensitivity of 1-1.5 $μΦ_0/\sqrt{Hz}$. With flux-ramp modulation, low-frequency 1/f noise is suppressed, and the flux sensitivity is around 3-4 $μΦ_0/\sqrt{Hz}$, corresponding to a current sensitivity of 24-33 $pA/\sqrt{Hz}$ at the input coil. We further demonstrate a reduction in readout noise by incorporating a Josephson traveling-wave parametric amplifier (JTWPA) between the $μ$MUX and the HEMT. This achieves an open-loop flux sensitivity of 0.3-0.6 $μΦ_0/\sqrt{Hz}$ and an effective system noise temperature below 1 K. These results establish aluminum $μ$MUX devices as a viable and extensible readout technology for low-noise cryogenic detector arrays.

physics.ins-det↗

arXiv2026

Characterization of Radiation-Induced Errors in Superconducting Qubits Protected with Various Gap-Engineering Strategies

Impacts from high-energy particles cause correlated errors in superconducting qubits by increasing the quasiparticle density in the vicinity of the Josephson junctions (JJs). Such errors are particularly harmful as they cannot be easily remedied via conventional error correcting codes. Recent experiments reduced correlated errors by making the difference in superconducting gap energy across the JJ larger than the qubit transition energy. In this work, we assess gap engineering near the JJ ($δΔ_{\mathrm{JJ}}$) and the capacitor/ground-plane ($δΔ_{\mathrm{M1}}$) by exposing arrays of transmon qubits to two sources of radiation. For $α$-particles from an $^{241}$Am source, we observe $T_1$ errors correlated in space and time, supporting a hypothesis that hadronic cosmic rays are a major contributor to the $10^{-10}$ error floor observed in Ref. 1. For electrons from a pulsed linear accelerator, we observe temporally correlated $T_1$ and $T_2$ errors, this measurement is insensitive to spatial correlations. We observe that the severity of correlated $T_1$ errors is reduced for qubit arrays with a greater degree of gap engineering at the JJ. For both $T_1$ and $T_2$ errors, the recovery time is hastened by an increased $δΔ_{\mathrm{M1}}$, which we attribute to the trapping of quasiparticles into the capacitor/ground-plane. We construct a model of quasiparticle dynamics that qualitatively agrees with our observations. This work reinforces the multifaceted influence of radiation on superconducting qubits and provides strategies for improving radiation resilience.

quant-ph↗

arXiv2025

Improving Transmon Qubit Performance with Fluorine-based Surface Treatments

Reducing materials and processing-induced decoherence is critical to the development of utility-scale quantum processors based on superconducting qubits. Here we report on the impact of two fluorine-based wet etches, which we use to treat the silicon surface underneath the Josephson junctions (JJs) of fixed-frequency transmon qubits made with aluminum base metallization. Using several materials analysis techniques, we demonstrate that these surface treatments can remove germanium residue introduced by our JJ fabrication with no other changes to the overall process flow. These surface treatments result in significantly improved energy relaxation times for the highest performing process, with median $T_1=334~μ$s, corresponding to quality factor $Q=6.6\times10^6$. This result suggests that the metal-substrate interface directly underneath the JJs was a major contributor to microwave loss in these transmon qubit circuits prior to integration of these surface treatments. Furthermore, this work illustrates how materials analysis can be used in conjunction with quantum device performance metrics to improve performance in superconducting qubits.

quant-ph↗

arXiv2023

Characterization of superconducting through-silicon vias as capacitive elements in quantum circuits

The large physical size of superconducting qubits and their associated on-chip control structures presents a practical challenge towards building a large-scale quantum computer. In particular, transmons require a high-quality-factor shunting capacitance that is typically achieved by using a large coplanar capacitor. Other components, such as superconducting microwave resonators used for qubit state readout, are typically constructed from coplanar waveguides which are millimeters in length. Here we use compact superconducting through-silicon vias to realize lumped element capacitors in both qubits and readout resonators to significantly reduce the on-chip footprint of both of these circuit elements. We measure two types of devices to show that TSVs are of sufficient quality to be used as capacitive circuit elements and provide a significant reductions in size over existing approaches.

quant-ph↗

arXiv2023

Visualizing the atomic-scale origin of metallic behavior in Kondo insulators

A Kondo lattice is often electrically insulating at low temperatures. However, several recent experiments have detected signatures of bulk metallicity within this Kondo insulating phase. Here we visualize the real-space charge landscape within a Kondo lattice with atomic resolution using a scanning tunneling microscope. We discover nanometer-scale puddles of metallic conduction electrons centered around uranium-site substitutions in the heavy-fermion compound URu$_2$Si$_2$, and around samarium-site defects in the topological Kondo insulator SmB$_6$. These defects disturb the Kondo screening cloud, leaving behind a fingerprint of the metallic parent state. Our results suggest that the mysterious 3D quantum oscillations measured in SmB$_6$ could arise from these Kondo-lattice defects, although we cannot rule out other explanations. Our imaging technique could enable the development of atomic-scale charge sensors using heavy-fermion probes.

cond-mat.str-el↗

arXiv2023

Bistable electric field control of single-atom magnetocrystalline anisotropy

We reversibly switch the polar environment of an individual magnetic atom with an electric field to control the energy barrier for reversal of magnetization. By applying an electric field in the gap between the tip and sample of a scanning tunneling microscope, we induce bistable changes in the polarization of the region surrounding a chlorine vacancy in a monolayer of sodium chloride on copper terminated by a monolayer of copper nitride. The displacement of the sodium chloride ions alters the local electric polarization and modifies the magnetocrystalline anisotropy experienced by a single cobalt atom. When a cobalt atom is near a chlorine vacancy, spin-sensitive inelastic electron tunneling spectroscopy measurements can reveal the change in anisotropy. The demonstration of atomic-scale control of magnetic properties with electric fields opens new possibilities for probing the origins of magnetoelectric coupling and will stimulate the development of model artificial mutliferroic systems.

cond-mat.mes-hall↗

arXiv2022

Demonstration of tunable three-body interactions between superconducting qubits

Nonpairwise multi-qubit interactions present a useful resource for quantum information processors. Their implementation would facilitate more efficient quantum simulations of molecules and combinatorial optimization problems, and they could simplify error suppression and error correction schemes. Here we present a superconducting circuit architecture in which a coupling module mediates 2-local and 3-local interactions between three flux qubits by design. The system Hamiltonian is estimated via multi-qubit pulse sequences that implement Ramsey-type interferometry between all neighboring excitation manifolds in the system. The 3-local interaction is coherently tunable over several MHz via the coupler flux biases and can be turned off, which is important for applications in quantum annealing, analog quantum simulation, and gate-model quantum computation.

quant-ph↗

arXiv2021

Distinguishing multi-spin interactions from lower-order effects

Multi-spin interactions can be engineered with artificial quantum spins. However, it is challenging to verify such interactions experimentally. Here we describe two methods to characterize the $n$-local coupling of $n$ spins. First, we analyze the variation of the transition energy of the static system as a function of local spin fields. Standard measurement techniques are employed to distinguish $n$-local interactions between up to five spins from lower-order contributions in the presence of noise and spurious fields and couplings. Second, we show a detection technique that relies on time dependent driving of the coupling term. Generalizations to larger system sizes are analyzed for both static and dynamic detection methods, and we find that the dynamic method is asymptotically optimal when increasing the system size. The proposed methods enable robust exploration of multi-spin interactions across a broad range of both coupling strengths and qubit modalities.

quant-ph↗

arXiv2020

Characterizing and optimizing qubit coherence based on SQUID geometry

The dominant source of decoherence in contemporary frequency-tunable superconducting qubits is 1/$f$ flux noise. To understand its origin and find ways to minimize its impact, we systematically study flux noise amplitudes in more than 50 flux qubits with varied SQUID geometry parameters and compare our results to a microscopic model of magnetic spin defects located at the interfaces surrounding the SQUID loops. Our data are in agreement with an extension of the previously proposed model, based on numerical simulations of the current distribution in the investigated SQUIDs. Our results and detailed model provide a guide for minimizing the flux noise susceptibility in future circuits.

quant-ph↗

arXiv2017

Gating classical information flow through spin chains by quantum phase transitions

To push commercial electronics beyond its current size limits, atomic-scale communication channels and logic units need to be designed, making the use of quantum entities an imperative. In this regime, quantum fluctuations naturally become prominent, and are generally considered to be detrimental. Here we show that for spin-based information processing, these fluctuations can be uniquely exploited to gate the flow of classical binary information across a magnetic chain. Moreover, this information flow can be controlled with a modest external magnetic field that drives the system through different many-body quantum phases in which the orientation of the final spin does or does not reflect the orientation of the initial input. Our results are general for a wide class of anisotropic spin chains that act as magnetic cellular automata, and suggest that quantum fluctuations may play a unique role in driving classical information flow at the atomic scale.

cond-mat.mes-hall↗

arXiv2016

Sub-molecular modulation of a 4f driven Kondo resonance by surface-induced asymmetry

Coupling between a magnetic impurity and an external bath can give rise to many-body quantum phenomena, including Kondo and Hund's impurity states in metals, and Yu-Shiba-Rusinov states in superconductors. While advances have been made in probing the magnetic properties of d-shell impurities on surfaces, the confinement of f orbitals makes them difficult to access directly. Here we show that a 4f driven Kondo resonance can be modulated spatially by asymmetric coupling between a metallic surface and a molecule containing a 4f-like moment. Strong hybridisation of dysprosium double-decker phthalocyanine with Cu(001) induces Kondo screening of the central magnetic moment. Misalignment between the symmetry axes of the molecule and the surface induces asymmetry in the molecule's electronic structure, spatially mediating electronic access to the magnetic moment through the Kondo resonance. This work demonstrates the important role that molecular ligands play in mediating electronic and magnetic coupling and in accessing many-body quantum states.

cond-mat.mes-hall↗

arXiv2015

Tunable magnetoresistance in an asymmetrically coupled single molecule junction

Phenomena that are highly sensitive to magnetic fields can be exploited in sensors and non-volatile memories. The scaling of such phenomena down to the single molecule level may enable novel spintronic devices. Here we report magnetoresistance in a single molecule junction arising from negative differential resistance that shifts in a magnetic field at a rate two orders of magnitude larger than Zeeman shifts. This sensitivity to the magnetic field produces two voltage-tunable forms of magnetoresistance, which can be selected via the applied bias. The negative differential resistance is caused by transient charging of an iron phthalocyanine (FePc) molecule on a single layer of copper nitride (Cu2N) on a Cu(001) surface, and occurs at voltages corresponding to the alignment of sharp resonances in the filled and empty molecular states with the Cu(001) Fermi energy. An asymmetric voltage-divider effect enhances the apparent voltage shift of the negative differential resistance with magnetic field, which inherently is on the scale of the Zeeman energy. These results illustrate the impact that asymmetric coupling to metallic electrodes can have on transport through molecules, and highlight how this coupling can be used to develop molecular spintronic applications.

cond-mat.mes-hall↗

arXiv2014

Control of single-spin magnetic anisotropy by exchange coupling

The properties of quantum systems interacting with their environment, commonly called open quantum systems, can be strongly affected by this interaction. While this can lead to unwanted consequences, such as causing decoherence in qubits used for quantum computation, it can also be exploited as a probe of the environment. For example, magnetic resonance imaging is based on the dependence of the spin relaxation times of protons in water molecules in a host's tissue. Here we show that the excitation energy of a single spin, which is determined by magnetocrystalline anisotropy and controls its stability and suitability for use in magnetic data storage devices, can be modified by varying the exchange coupling of the spin to a nearby conductive electrode. Using scanning tunnelling microscopy and spectroscopy, we observe variations up to a factor of two of the spin excitation energies of individual atoms as the strength of the spin's coupling to the surrounding electronic bath changes. These observations, combined with calculations, show that exchange coupling can strongly modify the magnetic anisotropy. This system is thus one of the few open quantum systems in which the energy levels, and not just the excited-state lifetimes, can be controllably renormalized. Furthermore, we demonstrate that the magnetocrystalline anisotropy, a property normally determined by the local structure around a spin, can be electronically tuned. These effects may play a significant role in the development of spintronic devices5 in which an individual magnetic atom or molecule is coupled to conducting leads.

cond-mat.mes-hall↗

arXiv2013

Investigating individual arsenic dopant atoms in silicon using low-temperature scanning tunnelling microscopy

We study sub-surface arsenic dopants in a hydrogen terminated Si(001) sample at 77 K, using scanning tunnelling microscopy and spectroscopy. We observe a number of different dopant related features that fall into two classes, which we call As1 and As2. When imaged in occupied states the As1 features appear as anisotropic protrusions superimposed on the silicon surface topography, and have maximum intensities lying along particular crystallographic orientations. In empty-state images the features all exhibit long-range circular protrusions. The images are consistent with buried dopants that are in the electrically neutral (D0) charge state when imaged in filled states, but become positively charged (D+) through electrostatic ionisation when imaged under empty state conditions, similar to previous observations of acceptors in GaAs. Density functional theory (DFT) calculations predict that As dopants in the third layer of the sample induce two states lying just below the conduction band edge, which hybridize with the surface structure creating features with the surface symmetry consistent with our STM images. The As2 features have the surprising characteristic of appearing as a protrusion in filled state images and an isotropic depression in empty state images, suggesting they are negatively charged at all biases. We discuss the possible origins of this feature.

cond-mat.mes-hall↗

arXiv2008

The role of magnetic anisotropy in the Kondo effect

In the Kondo effect, a localized magnetic moment is screened by forming a correlated electron system with the surrounding conduction electrons of a non-magnetic host. Spin S=1/2 Kondo systems have been investigated extensively in theory and experiments, but magnetic atoms often have a larger spin. Larger spins are subject to the influence of magnetocrystalline anisotropy, which describes the dependence of the magnetic moment's energy on the orientation of the spin relative to its surrounding atomic environment. Here we demonstrate the decisive role of magnetic anisotropy in the physics of Kondo screening. A scanning tunnelling microscope is used to simultaneously determine the magnitude of the spin, the magnetic anisotropy and the Kondo properties of individual magnetic atoms on a surface. We find that a Kondo resonance emerges for large-spin atoms only when the magnetic anisotropy creates degenerate ground-state levels that are connected by the spin flip of a screening electron. The magnetic anisotropy also determines how the Kondo resonance evolves in a magnetic field: the resonance peak splits at rates that are strongly direction dependent. These rates are well described by the energies of the underlying unscreened spin states.

cond-mat.str-el↗

arXiv2007

Spin-texture and magneto-roton excitations at nu=1/3

Neutral spin texture ST excitations at nu=1/3 are directly observed for the first time by resonant inelastic light scattering. They are determined to involve two simultaneous spin- flips. At low magnetic fields, the ST energy is below that of the magneto-roton minimum. With increasing in-plane magnetic field these modes energies cross at a critical ratio of the Zeeman and Coulomb energies of eta_c=0.020 +- 0.001. Surprisingly, the intensity of the ST mode grows with temperature in the range in which the magneto-roton modes collapse. The temperature dependence is interpreted in terms of a competition between coexisting phases supporting different excitations. We consider the role of the ST excitations in activated transport at nu=1/3.

cond-mat.str-el↗