Searcharxiv⌕ Search

arXiv subjects

D. G. Hinks

Publications and source records attributed to D. G. Hinks.

At least 55 records · Page 3Linked to original sources

On the Doping and Temperature Dependence of the Mass Enhancement Observed in the Cuprate Bi2212

High-resolution photoemission is used to study the electronic structure of the cuprate superconductor, Bi2212, as a function of hole doping and temperature. A kink observed in the band dispersion in the nodal direction in the superconducting state is associated with coupling to a resonant mode observed in neutron scattering. From the measured real part of the self energy it is possible to extract a coupling constant which is largest in the underdoped regime, then decreasing continuously into the overdoped regime.

cond-mat.supr-con↗

Dependence of the Superconducting Transition Temperature of MgB2 on Pressure to 20 GPa

The dependence of Tc on nearly hydrostatic pressure has been measured for an isotopically pure (11B) MgB2 sample in a helium-loaded diamond-anvil-cell to nearly 20 GPa. Tc decreases monotonically with pressure from 39.1 K at ambient pressure to 20.9 K at 19.2 GPa. The initial dependence is the same as that obtained earlier (dTc/dP = -1.11(2) K/GPa) on the same sample in a He-gas apparatus to 0.7 GPa. The observed pressure dependence Tc(P) to 20 GPa can be readily described in terms of simple lattice stiffening within standard phonon-mediated BCS superconductivity.

cond-mat.supr-con↗

The Dependence of Tc on Hydrostatic Pressure in Superconducting MgB2

The dependence of Tc on hydrostatic (He-gas) pressure has been determined to 0.7 GPa. We find that Tc decreases linearly and reversibly under pressure at the rate dTc/dP = -1.11 +- 0.02 K/GPa. These studies were carried out on the same sample used in earlier structural studies under He-gas pressure which yielded the bulk modulus B = 147.2 +- 0.7 GPa. The value of the logarithmic volume derivative of Tc is thus accurately determined, dlnTc/dlnV = +4.16 +- 0.08, allowing quantitative comparison with theory. The present results support the emerging picture that MgB2 is a BCS superconductor with electron-phonon pairing interaction.

cond-mat.supr-con↗

Quasiparticle Liquid in the Highly Overdoped Bi2212

We present results from the study of a highly overdoped (OD) Bi2212 with a $T_{c}=51$K using high resolution angle-resolved photoemission spectroscopy. The temperature dependent spectra near the ($π,0$) point show the presence of the sharp peak well above $T_{c}$. From the nodal direction, we make comparison of the self-energy with the optimally doped and underdoped cuprates, and the Mo(110) surface state. We show that this OD cuprate appears to have properties that approach that of the Mo. Further analysis shows that the OD has a more $k$-independent lineshape at the Fermi surface than the lower-doped cuprates. This allows for a realistic comparison of the nodal lifetime values to the experimental resistivity measurements via Boltzmann transport formulation. All these observations point to the validity of the quasiparticle picture for the OD even in the normal state within a certain energy and momentum range.

cond-mat.supr-con↗

The reduced total isotope effect and its implications on the nature of superconductivity in MgB2

The recent discovery of superconductivity at ~39 K in MgB2, by Nagamatsu et al. establishes this simple binary compound as having the highest bulk superconducting transition temperature, Tc, of any non-copper-oxide material. Much of the initial research has focused on whether MgB2 is a conventional BCS, electron-phonon mediated superconductor, and, if it is, why Tc is so high. Isotope effect measurements, in which the atom masses are manipulated to systematically change the phonon frequencies, are one of the fundamental experimental tests of electron-phonon mediated superconductivity. One would expect the total isotope effect coefficient, i.e. the sum of both the Mg and B coefficients, to be 1/2 for a high- Tc, phonon mediated, simple sp orbital superconductor like MgB2. We find a value of 0.32(1), much reduced from the canonical BCS value of 0.5. This requires large values of l (electron-phonon coupling constant) and m* (repulsive electron-electron pseudopotential) to account for the high Tc and, thus, constrains any theoretical model for superconductivity in MgB2.

cond-mat.supr-con↗

Specific Heat of Mg ^{11}B_2

Measurements of the specific heat of Mg ^{11}B_2 (MgB2), from 1 to 50 K, in magnetic fields to 9 T, give the Debye temperature, $Θ$ = 1050 K, the coefficient of the normal-state electron contribution, $γ_n$ = 2.6 mJ mol^{-1} K^{-2}, and a discontinuity in the zero-field specific heat of 133 mJ mol^{-1} K^{-1} at $T_c$ = 38.7 K. The estimated value of the electron-phonon coupling parameter, $λ$ = 0.62, could account for the observed $T_c$ only if the important phonon frequencies are unusually high relative to $Θ$. At low $T$, there is a strongly field-dependent feature that suggests the existence of a second energy gap, about four times smaller than the major gap.

cond-mat.supr-con↗

Experimental study of MgB2 decomposition

The thermal stability of MgB2 has been studied experimentally to determine the role of thermodynamic and kinetic barriers in the decomposition process. The MgB2 decomposition rate approaches one monolayer per second at 650 C and has an activation energy of 2.0 eV. The evaporation coefficient is inferred to be ~ 10(-4), indicating that this process is kinetically limited. These values were inferred from in-situ measurements using a quartz crystal microbalance and a residual gas analyzer, in conjunction with ex-situ measurements of re-deposited material by Rutherford Backscattering Spectroscopy. The presence of a large kinetic barrier to decomposition indicates that the synthesis of MgB2 thin films conditions may be possible with vacuum processing, albeit within a narrow window in the reactive growth conditions.

cond-mat.supr-con↗

Lattice Properties of MgB2 versus Temperature and Pressure

We have determined the structural properties of the superconducting compound MgB2 as a function of temperature from 11 K to 297 K and as a function of hydrostatic pressure up to 0.62 GPa using neutron powder diffraction. This compound, when compared to other diborides with the same structure, is characterized by unusually large anisotropies of both the thermal expansion and compressibility, with the c-axis responses being substantially larger in both cases. We speculate that the comparatively weaker metal-boron bonding in MgB2, manifest by these lattice responses, is important for establishing the structural features that give rise to high Tc superconductivity in this structure type.

cond-mat.supr-con↗

Phonon Density-of-States in MgB2

We report inelastic neutron scattering measurements of the phonon density-of-states in Mg11B2, which has a superconducting transition at 39.2 K. The acoustic phonons extend in energy to 36 meV, and there are highly dispersive optic branches peaking at 54, 78, 89 and 97 meV. A simple Born-von Karman model is able to reproduce the mode energies, and provides an estimate of the electron-phonon coupling of lambda~0.9. The estimated boron and magnesium contributions to the isotope effect are in qualitative agreement with experiment. The data confirm that a conventional phonon mechanism, with moderately strong electron-phonon coupling, can explain the observed superconductivity.

cond-mat.supr-con↗

Correlation of Tunneling Spectra in Bi2Sr2CaCu2O(8+delta) with the Resonance Spin Excitation

New break-junction tunneling data are reported in Bi2Sr2CaCu2O(8+delta) over a wide range of hole concentration from underdoped (Tc = 74 K) to optimal doped (Tc = 95 K) to overdoped (Tc = 48 K). The conductances exhibit sharp dips at a voltage, Omega/e, measured with respect to the superconducting gap. Clear trends are found such that the dip strength is maximum at optimal doping and that Omega scales as 4.9 kTc over the entire doping range. These features link the dip to the resonance spin excitation and suggest quasiparticle interactions with this mode are important for superconductivity.

cond-mat.supr-con↗

Energy Gap from Tunneling and Metallic Sharvin Contacts onto MgB2: Evidence for a Weakened Surface Layer

Point-contact tunnel junctions using a Au tip on sintered MgB2 pellets reveal a sharp superconducting energy gap that is confirmed by subsequent metallic Sharvin contacts made on the same sample. The peak in the tunneling conductance and the Sharvin contact conductance follow the BCS form, but the gap values of 4.3 meV are less than the weak-coupling BCS value of 5.9 meV for the bulk Tc of 39 K. The low value of Delta compared to the BCS value for the bulk Tc is possibly due to chemical reactions at the surface.

cond-mat.supr-con↗

Scanning Tunneling Spectroscopy in MgB2

We present scanning tunneling microscopy measurements of the surface of superconducting MgB2 with a critical temperature of 39K. In zero magnetic field the conductance spectra can be analyzed in terms of the standard BCS theory with a smearing parameter Gamma. The value of the superconducting gap is 5.2 meV at 4.2 K, with no experimentally significant variation across the surface of the sample. The temperature dependence of the gap follows the BCS form, fully consistent with phonon-mediated superconductivity in this novel superconductor. The application of a magnetic field induces strong pair-breaking as seen in the conductance spectra in fields up to 6 T.

cond-mat.supr-con↗

Coherent quasiparticle weight and its connection to high-T_c superconductivity from angle-resolved photoemission

In conventional superconductors, the pairing energy gap (Δ) and superconducting phase coherence go hand-in-hand. As the temperature is lowered, both the energy gap and phase coherence appear at the transition temperature T_c. In contrast, in underdoped high-T_c superconductors (HTSCs), a pseudogap appears at a much higher temperature T^*, smoothly evolving into the superconducting gap at T_c. Phase coherence on the other hand is only established at T_c, signaled by the appearance of a sharp quasiparticle (QP) peak in the excitation spectrum. Another important difference between the two types of superconductors is in the ratio of 2Δ/ T_c=R. In BCS theory, R~3.5, is constant. In the HTSCs this ratio varies widely, continuing to increase in the underdoped region, where the gap increases while T_c decreases. Here we report that in HTSCs it is the ratio z_AΔ_m/T_c which is approximately constant, where Δ_m is the maximum value of the d-wave gap, and z_A is the weight of the coherent excitations in the spectral function. This is highly unusual, since in nearly all phase transitions, T_c is determined by an energy scale alone. We further show that in the low-temperature limit, z_{\it A} increases monotonically with increasing doping x. The growth is linear, i.e. z_A(x)\propto x, in the underdoped to optimally doped regimes, and slows down in overdoped samples. The reduction of z_A with increasing temperature resembles that of the c-axis superfluid density.

cond-mat.supr-con↗

Measurements of the absolute value of the penetration depth in high-$ T_c$ superconductors using a tunnel diode resonator

A method is presented to measure the absolute value of the London penetration depth, $λ$, from the frequency shift of a resonator. The technique involves coating a high-$T_c$ superconductor (HTSC) with film of low - Tc material of known thickness and penetration depth. The method is applied to measure London penetration depth in YBa2Cu3O{7-δ} (YBCO) Bi2Sr2CaCu2O{8+δ} (BSCCO) and Pr{1.85}Ce{0.15}CuO{4-δ}$ (PCCO). For YBCO and BSCCO, the values of $λ(0)$ are in agreement with the literature values. For PCCO $λ\approx 2790$ Å, reported for the first time.

cond-mat.supr-con↗

Nonequilibrium Campbell length: probing the vortex pinning potential

The $AC$ magnetic penetration depth $λ(T,H,j)$ was measured in presence of a macroscopic $DC$ (Bean) supercurrent, $j$. In single crystal BSCCO below approximately 28 K, $λ(T,H,j)$ exhibits thermal hysteresis. The irreversibility arises from a shift of the vortex position within its pinning well as $j$ changes. It is demonstrated that below a new irreversibility temperature, the nonequilibrium Campbell length depends upon the ratio $j/j_c$. $λ(T,H,j)$ {\it increases} with $j/j_c$ as expected for a non-parabolic potential well whose curvature {\it decreases} with the displacement. Qualitatively similar results are observed in other high-$T_{c}$ and conventional superconductors.

cond-mat.supr-con↗

Low temperature vortex phase diagram of Bi2Sr2CaCu2O8 : a magnetic penetration depth study

We report measurements of the magnetic penetration depth λ_m(T) in the presence of a DC magnetic field in optimally doped BSCCO-2212 single crystals. Warming, after magnetic field is applied to a zero-field cooled sample, results in a non-monotonic λ_m(T), which does not coincide with a curve obtained upon field cooling, thus exhibiting a hysteretic behaviour. We discuss the possible relation of our results to the vortex decoupling, unbinding, and dimensional crossover.

cond-mat.supr-con↗

Electronic Spectra and Their Relation to the (pi,pi) Collective Mode in High-Tc Superconductors

Photoemission spectra of Bi2Sr2CaCu2O8 reveal that the high energy feature near (pi,0), the "hump", scales with the superconducting gap and persists above Tc in the pseudogap phase. As the doping decreases, the dispersion of the hump increasingly reflects the wavevector (pi,pi) characteristic of the undoped insulator, despite the presence of a large Fermi surface. This can be understood from the interaction of the electrons with a collective mode, supported by our observation that the doping dependence of the resonance observed by neutron scattering is the same as that inferred from our data.

cond-mat.supr-con↗

Tunneling Spectroscopy of Tl2Ba2CuO6

New results from tunneling spectroscopies on near optimally-doped single crystals of Tl_{2}Ba_{2}CuO_{6} (Tl-2201) junctions are presented. The superconductor-insulator-normal metal (SIN) tunnel junctions are obtained using the point-contact technique with a Au tip. The tunneling conductances reproducibly show a sharp cusp-like subgap, prominent quasiparticle peaks with a consistent asymmetry, and weakly decreasing backgrounds. A rigorous analysis of the SIN tunneling data is performed using two different models for the $d_{x^{2}-y^{2}}$ (d-wave) density of states (DOS). Based on these and earlier results, the tunneling DOS of Tl-2201 have exhibited the most reproducible data that are consistent with a d-wave gap symmetry. We show that the dip feature at $2Δ$ that is clearly seen in SIN tunneling data of Bi_{2}Sr_{2}CaCu_{2}O_{8+δ} is also present in Tl-2201, but at a weaker level. The gap values for crystals with a bulk T_c = 86 K are in the range of 19-25 meV.

cond-mat.supr-con↗